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clusters in dilute neutron-rich matterTanaka, Junki*; Yang, Z.*; Typel, S.*; Adachi, Satoshi*; Bai, S.*; Van Beek, P.*; Beaumel, D.*; Fujikawa, Yuki*; Han, J.*; Heil, S.*; et al.
Science, 371(6526), p.260 - 264, 2021/01
Times Cited Count：25 Percentile：98.55(Multidisciplinary Sciences)By employing quasi-free -cluster-knockout reactions, we obtained direct experimental evidence for the formation of clusters at the surface of neutron-rich tin isotopes. The observed monotonous decrease of the reaction cross sections with increasing mass number, in excellent agreement with the theoretical prediction, implies a tight interplay between -cluster formation and the neutron skin.
CoLokotko, T.*; Leblond, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Poves, A.*; Nowacki, F.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Authelet, G.*; et al.
Physical Review C, 101(3), p.034314_1 - 034314_7, 2020/03
Times Cited Count：7 Percentile：73.84(Physics, Nuclear)The structures of the neutron-rich Co isotopes were investigated via (
) knockout reactions at the Radioactive Isotope Beam Factory, RIKEN. Level schemes were reconstructed using the 
coincidence technique, with tentative spin-parity assignments based on the measured inclusive and exclusive cross sections. Comparison with shell-model calculations suggests coexistence of spherical and deformed shapes at low excitation energies in the Co isotopes.
Ni from the (
,
) reactionElekes, Z.*; Kripk
, 
*; Sohler, D.*; Sieja, K.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Doornenbal, P.*; Obertelli, A.*; Authelet, G.*; Baba, Hidetada*; et al.
Physical Review C, 99(1), p.014312_1 - 014312_7, 2019/01
Times Cited Count：7 Percentile：65.88(Physics, Nuclear)The nuclear structure of the Ni nucleus was investigated by (,) reaction using a NaI(Tl) array to detect the deexciting prompt 
rays. A new transition with an energy of 2227 keV was identified by 
and 
coincidences. Our shell-model calculations using the Lenzi, Nowacki, Poves, and Sieja interaction produced good candidates for the experimental proton hole states in the observed energy region, and the theoretical cross sections showed good agreement with the experimental values. Although we could not assign all the experimental states to the theoretical ones unambiguously, the results are consistent with a reasonably large Z = 28 shell gap for nickel isotopes in accordance with previous studies.
=28 and 
=50; Spectroscopy of 
ZnShand, C. M.*; Podoly
k, Zs.*; Grska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.
Physics Letters B, 773, p.492 - 497, 2017/10
Times Cited Count：22 Percentile：87.77(Astronomy & Astrophysics)Kirishima, Akira*; Kuno, Atsushi*; Amamiya, Hiroki; Kubota, Takumi*; Kimuro, Shingo*; Amano, Yuki; Miyakawa, Kazuya; Iwatsuki, Teruki; Mizuno, Takashi; Sasaki, Takayuki*; et al.
Chemosphere, 168, p.798 - 806, 2017/02
Times Cited Count：3 Percentile：11.4(Environmental Sciences)For better understanding of the migration behavior of minor actinides (MA) in deep groundwater, the interaction of doped rare earth elements (REEs) and components in Horonobe deep groundwater was studied. Appx. 10 ppb of rare earth elements, i.e., Y, La, Ce, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Er, Tm and Yb were doped to the sample groundwater collected from a packed sections in borehole drilled from 140 m depth experiment drift of Horonobe underground research laboratory (URL), Hokkaido, Japan. Then, that groundwater was sequentially filtrated by 0.2 micron pore filter, 10 kDa, 3 kDa and 1 kDa of nominal molecular weight limit (NMWL) ultrafilters by keeping inert condition. After that, the filtrate solutions were analyzed by ICP-MS to determine the concentrations of retained REEs at each filtration steps, while the used filters were analyzed by the neutron activation analysis (NAA) and TOF-SIMS element mapping to know the amount and chemical speciation of trapped fraction of the REEs on each filter. A remarkable relation between the retention ratios of REEs in the filtrate solutions and the ionic radius was observed, i.e., smaller rare earth element solves more in liquid phase under the Horonobe groundwater condition. NAA and TOF-SIMS analyses revealed that certain portions of REEs were trapped by 0.2 micron pore filters as rare earth phosphates which corresponded with the predicted predominant species by a chemical equilibrium calculation for the Horonobe groundwater condition, while small portions of colloidal REEs were trapped by 10 kDa and 3 kDa NMWL ultrafilters. The result suggested that phosphate anion plays an important role in the chemical behavior of REEs in saline (seawater based) groundwater, which could be referred for the prediction of migration behavior of trivalent actinide released from the repository of radioactive waste in far future.
Kada, Wataru*; Kambayashi, Yuya*; Miura, Kenta*; Saruya, Ryota*; Kubota, Atsushi*; Sato, Takahiro; Koka, Masashi; Kamiya, Tomihiro; Hanaizumi, Osamu*
Key Engineering Materials, 643, p.15 - 19, 2015/05
Kada, Wataru*; Miura, Kenta*; Kato, Hijiri*; Saruya, Ryota*; Kubota, Atsushi*; Sato, Takahiro; Koka, Masashi; Ishii, Yasuyuki; Kamiya, Tomihiro; Nishikawa, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research B, 348, p.218 - 222, 2015/04
Times Cited Count：6 Percentile：48.5(Instruments & Instrumentation)Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Kitamura, Akira; Yoshikawa, Hideki; Oda, Chie; Ishidera, Takamitsu; et al.
JAEA-Research 2014-030, 457 Pages, 2015/03
JAEA-Research-2014-030.pdf:199.23MB
JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and post-closure performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, based on some examples of developing method of hydro-geological structure model, acquired knowledge are arranged using the tree diagram, and model uncertainty and its influence on the evaluation items were discussed. With regard to (2) study on scenario development, the developed approach for "defining conditions" has been reevaluated and improved from practical viewpoints. In addition, the uncertainty evaluation for the effect of use of cementitious material, as well as glass dissolution model, was conducted with analytical evaluation. With regard to (3) study on setting radionuclide migration parameters, based on survey of precedent procedures, multiple-approach for distribution coefficient of rocks was established, and the adequacy of the approach was confirmed though its application to sedimentary rock and granitic rock. Besides, an approach for solubility setting was developed including the procedure of selection of solubility limiting solid phase. The adequacy of the approach was confirmed though its application to key radionuclides.
Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Hayano, Akira; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.
JAEA-Research 2013-037, 455 Pages, 2013/12
JAEA-Research-2013-037.pdf:42.0MB
Following FY2011, JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, the tree diagram of methodology of groundwater travel time has been extended for crystalline rock, in addition, tree diagram for sedimentary rock newly has been organized. With regard to (2) study on scenario development, the existing approach has been improved in terms of a practical task, and applied and tested for near field focusing on the buffer. In addition, the uncertainty of some important processes and its impact on safety functions are discussed though analysis. With regard to (3) study on setting radionuclide migration parameters, the approaches for parameter setting have been developed for sorption for rocks and solubility, and applied and tested through parameter setting exercises for key radionuclides.
Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Hayano, Akira; Mitsui, Seiichiro; Taniguchi, Naoki; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.
JAEA-Research 2012-032, 298 Pages, 2012/09
JAEA-Research-2012-032.pdf:33.68MB
JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation phase. The topics and the conducted research are follows; (1) Study on selection of host rock: in terms of hydraulic properties, items for assessing rock property, and assessment methodology of groundwater travel time has been organized with interaction from site investigation. (2) Study on development of scenario: the existing approach has been embodied, in addition, the phenomenological understanding regarding dissolution of and nuclide release from vitrified waste, corrosion of the overpack, long-term performance of the buffer are summarized. (3) Study on setting nuclide migration parameters: the approach for parameter setting has been improved for sorption and diffusion coefficient of buffer/rock, and applied and tested for parameter setting of key radionuclides. (4) Study on ensuring quality of knowledge: framework for ensuring quality of knowledge has been studied and examined aimed at the likely disposal facility condition.
; Comparison with LaFePONishi, Ichiro*; Ishikado, Motoyuki; Ideta, Shinichiro*; Malaeb, W.*; Yoshida, Teppei*; Fujimori, Atsushi*; Kotani, Yoshinori*; Kubota, Masato*; Ono, Kanta*; Yi, M.*; et al.
Physical Review B, 84(1), p.014504_1 - 014504_5, 2011/07
Times Cited Count：22 Percentile：66.85(Materials Science, Multidisciplinary)We have performed an angle-resolved photoemission spectroscopy (ARPES) study of the iron-based superconductor PrFeAsO and examined the Fermi surfaces and band dispersions near the fermi level. Heavily hole-doped electronic states have been observed due to the polar nature of the cleaved surfaces. Nevertheless, we have found that the ARPES spectra basically agree with band dispersions calculated in the local density approximation (LDA) if the bandwidth is reduced by a factor of 
2.5 and then the chemical potential is lowered by 70 meV. Comparison with previous ARPES results on LaFePO reveals that the energy positions of the 
- and 
-derived bands are considerably different between the two materials, which we attribute to the different pnictogen height as predicted by the LDA calculation.
Shiotani, Hiroki; Ohtaki, Akira; Ono, Kiyoshi; Hirao, Kazunori; Kato, Atsushi; Yasumatsu, Naoto*; Kubota, Sadae*
JNC TN9400 2004-052, 514 Pages, 2004/09
JNC-TN9400-2004-052.pdf:8.85MB
This report presents the outline of the development and the results of characteristic evaluation on the candidate Fast Reactor (FR) cycle system concepts, scenario study on FR cycle deployment and cost-benefit analysis on the candidate FR cycle system concepts in the interim evaluation (FY2001 through FY2003) of the second phase of the Japanese "Feasibility Study on Commercialization of Fast Breeder Reactor Cycle System (FS)".
Matsukado, Koji*; Esirkepov, T. Z.; Kinoshita, Kenichi*; Daido, Hiroyuki; Utsumi, Takayuki*; Li, Z.*; Fukumi, Atsushi*; Hayashi, Yukio; Orimo, Satoshi; Nishiuchi, Mamiko; et al.
Physical Review Letters, 91(21), p.215001_1 - 215001_4, 2003/11
Times Cited Count：136 Percentile：95.38(Physics, Multidisciplinary)no abstracts in English
Takeshita, Isao; Maeda, Mitsuru; Miyoshi, Yoshinori; Ono, Akio; Okazaki, Shuji; Nakajima, Ken; Fujine, Sachio; Kubota, Masumitsu; Muraoka, Susumu; Ara, Katsuyuki; et al.
Genshiryoku Kogyo, 43(9), p.1 - 37, 1997/09
no abstracts in English
Kato, Atsushi; Mukaida, Kyoko; Ohtaki, Akira; Shiotani, Hiroki; Ono, Kiyoshi; Yasumatsu, Naoto*; Kubota, Sadae*
no journal, ,
no abstracts in English
Hayano, Akira; Sawada, Atsushi; Goto, Junichi*; Ishii, Eiichi*; Moriya, Toshifumi*; Inagaki, Manabu*; Kubota, Shigeru*; Ebashi, Takeshi*
no journal, ,
Detailed Investigation Areas have to be selected with focusing on suitability of the host rock in the siting process for high-level radioactive waste disposal in Japan. The suitability of the host rock is evaluated in terms of the preferable disposal condition such as thermal, hydraulic, mechanical and geochemical condition, and the feasibility of the geological disposal project relevant to volumetric capacity of host rock and economics, based on the site model. However, due to a limited number of surveys at relatively early stage of the investigation, the lack of understanding of geological environment at the site causes an uncertainty of the site model. It is essential to clarify an association the important factors relevant to safety assessment (SA) and a repository design (Design) with the information obtained by the site investigation through the site model. In this study, the methodology not only for defining evaluation factors relevant to SA in term of hydrogeology, but also for visualizing the methods to evaluate the factors through the site model is organized into a tree diagram. A method to evaluate groundwater travel time which is one of evaluation factors in granitic rock is organized into a first version of the tree diagram.
Miura, Kenta*; Sato, Takahiro; Ishii, Yasuyuki; Koka, Masashi; Takano, Katsuyoshi*; Okubo, Takeru; Yamazaki, Akiyoshi; Kada, Wataru; Yokoyama, Akihito; Kamiya, Tomihiro; et al.
no journal, ,
Kirishima, Akira*; Kuno, Atsushi*; Amamiya, Hiroki; Murakami, Hiroaki; Amano, Yuki; Iwatsuki, Teruki; Mizuno, Takashi; Kubota, Takumi*; Sasaki, Takayuki*; Sato, Nobuaki*
no journal, ,
For understanding of the migration behavior of minor actinides (MA) in groundwater, the interaction of rare earth elements and suspended matters contained in Horonobe deep groundwater was studied. From this chemical analog study, it is suggested that the migration behavior of MA in the Horonobe groundwater system seems to be regulated by the formation of phosphate precipitation and small percentage of MA would be carried in the groundwater as pseudo colloids like MA-humic substance complex.
Amano, Yuki; Amamiya, Hiroki; Murakami, Hiroaki; Iwatsuki, Teruki; Terashima, Motoki; Mizuno, Takashi; Kirishima, Akira*; Kuno, Atsushi*; Sasaki, Takayuki*; Kubota, Takumi*; et al.
no journal, ,
no abstracts in English
Kirishima, Akira*; Kuno, Atsushi*; Amamiya, Hiroki; Murakami, Hiroaki; Amano, Yuki; Iwatsuki, Teruki; Mizuno, Takashi; Kubota, Takumi*; Sasaki, Takayuki*; Sato, Nobuaki*
no journal, ,
no abstracts in English
