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Journal Articles

Assessment of caesium-137 detections at CTBTO radionuclide monitoring stations in East Asia and their relationship to Asian dust dispersion

Furuno, Akiko; Omori, Ryuta*; Tateoka, Hisanori*; Minakawa, Yuya*; Kurihara, Toshiyuki; Yamamoto, Yoichi; Tomita, Yutaka

Pure and Applied Geophysics, 182(12), p.5175 - 5188, 2025/12

 Times Cited Count:2 Percentile:23.61(Geochemistry & Geophysics)

The Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) Okinawa radionuclide monitoring station (JPP37) is located on a hill facing the East China Sea at the center of the main island of Okinawa. It occasionally detects Cs-137, although no nuclear facilities are located on the island. This study focused on the detection of Cs-137 at JPP37 and examined the ratio of simultaneous detections at nearby stations of the International Monitoring System (IMS) of the CTBTO and the relationship with Asian dust from inland East Asia. The detection of Cs-137 in JPP37 from 2020 to 2023, which motivated this study, was high in spring. Among the nine IMS radionuclide stations in East Asia, the detections in Beijing, Lanzhou, and Ulaanbaatar, Mongolia, were also high in spring. This suggested a high association with the detection of Asian dust in East Asia. Thus, we confirmed the detection of Cs-137 at nine nearby IMS stations when Asian dust was observed at any of the sites in Japan. In addition, we observed that the detection rates were high in Takasaki, Beijing, Lanzhou, and Ulaanbaatar. It can be inferred that the Cs-137 observed mainly in spring at the IMS particulate radionuclide stations in the East Asian region around Japan were likely to pick up the effects of global fallout conveyed by Asian dust. Thereafter, we conducted a preliminary source estimation analysis for Asian dust arrival near Japan. Atmospheric dispersion simulations explained the detection of Cs-137 at nearby IMS particulate radionuclide stations, assuming that Cs-137 was emitted from the desert, the source of the Asian dust.

Journal Articles

Speciation of cesium in a radiocesium-bearing microparticle emitted from Unit 1 during the Fukushima nuclear accident by XANES spectroscopy using transition edge sensor

Takahashi, Yoshio*; Miura, Hikaru*; Yamada, Shinya*; Sekizawa, Oki*; Nitta, Kiyofumi*; Hashimoto, Tadashi*; Yomogida, Takumi; Yamaguchi, Akiko; Okada, Shinji*; Itai, Takaaki*; et al.

Journal of Hazardous Materials, 495, p.139031_1 - 139031_19, 2025/09

 Times Cited Count:6 Percentile:80.81(Engineering, Environmental)

In this presentation, we analyzed the chemical state of cesium in radiocesium-bearing microparticles (CsMPs) released during the 2011 Fukushima Daiichi Nuclear Power Plant accident using high-resolution X-ray absorption spectroscopy (XANES) and micro X-ray fluorescence ($$mu$$-XRF). The results identified two forms of cesium: one dissolved in glass and the other enriched on the surfaces of internal voids. The latter is considered to have originally existed as a gas and became concentrated during the cooling and solidification of the molten glass. These findings are crucial for understanding the formation process of CsMPs during the accident, as well as for future decommissioning and safety assessments.

Journal Articles

Beam commissioning of the linac for iBNCT

Naito, Fujio*; Anami, Shozo*; Ikegami, Kiyoshi*; Uota, Masahiko*; Ouchi, Toshikatsu*; Onishi, Takahiro*; Oba, Toshiyuki*; Obina, Takashi*; Kawamura, Masato*; Kumada, Hiroaki*; et al.

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1244 - 1246, 2016/11

The proton linac installed in the Ibaraki Neutron Medical Research Center is used for production of the intense neutron flux for the Boron Neutron Capture Therapy (BNCT). The linac consists of the 3-MeV RFQ and the 8-MeV DTL. Design average beam current is 10mA. Target is made of Beryllium. First neutron production from the Beryllium target was observed at the end of 2015 with the low intensity beam as a demonstration. After the observation of neutron production, a lot of improvement s was carried out in order to increase the proton beam intensity for the real beam commissioning. The beam commissioning has been started on May 2016. The status of the commissioning is summarized in this report.

Journal Articles

3D geostatistical modeling of fracture system in a granitic massif to characterize hydraulic properties and fracture distribution

Koike, Katsuaki*; Kubo, Taiki*; Liu, C.*; Masoud, A.*; Amano, Kenji; Kurihara, Arata*; Matsuoka, Toshiyuki; Lanyon, B.*

Tectonophysics, 660, p.1 - 16, 2015/10

 Times Cited Count:32 Percentile:65.31(Geochemistry & Geophysics)

This study integrates 3D models of rock fractures from different sources and hydraulic properties aimed at identifying relationships between fractures and permeability. A geostatistical method (GEOFRAC) that can incorporate orientations of sampled data was applied to 50,900 borehole fractures for spatial modeling of fractures over a 12 km by 8 km area, to a depth of 1.5 km. GEOFRAC produced a plausible 3D fracture model, in that the orientations of simulated fractures correspond to those of the sample data and the continuous fractures appeared near a known fault. Small-scale fracture distributions with dominant orientations were also characterized around the two shafts using fracture data from the shaft walls. By integrating the 3D model of hydraulic conductivity using sequential Gaussian simulation with the GEOFRAC fractures from the borehole data, the fracture sizes and directions that strongly affect permeable features were identified.

Journal Articles

3D hydraulic conductivity modeling of fractured granitic body using geostatistical techniques and its application to regional groundwater flow analysis

Kubo, Taiki*; Koike, Katsuaki*; Liu, C.*; Kurihara, Arata*; Matsuoka, Toshiyuki

Chigaku Zasshi, 122(1), p.139 - 158, 2013/03

Numerical simulations have been the most effective method for estimating flow pattern, flux, and flow velocity of the groundwater to precisely characterize large-scale groundwater systems. Spatial modeling of the 3D distribution of hydraulic conductivity over a study area is indispensable to obtain accurate simulation results. However, such spatial modeling is difficult in most cases due to the limitations of hydraulic conductivity data in terms of their volume and location. To overcome these problems and establish an advanced technique, we adopt geostatistics and combine a fracture distribution model with measured conductivity data, selecting the Tono area situated in Gifu Prefecture, central Japan for the field study. The size of the main target area covers 12 km (E-W) by 8 km (N-S), with a depth range of 1.5 km, and it is chiefly underlain by Cretaceous granite. Because the distribution of 395 hydraulic test data acquired along the 25 deep boreholes was biased, the data values were compared to the dimensions of simulated fractures using GEOFRAC. As a result, a positive correlation was identified. Using a regression equation for the correlation, hydraulic conductivity values were assigned to every simulated fracture. Then, a sequential Gaussian simulation (SGS) was applied to construct a 3D spatial model of hydraulic conductivity using those assumed values and actual test data. The plausibility of the resulting model was confirmed through the continuity of high and low permeable zones. The next step is a groundwater flow simulation using MODFLOW and the model. The simulation results were regarded to be appropriate because distribution of hydraulic head, locations of major discharge points, and anisotropy of hydraulic behavior of the Tsukiyoshi fault correspond to the results of observations.

Journal Articles

Geological investigations for geological model of deep underground geoenvironment at the Mizunami Underground Research Laboratory (MIU)

Tsuruta, Tadahiko; Tagami, Masahiko; Amano, Kenji; Matsuoka, Toshiyuki; Kurihara, Arata; Yamada, Yasuhiro*; Koike, Katsuaki*

Chishitsugaku Zasshi, 119(2), p.59 - 74, 2013/02

Japan Atomic Energy Agency (JAEA) is developing a geoscientific research project, Mizunami Underground Research Laboratory (MIU) project, in order to establish scientific and technological basis for geological disposal of HLW. A series of geological mapping, reflection seismic survey, borehole investigation and geological investigations around research galleries are carried out to identify the distribution and the heterogeneity of fractures and faults that are potential major flow-pass of groundwater as field investigations. This paper describes geological investigations in the MIU project, focused on the evaluation of their effectiveness in order to understand the deep underground geological environment.

JAEA Reports

Development of geological models in the Mizunami Underground Research Laboratory Project; Updating from "Shaft180 geological model" to "Stage300 geological model" in Phase 2

Ishibashi, Masayuki; Kurihara, Arata*; Matsuoka, Toshiyuki; Sasao, Eiji

JAEA-Research 2012-018, 48 Pages, 2012/07

JAEA-Research-2012-018.pdf:8.48MB
JAEA-Research-2012-018(errata).pdf:1.13MB
JAEA-Research-2012-018-appendix(CD-ROM).zip:13.81MB

This document presents about updating of geological models at the Phase 2 in the Mizunami underground research laboratory project. In the phase 2, the geological models has been updated four times (Shaft180 geological model, Pilot500 geological model, Sustage200 geological model, Stage300 geological model) based on geological mapping date and/or some borehole investigation data at the shafts and research galleries. These geological models represent distributions of lithofacies and/or geological structures based on each geological investigation. In order to evaluate relationship between understanding of geological environments and progress of investigations, to organize the history of geological models updating is important.

Journal Articles

Geostatistic analysis for groundwater flow and hydraulic parameters in deep granitic body

Kubo, Taiki*; Koike, Katsuaki*; Kurihara, Arata*; Matsuoka, Toshiyuki

Heisei-23 Nendo (2011 Nen) Shigen, Sozai Gakkai Shuki Taikai Koenshu, p.369 - 370, 2011/09

no abstracts in English

JAEA Reports

Study on Geology on Mizunami Underground Research Laboratory Project; Annual report for fiscal year 2008

Tsuruta, Tadahiko; Matsuoka, Toshiyuki; Hodotsuka, Yasuyuki; Tagami, Masahiko; Ishida, Hideaki; Hayano, Akira; Kurihara, Arata; Yuguchi, Takashi

JAEA-Research 2010-039, 131 Pages, 2011/01

JAEA-Research-2010-039.pdf:25.36MB

Tono Geoscientific Unit of Geological Isolation and Development Directoratte is performing Mizunami Underground Research Laboratory (MIU) Project, which is a broad scientific study of the deep geological environment as a basis of research and development for geological disposal of nuclear wastes, in order to establish comprehensive techniques for the investigation, analysis and assessment of the deep geological environment in fractured crystalline rock. The MIU Project has three overlapping 3 phases, with a total duration of 20 years. The project goals of the MIU Project from Phase I through to Phase III are: to establish techniques for investigation, analysis and assessment of the deep geological environment, and to develop a range of engineering for deep underground application. Currently, the project is under the Phase II. This document presents the overview of results of the research and development on "geology" performed in fiscal year 2008, with regard to the Phase II goal.

Journal Articles

Commentaries for third secondary national examination on fiscal 2010 for the professional engineer of nuclear and radiation; Commentaries (Part 1) including key point for elective examinations

Sasaki, Satoru; Suto, Toshiyuki; Harada, Akio; Kurihara, Ryoichi; Yamamoto, Kazuyoshi; Tsuchida, Noboru; Shimizu, Isamu; Nomura, Toshibumi

Genshiryoku eye, 57(1), p.66 - 75, 2011/01

no abstracts in English

Journal Articles

A Neutron crystallographic analysis of a cubic porcine insulin at pD 6.6

Ishikawa, Takuya*; Chatake, Toshiyuki*; Onishi, Yuki*; Tanaka, Ichiro*; Kurihara, Kazuo; Kuroki, Ryota; Niimura, Nobuo*

Chemical Physics, 345(2-3), p.152 - 158, 2008/04

 Times Cited Count:14 Percentile:42.35(Chemistry, Physical)

Journal Articles

Design study of the JT-60SA supervisory control system

Kawamata, Yoichi; Naito, Osamu; Kiyono, Kimihiro; Itami, Kiyoshi; Totsuka, Toshiyuki; Akasaka, Hiromi; Sueoka, Michiharu; Sato, Tomoki; Oshima, Takayuki; Sakata, Shinya; et al.

Fusion Engineering and Design, 83(2-3), p.198 - 201, 2008/04

 Times Cited Count:3 Percentile:21.81(Nuclear Science & Technology)

The design activity of JT-60SA (JT-60 Super Advanced) which is remodeled to a superconducting tokamak device has been starting under the JA-EU collaborative ITER-BA project. For the JT-60SA control system, the existing system should be reused as much as possible from the viewpoint of cost-effectiveness. We have just begun to discuss the configuration of the advanced Supervisory Control System (SVCS) including the following systems: (1) ultimately flexible real-time control system, (2) precise timing system enough to clarify cause and effect, and (3) safety shutdown control system. In this report, we present the design study of the JT-60SA SVCS with focusing on these systems.

Journal Articles

Development of the supervisory discharge operation monitoring system for JT-60

Sueoka, Michiharu; Totsuka, Toshiyuki; Kawamata, Yoichi; Kurihara, Kenichi; Seki, Akiyuki

Fusion Engineering and Design, 83(2-3), p.283 - 286, 2008/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

For safety and efficient operation of a fusion device, appropriate information should be provided to the personnel related to experiment. In order to realize this, we have newly developed highlight screens displaying the plasma movie, the status of discharge sequence, the discharge schedule, the present status of trouble, etc., with the large (65 inch) monitor TV in front of the central consoles. These highlight screens are automatically switched according to the timing signal of JT-60 discharge sequence and/or the operator's request. We call this system the supervisory discharge operation monitoring system. This report deals with the technical details of this system including the plasma movie database system and the discharge information management system.

Journal Articles

Protonation states of buried histidine residues in human deoxyhemoglobin revealed by neutron crystallography

Chatake, Toshiyuki*; Shibayama, Naoya*; Park, S. Y.*; Kurihara, Kazuo; Tamada, Taro; Tanaka, Ichiro*; Niimura, Nobuo*; Kuroki, Ryota; Morimoto, Yukio*

Journal of the American Chemical Society, 129(48), p.14840 - 14841, 2007/12

 Times Cited Count:27 Percentile:60.67(Chemistry, Multidisciplinary)

Journal Articles

Recent results on hydrogen and hydration in biology studied by neutron macromolecular crystallography

Niimura, Nobuo; Arai, Shigeki; Kurihara, Kazuo; Chatake, Toshiyuki*; Tanaka, Ichiro*; Bau, R.*

Cellular and Molecular Life Sciences, 63(3), p.285 - 300, 2006/02

 Times Cited Count:41 Percentile:36.50(Biochemistry & Molecular Biology)

Neutron diffraction provides an experimental method of directly locating hydrogen atoms in proteins and DNA oligomers. Three different types of high resolution neutron diffractometers for biological macromolecules have been constructed in Japan, France and the U.S.A., and they have all been actively used in recent years to determine the crystal structures of numerous proteins. Examples include the detailed geometries of hydrogen bonds, information on H/D exchange in proteins, the unambiguous location of protons, the role of key hydrogen atoms in enzymatic activity and thermostability, and the dynamical behavior of hydration structures, all of which have been extracted from these structural results and reviewed in this article. Other important techniques, such as the optimization of growth of large single crystals using phase diagrams, the preparation of fully deuterated proteins, the introduction of cryogenic techniques to neutron protein crystallography, and the establishment of a "hydrogen and hydration in proteins" database, will also be described in this paper.

Journal Articles

Complicated water orientations in the minor groove of the B-DNA decamer d(CCATTAATGG)$$_{2}$$ observed by neutron diffraction measurements

Arai, Shigeki; Chatake, Toshiyuki*; Ohara, Takashi; Kurihara, Kazuo; Tanaka, Ichiro*; Suzuki, Nobuhiro*; Fujimoto, Zui*; Mizuno, Hiroshi*; Niimura, Nobuo

Nucleic Acids Research, 33(9), p.3017 - 3024, 2005/05

 Times Cited Count:94 Percentile:81.78(Biochemistry & Molecular Biology)

It has long been suspected that the structure and function of a DNA duplex can be strongly dependent on its degree of hydration. By neutron diffraction experiments, we have succeeded in determining most of the hydrogen (H) and deuterium (D) atomic positions in the d(CCATTAATGG)$$_{2}$$ duplex. Moreover, the D positions in 27 D$$_{2}$$O molecules have been determined. In particular, the complex water network in the minor groove has been observed in detail. By a combined structural analysis using 2.0 Å resolution X-ray and 3.0 Å resolution neutron data, it is clear that the spine of hydration is built up, not only by a simple hexagonal hydration pattern (as reported in prior X-ray studies), but also by many other water bridges hydrogen-bonded to the DNA strands. The complexity of the hydration pattern in the minor groove is derived from an extraordinary variety of orientations displayed by the water molecules.

Journal Articles

Hydrogen and hydration in proteins and nucleic acids; Neutron diffraction from bio-macromolecules at JAERI

Niimura, Nobuo; Arai, Shigeki; Kurihara, Kazuo; Chatake, Toshiyuki*; Tanaka, Ichiro*; Bau, R.*

Hydrogen- and Hydration-Sensitive Structural Biology, p.17 - 35, 2005/00

At the JAERI, we have constructed several high-resolution neutron diffractometers dedicated to biological macromolecules (called BIX-type diffractometers), which use a monochromatized neutron beam and a neutron imaging plate detector. In this paper, we review several interesting results regarding hydrogen positions and hydration in proteins, obtained using the two BIX-type diffractometers in JAERI. The general subject of neutron protein crystallography has been reviewed by several authors, and several selected topics have been discussed.

Journal Articles

A Neutron crystallographic analysis of a rubredoxin mutant at 1.6 ${AA}$ resolution

Chatake, Toshiyuki*; Kurihara, Kazuo; Tanaka, Ichiro*; Tsyba, I.*; Bau, R.*; Jenney, F. E. Jr.*; Adams, M. W. W.*; Niimura, Nobuo

Acta Crystallographica Section D, 60(8), p.1364 - 1373, 2004/08

 Times Cited Count:34 Percentile:88.04(Biochemical Research Methods)

A neutron diffraction study has been carried out at 1.6 ${AA}$ resolution on a mutant rubredoxin from ${it Pyrococcus furiosus}$ using the BIX-3 single-crystal diffractometer at the JRR-3 reactor of JAERI. In order to study the unusual thermostability of rubredoxin from ${it P. furiosus}$, the hydrogen-bonding patterns were compared between the native and a 'triple-mutant' variant where three residues were changed so that they are identical to those in a mesophilic rubredoxin. In the present study, some minor changes were found between the wild-type and mutant proteins in the hydrogen-bonding patterns of the Trp3/Tyr3 region. The H/D-exchange ratios in the protein were also studied. The results suggest that the backbone amide bonds near the four Cys residues of the FeS$$_{4}$$ redox center are most resistant to H/D exchange. In addition, the 1.6 ${AA}$ resolution of the present neutron structure determination has revealed a more detailed picture than previously available of some portions of the water structure, including ordered and disordered O-D bonds.

Journal Articles

Neutron crystallographic study on rubredoxin from ${it Pyrococcus furiosus}$ by BIX-3, a single-crystal diffractometer for biomacromolecules

Kurihara, Kazuo; Tanaka, Ichiro*; Chatake, Toshiyuki*; Adams, M. W. W.*; Jenney, F. E. Jr.*; Moiseeva, N.*; Bau, R.*; Niimura, Nobuo

Proceedings of the National Academy of Sciences of the United States of America, 101(31), p.11215 - 11220, 2004/08

 Times Cited Count:52 Percentile:62.17(Multidisciplinary Sciences)

The structure of a rubredoxin (Rd) from ${it Pyrococcus furiosus}$, an organism that grows optimally at 100 $$^{circ}$$C, was determined using the neutron single-crystal diffractometer for biological macromolecules (BIX-3) at the JRR-3 reactor of JAERI. Data were collected at room temperature up to a resolution of 1.5 ${AA}$, and the completeness of the data set was 81.9 %. The model contains 306 H atoms and 50 D atoms. A total of 37 hydration water molecules were identified. The model has been refined to final agreement factors of ${it R}$ = 18.6 % and ${it R}$$$_{free}$$ = 21.7 %. Several orientations of the O-D bonds of side chains, whose assignments from X-ray data were previously ambiguous, were clearly visible in the neutron structure. While most backbone N-H bonds had undergone some degree of H/D exchange throughout the molecule, five H atom positions still had distinctly negative (H) peaks. The neutron Fourier maps clearly showed the details of an extensive set of H bonds involving the ND$$_{3}$$$$^{+}$$ terminus that may contribute to the unusual thermostability of this molecule.

Journal Articles

Hydrogen and hydration in proteins

Niimura, Nobuo; Chatake, Toshiyuki; Kurihara, Kazuo; Maeda, Mitsuru

Cell Biochemistry and Biophysics, 40(3), p.351 - 369, 2004/06

 Times Cited Count:24 Percentile:24.51(Biochemistry & Molecular Biology)

Neutron diffraction provides an experimental method of directly locating hydrogen atoms in proteins. High resolution neutron diffractometers dedicated to biological macromolecules (BIX-type diffractometer) have been constructed at the Japan Atomic Energy Research Institute (JAERI) and they have been used in the 1.5 AA -resolution crystal structure analyses of several proteins.

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