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Journal Articles

Birchite Cd$$_{2}$$Cu$$_{2}$$(PO$$_{4}$$)$$_{2}$$SO$$_{4}$$ $$cdot$$ 5H$$_{2}$$O as a model antiferromagnetic spin-1/2 Heisenberg $${it J}$$$$_{1}$$-$${it J}$$$$_{2}$$ chain

Fujihara, Masayoshi; Jeschke, H. O.*; Morita, Katsuhiro*; Kuwai, Tomohiko*; Koda, Akihiro*; Okabe, Hirotaka*; Matsuo, Akira*; Kindo, Koichi*; Mitsuda, Setsuo*

Physical Review Materials (Internet), 6(11), p.114408_1 - 114408_8, 2022/11

https://doi.org/10.1103/PhysRevMaterials.6.114408
 Times Cited Count：2 Percentile：12.90(Materials Science, Multidisciplinary)

$${it S}$$ = 1/2 Heisenberg $${it J}$$$$_{1}$$-$${it J}$$$$_{2}$$ chain antiferromagnets have been investigated extensively due to their exotic magnetic states. Here, we report the magnetic behavior of birchite Cd$$_{2}$$Cu$$_{2}$$(PO$$_{4}$$)$$_{2}$$SO$$_{4}$$$$cdot$$5H$$_{2}$$O and its effective spin model. Experimental studies by magnetic susceptibility, magnetization, heat capacity, and $$mu$$SR measurements indicate the absence of long-range order down to 0.4 K. Theoretical studies reveal that birchite is a model compound for the $${it J}$$$$_{1}$$-$${it J}$$$$_{2}$$ antiferromagnetic chain: the intrachain interactions $${it J}$$$$_{1}$$ and $${it J}$$$$_{2}$$ are antiferromagnetic and their magnitude is about 100 times larger than the interchain interactions. The magnitude of $${it J}$$$$_{2}$$ is two to three times larger than that of $${it J}$$$$_{1}$$, thus the spin gap is expected to be only a few percent of that of $${it J}$$$$_{1}$$. The temperature dependence of the specific heat shows a broad peak at about 1 K ($$simeq$$ 0.036 $${it J}$$$$_{1}$$), which suggests the presence of a spin gap.

Journal Articles

Gapless spin liquid in a square-kagome lattice antiferromagnet

Fujihara, Masayoshi*; Morita, Katsuhiro*; Mole, R.*; Mitsuda, Setsuo*; Toyama, Takami*; Yano, Shinichiro*; Yu, D.*; Sota, Shigetoshi*; Kuwai, Tomohiko*; Koda, Akihiro*; et al.

Nature Communications (Internet), 11, p.3429_1 - 3429_7, 2020/07

https://doi.org/10.1038/s41467-020-17235-z
 Times Cited Count：51 Percentile：92.31(Multidisciplinary Sciences)

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