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CoSi山内 宏樹; Sari, D. P.*; 安井 幸夫*; 坂倉 輝俊*; 木村 宏之*; 中尾 朗子*; 大原 高志; 本田 孝志*; 樹神 克明; 井川 直樹; et al.
Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02
-Mn-type family alloys Mn
have three-dimensional antiferromagnetic (AFM) corner-shared triangular network. The antiferromagnet MnRhSi shows magnetic short-range order (SRO) over a wide temperature range of approximately 500 K above the N
el temperature 
= 190 K. MnCoSi has the smallest lattice parameter and the lowest in the family compounds. The quantum critical point (QCP) from AFM to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 
of MnCoSi is only 140 K, quantum critical behavior is observed in MnCoSi as the enhancement of the electronic specific heat coefficient 
. We study how the magnetic SRO appears in MnCoSi by using neutron scattering, 
SR, and physical property measurements. The experimental results show that the neutron scattering intensity of the magnetic SRO does not change much regardless of the suppressed magnetic moment in the long-range magnetic ordered state compared to those of MnRhSi. The initial asymmetry drop ratio of SR above becomes small, and the magnetic SRO temperature 
is suppressed to 240 K. The results suggest that the MnCoSi is close to the QCP in the Mn system.
飯田 一樹*; 樹神 克明; 稲村 泰弘; 中村 充孝; Chang, L.-J.*; 社本 真一
Scientific Reports (Internet), 12, p.20663_1 - 20663_7, 2022/12
被引用回数：2 パーセンタイル：20.84(Multidisciplinary Sciences)イルメナイトFeTiO
粉末サンプルのスピン励起を、飛行時間非弾性中性子散乱によって測定し、動的磁気ペア密度関数
を、動的磁気構造因子
からフーリエ変換によって初めて得ることに成功した。
RhSi樹神 克明; 本田 孝志*; 山内 宏樹; 社本 真一*; 池田 一貴*; 大友 季哉*
Journal of the Physical Society of Japan, 90(7), p.074710_1 - 074710_7, 2021/07
被引用回数：4 パーセンタイル：31.87(Physics, Multidisciplinary)Magnetic pair distribution function (mPDF) of intermetallic antiferromagnet MnRhSi is estimated from the powder neutron diffraction data. The mPDF exhibits negative peak at about 
= 2.7 
corresponding to the nearest neighbor Mn-Mn distance above the antiferromagnetic transition temperature 
. Below , the mPDF is a superposition of the mPDF with the negative peak at about = 2.7 and the mPDF calculated from the antiferromagnetic structure which is determined by the previous neutron diffraction study, indicating the coexistence of the short range ordering and the antiferromagnetic long range ordering. The mPDF of the short range ordering is not reproduced by the magnetic structure model with the symmetry consistent with that of the crystal structure. The possible magnetic structure which can reproduce the observed mPDF of the short range ordering is proposed.
FeTiO樹神 克明; 本田 孝志*; 池田 一貴*; 社本 真一; 大友 季哉*
JPS Conference Proceedings (Internet), 33, p.011059_1 - 011059_6, 2021/03
We have performed powder diffraction measurement on the typical spin-glass system MnFeTiO using the neutron total scattering spectrometer NOVA installed in J-PARC to apply the mPDF analysis to the short-range correlation in the spin-glass phase. The mPDF obtained from the magnetic scattering intensity can be reproduced by the linear combination of the mPDFs calculated from the antiferromagnetic structures of MnTiO and FeTiO, consistent with the coexistence of two different antiferromagnetic correlations in the spin-glass phase.
Se studied by inelastic neutron scattering石角 元志*; 樹神 克明; 梶本 亮一; 中村 充孝; 稲村 泰弘; 池内 和彦*; Ji, S.*; 新井 正敏*; 社本 真一
Condensed Matter (Internet), 4(3), p.69_1 - 69_10, 2019/09
中性子非弾性散乱により観測された磁気共鳴モードのQ依存性という初めての手法で、FeTeSeの超伝導対称性がs
波であることを実験的に示した。
iron-based superconductor LaFePO
石角 元志*; 社本 真一; 樹神 克明; 梶本 亮一; 中村 充孝; Hong, T.*; Mutka, H.*
Scientific Reports (Internet), 8, p.16343_1 - 16343_6, 2018/11
被引用回数：3 パーセンタイル：24.41(Multidisciplinary Sciences)磁気揺らぎはBCS理論に従わない非従来型超伝導で最も可能性のある機構として重要な役割を担うと考えられてきた。今回、これまで磁気ゆらぎが見つかっていない5Kという低い超伝導転移温度の鉄リン系超伝導体LaFePOで、30-50meVの高エネルギーで磁気ゆらぎを見つけた。これはこれまで考えられてきた高エネルギー磁気揺らぎで、高い超伝導転移温度になるという考えとは矛盾することから、超伝導機構の理解に向けて重要な発見である。
社本 真一; 伊藤 孝; 大西 弘明; 山内 宏樹; 稲村 泰弘; 松浦 直人*; 赤津 光洋*; 樹神 克明; 中尾 朗子*; 茂吉 武人*; et al.
Physical Review B, 97(5), p.054429_1 - 054429_9, 2018/02
被引用回数：30 パーセンタイル：70.79(Materials Science, Multidisciplinary)イットリウム鉄ガーネットの核および磁気構造と全マグノン分散を中性子散乱により調べた。低エネルギーの分散は強磁性マグノンで期待されるように14meVまで2次関数の分散を示した。
積分した動的磁化率
"(
)の虚部は低エネルギーで平方根のエネルギー依存性を示した。"()から絶対値でマグノン状態密度を求めた。その値は理論的に予想されるマグノン分散でひとつのカラリティーモードに対応する。
樹神 克明; 池田 一貴*; 社本 真一; 大友 季哉*
Journal of the Physical Society of Japan, 86(12), p.124708_1 - 124708_8, 2017/12
被引用回数：11 パーセンタイル：56.28(Physics, Multidisciplinary)We derive an alternative equation of magnetic pair distribution function (mPDF) related to the mPDF equation given in a preceding study (B. A. Frandsen, X. Yang, and S. J. L. Billinge, Acta Crystallogr. A, 
, 3 (2014)) for quantitative analysis of realistic experimental data. The additional term related to spontaneous magnetization included in the equation is particularly important for the mPDF analysis of ferromagnetic materials. Quantitative estimation of mPDF from neutron diffraction data is also shown. The experimental mPDFs estimated from the neutron diffraction data of the ferromagnet MnSb and the antiferromagnet MnF
are quantitatively consistent with the mPDFs calculated using the presented equation.
樹神 克明; 池田 一貴*; 礒部 正彦*; 武田 晃*; 伊藤 正行*; 上田 寛*; 社本 真一; 大友 季哉*
Journal of the Physical Society of Japan, 85(9), p.094709_1 - 094709_5, 2016/09
被引用回数：4 パーセンタイル：30.64(Physics, Multidisciplinary)We have performed powder neutron diffraction on the half-metallic ferromagnet CrO which has a rutile-type crystal structure with a tetragonal unit cell. Although the powder diffraction pattern can be fitted by the reported crystal structure including a single Cr site, the atomic pair distribution function (PDF) can be fitted by the structural model with an orthorhombic unit cell including two kinds of inequivalent Cr sites. The difference between the valences of the two inequivalent Cr sites, 
of Cr
, estimated from the local structural parameters is about 0.06. The shapes of the two CrO
octahedra are slightly different, suggesting the short-range orbital ordering of the Cr 3
orbitals. The lattice distortion and the improvement of the fitting to the PDF obtained using the locally distorted structure model are apparent in the region below about 10 , suggesting that the domain size or correlation length of the locally distorted structure is about 10 , roughly corresponding to the size of two unit cells.
樹神 克明; 井川 直樹; 社本 真一; 池田 一貴*; 大下 英敏*; 金子 直勝*; 大友 季哉*; 鈴谷 賢太郎; 星川 晃範*; 石垣 徹*
JPS Conference Proceedings (Internet), 8, p.034002_1 - 034002_6, 2015/09
Cubic spinel compound LiMnO
with the mixed valence of Mn
has non-metallic conductivity. The local structure determined by the PDF analysis has an orthorhombic lattice distortion and includes inequivalent Mn
and Mn
sites. YBaCoO
also exhibits non-metallic conductivity although the Co has the mixed valence of +2.5 above 220 K which corresponds with charge ordering temperature. The PDF obtained at 450 K is not reproduced by the PDF calculated for the averaged structure and can be reproduced by the PDF calculated for the structure model corresponding to the charge ordering state. These results suggest that the valence electrons are localized with short-range periodicity, resulting in the non-metallic conductivities in these materials.
As樹神 克明; 石角 元志*; 脇本 秀一; 木方 邦宏*; Lee, C.-H.*; 伊豫 彰*; 永崎 洋*; 社本 真一
Physical Review B, 90(14), p.144510_1 - 144510_5, 2014/10
被引用回数：1 パーセンタイル：4.13(Materials Science, Multidisciplinary)We have performed neutron diffraction measurements at 12K on a single crystal of BaFeAs, which serves as the parent compound of iron-based superconductor. To investigate the in-plane anisotropy of the magnetic form factor in the antiferromagnetic phase, the single crystal was detwinned. The magnetic structure factor and magnetic form factor are well explained by the spin densities comprising 
electrons with a fraction of approximately 40% and electrons in the other four 
orbitals each with a fraction of approximately 15%. It is a direct observation of the largely anisotropic spin density relative to the small orthorhombic lattice distortion, 
0.3%.
IrSiPyon, S.*; 工藤 一貴*; 松村 純一*; 石井 博文*; 松尾 元太*; 野原 実*; 北條 元*; 岡 研吾*; 東 正樹*; Garlea, V. O.*; et al.
Journal of the Physical Society of Japan, 83(9), p.093706_1 - 093706_5, 2014/09
被引用回数：36 パーセンタイル：81.48(Physics, Multidisciplinary)The effects of lithium absorption on the crystal structure and electronic properties of IrSi, a binary silicide with a noncentrosymmetric crystal structure, were studied. X-ray and neutron diffraction experiments revealed that hexagonal IrSi (space group 
) transforms into trigonal LiIrSi (space group 
) upon lithium absorption. The structure of LiIrSi is found to consist of a planar kagome network of silicon atoms with Li and Ir spaced at unequal distances between the kagome layers, resulting in a polar structure along the c-axis. LiIrSi exhibited type-II superconductivity with a transition temperature 
of 3.8 K, displaying a structure type that no previous superconductors have been reported to have.
O樹神 克明; 井川 直樹; 社本 真一; 池田 一貴*; 大下 英敏*; 金子 直勝*; 大友 季哉*; 鈴谷 賢太郎; 星川 晃範*; 石垣 徹*
JPS Conference Proceedings (Internet), 3, p.013012_1 - 013012_6, 2014/06
LiMnO has a cubic spinel structure with a single Mn site whose valence is +3.5. Below about 260 K, the compound exhibits a charge ordering and has inequivalent Mn sites with valences of +3 and +4. However, even in the cubic phase without the charge ordering, temperature dependence of the electrical conductivity is non-metallic. We have performed PDF (atomic pair distribution function) analysis on powder neutron diffraction data of LiMnO obtained above 300 K where the compound has cubic structure. The local structure determined by PDF analysis has an orthorhombic lattice distortion and includes the inequivalent Mn sites with valences of +3 and +4 up to, at least, about 450 K. These results indicate that valence electrons are localized at Mn sites with short range periodicity, resulting in the non-metallic electrical conductivity. It can be regarded as a glass state of valence electrons whereas a charge ordering can be regarded as a crystallization of valence electrons.
Zhidkov, A.*; 益田 伸一*; Bulanov, S. S.*; Koga, J. K.; 細貝 知直*; 兒玉 了祐*
Physical Review Special Topics; Accelerators and Beams, 17(5), p.054001_1 - 054001_7, 2014/05
被引用回数：12 パーセンタイル：58.46(Physics, Nuclear)Nonlinear cascade scattering of intense tightly focused laser pulses by relativistic electrons is studied numerically including the classical radiation damping. The electron energy loss, along with its side scattering by the ponderomotive force makes the scattering in the vicinity of high laser field nearly impossible at high electron energies. The use of a second co-propagating laser pulse as a booster is shown to solve this problem.
社本 真一; 樹神 克明; 伊巻 正*; 中谷 健; 大下 英敏*; 金子 直勝*; 増子 献児*; 坂本 健作; 山口 憲司; 鈴谷 賢太郎; et al.
JPS Conference Proceedings (Internet), 1, p.014011_1 - 014011_5, 2014/03
アンモナイト化石の2次元回折イメージングをJ-PARCにおける高強度全散乱装置NOVAで行った。観測された回折プロファイルはカルサイト,シデライトとアモルファス構造からなっていることがわかった。
Park, S.-W.*; 溝口 拓*; 樹神 克明; 社本 真一; 大友 季哉*; 松石 聡*; 神谷 利夫*; 細野 秀雄*
Inorganic Chemistry, 52(23), p.13363 - 13368, 2013/12
被引用回数：36 パーセンタイル：82.97(Chemistry, Inorganic & Nuclear)We report the synthesis, structure, and electromagnetic properties of Cr-based layered oxyarsenides LnCrAsO (Ln = La, Ce, Pr, and Nd) with a ZrCuSiAs-type structure. All LnCrAsO samples showed metallic electronic conduction. Electron doping in LaCrAsO by Mnsubstitution for the Cr sites gave rise to a metal-insulator transition. Analysis of powder neutron diffraction data revealed that LaCrAsO had Gtype antiferromagnetic (AFM) ordering, i.e., a checkerboard-type AFM ordering in the CrAs plane and antiparallel spin coupling between the adjacent CrAs planes, at 300 K with a large spin moment of 1.57 
along the c axis. The magnetic susceptibility of LaCrAsO was very small (on the order of 10
emu/mol) and showed a broad hump at 550 K. First-principles density functional theory calculations of LaCrAsO explained its crystal structure and metallic nature well, but could not replicate the antiparallel spin coupling between the CrAs layers. The electronic structure of LaCrAsO is discussed with regard to those of related compounds LaFeAsO and LaMnAsO.
O樹神 克明; 井川 直樹; 社本 真一; 池田 一貴*; 大下 英敏*; 金子 直勝*; 大友 季哉*; 鈴谷 賢太郎
Journal of the Physical Society of Japan, 82(9), p.094601_1 - 094601_6, 2013/09
被引用回数：11 パーセンタイル：55.24(Physics, Multidisciplinary)We have performed powder neutron diffraction on 
LiMnO at 300 K. The crystal structure determined by Rietveld analysis is a cubic spinel with space group of 
in which all Mn atoms are crystallograghically equivalent, consistent with many preceding studies. However, the atomic pair distribution function (PDF) of this compound cannot be fitted by the cubic structure satisfactorily, and it can be reproduced by the orthorhombic structure with 
. It corresponds with the structure of charge ordered phase below about 260 K, indicating a short range charge ordering. In the local structure determined by PDF analysis, two types of MnO octahedra with long and short atomic distances between Mn and O atoms exist and their Mn-O distances are almost consistent with the distances in the charge ordered phase. From these results, valence electrons are localized at Mn sites like a glass even in the cubic phase, resulting in the non-metallic electrical conductivity.
半那 拓*; 松石 聡*; 樹神 克明; 大友 季哉*; 社本 真一; 細野 秀雄*
Physical Review B, 87(2), p.020401_1 - 020401_5, 2013/01
被引用回数：37 パーセンタイル：77.41(Materials Science, Multidisciplinary)Manganese oxyarsenide hydrides LaMnAsO
H
(
= 0-0.73) were synthesized by a solid state reaction under a high pressure of 2 GPa. The hydride ions H
in O
sites induced an insulator-to-metal conversion and suppressed the antiferromagnetic ordering of Mn spins. Instead, ferromagnetism with negative magnetoresistance was observed. The Curie temperature and saturated moment per Mn increased with up to 264 K and 1.5 , respectively, at = 0.73. These results indicate that H donate conduction electrons to the MnAs layer, mediating a direct ferromagnetic interaction between Mn atoms.
水田 好雄*; 細貝 知直*; 益田 伸一*; Zhidkov, A.*; 牧戸 啓悟*; 中新 信彦*; 梶野 祥平*; 西田 明憲*; 神門 正城; 森 道昭; et al.
Physical Review Special Topics; Accelerators and Beams, 15(12), p.121301_1 - 121301_10, 2012/12
被引用回数：21 パーセンタイル：69.15(Physics, Nuclear)Laser wakefield acceleration is capable of generating electron bunches with high quality: quasi-monoenergetic, low in emittance, and a very short duration of the order of ten femto-seconds. Such femtosecond bunches can be used to measure ultrafast phenomena. We conducted experiments for controllable electron bunch generation. Short-lived, 10 ps, deep plasma channels, with their lengths of 1 mm and diameters of 20 m, are observed and characterized in Ar gas jets irradiated by moderate intensity, 10
W/cm
, laser pulses with a duration from subpicosecond to several picoseconds. The channels, upon 2D particle-in-cell simulations including ionization, fit well in the guiding of high intensity femtosecond laser pulses and, therefore, in laser wakefield acceleration with a controllable electron self-injection.
社本 真一; 樹神 克明
JAEA-Review 2012-029, 264 Pages, 2012/08
JAEA-Review-2012-029.pdf:50.76MB
物質・材料研究機構,理化学研究所及び日本原子力研究開発機構の三機関での「超伝導と磁性とフォノン」に関する特徴的な技術,装置,優れた研究やこれまでの三機関での共同研究結果等について、今後の方向性を含めて、講演及び議論した。本報告書は本研究会の講演要旨及び講演で使用された発表資料を収録したものである。
