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Journal Articles

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

 Times Cited Count:1 Percentile:0.02(Astronomy & Astrophysics)

Gamma decays were observed in $$^{56}$$Ca and $$^{58}$$Ca following quasi-free one-proton knockout reactions from $$^{57,59}$$Sc. For $$^{56}$$Ca, a $$gamma$$ ray transition was measured to be 1456(12) keV, while for $$^{58}$$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $$2^{+}_{1} rightarrow 0^{+}_{gs}$$ decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $$2^{+}_{1}$$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the $$0_{f5/2}$$ and $$0_{g9/2}$$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $$^{60}$$Ca and potentially drives the dripline of Ca isotopes to $$^{70}$$Ca or even beyond.

Journal Articles

Structural phase transition in cobalt oxyfluoride Co$$_{3}$$Sb$$_{4}$$O$$_{6}$$F$$_{6}$$ observed by high-resolution synchrotron and neutron diffraction

Shimono, Seiya*; Ishibashi, Hiroki*; Nagayoshi, Yusuke*; Ikeno, Hidekazu*; Kawaguchi, Shogo*; Hagihara, Masato; Torii, Shuki*; Kamiyama, Takashi*; Ichihashi, Katsuya*; Nishihara, Sadafumi*; et al.

Journal of Physics and Chemistry of Solids, 163, p.110568_1 - 110568_7, 2022/04

 Times Cited Count:1 Percentile:15.7(Chemistry, Multidisciplinary)

Journal Articles

Microstructures and interface magnetic moments in Mn$$_{2}$$VAl/Fe layered films showing exchange bias

Kubota, Takahide*; Shimada, Yusuke*; Tsuchiya, Tomoki*; Yoshikawa, Tomoki*; Ito, Keita*; Takeda, Yukiharu; Saito, Yuji; Konno, Toyohiko*; Kimura, Akio*; Takanashi, Koki*

Nanomaterials (Internet), 11(7), p.1723_1 - 1723_11, 2021/07

 Times Cited Count:2 Percentile:17.84(Chemistry, Multidisciplinary)

Journal Articles

Quasifree neutron knockout reaction reveals a small $$s$$-Orbital component in the Borromean nucleus $$^{17}$$B

Yang, Z. H.*; Kubota, Yuki*; Corsi, A.*; Yoshida, Kazuki; Sun, X.-X.*; Li, J. G.*; Kimura, Masaaki*; Michel, N.*; Ogata, Kazuyuki*; Yuan, C. X.*; et al.

Physical Review Letters, 126(8), p.082501_1 - 082501_8, 2021/02

AA2020-0819.pdf:1.29MB

 Times Cited Count:43 Percentile:96.7(Physics, Multidisciplinary)

A quasifree ($$p$$,$$pn$$) experiment was performed to study the structure of the Borromean nucleus $$^{17}$$B, which had long been considered to have a neutron halo. By analyzing the momentum distributions and exclusive cross sections, we obtained the spectroscopic factors for $$1s_{1/2}$$ and $$0d_{5/2}$$ orbitals, and a surprisingly small percentage of 9(2)% was determined for $$1s_{1/2}$$. Our finding of such a small $$1s_{1/2}$$ component and the halo features reported in prior experiments can be explained by the deformed relativistic Hartree-Bogoliubov theory in continuum, revealing a definite but not dominant neutron halo in $$^{17}$$B. The present work gives the smallest $$s$$- or $$p$$-orbital component among known nuclei exhibiting halo features and implies that the dominant occupation of $$s$$ or $$p$$ orbitals is not a prerequisite for the occurrence of a neutron halo.

Journal Articles

Repeatability and reproducibility of measurements of low dissolved radiocesium concentrations in freshwater using different pre-concentration methods

Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11

 Times Cited Count:2 Percentile:21.58(Chemistry, Analytical)

We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the $$^{137}$$Cs results were within $$pm$$2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.

JAEA Reports

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Compilation of groundwater chemistry data in the Mizunami group and the Toki granite (fiscal year 2016)

Watanabe, Yusuke; Hayashida, Kazuki; Kato, Toshihiro; Kubota, Mitsuru; Aosai, Daisuke*; Kumamoto, Yoshiharu*; Iwatsuki, Teruki

JAEA-Data/Code 2018-002, 108 Pages, 2018/03

JAEA-Data-Code-2018-002.pdf:6.53MB

Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the effect of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2016 and 2014 to 2016, respectively. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.

Journal Articles

Application of ionic liquids to extraction separation of rare earth metals with an effective diglycol amic acid extractant

Kubota, Fukiko*; Shimobori, Yosuke*; Baba, Yuzo*; Koyanagi, Yusuke*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

Journal of Chemical Engineering of Japan, 44(5), p.307 - 312, 2011/05

 Times Cited Count:57 Percentile:82.68(Engineering, Chemical)

The application of ionic liquids as alternatives to conventional organic solvents in extraction processes has been actively investigated. A crucial step towards the practical use of ionic liquids is the development of extractants that work effectively within these new media. In the present study, the extraction separation of rare earth metals into ionic liquids, 1-butyl, 1-octyl, and l-dodecyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide ([C$$_{n}$$ min][Tf$$_{2}$$N], ${it n}$ = 4, 8, 12), was performed using a novel extractant, ${it N}$,${it N}$-dioctyldiglycol amic acid (DODGAA). Quantitative extraction of metal ions such as Y$$^{3+}$$ and Eu$$^{3+}$$ was selectively achieved in the presence of the base metal ion Zn$$^{2+}$$, which was not extracted at all under the present experimental conditions. The extraction efficiency was enhanced for the shorter-alkyl-chain imidazolium ionic liquid [C$$_{4}$$mim] [Tf$$_{2}$$N] compared to that for a conventional organic solvent system. Extraction mechanism studies elucidated that the metal extraction proceeds via proton exchange reactions between DODGAA and the metal ions in the ionic liquid (the same mechanism as in the conventional organic solvent). The stripping reaction, or recovery, of the metal ions from the extracting phase was readily accomplished with an acid solution such as nitric acid.

Journal Articles

Uphill transport of rare-earth metals through a highly stable supported liquid membrane based on an ionic liquid

Kubota, Fukiko*; Shimobori, Yosuke*; Koyanagi, Yusuke*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

Analytical Sciences, 26(3), p.289 - 290, 2010/03

 Times Cited Count:49 Percentile:82.68(Chemistry, Analytical)

We have developed a highly stable supported liquid membrane based on ionic liquids (ILs) for the separation of rare-earth metals, employing $$N,N$$-dioctyldiglycol amic acid as a mobile carrier. The quantitative transport of Y and Eu through the membrane was successfully attained, and separation from metal impurities, Zn, was efficiently accomplished. A membrane stable enough for long-term operation was constructible from imidazolium-based ILs having a longer alkyl chain, such as octyl or dodecyl groups in an imidazolium cation.

Journal Articles

Extraction behavior of indium with TOPO into ionic liquids

Kubota, Fukiko*; Shimobori, Yosuke*; Koyanagi, Yusuke*; Nakashima, Kazunori*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

Solvent Extraction Research and Development, Japan, 16, p.142 - 146, 2009/00

Journal Articles

Extraction of lanthanide ions with an organophosphorous extractant into ionic liquids

Kubota, Fukiko*; Koyanagi, Yusuke*; Nakashima, Kazunori*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

Solvent Extraction Research and Development, Japan, 15, p.81 - 87, 2008/00

Extraction of lanthanide ions was carried out with the organophosphorous extractant PC-88A dissolved in an imidazolium-based ionic liquid. PC-88A was soluble in ionic liquids having long-chain alkyl substituents such as octyl and dodecyl groups, [C$$_{8}$$mim] and [C$$_{12}$$mim][TFSI], although short-chain imidazolium ionic liquids could not solubilize the extractant. The extraction equilibrium observed in the ionic liquid system was similar to that in the n-dodecane system, and the extraction behavior could be explained by the same proton exchange mechanism as for the conventional organic solvent system, although the extraction efficiency was not improved. An ionic liquid having shorter alkyl chain [C$$_{8}$$mim] showed a higher extraction ability than [C$$_{12}$$mim][TFSI]. Stripping of the metal ions from the ionic liquids was also examined. Quantitative stripping of the metal ions was achieved by nitric acid in the [C$$_{12}$$mim][TFSI] system.

Journal Articles

Extraction of cytochrome c by a functionalized ionic liquid containing a crown ether

Kubota, Fukiko*; Koyanagi, Yusuke*; Nakashima, Kazunori*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

Solvent Extraction Research and Development, Japan, 14, p.115 - 120, 2007/00

We carried out the extraction of a protein cytochrome c (Cyt-c) with an ionic liquid with an attached crown ether moiety in the imidazolium cation. The functional ionic liquid, [18C6mim][PF$$_{6}$$], was dissolved in two different ionic liquids as diluents, one having a hydroxyethyl group, [C$$_{2}$$OHmim][Tf$$_{2}$$N], and the other an ethyl group, [C$$_{2}$$mim][Tf$$_{2}$$N], respectively. The transfer of Cyt-c from the aqueous phase to the ionic liquid phase took place with [18C6mim][PF$$_{6}$$] in the [C$$_{2}$$OHmim][Tf$$_{2}$$N] system. Although the extraction ability was lower than that of dicyclohexano-18-crown-6 (DCH18C6), the functionalized ionic liquid system gave a better stripping performance than the ordinary crown ether system. The extraction efficiency was not influenced by operating temperature when the concentration of [18C6mim] was high whereas it was greatly affected by temperature at low [18C6mim] concentration.

Journal Articles

High heat load test of molybdenum

Tanabe, Tetsuro*; Fujine, Michihiko*; Noguchi, Hiroshi*; Yagi, Yasufumi*; Hirano, Yoichi*; Shimizu, Hajime*; Akiba, Masato; Araki, Masanori; Kubota, Yusuke*; Miyahara, Akira*

Journal of Nuclear Materials, 200(1), p.120 - 127, 1993/03

 Times Cited Count:9 Percentile:66.93(Materials Science, Multidisciplinary)

no abstracts in English

Oral presentation

Extraction of protein by functionalized ionic liquid

Kubota, Fukiko*; Koyanagi, Yusuke*; Nakashima, Kazunori*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

no journal, , 

no abstracts in English

Oral presentation

Extraction of Cyt-c by functionalized ionic liquid with crown ether

Kubota, Fukiko*; Koyanagi, Yusuke*; Nakashima, Kazunori*; Shimojo, Kojiro; Kamiya, Noriho*; Goto, Masahiro*

no journal, , 

no abstracts in English

Oral presentation

Mach-Zehnder type thermo-optic switch fabricated by proton beam writing

Ozawa, Yusuke*; Kubota, Hitoshi*; Miura, Kenta*; Hanaizumi, Osamu*; Noguchi, Katsuya*; Sato, Takahiro; Ishii, Yasuyuki; Koka, Masashi; Takano, Katsuyoshi*; Okubo, Takeru; et al.

no journal, , 

Oral presentation

Prototype of thermo-optic switch consisting of Mach-Zehnder polymer waveguide drawn by focused proton beam

Miura, Kenta*; Sato, Takahiro; Ishii, Yasuyuki; Koka, Masashi; Takano, Katsuyoshi*; Okubo, Takeru; Yamazaki, Akiyoshi; Kada, Wataru; Yokoyama, Akihito; Kamiya, Tomihiro; et al.

no journal, , 

Oral presentation

Development of fabrication technique of optical functional devices by ion beam irradiation

Miura, Kenta*; Hanaizumi, Osamu*; Kada, Wataru*; Ozawa, Yusuke*; Inada, Kazuki*; Kubota, Atsushi*; Kawashima, Akihiro*; Sato, Takahiro; Ishii, Yasuyuki; Koka, Masashi; et al.

no journal, , 

no abstracts in English

Oral presentation

The Activity Report of review working group for simple radiation shielding "V&V activity with benchmark experiment of Mutsu"

Nobuhara, Fumiyoshi*; Matsuda, Norihiro; Onishi, Seiki*; Matsui, Yusuke*; Kubota, Osamu*; Sakamoto, Yukio*; Hirao, Yoshihiro*

no journal, , 

no abstracts in English

18 (Records 1-18 displayed on this page)
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