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論文

On the adsorption and reactivity of element 114, flerovium

Yakushev, A.*; Lens, L.*; D$"u$llmann, Ch. E.*; Khuyagbaatar, J.*; J$"a$ger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; 浅井 雅人; Block, M.*; et al.

Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08

https://doi.org/10.3389/fchem.2022.976635
 被引用回数：9 パーセンタイル：79.28(Chemistry, Multidisciplinary)

114番元素フレロビウム(Fl)は現在その化学的性質が研究されている最も重い元素である。Flに関する最初の化学実験では、Flは貴ガス的な性質を持つ元素であると報告された。一方、2番目の研究では、Flは揮発性金属の性質を示すと報告された。より信頼性の高い結論を得るため、我々は更なる実験的研究を行い、二酸化ケイ素と金表面におけるFlの吸着挙動を調べた。その結果、Flは揮発性金属の水銀よりも高い揮発性と低い反応性を示し、一方、貴ガスのラドンよりは反応性が高いことを明らかにした。

論文

Competition between allowed and first-forbidden $$beta$$ decays of $$^{208}$$At and expansion of the $$^{208}$$Po level scheme

Brunet, M.*; Podoly$'a$k, Zs.*; Berry, T. A.*; Brown, B. A.*; Carroll, R. J.*; Lica, R.*; Sotty, Ch.*; Andreyev, A. N.; Borge, M. J. G.*; Cubiss, J. G.*; et al.

Physical Review C, 103(5), p.054327_1 - 054327_13, 2021/05

https://doi.org/10.1103/PhysRevC.103.054327
 被引用回数：4 パーセンタイル：57.13(Physics, Nuclear)

The structure of $$^{208}$$Po populated through the EC/$$beta^{+}$$ decay of $$^{208}$$At is investigated using $$gamma$$-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed $$gamma$$ rays which have been (re)assigned a position. Through the analysis using the shell model calculations approximately half of the $$beta$$-decay strength of $$^{208}$$At is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations.

論文

Identification of a 6.6$$mu$$s isomeric state in $$^{175}$$Ir

Gillespie, S. A.*; Andreyev, A. N.; Al Monthery, M.*; Barton, C. J.*; Antalic, S.*; Auranen, K.*; Badran, H.*; Cox, D.*; Cubiss, J. G.*; O'Donnell, D.*; et al.

Physical Review C, 99(6), p.064310_1 - 064310_6, 2019/06

https://doi.org/10.1103/PhysRevC.99.064310
 被引用回数：3 パーセンタイル：32.64(Physics, Nuclear)

An experiment has been performed to study excited states in the neutron-deficient nucleus $$^{175}$$Ir via the use of the JUROGAM II high-purity germanium detector array and the RITU gas-filled separator at JYFL, Jyv$"a$skyl$"a$. By using isomer tagging, an isomeric state with a half-life of 6.58(15) $$mu$$s has been observed in $$^{175}$$Ir for the first time. It has been established that the isomer decays via a 45.2 ($$E1$$) - 26.1 ($$M1$$) keV cascade to new states below the previously reported ground state in $$^{175}$$Ir with $$I^{pi} = (5/2^{-})$$. We now reassign this $$(5/2^{-})$$ state to the isomeric state discovered in this study.

論文

Investigation of the $$Delta$$$$n$$ = 0 selection rule in Gamow-Teller transitions; The $$beta$$-decay of $$^{207}$$Hg

Berry, T. A.*; Podoly$'a$k, Zs.*; Carroll, R. J.*; Lic$u{a}$, R.*; Grawe, H.*; Timofeyuk, N. K.*; Alexander, T.*; Andreyev, A. N.; Ansari, S.*; Borge, M. J. G.*; et al.

Physics Letters B, 793, p.271 - 275, 2019/06

https://doi.org/10.1016/j.physletb.2019.04.039
 被引用回数：5 パーセンタイル：47.88(Astronomy & Astrophysics)

Gamow-Teller $$beta$$ decay is forbidden if the number of nodes in the radial wave functions of the initial and final states is different. This $$Delta$$$$n$$ = 0 requirement plays a major role in the $$beta$$ decay of heavy neutron-rich nuclei, affecting the nucleosynthesis through the increased half-lives of nuclei on the astrophysical $$r$$-process pathway below both $$Z$$ = 50 (for $$N >$$ 82) and $$Z$$ = 82 (for $$N >$$ 126). The level of forbiddenness of the $$Delta$$$$n$$ = 1 $$nu$$1$$g_{9/2} rightarrow pi$$0$$g_{7/2}$$ transition has been investigated from the $$beta^{-}$$ decay of the ground state of $$^{207}$$Hg into the single-proton-hole nucleus $$^{207}$$Tl in an experiment at the ISOLDE Decay Station. From statistical observational limits on possible $$gamma$$-ray transitions depopulating the $$pi$$0$$g^{-1}_{7/2}$$ state in $$^{207}$$Tl, an upper limit of 3.9$$times$$10$$^{-3}$$ % was obtained for the probability of this decay, corresponding to log$$ft >$$ 8.8 within a 95% confidence limit. This is the most stringent test of the $$Delta$$$$n$$ = 0 selection rule to date.

論文

Shape coexistence in $$^{178}$$Hg

M$"u$ller-Gatermann, C.*; Dewald, A.*; Fransen, C.*; Auranen, K.*; Badran, H.*; Beckers, M.*; Blazhev, A.*; Braunroth, T.*; Cullen, D. M.*; Fruet, G.*; et al.

Physical Review C, 99(5), p.054325_1 - 054325_7, 2019/05

https://doi.org/10.1103/PhysRevC.99.054325
 被引用回数：8 パーセンタイル：64.15(Physics, Nuclear)

陽子過剰核$$^{178}$$Hgにおける変形共存を調べることを目的として、ユヴァスキュラ大学の加速器において$$^{103}$$Rh($$^{78}$$Kr, $$p2n$$)反応によって$$^{178}$$Hgを生成し、その原子核の励起状態からの脱励起の寿命を測定した。実験データを理論計算と比較した結果、$$^{178}$$Hgでは$$^{180}$$Hgに比べ、プロレート変形した状態がより高い励起状態へとシフトするとともに、変形度が増大することがわかった。

論文

Online chemical adsorption studies of Hg, Tl, and Pb on SiO$$_{2}$$ and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCA

Lens, L.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; 浅井 雅人; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.

Radiochimica Acta, 106(12), p.949 - 962, 2018/12

AA2018-0417.pdf:0.99MB

https://doi.org/10.1515/ract-2017-2914
 被引用回数：8 パーセンタイル：62.99(Chemistry, Inorganic & Nuclear)

半減期4$$sim$$49秒の短寿命同位体を用いて、水銀(Hg), タリウム(Tl), 鉛(Pb)の単一原子レベルでのSiO$$_{2}$$及びAu表面への固体吸着挙動をオンライン気相実験により調べた。超重元素Cn, Nh, Flの吸着エンタルピー測定のためのモデル実験として実施した。短寿命同位体はドイツ重イオン研究所の反跳核分離装置TASCAを用いて生成・分離した。生成核はヘリウムガス中に捕集された後、SiO$$_{2}$$あるいはAuで表面を覆われたSi検出器で作製されたガスクロマトグラフィーカラムへと導入した。短寿命Tl及びPb同位体は室温においてSiO$$_{2}$$表面に吸着し、Si検出器で測定することに成功した。一方、HgはSiO$$_{2}$$表面には吸着せず、Au表面に吸着した。この結果より、本実験のセットアップを用いることで短寿命Hg, Tl, Pb同位体の吸着特性を調べることができると証明され、この手法がCn, Nh, Flの実験にも適用できることが確認された。

論文

Identification of the crossing point at $$N$$ = 21 between normal and intruder configurations

Lic$u{a}$, R.*; Rotaru, F.*; Borge, M. J. G.*; Gr$'e$vy, S.*; Negoita, F.*; Poves, A.*; Sorlin, O.*; Andreyev, A. N.; Borcea, R.*; Costache, C.*; et al.

Physical Review C, 95(2), p.021301_1 - 021301_6, 2017/02

https://doi.org/10.1103/PhysRevC.95.021301
 被引用回数：18 パーセンタイル：79.42(Physics, Nuclear)

The $$beta^{-}$$ decay of $$^{34}$$Mg was used to study the $$^{34}$$Al nucleus through $$gamma$$ spectroscopy at the Isotope Separator On-Line facility of CERN. Previous studies identified two $$beta$$-decaying states in $$^{34}$$Al having spin-parity assignments $$J^{pi}$$=4$$^{-}$$ dominated by the normal configuration $$pi$$(d5/2)$$^{-1}$$ $$bigoplus$$ $$nu$$(f7/2) and $$J^{pi}$$ = 1$$^{+}$$ by the intruder configuration $$pi$$(d5/2)$$^{-1}$$ $$bigoplus$$ $$nu$$(d3/2)$$^{-1}$$(f7/2)$$^{2}$$. Their unknown ordering and relative energy have been the subject of debate for the placement of $$^{34}$$Al inside or outside the $$N$$ = 20 "island of inversion". We report here that the 1$$^{+}$$ intruder lies only 46.6 keV above the 4$$^{-}$$ ground state. In addition, a new half-life of $$T_{1/2}$$=44.9(4)ms, that is twice as long as thepreviously measured 20(10) ms, has been determined for $$^{34}$$Mg. Large-scale shell-model calculations with the recently developed SDPF-U-MIX interaction are compared with the new data and used to interpret the mechanisms at play at the very border of the $$N$$ = 20 island of inversion.

論文

Towards saturation of the electron-capture delayed fission probability; The New isotopes $$^{240}$$Es and $$^{236}$$Bk

Konki, J.*; Khuyagbaatar, J.*; Uusitalo, J.*; Greenlees, P. T.*; Auranen, K.*; Badran, H.*; Block, M.*; Briselet, R.*; Cox, D. M.*; Dasgupta, M.*; et al.

Physics Letters B, 764, p.265 - 270, 2017/01

https://doi.org/10.1016/j.physletb.2016.11.038
 被引用回数：17 パーセンタイル：79.42(Astronomy & Astrophysics)

The new neutron-deficient nuclei $$^{240}$$Es and $$^{236}$$Bk were synthesised at the gas-filled recoil separator RITU. They were identified by their radioactive decay chains starting from $$^{240}$$Es produced in the fusion-evaporation reaction $$^{209}$$Bi($$^{34}$$S,3n)$$^{240}$$Es. Half-lives of 6(2)s and 22$$^{+13}_{-6}$$s were obtained for $$^{240}$$Es and $$^{236}$$Bk, respectively. Two groups of $$alpha$$ particles with energies $$E_{alpha}$$=8.19(3) MeV and 8.09(3) MeV were unambiguously assigned to $$^{240}$$Es. Electron-capture delayed fission branches with probabilities of 0.16(6) and 0.04(2) were measured for $$^{240}$$Es and $$^{236}$$Bk, respectively. These new data show a continuation of the exponential increase of ECDF probabilities in more neutron-deficient isotopes.

論文

Beta-delayed proton emission from $$^{20}$$Mg

Lund, M. V.*; Andreyev, A. N.; Borge, M. J. G.*; Cederk$"a$ll, J.*; De Witte, H.*; Fraile, L. M.*; Fynbo, H. O. U.*; Greenlees, P. T.*; Harkness-Brennan, L. J.*; Howard, A. M.*; et al.

European Physical Journal A, 52(10), p.304_1 - 304_14, 2016/10

https://doi.org/10.1140/epja/i2016-16304-x
 被引用回数：17 パーセンタイル：75.78(Physics, Nuclear)

Beta-delayed proton emission from $$^{20}$$Mg has been measured at ISOLDE, CERN, with the ISOLDE Decay Station setup including both charged-particle and $$gamma$$-ray detection capabilities. A total of 27 delayed proton branches were measured including seven so far unobserved. An updated decay scheme, including three new resonances above the proton separation energy in $$^{20}$$Na and more precise resonance energies, is presented. Beta-decay feeding to two resonances above the Isobaric Analogue State in $$^{20}$$Na is observed. This may allow studies of the 4032.9(2.4) keV resonance in $$^{19}$$Ne through the beta decay of $$^{20}$$Mg, which is important for the astrophysically relevant reaction $$^{15}$$O($$alpha$$,$$gamma$$)$$^{19}$$Ne. Beta-delayed protons were used to obtain a more precise value for the half-life of $$^{20}$$Mg, 91.4(1.0) ms.

論文

Spectroscopy of $$^{46}$$Ar by the ($$t,p$$) two-neutron transfer reaction

Nowak, K.*; Wimmer, K.*; Hellgartner, S.*; M$"u$cher, D.*; Bildstein, V.*; Diriken, J.*; Elseviers, J.*; Gaffney, L. P.*; Gernh$"a$user, R.*; Iwanicki, J.*; et al.

Physical Review C, 93(4), p.044335_1 - 044335_10, 2016/04

https://doi.org/10.1103/PhysRevC.93.044335
 被引用回数：18 パーセンタイル：77.39(Physics, Nuclear)

The $$^{44}$$Ar($$t,p$$)$$^{46}$$Ar two-neutron transfer reaction at 2.16 MeV/u was studied at CERN using a $$^{44}$$Ar radioactive beam and a tritium loaded radioactive target. Angular distributions for three final states were measured and based on the shape of the differential cross section an excited state at 3695 keV was identified as the first excited 0$$+$$ state. The differential cross-sections for the 0$$^+$$-ground state, and first excited 2$$^+$$ and 0$$^+$$ states are compared to DWBA calculations including two-step reactions through the intermediate nucleus $$^{45}$$Ar. By comparison large scale shell model calculations using state-of-the-art effective interactions, with and without the tensor components of the interactions, it was observed that the cross-shell proton-neutron tensor interaction has measurable effects on the observables at low excitation energy in $$^{46}$$Ar.

論文

Fast-timing study of the $$l$$-forbidden 1/2$$^+$$ $$rightarrow$$ 3/2$$^+$$ $$M1$$ transition in $$^{129}$$Sn

Lic$u{a}$, R.*; Mach, H.*; Fraile, L. M.*; Gargano, A.*; Borge, M. J. G.*; M$u{a}$rginean, N.*; Sotty, C. O.*; Vedia, V.*; Andreyev, A. N.; Benzoni, G.*; et al.

Physical Review C, 93(4), p.044303_1 - 044303_7, 2016/04

https://doi.org/10.1103/PhysRevC.93.044303
 被引用回数：5 パーセンタイル：39.53(Physics, Nuclear)

The levels in $$^{129}$$Sn populated from the $$beta^-$$ decay of $$^{129}$$In isomers were investigated at the ISOLDE facility of CERN using the newly commissioned ISOLDE Decay Station. The lowest 1/2$$^+$$ state and the 3/2$$^+$$ ground state in $$^{129}$$Sn are expected to have configurations dominated by the neutron $$s_{1/2}$$ ($$l$$=0) and $$d_{3/2}$$ ($$l$$=2) single-particle states, respectively. Consequently, these states should be connected by a somewhat slow $$l$$-forbidden $$M1$$ transition. Using fast-timing spectroscopy we have measured the half-life of the 1/2$$^+$$ 315.3-keV state, $$T_{1/2}$$ = 19(10) ps, which corresponds to a moderately fast $$M1$$ transition. Shell-model calculations using the CD-Bonn effective interaction, with standard effective charges and $$g$$ factors, predict a 4-ns half-life for this level. We can reconcile the shell-model calculations to the measured $$T_{1/2}$$ value by the renormalization of the $$M1$$ effective operator for neutron holes.

論文

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Gaffney, L. P.*; Robinson, A. P.*; Jenkins, D. G.*; Andreyev, A. N.; Bender, M.*; Blazhev, A.*; Bree, N.*; Bruyneel, B.*; Butler, P.*; Cocolios, T. E.*; et al.

Physical Review C, 91(6), p.064313_1 - 064313_11, 2015/06

https://doi.org/10.1103/PhysRevC.91.064313
 被引用回数：8 パーセンタイル：50.7(Physics, Nuclear)

Radioactive ion beams of $$^{202,204}$$Rn were studied by means of low-energy Coulomb excitation at REX-ISOLDE, CERN. The electric-quadrupole (E2) matrix elements connecting the first excited 2$$^+$$ to the ground state of these nuclei was extracted, which permits to determine the collectivity of these isotopes, which in both cases is deduced to be weak, as expected from the low-lying level-energy scheme. Comparisons were also made with beyond-mean-field model calculations and the magnitude of the transitional quadrupole moments are well reproduced.

論文

Single-neutron orbits near $$^{78}$$Ni; Spectroscopy of the N=49 isotope $$^{79}$$Zn

Orlandi, R.; M$"u$cher, D.*; Raabe, R.*; Jungclaus, A.*; Pain, S. D.*; Bildstein, V.*; Chapman, R.*; De Angelis, G.*; Johansen, J. G.*; Van Duppen, P.*; et al.

Physics Letters B, 740, p.298 - 302, 2015/01

https://doi.org/10.1016/j.physletb.2014.12.006
 被引用回数：29 パーセンタイル：85.36(Astronomy & Astrophysics)

Single-neutron states in $$^{79}$$Zn have been populated using the reaction $$^{78}$$Zn(d,p) at REX-Isolde, CERN. The analysis reveals that the lowest excited states in $$^{79}$$Zn lie at approximately 1 MeV, and involve neutron orbits above the N=50 shell gap. A 5/2$$^{+}$$ configuration was assigned to the 983-keV state. Comparison with large-scale shell model calculations supports a robust neutron N=50 shell closure for $$^{78}$$Ni. These data constitute an important step towards the understanding the magicity of $$^{78}$$Ni and the structure of nuclei in the region.

口頭

Low-energy states in $$^{79}$$Zn and the structure of $$^{78}$$Ni

Orlandi, R.; M$"u$cher, D.*; Raabe, R.*; Jungclaus, A.*; Pain, S. D.*; Bildstein, V.*; Chapman, R.*; De Angelis, G.*; Johansen, J. G.*; Van Duppen, P.*; et al.

no journal, , 

Single-neutron states in the $$N$$ = 49 isotope $$^{79}$$Zn were populated in the $$^{78}$$Zn(d,p)$$^{79}$$Zn transfer reaction at REX-ISOLDE, CERN. The combined detection of protons ejected in the reaction and of $$gamma$$ rays emitted by $$^{79}$$Zn permitted the identification of the lowest-lying 5/2$$^+$$ and 1/2$$^+$$ excited states. The analysis of proton angular distributions links these states to a significant amount of single-particle strength around 1 MeV, and specifically to the $$nu$$d$$_{5/2}$$ and $$nu$$s$$_{1/2}$$ neutron orbits, which lie above the $$N$$ = 50 neutron shell gap. Comparison with large-scale-shell-model calculations supports a robust $$N$$ = 50 shell-closure for $$^{78}$$Ni. These data constitute a considerable step towards the understanding of the magicity of $$^{78}$$Ni and of the structure of isotopes in the region.

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