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; Bandgap narrowing, metallization, and remarkable enhancement of photoelectric activityFang, Y.*; Kong, L.*; Wang, R.*; Zhang, Z.*; Li, Z.*; Wu, Y.*; Bu, K.*; Liu, X.*; Yan, S.*; Hattori, Takanori; et al.
Materials Today Physics (Internet), 34, p.101083_1 - 101083_7, 2023/05
Times Cited Count：1 Percentile：0(Materials Science, Multidisciplinary)The layered van der Waals halides are particularly sensitive to external pressure, suggesting a feasible route to pinpoint their structure with extraordinary behavior. However, a very sensitive pressure response usually lead to a detrimental phase transition and/or lattice distortion, making the approach of materials manipulation in a continuous manner remain challenging. Here, the extremely weak interlayer coupling and high tunability of layered RhI crystals are observed. A pressure-driven phase transition occurs at a moderate pressure of 5 GPa, interlinking to a change of layer stack mode. Strikingly, such a phase transition does not affect the tendency of quasi-linear bandgap narrowing, and a metallization with an ultra-broad tunability of 1.3 eV redshift is observed at higher pressures. Moreover, the carrier concentration increases by 4 orders of magnitude at 30 GPa, and the photocurrent enhances by 5 orders of magnitude at 7.8 GPa. These findings create new opportunities for exploring, tuning, and understanding the van der Waals halides by harnessing their unusual feature of a layered structure, which is promising for future devices based on materials-by-design that are atomically thin.
Kong, L.*; Gong, J.*; Hu, Q.*; Capitani, F.*; Celeste, A.*; Hattori, Takanori; Sano, Asami; Li, N.*; Yang, W.*; Liu, G.*; et al.
Advanced Functional Materials, 31(9), p.2009131_1 - 2009131_12, 2021/02
Times Cited Count：22 Percentile：80.38(Chemistry, Multidisciplinary)The soft nature of organic-inorganic halide perovskites renders their lattice particularly tunable to external stimuli such as pressure, undoubtedly offering an effective way to modify their structure for extraordinary optoelectronic properties. However, these soft materials meanwhile feature a general characteristic that even a very mild pressure will lead to detrimental lattice distortion and weaken the critical light-matter interaction, thereby triggering the performance degradation. Here, using the methylammonium lead iodide as a representative exploratory platform, we observed the pressure-driven lattice disorder can be significantly suppressed via hydrogen isotope effect, which is crucial for better optical and mechanical properties previously unattainable.
Yang, H. L.*; Kim, Y. S.*; Park, Y. M.*; Bae, Y. S.*; Kim, H. K.*; Kim, K. M.*; Lee, K. S.*; Kim, H. T.*; Bang, E. N.*; Joung, M.*; et al.
Proceedings of 23rd IAEA Fusion Energy Conference (FEC 2010) (CD-ROM), 8 Pages, 2011/03
Because the 2010 operation of Korea Superconducting Tokamak Advanced Research (KSTAR) mainly aims to achieve strongly elongated and diverted plasma, all the necessary hardware systems to provide an essential circumstance for the plasma shaping were newly installed and upgraded in 2010. In this paper, general configuration of the upgraded systems described earlier will be outlined. Moreover, several key performances and test results of the systems will be also reported in summary.
Ostermeyer, M.*; Kong, H.-J.*; Kovalev, V. I.*; Harrison, R. G.*; Fotiadi, A. A.*; M
gret, P.*; Kalal, M.*; Slezak, O.*; Yoon, J. W.*; Shin, J. S.*; et al.
Laser and Particle Beams, 26(3), p.297 - 362, 2008/09
Times Cited Count：41 Percentile：55.6(Physics, Applied)