Molecular geochemistry of radium; A key to understanding cation adsorption reaction on clay minerals

Yamaguchi, Akiko; Kurihara, Yuichi*; Nagata, Kojiro*; Tanaka, Kazuya; Higaki, Shogo*; Kobayashi, Toru; Tanida, Hajime; Ohara, Yoshiyuki*; Yokoyama, Keiichi; Yaita, Tsuyoshi; et al.

Journal of Colloid and Interface Science, 661, p.317 - 332, 2024/05

https://doi.org/10.1016/j.jcis.2024.01.120

no abstracts in English

Extended X-ray absorption fine structure spectroscopy measurements and molecular dynamics simulations reveal the hydration structure of the radium(II) ion

Yamaguchi, Akiko; Nagata, Kojiro*; Kobayashi, Keita; Tanaka, Kazuya; Kobayashi, Toru; Tanida, Hajime; Shimojo, Kojiro; Sekiguchi, Tetsuhiro; Kaneta, Yui; Matsuda, Shohei; et al.

iScience (Internet), 25(8), p.104763_1 - 104763_12, 2022/08

https://doi.org/10.1016/j.isci.2022.104763

no abstracts in English

Hydration structures of barium ions; molecular dynamics simulations using the SCAN meta-GGA density functional and EXAFS spectroscopy studies

Yamaguchi, Akiko; Kobayashi, Keita; Takahashi, Yoshio*; Machida, Masahiko; Okumura, Masahiko

Chemical Physics Letters, 780, p.138945_1 - 138945_5, 2021/10

https://doi.org/10.1016/j.cplett.2021.138945

no abstracts in English

Multi-step magnetic transitions in EuNiIn

Ikeda, Shugo*; Kaneko, Koji; Tanaka, Yuki*; Kawasaki, Takuro; Hanashima, Takayasu*; Munakata, Koji*; Nakao, Akiko*; Kiyanagi, Ryoji; Ohara, Takashi; Mochizuki, Kensei*; et al.

Journal of the Physical Society of Japan, 89(1), p.014707_1 - 014707_7, 2020/01

https://doi.org/10.7566/JPSJ.89.014707

Submesoscale mixing on initial dilution of radionuclides released from the Fukushima Daiichi Nuclear Power Plant

Kamidaira, Yuki; Uchiyama, Yusuke*; Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko

Journal of Geophysical Research; Oceans (Internet), 123(4), p.2808 - 2828, 2018/04

https://doi.org/10.1002/2017JC013359

We developed a submesoscale eddy-resolving oceanic dispersal modeling system consisting of a double nested oceanic downscaling model and an offline oceanic radionuclides dispersion model to investigate influences of submesoscale coherent structures (SCSs) and associated ageostrophic secondary circulations (ASCs) on the three-dimensional (3D) dispersal and initial dilution of the dissolved radioactive Cs accidentally released from the Fukushima Daiichi Nuclear Power Plant (FNPP1) occurred since March 2011. The extensive model-data comparison demonstrates that the elaborated innermost high-resolution model at a lateral grid resolution of 1 km successfully reproduces transient mesoscale oceanic structures, the Kuroshio path and stratification, and spatiotemporal variations of 3D Cs concentrations. These SCSs and ASCs occurred primarily due to shear instability with baroclinic instability as the secondary mechanism, according to energy conversion and spectral analyses. The vertical Cs flux analysis was performed with decomposition of the variables into the mean, mesoscale, and submesoscale components using frequency and wavenumber filters. The vertical Cs flux analysis explained that 84% of the FNPP1-derived Cs was transported downward below the mixed layer by eddies, with the major contributions from ASCs induced by submesoscale eddies.

Oceanic dispersion of Fukushima-derived Cs-137 simulated by multiple oceanic general circulation models

Kawamura, Hideyuki; Furuno, Akiko; Kobayashi, Takuya; In, Teiji*; Nakayama, Tomoharu*; Ishikawa, Yoichi*; Miyazawa, Yasumasa*; Usui, Norihisa*

Journal of Environmental Radioactivity, 180, p.36 - 58, 2017/12

https://doi.org/10.1016/j.jenvrad.2017.09.020

This study simulates the oceanic dispersion of Fukushima-derived Cs-137 by an oceanic dispersion model and multiple oceanic general circulation models. The models relatively well reproduced the observed Cs-137 concentrations in the coastal, offshore, and open oceans. Multiple simulations in the coastal, offshore, and open oceans consistently suggested that Cs-137 dispersed along the coast in the north-south direction during the first few months post-disaster, and were subsequently dispersed offshore by the Kuroshio Current and Kuroshio Extension. Quantification of the Cs-137 amounts suggested that Cs-137 actively dispersed from the coastal and offshore oceans to the open ocean, and from the surface layer to the deeper layers in the North Pacific.

Behavior of tritium in the vacuum vessel of JT-60U

Kobayashi, Kazuhiro; Torikai, Yuji*; Saito, Makiko; Alimov, V. Kh.*; Miya, Naoyuki; Ikeda, Yoshitaka

Fusion Science and Technology, 67(2), p.428 - 431, 2015/03

https://doi.org/10.13182/FST14-T46

Disassembly of the JT-60U torus was started in 2010 after 18 years deuterium operations. In the disassembly of the JT-60U torus, tritium retention in the vacuum vessel of the JT-60U is one of the most important safety issues for the fusion reactor. It was very important to study the tritium behavior in Inconel 625 from viewpoint of the clearance procedure in the future plan. After the tritium release for about 1 year at 298 K, the residual tritium in the specimen was released by heating up to 1073 K, and then the residual tritium in the specimen was measured by chemical etching method. Most of the chemical form of the released tritium was HTO. The contaminated specimen by tritium was released continuously the diffusible tritium under the ambient condition. In the tritium release experiment, most of tritium in the specimen was released during 1 year.

Nonhomologous end-joining repair plays a more important role than homologous recombination repair in defining radiosensitivity after exposure to high-LET radiation

Takahashi, Akihisa*; Kubo, Makoto*; Ma, H.*; Nakagawa, Akiko*; Yoshida, Yukari*; Isono, Mayu*; Kanai, Tatsuaki*; Ono, Tatsuya*; Furusawa, Yoshiya*; Funayama, Tomoo; et al.

Radiation Research, 182(3), p.338 - 344, 2014/09

https://doi.org/10.1667/RR13782.1

To clarify whether high-LET radiation inhibits all repair pathways or specifically one repair pathway, studies were designed to examine the effects of radiation with different LET values on DNA DSB repair and radiosensitivity. Embryonic fibroblasts bearing repair gene KO were exposed to X rays, carbon-, iron-, neon- and argon-ion beams. Cell survival was measured with colony-forming assays. The sensitization enhancement ratio (SER) values were calculated using the 10% survival dose of wild-type cells and repair-deficient cells. Cellular radiosensitivity was listed in descending order: double-KO cells NHEJ-KO cells HR-KO cells wild-type cells. Although HR-KO cells had an almost constant SER value, NHEJ-KO cells showed a high-SER value when compared to HR-KO cells, even with increasing LET values. These results suggest that with carbon-ion therapy, targeting NHEJ repair yields higher radiosensitivity than targeting homologous recombination repair.

Intercomparison of numerical simulations on oceanic dispersion of the radioactive cesium released because of the Fukushima disaster

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; Usui, Norihisa*; Kamachi, Masafumi*; Nishikawa, Shiro*; Ishikawa, Yoichi*

Proceedings of 19th Pacific Basin Nuclear Conference (PBNC 2014) (USB Flash Drive), 7 Pages, 2014/08

Numerical simulations on oceanic dispersion of the radioactive cesium in the North Pacific from March 2011 to September 2013 were conducted to clarify the concentration of the radioactive cesium released from the Fukushima Daiichi Nuclear Power Plant. We implemented the oceanic dispersion simulations with two independent ocean reanalysis dataset. It was suggested that the Cs concentration in the North Pacific was lower than the pre-Fukushima background level about two years after the Fukushima disaster. The intercomparison revealed that meso-scale eddies in the Kuroshio Extension region may have efficiently diluted the radioactive cesium concentration at the sea surface. In addition, it was suggested that the enhanced downward current accompanied by the meso-scale eddies played an important role in transporting the radioactive cesium into the intermediate layer.

Numerical experiments on dispersion of radionuclides in the ocean released from the Fukushima Daiichi Nuclear Power Plant

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; In, Teiji*; Ishikawa, Yoichi*; Nakayama, Tomoharu*; Shima, Shigeki*; Awaji, Toshiyuki*

Reports of Research Institute for Applied Mechanics, Kyushu University, (143), p.111 - 117, 2012/09

Because of the Fukushima Dai-ichi Nuclear Power Plant disaster, some radionuclides were released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant. In response to this situation, numerical experiments were carried out at Japan Atomic Energy Agency using an oceanic dispersion model and an ocean general circulation model to estimate an effect of the radionuclides on marine environment. It was suggested that the radionuclides deposited from the atmosphere mainly in the middle of March after the disaster spread over a comparatively wide area of the Pacific Ocean east of Japan. On the other hand the radionuclides directly released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant were carried along the coast and then spread along the Kuroshio extension.