Development of nondestructive elemental analysis system for Hayabusa2 samples using muonic X-rays

Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.

ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04

https://doi.org/10.1021/acsearthspacechem.2c00303

The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.

Spallation and fragmentation cross sections for 168 MeV/nucleon Xe ions on proton, deuteron, and carbon targets

Sun, X. H.*; Wang, H.*; Otsu, Hideaki*; Sakurai, Hiroyoshi*; Ahn, D. S.*; Aikawa, Masayuki*; Fukuda, Naoki*; Isobe, Tadaaki*; Kawakami, Shunsuke*; Koyama, Shumpei*; et al.

Physical Review C, 101(6), p.064623_1 - 064623_12, 2020/06

https://doi.org/10.1103/PhysRevC.101.064623

The spallation and fragmentation reactions of Xe induced by proton, deuteron and carbon at 168 MeV/nucleon were studied at RIKEN Radioactive Isotope Beam Factory via the inverse kinematics technique. The cross sections of the lighter products are larger in the carbon-induced reactions due to the higher total kinetic energy of carbon. The energy dependence was investigated by comparing the newly obtained data with previous results obtained at higher reaction energies. The experimental data were compared with the results of SPACS, EPAX, PHITS and DEURACS calculations. These data serve as benchmarks for the model calculations.

Conceptual study on parasitic low-energy RI beam production with in-flight separator BigRIPS and the first stopping examination for high-energy RI beams in the parasitic gas cell

Sonoda, Tetsu*; Katayama, Ichiro*; Wada, Michiharu*; Iimura, Hideki; Sonnenschein, V.*; Iimura, Shun*; Takamine, Aiko*; Rosenbusch, M.*; Kojima, Takao*; Ahn, D. S.*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(11), p.113D02_1 - 113D02_12, 2019/11

AA2019-0315.pdf:1.37MB

https://doi.org/10.1093/ptep/ptz120

An in-flight separator, BigRIPS, at RIBF in RIKEN provides each experiment with specific nuclides separated from many nuclides produced by projectile fragmentation or in-flight fission. In this process, nuclides other than separated ones are discarded on the slits in BigRIPS, although they include many nuclides interested from the view point of nuclear structure. In order to extract these nuclides for parasitic experiments, we are developing a method using laser ion-source (PALIS). A test experiment with Se beam from RIBF has been performed by using a gas cell set in BigRIPS. Unstable nuclides around Se were stopped in the gas cell in accordance with a calculation using LISE code. The stopping efficiency has been estimated to be about 30%. As a next step, we will establish the technique for extracting reaction products from the gas cell.

Observation of a -decaying millisecond isomeric state in Cd

Jungclaus, A.*; Grawe, H.*; Nishimura, Shunji*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstrm, P.-A.*; Sumikama, Toshiyuki*; Taprogge, J.*; Xu, Z. Y.*; et al.

Physics Letters B, 772, p.483 - 488, 2017/09

https://doi.org/10.1016/j.physletb.2017.07.006

First observation of rays emitted from excited states south-east of Sn; The g multiplet of In

Jungclaus, A.*; Gargano, A.*; Grawe, H.*; Taprogge, J.*; Nishimura, Shunji*; Doornenbal, P.*; Lorusso, G.*; Shimizu, Y.*; Simpson, G. S.*; Sderstrm, P.-A.*; et al.

Physical Review C, 93(4), p.041301_1 - 041301_6, 2016/04

https://doi.org/10.1103/PhysRevC.93.041301

decay of Cd and excited states in In

Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; Nishimura, Shunji*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstrm, P.-A.*; Sumikama, Toshiyuki*; Xu, Z. Y.*; et al.

Physical Review C, 91(5), p.054324_1 - 054324_11, 2015/05

https://doi.org/10.1103/PhysRevC.91.054324

Identification of a millisecond isomeric state in Cd via the detection of internal conversion and Compton electrons

Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; Nishimura, Shunji*; Xu, Z. Y.*; Doornenbal, P.*; Lorusso, G.*; Ncher, E.*; Simpson, G. S.*; Sderstrm, P.-A.*; et al.

Physics Letters B, 738, p.223 - 227, 2014/11

https://doi.org/10.1016/j.physletb.2014.09.047

Monopole-driven shell evolution below the doubly magic nucleus Sn explored with the long-lived isomer in Pd

Watanabe, H.*; Lorusso, G.*; Nishimura, Shunji*; Otsuka, T.*; Ogawa, K.*; Xu, Z. Y.*; Sumikama, Toshiyuki*; Sderstrm, P.-A.*; Doornenbal, P.*; Li, Z.*; et al.

Physical Review Letters, 113(4), p.042502_1 - 042502_6, 2014/07

https://doi.org/10.1103/PhysRevLett.113.042502

Deformation-driven -wave halos at the drip-line; Ne

Nakamura, Takashi*; Kobayashi, Nobuyuki*; Kondo, Yosuke*; Sato, Yoshiteru*; Tostevin, J. A.*; Utsuno, Yutaka; Aoi, Nori*; Baba, Hidetada*; Fukuda, Naoki*; Gibelin, J.*; et al.

Physical Review Letters, 112(14), p.142501_1 - 142501_5, 2014/04

https://doi.org/10.1103/PhysRevLett.112.142501

no abstracts in English

3D hydraulic conductivity modeling of fractured granitic body using geostatistical techniques and its application to regional groundwater flow analysis

Kubo, Taiki*; Koike, Katsuaki*; Liu, C.*; Kurihara, Arata*; Matsuoka, Toshiyuki

Chigaku Zasshi, 122(1), p.139 - 158, 2013/03

https://doi.org/10.5026/jgeography.2012ap02

Numerical simulations have been the most effective method for estimating flow pattern, flux, and flow velocity of the groundwater to precisely characterize large-scale groundwater systems. Spatial modeling of the 3D distribution of hydraulic conductivity over a study area is indispensable to obtain accurate simulation results. However, such spatial modeling is difficult in most cases due to the limitations of hydraulic conductivity data in terms of their volume and location. To overcome these problems and establish an advanced technique, we adopt geostatistics and combine a fracture distribution model with measured conductivity data, selecting the Tono area situated in Gifu Prefecture, central Japan for the field study. The size of the main target area covers 12 km (E-W) by 8 km (N-S), with a depth range of 1.5 km, and it is chiefly underlain by Cretaceous granite. Because the distribution of 395 hydraulic test data acquired along the 25 deep boreholes was biased, the data values were compared to the dimensions of simulated fractures using GEOFRAC. As a result, a positive correlation was identified. Using a regression equation for the correlation, hydraulic conductivity values were assigned to every simulated fracture. Then, a sequential Gaussian simulation (SGS) was applied to construct a 3D spatial model of hydraulic conductivity using those assumed values and actual test data. The plausibility of the resulting model was confirmed through the continuity of high and low permeable zones. The next step is a groundwater flow simulation using MODFLOW and the model. The simulation results were regarded to be appropriate because distribution of hydraulic head, locations of major discharge points, and anisotropy of hydraulic behavior of the Tsukiyoshi fault correspond to the results of observations.