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JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2024)

Niwa, Masakazu; Shimada, Akiomi; Asamori, Koichi; Sueoka, Shigeru; Komatsu, Tetsuya; Nakajima, Toru; Ogata, Manabu; Uchida, Mao; Nishiyama, Nariaki; Tanaka, Kiriha; et al.

JAEA-Review 2024-035, 29 Pages, 2024/09

JAEA-Review-2024-035.pdf:1.24MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2024. The objectives and contents of this research are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:49 Percentile:96.63(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Experimental study of Di-quark correlation by charmed baryon spectroscopy at J-PARC high-momentum secondary beam line

Komatsu, Yusuke*; Ichikawa, Yudai; Naruki, Megumi*; Tanida, Kiyoshi; 24 of others*

JPS Conference Proceedings (Internet), 26, p.022029_1 - 022029_4, 2019/11

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:282 Percentile:99.70(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Pressure-induced stacking disorder in boehmite

Ishii, Yusuke*; Komatsu, Kazuki*; Nakano, Satoshi*; Machida, Shinichi*; Hattori, Takanori; Sano, Asami; Kagi, Hiroyuki*

Physical Chemistry Chemical Physics, 20(24), p.16650 - 16656, 2018/06

 Times Cited Count:5 Percentile:21.14(Chemistry, Physical)

The structure of an aluminum layered hydroxide, boehmite ($$gamma$$-AlOOH), as a function of pressure was studied by using ${it in situ}$ synchrotron X-ray and neutron diffraction. Peak broadening and subsequent splitting, which are only found for hkl (h $$neq$$ 0) peaks in the X-ray diffraction patterns above 25 GPa, are explained by stacking disorder accompanied with a continuously increasing displacement of the AlO$$_{6}$$ octahedral layer along a-axis. This finding could be the first experimental result for the pressure-induced stacking disorder driven by the continuous layer displacement. The magnitude of the layer displacement was estimated from the X-ray scattering profile calculation based on the stacking disordered structure model. Hydrogen bond geometries of boehmite, obtained by structure refinements on the observed neutron diffraction patterns for deuterated sample up to 10 GPa, show linearly approaching O-D covalent and D$$cdots$$O hydrogen bond distances and they could merge below 26 GPa. The pressure-induced stacking disorder would make the electrostatic potential of hydrogen bonds asymmetric, yielding less chance for the proton-tunnelling.

Journal Articles

An Evaluation method of reflectance spectra to be obtained by Hayabusa2 Near-Infrared Spectrometer (NIRS3) based on laboratory measurements of carbonaceous chondrites

Matsuoka, Moe*; Nakamura, Tomoki*; Osawa, Takahito; Iwata, Takahiro*; Kitazato, Kohei*; Abe, Masanao*; Nakauchi, Yusuke*; Arai, Takehiko*; Komatsu, Mutsumi*; Hiroi, Takahiro*; et al.

Earth, Planets and Space (Internet), 69(1), p.120_1 - 120_12, 2017/12

AA2017-0327.pdf:1.53MB

 Times Cited Count:6 Percentile:20.07(Geosciences, Multidisciplinary)

We have conducted ground-based performance evaluation tests of the Near-Infrared Spectrometer (NIRS3) onboard Hayabusa2 spacecraft and established a method for evaluating its measured reflectance spectra. Reflectance spectra of nine powdered carbonaceous chondrite samples were measured by both NIRS3 and a FT-IR spectrometer. Since raw data obtained by NIRS3 had considerable spectral distortion caused by systematic offsets in sensitivity of individual pixels, we have established two methods for correcting the NIRS3 data by comparing them with the corresponding FT-IR data. In order to characterize the absorption bands in NIRS3 spectra, the depth of each band component D$$lambda$$ is defined for each wavelength $$lambda$$ ($$mu$$m). Reflectance spectra of asteroid Ryugu, the target asteroid of Hayabusa2, to be recorded by the NIRS3 are expected to reveal the characteristics of the surface materials by using the evaluation technique.

Journal Articles

NIRS3; The Near Infrared Spectrometer on Hayabusa2

Iwata, Takahiro*; Kitazato, Kohei*; Abe, Masanao*; Otake, Makiko*; Arai, Takehiko*; Arai, Tomoko*; Hirata, Naru*; Hiroi, Takahiro*; Honda, Chikatoshi*; Imae, Naoya*; et al.

Space Science Reviews, 208(1-4), p.317 - 337, 2017/07

 Times Cited Count:54 Percentile:69.65(Astronomy & Astrophysics)

NIRS3: The Near Infrared Spectrometer is installed on the Hayabusa2 spacecraft to observe the target C-type asteroid 162173 Ryugu at near infrared wavelengths of 1.8 to 3.2 micrometer. It aims to obtain reflectance spectra in order to detect absorption bands of hydrated and hydroxide minerals in the 3 micrometer-band. We adopted a linear-image sensor with indium arsenide (InAs) photo diodes and a cooling system with a passive radiator to achieve an optics temperature of 188 K, which enables to retaining sufficient sensitivity and noise level in the 3 micrometer wavelength region. We conducted ground performance tests for the NIRS3 flight model (FM) to confirm its baseline specifications. The results imply that the properties such as the signal-to-noise ratio (SNR) conform to scientific requirements to determine the degree of aqueous alteration, such as CM or CI chondrite, and the stage of thermal metamorphism on the asteroid surface.

Journal Articles

Design and performance of high-pressure PLANET beamline at pulsed neutron source at J-PARC

Hattori, Takanori; Sano, Asami; Arima, Hiroshi*; Komatsu, Kazuki*; Yamada, Akihiro*; Inamura, Yasuhiro; Nakatani, Takeshi; Seto, Yusuke*; Nagai, Takaya*; Utsumi, Wataru; et al.

Nuclear Instruments and Methods in Physics Research A, 780, p.55 - 67, 2015/04

 Times Cited Count:82 Percentile:99.02(Instruments & Instrumentation)

PLANET is a time-of-flight (ToF) neutron beamline dedicated to high-pressure and high-temperature experiments. The large six-axis multi-anvil high-pressure press designed for ToF neutron diffraction experiments enables routine data collection at high pressures and high temperatures up to 10 GPa and 2000 K, respectively. To obtain clean data, the beamline is equipped with the incident slits and receiving collimators to eliminate parasitic scattering from the high-pressure cell assembly. The high performance of the diffractometer for the resolution ($$Delta$$ $$d$$/$$d$$ $$sim$$ 0.6%) and the accessible $$d$$-spacing range (0.2-8.4 ${AA}$) together with low-parasitic scattering characteristics enables precise structure determination of crystals and liquids under high pressure and temperature conditions.

Journal Articles

Stoichiometric study of the dielectric and magnetic properties in charge frustrated system LuFe$$_{2}$$O$$_{4}$$

Michiuchi, Takamasa*; Yokota, Yusuke*; Komatsu, Takuma*; Hayakawa, Hironori*; Kuroda, Tomoko*; Maeda, Daisuke*; Matsuo, Yoji*; Mori, Shigeo*; Yoshii, Kenji; Hanasaki, Noriaki*; et al.

Ferroelectrics, 378(1), p.175 - 180, 2009/00

 Times Cited Count:18 Percentile:58.73(Materials Science, Multidisciplinary)

We have synthesized the samples of LuFe$$_{2}$$O$$_{4}$$, which shows the ferroelectricity due to charge ordering of Fe ions, under several different reducing conditions using a CO$$_{2}$$-CO flow. The reducing condition was changed by changing a flow ratio of CO$$_{2}$$ and CO. It was found that the flow ratio of CO$$_{2}$$/CO of about 5 provided the sample with the highest magnetic transition temperature of 240-250 K. This sample showed the dielectric constant of 10000 at room temperature. The imaginary part of the dielectric response offered the activation energy of 0.4-0.5 eV, which is slightly larger than that reported previously (about 0.3 eV). We will perform further investigation of the physical properties of this sample to clarify full details and their origin of LuFe$$_{2}$$O$$_{4}$$.

Journal Articles

Magnetic and dielectric properties of HoFe$$_{2}$$O$$_{4}$$ and R$$_{1-x}$$R'$$_{x}$$Fe$$_{2}$$O$$_{4}$$ (R, R': rare earths)

Yoshii, Kenji; Yoneda, Yasuhiro; Maeda, Daisuke*; Yokota, Yusuke*; Michiuchi, Takamasa*; Komatsu, Takuma*; Ikeda, Naoshi*; Matsuo, Yoji*; Mori, Shigeo*

Japanese Journal of Applied Physics, 47(9), p.7599 - 7602, 2008/09

 Times Cited Count:8 Percentile:32.87(Physics, Applied)

We have investigated the physical properties of HoFe$$_{2}$$O$$_{4}$$ and R$$_{1-x}$$R'$$_{x}$$Fe$$_{2}$$O$$_{4}$$ (R, R': rare earths). Dielectric measurements showed their dielectric constants of 1000 at around room temperature, which is characteristic of the RFe$$_{2}$$O$$_{4}$$ series (R: rare earths). However, the magnetic transition temperatures and the coherency in dielectric response were found to be different from those of RFe$$_{2}$$O$$_{4}$$ reported so far. Interestingly, these materials suggested higher ferroelectric temperatures than those reported so far, suggesting a possibility of application of these materials.

Oral presentation

Remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris; Prototype experiments

Matsuhira, Nobuto*; Komatsu, Ren*; Nakashima, Shinsuke*; Yamashita, Atsushi*; Fukui, Rui*; Takahashi, Hiroyuki*; Shimazoe, Kenji*; Woo, H.*; Tamura, Yusuke*; Takashi, Takayuki*; et al.

no journal, , 

This research aims to develop human resources in the field of remote technology for the decommissioning of the Fukushima Daiichi Nuclear Power Plant. We conduct research on a monitoring platform for fuel debris removal. Here, the developments on prototype experiments were described. We expect to develop research personnel through participation in projects, lectures, and facility tours.

Oral presentation

Dating marine terraces by terrestrial cosmogenic nuclides; Applicability and limitations

Matsushi, Yuki*; Komatsu, Tetsuya; Sueoka, Shigeru; Yonaga, Yusuke; Ogawa, Yumi*; Fujita, Natsuko; Kokubu, Yoko

no journal, , 

no abstracts in English

Oral presentation

Dating of marine erosional terraces using cosmogenic nuclides; A Case study of the Hyuga City, Miyazaki Prefecture, southwest Japan (preliminary results)

Sueoka, Shigeru; Komatsu, Tetsuya; Matsushi, Yuki*; Yonaga, Yusuke; Sano, Naomi; Hirao, Noriaki*; Ueki, Tadamasa; Fujita, Natsuko; Kokubu, Yoko; Niwa, Masakazu

no journal, , 

no abstracts in English

Oral presentation

Spectral characteristics of asteroid (162173) Ryugu with Hayabusa2 NIRS3

Takir, D.*; Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; et al.

no journal, , 

JAXA spacecraft and sample return mission Hayabusa2 has arrived at the near-Earth asteroid 162173 Ryugu, which is classified a primitive carbonaceous object. Here we report recent results of near-infrared spectrometer (NIRS3) on the Hayabusa2 spacecraft. The observations provide direct measurements of the surface composition of Ryugu and context for the returned samples. NIRS3 has detected a weak and narrow absorption feature centered at 2.72 micrometer across entire observed surface. This absorption feature is attributed to the presence of OH-bearing minerals. The NIRS3 observations also revealed that Ryugu is the darkest object to be observed up-close by a visiting spacecraft. The intensity of the OH feature and low albedo are consistent with thermally-and/or shock-metamorphosed, and/or carbon-rich space-weathered primitive and hydrated carbonaceous chondrites.

Oral presentation

Environmental changes in the center of the Kanto plane around the Sashima and Takaragi uplands based on diatom analysis

Noguchi, Marie*; Miyamoto, Tatsuki*; Sugai, Toshihiko*; Nakanishi, Toshimichi*; Komatsu, Tetsuya; Suginaka, Yusuke*; Endo, Kunihiko*

no journal, , 

Discussions on the history of crustal development based on sedimentary facies analysis using the boring cores GC-NG-1, GC-OY-1, and GC-OY-2 in the central Kanto Plain, from the Sarushima Plateau to the Takaragi Plateau, are underway. In the study, paleoenvironmental restoration based on diatom analysis was performed. These core samples are likely to preserve sea-level changes and landing processes since MIS9. From the results of the diatom community analysis, the paleoenvironment in each core was found to change according to the boring site, such as inner bay, brackish water to freshwater, freshwater, lakes, river environment, and land environment. We also attempted to objectively present changes in community composition by cluster analysis of diatom analysis results.

Oral presentation

Remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris

Matsuhira, Nobuto*; Komatsu, Ren*; Nakashima, Shinsuke*; Yamashita, Atsushi*; Fukui, Rui*; Takahashi, Hiroyuki*; Shimazoe, Kenji*; Woo, H.*; Tamura, Yusuke*; Takashi, Takayuki*; et al.

no journal, , 

Oral presentation

Remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris; Integrated experiments

Matsuhira, Nobuto*; Komatsu, Ren*; Nakashima, Shinsuke*; Yamashita, Atsushi*; Fukui, Rui*; Takahashi, Hiroyuki*; Shimazoe, Kenji*; Woo, H.*; Tamura, Yusuke*; Takashi, Takayuki*; et al.

no journal, , 

17 (Records 1-17 displayed on this page)
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