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Tonna, Ryutaro*; Sasaki, Takayuki*; Okamoto, Yoshihiro; Kobayashi, Taishi*; Akiyama, Daisuke*; Kirishima, Akira*; Sato, Nobuaki*
Journal of Nuclear Materials, 589, p.154862_1 - 154862_10, 2024/02
Times Cited Count：2 Percentile：31.89(Materials Science, Multidisciplinary)The dissolution behavior of FeUO
compounds formed by a high-temperature reaction of UO
with iron, a stainless-steel component of reactor structural materials, was investigated under atmospheric conditions. The compounds were prepared in an electric furnace using U
O
and FeO as starting materials, and their solid states were analyzed using X-ray diffraction, scanning electron microscopy energy dispersive X-ray spectroscopy, and X-ray absorption fine structure spectroscopy. The concentration of nuclides dissolved in water was examined by performing static leaching tests of FeUO compounds for up to three months. A redox reaction was proposed to occur between trivalent Fe and pentavalent U ions in the early stage of FeUO dissolution. It was thermodynamically deduced that the reduced divalent Fe ion was finally oxidized into a trivalent ion in the presence of dissolved oxygen, and iron hydroxide limited the solubility of Fe. Meanwhile, the concentration of hexavalent U (i.e., uranyl ion) was limited owing to the presence of secondary minerals such as metaschoepite and sodium uranate and subsequently decreased, possibly owing to sorption on Fe oxides, for example. The concentrations of multivalent ions of fission products, such as Ru and Ce, also decreased, likely for the reason above. By contrast, the concentration of soluble Cs ions did not decrease. The validity of this interpretation was supported by comparing the results with the dissolution behavior of a reference sample (Fe-free UO).
Be ground-state molecular structure using Be(
)
He triple differential reaction cross-section measurementsLi, P. J.*; Beaumel, D.*; Lee, J.*; Assi
, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; Kanada-En'yo, Yoshiko*; et al.
Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11
Times Cited Count：13 Percentile：91.04(Physics, Multidisciplinary)The cluster structure of the neutron-rich isotope Be has been probed via the () reaction. The triple differential cross-section was extracted and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using the Tohsaki-Horiuchi-Schuck-R
pke wave function and the wave function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the description of the Be ground-state as a rather compact nuclear molecule.
Umino, Yoshinori; Kato, Keisuke; Tanigawa, Masafumi; Kobayashi, Daisuke; Obu, Tomoyuki; Kimura, Yuichi*; Nemoto, Ryo*; Tajiri, Kazuma*
Nihon Hozen Gakkai Dai-19-Kai Gakujutsu Koenkai Yoshishu, p.33 - 36, 2023/08
In the basic laboratory of the Plutonium Conversion Development Facility in Tokai Reprocessing Plant, tests had been conducted to obtain effective data for manufacturing mixed plutonium and uranium oxide powder by irradiating a mixture of plutonium and uranium solution with microwaves. The test has already been completed, and we are currently dismantling and removing equipment. In this paper, techniques related to equipment renewal, dismantling and removal works inside the glove-box are discussed.
Yamamoto, Masahiko; Nishida, Naoki; Kobayashi, Daisuke; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kitao, Takahiko; Kuno, Takehiko
JAEA-Technology 2023-004, 30 Pages, 2023/06
JAEA-Technology-2023-004.pdf:1.94MB
Glove-box gloves, that are used for handling nuclear fuel materials at the Tokai Reprocessing Plant (TRP) of the Japan Atomic Energy Agency, have an expiration date by internal rules. All gloves are replaced at a maximum of every 4-year. However, degrees of glove deterioration varies depending on its usage environment such as frequency, chemicals, and radiation dose. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured and technical evaluation method for the glove life-time is established. It was found that gloves without any defects in its appearance have enough physical properties and satisfies the acceptance criteria values of new gloves. Thus, it was considered that the expired gloves could be used for total of 8-year, by adding 4-year of new glove life-time. In addition, the results of extrapolation by plotting the glove's physical properties versus the used years showed that the physical properties at 8-year is on the safer side than the reported physical properties of broken glove. Also, the data are not significantly different from the physical properties of the long-term storage glove (8 and 23 years). Based on these results, life-time of gloves at TRP is set to be 8-year. The frequency of glove inspections are not changed, and if any defects is found, the glove is promptly replaced. Thus, the risk related to glove usage is not increased. The cost of purchasing gloves, labor for glove replacement, and the amount of generated waste can be reduced by approximately 40%, respectively, resulting in more efficient and rationalized glove management.
, Zr, and stainless steel and leaching behavior of the fission products and matrix elementsTonna, Ryutaro*; Sasaki, Takayuki*; Kodama, Yuji*; Kobayashi, Taishi*; Akiyama, Daisuke*; Kirishima, Akira*; Sato, Nobuaki*; Kumagai, Yuta; Kusaka, Ryoji; Watanabe, Masayuki
Nuclear Engineering and Technology, 55(4), p.1300 - 1309, 2023/04
Times Cited Count：5 Percentile：79.63(Nuclear Science & Technology)Simulated debris was synthesized using UO, Zr, and stainless steel and a heat treatment method under inert or oxidizing conditions. The primary U solid phase of the debris synthesized at 1473 K under inert conditions was UO, whereas a (U,Zr)O solid solution formed at 1873 K. Under oxidizing conditions, a mixture of UO and (Fe,Cr)UO phases formed at 1473 K whereas a (U,Zr)O
solid solution formed at 1873 K. The leaching behavior of the fission products from the simulated debris was evaluated using two methods: the irradiation method, for which fission products were produced via neutron irradiation, and the doping method, for which trace amounts of non-radioactive elements were doped into the debris. The dissolution behavior of U depended on the properties of the debris and aqueous medium the debris was immersed in. Cs, Sr, and Ba leached out regardless of the primary solid phases. The leaching of high-valence Eu and Ru ions was suppressed, possibly owing to their solid-solution reaction with or incorporation into the uranium compounds of the simulated debris.
100 MeV/nucleonPohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G
mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.
Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04
Times Cited Count：11 Percentile：89.82(Physics, Multidisciplinary)We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient 
O nucleus with large Fermi-surface asymmetry at 100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.
Kobayashi, Daisuke; Yamamoto, Masahiko; Nishida, Naoki; Miyoshi, Ryuta; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kato, Keisuke; Nishino, Saki; Kuno, Takehiko; Kitao, Takahiko; et al.
Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.237 - 240, 2022/07
All gloves attached to glove-box in Tokai Reprocessing Plant have a fixed expiration date and have to be replaced every 4-year. However, degrees of glove deterioration are different depending on its usage environment (frequency, chemicals, radiation, etc.), because of rubber products. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured, and the life-time of gloves are estimated. As a result, gloves without any defects in its appearance have enough physical property for acceptance criteria of new glove. The extrapolated physical property of glove is sufficiently larger than the reported values of damaged glove. No deterioration in physical properties of gloves, that are periodically replaced without any defects in its appearance, is observed and the usable life-time of the glove is estimated to be 8 years.
Tochio, Daisuke; Nagasumi, Satoru; Inoi, Hiroyuki; Hamamoto, Shimpei; Ono, Masato; Kobayashi, Shoichi; Uesaka, Takahiro; Watanabe, Shuji; Saito, Kenji
JAEA-Technology 2021-014, 80 Pages, 2021/09
JAEA-Technology-2021-014.pdf:5.87MB
In response to the new regulatory standards established in response to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station in March 2011, measures and impact assessments related to internal flooding at HTTR were carried out. In assessing the impact, considering the characteristics of the high-temperature gas-cooled reactor, flooding due to assumed damage to piping and equipment, flooding due to water discharge from the system installed to prevent the spread of fire, and flooding due to damage to piping and equipment due to an earthquake. The effects of submersion, flooding, and flooding due to steam were evaluated for each of them. The impact of the overflow of liquids containing radioactive materials outside the radiation-controlled area was also evaluated. As a result, it was confirmed that flooding generated at HTTR does not affect the safety function of the reactor facility by taking measures.
SGo, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Aoi, Nori*; Azaiez, F.*; Furutaka, Kazuyoshi; Hatsukawa, Yuichi; Kimura, Atsushi; Kisamori, Keiichi*; Kobayashi, Motoki*; et al.
Physical Review C, 103(3), p.034327_1 - 034327_8, 2021/03
Times Cited Count：4 Percentile：46.48(Physics, Nuclear)
Sr and 
Cs in soils near the Fukushima Daiichi Nuclear Power StationSasaki, Takayuki*; Matoba, Daisuke*; Dohi, Terumi; Fujiwara, Kenso; Kobayashi, Taishi*; Iijima, Kazuki
Journal of Radioanalytical and Nuclear Chemistry, 326(1), p.303 - 314, 2020/10
Times Cited Count：9 Percentile：51.89(Chemistry, Analytical)
F from 
O
?Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.
Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05
Times Cited Count：18 Percentile：74.58(Physics, Multidisciplinary)The structure of a neutron-rich F nucleus is investigated by a quasifree (
) knockout reaction. The sum of spectroscopic factors of 
orbital is found to be 1.0 
0.3. The result shows that the O core of F nucleus significantly differs from a free O nucleus, and the core consists of 35% O
, and 65% excited O. The result shows that the O core of F nucleus significantly differs from a free O nucleus. The result may infer that the addition of the 
proton considerably changes the neutron structure in F from that in O, which could be a possible mechanism responsible for the oxygen dripline anomaly.
Kondo, Yasuhiro; Hirano, Koichiro; Ito, Takashi; Kikuzawa, Nobuhiro; Kitamura, Ryo; Morishita, Takatoshi; Oguri, Hidetomo; Okoshi, Kiyonori; Shinozaki, Shinichi; Shinto, Katsuhiro; et al.
Journal of Physics; Conference Series, 1350, p.012077_1 - 012077_7, 2019/12
Times Cited Count：2 Percentile：68.44(Physics, Particles & Fields)We have upgraded a 3-MeV linac at J-PARC. The ion source is same as the J-PARC linac's, and the old 30-mA RFQ is replaced by a spare 50-mA RFQ, therefore, the beam energy is 3 MeV and the nominal beam current is 50 mA. The main purpose of this system is to test the spare RFQ, but also used for testing of various components required in order to keep the stable operation of the J-PARC accelerator. The accelerator has been already commissioned, and measurement programs have been started. In this paper, present status of this 3-MeV linac is presented.
Nagai, Takayuki; Kobayashi, Hidekazu; Okamoto, Yoshihiro; Akiyama, Daisuke*; Sato, Nobuaki*; Uehara, Akihiro*; Fujii, Toshiyuki*; Sekimoto, Shun*
KURNS Progress Report 2018, P. 105, 2019/08
To understand this structural change of a borosilicate glass by a neutron irradiation in detail, the irradiation test was carried out in KUR in 2017FY. The glass structure was estimated by using Raman spectrometry in 2018FY. Comparing with the Raman spectra of glass samples before and after irradiation, it could be observed the change of peak height of Si-O bridging structure by the irradiation.
Tojo, Masayuki*; Kanazawa, Toru*; Nakashima, Kazuo*; Iwamoto, Tatsuya*; Kobayashi, Kensuke*; Goto, Daisuke*; Nemoto, Yoshiyuki; Kaji, Yoshiyuki
Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 13 Pages, 2019/05
In this study, fuel loading effects in BWR spent fuel rack accidents are widely investigated using three-dimensional analysis methods from both nuclear and thermal hydraulics viewpoints, including: (a) Decay heat of spent fuel after discharge, (b) The maximum temperature of spent fuel cladding in the spent fuel rack depending on heat transfer phenomena, and (c) Criticality of the spent fuel rack after collapsing of the fuel due to a severe accidents in the BWR spent fuel pool (SFP).
Nagai, Takayuki; Kobayashi, Hidekazu; Okamoto, Yoshihiro; Akiyama, Daisuke*; Sato, Nobuaki*
Photon Factory Activity Report 2017, 2 Pages, 2018/00
no abstracts in English
Mukai, Yasunobu; Nakamichi, Hideo; Kobayashi, Daisuke; Nishimura, Kazuaki; Fujisaku, Sakae; Tanaka, Hideki; Isomae, Hidemi; Nakamura, Hironobu; Kurita, Tsutomu; Iida, Masayoshi*; et al.
Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 8 Pages, 2017/04
TRP has stored the plutonium in solution state for long-term since the last PCDF operation in 2007 was finished. After the great east Japan earthquake in 2011, JAEA had investigated the risk against potential hazard of these solutions which might lead to make hydrogen explosion and/or boiling of the solution accidents with the release of radioactive materials to the public when blackout. To reduce the risk for storing Pu solution (about 640 kg Pu), JAEA planned to perform the process operation for the solidification and stabilization of the solution by converted into MOX powder at PCDF in 2013. In order to perform PCDF operation without adaption of new safety regulation, JAEA conducted several safety measures such as emergency safety countermeasures, necessary security and safeguards (3S) measures with understanding of NRA. As a result, the PCDF operation had stared on 28th April, 2014, and successfully completed to convert MOX powder on 3rd August, 2016 for about 2 years as planned.
As using high-resolution inelastic X-ray scatteringMurai, Naoki*; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.
Physical Review B, 93(2), p.020301_1 - 020301_5, 2016/01
Times Cited Count：7 Percentile：31.95(Materials Science, Multidisciplinary)SGo, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Kobayashi, Motoki*; Kisamori, Keiichi*; Takaki, Motonobu*; Miya, Hiroyuki*; Ota, Shinsuke*; Michimasa, Shinichiro*; Shimoura, Susumu*; et al.
JPS Conference Proceedings (Internet), 6, p.030005_1 - 030005_4, 2015/06
Ueda, Daisuke*; Shirai, Koji*; Funayama, Tomoo; Sakashita, Tetsuya; Yokota, Yuichiro; Kobayashi, Yasuhiko
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 84, 2015/03
In this study, we investigated the effects of irradiation to the silkworm eggs at various developmental stages. First, we tried the irradiation to the unfertilized eggs (at 1.5 hour after oviposition). At this stage, the female pronucleus and the sperm nucleus are observed in the eggs, but not fertilized. After irradiation, the irradiated eggs stopped the development after fertilization. About 2 hours after, the egg restarted the nuclear cleavage. This result indicates the DNA damage on pronuleus cannot prevent the fertilization. We also investigated the effects of irradiation to the egg at the nuclear cleavage stage (at 6 hour after oviposition). The egg also stopped the development after irradiation, but the duration time of the developmental arrest was almost two times longer (about 4 hours) than that of the egg irradiated at fertilization.
Tsutsumi, Tomoaki*; Adachi, Rika*; Takatsuki, Satoshi*; Nei, Daisuke*; Kameya, Hiromi*; Todoriki, Setsuko*; Kikuchi, Masahiro; Kobayashi, Yasuhiko; Matsuda, Rieko*; Teshima, Reiko*
Shokuhin Shosha, 49(1), p.9 - 15, 2014/12
no abstracts in English
