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Journal Articles

Multipole polaron in the devil's staircase of CeSb

Arai, Yosuke*; Kuroda, Kenta*; Nomoto, Takuya*; Tin, Z. H.*; Sakuragi, Shunsuke*; Bareille, C.*; Akebi, Shuntaro*; Kurokawa, Kifu*; Kinoshita, Yuto*; Zhang, W.-L.*; et al.

Nature Materials, 21(4), p.410 - 415, 2022/04

Journal Articles

The Joint evaluated fission and fusion nuclear data library, JEFF-3.3

Plompen, A. J. M.*; Cabellos, O.*; De Saint Jean, C.*; Fleming, M.*; Algora, A.*; Angelone, M.*; Archier, P.*; Bauge, E.*; Bersillon, O.*; Blokhin, A.*; et al.

European Physical Journal A, 56(7), p.181_1 - 181_108, 2020/07

 Times Cited Count:73 Percentile:99.41(Physics, Nuclear)

The Joint Evaluated Fission and Fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu, on $$^{241}$$Am and $$^{23}$$Na, $$^{59}$$Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yileds, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 is excellent for a wide range of nuclear technology applications, in particular nuclear energy.

Journal Articles

Clades of huge phages from across Earth's ecosystems

Al-Shayeb, B.*; Sachdeva, R.*; Chen, L.-X.*; Ward, F.*; Munk, P.*; Devoto, A.*; Castelle, C. J.*; Olm, M. R.*; Bouma-Gregson, K.*; Amano, Yuki; et al.

Nature, 578(7795), p.425 - 431, 2020/02

 Times Cited Count:83 Percentile:99.63(Multidisciplinary Sciences)

Journal Articles

$$alpha$$-decay properties of $$^{200,202}$$Fr

Ghys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.

Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11

 Times Cited Count:9 Percentile:86.57(Physics, Nuclear)

Journal Articles

Investigation of the $$Delta$$$$n$$ = 0 selection rule in Gamow-Teller transitions; The $$beta$$-decay of $$^{207}$$Hg

Berry, T. A.*; Podoly$'a$k, Zs.*; Carroll, R. J.*; Lic$u{a}$, R.*; Grawe, H.*; Timofeyuk, N. K.*; Alexander, T.*; Andreyev, A. N.; Ansari, S.*; Borge, M. J. G.*; et al.

Physics Letters B, 793, p.271 - 275, 2019/06

 Times Cited Count:3 Percentile:52.47(Astronomy & Astrophysics)

Journal Articles

Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $$^{217,218,219}$$At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero$'n$, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

 Times Cited Count:5 Percentile:69.53(Physics, Nuclear)

Journal Articles

Colossal barocaloric effects in plastic crystals

Li, B.*; Kawakita, Yukinobu; Kawamura, Seiko; Sugahara, Takeshi*; Wang, H.*; Wang, J.*; Chen, Y.*; Kawaguchi, Saori*; Kawaguchi, Shogo*; Ohara, Koji*; et al.

Nature, 567(7749), p.506 - 510, 2019/03

 Times Cited Count:85 Percentile:99.22(Multidisciplinary Sciences)

Refrigeration is of vital importance for modern society for example, for food storage and air conditioning- and 25 to 30% of the world's electricity is consumed for refrigeration. Current refrigeration technology mostly involves the conventional vapour compression cycle, but the materials used in this technology are of growing environmental concern because of their large global warming potential. As a promising alternative, refrigeration technologies based on solid-state caloric effects have been attracting attention in recent decades. However, their application is restricted by the limited performance of current caloric materials, owing to small isothermal entropy changes and large driving magnetic fields. Here we report colossal barocaloric effects (CBCEs) (barocaloric effects are cooling effects of pressure-induced phase transitions) in a class of disordered solids called plastic crystals. The obtained entropy changes in a representative plastic crystal, neopentylglycol, are about 389 joules per kilogram per kelvin near room temperature. Pressure-dependent neutron scattering measurements reveal that CBCEs in plastic crystals can be attributed to the combination of extensive molecular orientational disorder, giant compressibility and highly anharmonic lattice dynamics of these materials. Our study establishes the microscopic mechanism of CBCEs in plastic crystals and paves the way to next-generation solid-state refrigeration technologies.

Journal Articles

Conceptual uncertainties in modelling the interaction between engineered and natural barriers of nuclear waste repositories in crystalline rocks

Finsterle, S.*; Lanyon, B.*; ${AA}$kesson, M.*; Baxter, S.*; Bergstr$"o$m, M.*; Bockg${aa}$rd, N.*; Dershowitz, W.*; Dessirier, B.*; Frampton, A.*; Fransson, ${AA}$.*; et al.

Geological Society, London, Special Publications, No.482, p.261 - 283, 2019/00

 Times Cited Count:3 Percentile:57.07

Nuclear waste disposal in geological formations relies on a multi-barrier concept that includes engineered components which in many cases includes a bentonite buffer surrounding waste packages and the host rock. An SKB's (Swedish Nuclear Fuel and Waste Management Co.) Modelling Task Force project facilitated to improve the overall understanding of rock - bentonite interactions, as 11 teams used different conceptualisations and modelling tools to analyse the in-situ experiment at the $"A$ps$"o$ Hard Rock Laboratory. The exercise helped identify conceptual uncertainties that led to different assessments of the relative importance of the engineered and natural barrier subsystems and of aspects that need to be better understood to arrive at reliable predictions of bentonite wetting.

Journal Articles

Primary radiation damage; A Review of current understanding and models

Nordlund, K.*; Zinkle, S. J.*; Sand, A. E.*; Granberg, F.*; Averback, R. S.*; Stoller, R. E.*; Suzudo, Tomoaki; Malerba, L.*; Banhart, F.*; Weber, W. J.*; et al.

Journal of Nuclear Materials, 512, p.450 - 479, 2018/12

 Times Cited Count:141 Percentile:99.04(Materials Science, Multidisciplinary)

Scientific understanding of any kind of radiation effects starts from the primary damage. We consider the extensive experimental and computer simulation studies that have been performed over the past several decades on what the nature of the primary damage is. We review both the production of crystallographic or topological defects in materials as well as radiation mixing, i.e. the process where atoms in perfect crystallographic positions exchange positions with other ones in non-defective positions. We also consider the recent effort to provide alternatives to the current international standard for quantifying this energetic particle damage, the Norgett-Robinson-Torrens displacements per atom (NRT-dpa) model for metals. We present in detail new complementary displacement production estimators ("athermal recombination corrected dpa": arc-dpa) and atomic mixing ("replacements per atom": rpa) functions that extend the NRT-dpa, and discuss their advantages and limitations.

Journal Articles

Improving atomic displacement and replacement calculations with physically realistic damage models

Nordlund, K.*; Zinkle, S. J.*; Sand, A. E.*; Granberg, F.*; Averback, R. S.*; Stoller, R.*; Suzudo, Tomoaki; Malerba, L.*; Banhart, F.*; Weber, W. J.*; et al.

Nature Communications (Internet), 9, p.1084_1 - 1084_8, 2018/03

 Times Cited Count:117 Percentile:98.72(Multidisciplinary Sciences)

Atomic collision processes are fundamental to numerous advanced materials technologies such as electron microscopy, semiconductor processing and nuclear power generation. Experimental and computer simulation studies over the past several decades provide the physical basis for understanding the atomic-scale processes occurring during primary displacement events. The current international standard for quantifying this particle damage, the Norgett-Robinson-Torrens displacements per atom (NRT-dpa) model, has nowadays several well-known limitations. In particular, the number of radiation defects produced in energetic cascades in metals is only $$sim$$1/3 the NRT-dpa prediction, while the number of atoms involved in atomic mixing is about a factor of 30 larger than the dpa value. Here we propose two new complementary displacement production estimators.

Journal Articles

CIELO collaboration summary results; International evaluations of neutron reactions on uranium, plutonium, iron, oxygen and hydrogen

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Kahler, A. C.*; Talou, P.*; Plompen, A. J.*; Schillebeeckx, P.*; et al.

Nuclear Data Sheets, 148, p.189 - 213, 2018/02

 Times Cited Count:49 Percentile:98.76(Physics, Nuclear)

The CIELO collaboration has studied neutron cross sections on nuclides that significantly impact criticality in nuclear facilities - $$^{235}$$U, $$^{238}$$U, $$^{239}$$Pu, $$^{56}$$Fe, $$^{16}$$O and $$^{1}$$H - with the aim of improving the accuracy of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project, coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with support also from the IAEA, has motivated experimental and theoretical work and led to suites of new evaluated libraries that accurately reflect measured data and also perform well in integral simulations of criticality. This report summarizes our results and outlines plans for the next phase of this collaboration.

Journal Articles

EXILL; A High-efficiency, high-resolution setup for $$gamma$$-spectroscopy at an intense cold neutron beam facility

Jentschel, M.*; Blanc, A.*; de France, G.*; K$"o$ster, U.*; Leoni, S.*; Mutti, P.*; Simpson, G.*; Soldner, T.*; Ur, C.*; Urban, W.*; et al.

Journal of Instrumentation (Internet), 12(11), p.P11003_1 - P11003_33, 2017/11

 Times Cited Count:27 Percentile:86.8(Instruments & Instrumentation)

Journal Articles

The CIELO collaboration; Progress in international evaluations of neutron reactions on Oxygen, Iron, Uranium and Plutonium

Chadwick, M. B.*; Capote, R.*; Trkov, A.*; Kahler, A. C.*; Herman, M. W.*; Brown, D. A.*; Hale, G. M.*; Pigni, M.*; Dunn, M.*; Leal, L.*; et al.

EPJ Web of Conferences, 146, p.02001_1 - 02001_9, 2017/09

 Times Cited Count:6 Percentile:97.85

The CIELO collaboration has studied neutron cross sections on nuclides ($$^{16}$$O, $$^{56}$$Fe, $$^{235,238}$$U and $$^{239}$$Pu) that significantly impact criticality in nuclear technologies with the aim of improving the accuracy of the data and resolving previous discrepancies in our understanding. This multi-laboratory pilot project, coordinated via the OECD/NEA Working Party on Evaluation Cooperation (WPEC) Subgroup 40 with support also from the IAEA, has motivated experimental and theoretical work and led to suites of new evaluated libraries that accurately reflect measured data and also perform well in integral simulations of criticality.

Journal Articles

Ground-state configuration of neutron-rich $$^{35}$$Al via Coulomb breakup

Chakraborty, S.*; Datta, U.*; Aumann, T.*; Beceiro-Novo, S.*; Boretzky, K.*; Caesar, C.*; Carlson, B. V.*; Catford, W. N.*; Chartier, M.*; Cortina-Gil, D.*; et al.

Physical Review C, 96(3), p.034301_1 - 034301_9, 2017/09

 Times Cited Count:2 Percentile:14.2(Physics, Nuclear)

no abstracts in English

Journal Articles

Spontaneous decays of magneto-elastic excitations in non-collinear antiferromagnet (Y,Lu)MnO$$_{3}$$

Oh, J.*; Le, M. D.*; Nahm, H.-H.*; Sim, H.*; Jeong, J.*; Perring, T. G.*; Woo, H.*; Nakajima, Kenji; Kawamura, Seiko; Yamani, Z.*; et al.

Nature Communications (Internet), 7, p.13146_1 - 13146_6, 2016/10

 Times Cited Count:38 Percentile:85.96(Multidisciplinary Sciences)

Magnons and phonons are fundamental quasiparticles in a solid and can be coupled together to form a hybrid quasi-particle. However, detailed experimental studies on the underlying Hamiltonian of this particle are rare for actual materials. Moreover, the anharmonicity of such magnetoelastic excitations remains largely unexplored, although it is essential for a proper understanding of their diverse thermodynamic behaviour and intrinsic zero-temperature decay. Here we show that in non-collinear antiferromagnets, a strong magnon phonon coupling can significantly enhance the anharmonicity, resulting in the creation of magnetoelastic excitations and their spontaneous decay. By measuring the spin waves over the full Brillouin zone and carrying out anharmonic spin wave calculations using a Hamiltonian with an explicit magnon phonon coupling, we have identified a hybrid magnetoelastic mode in (Y,Lu)MnO$$_{3}$$ and quantified its decay rate and the exchange-striction coupling termrequired to produce it.

Journal Articles

Spin excitations in optimally P-doped BaFe$$_2$$(As$$_{0.7}$$P$$_{0.3}$$)$$_2$$ superconductor

Hu, D.*; Yin, Z.*; Zhang, W.*; Ewings, R. A.*; Ikeuchi, Kazuhiko*; Nakamura, Mitsutaka; Roessli, B.*; Wei, Y.*; Zhao, L.*; Chen, G.*; et al.

Physical Review B, 94(9), p.094504_1 - 094504_7, 2016/09

AA2016-0252.pdf:2.18MB

 Times Cited Count:14 Percentile:64.66(Materials Science, Multidisciplinary)

The temperature and energy dependence of spin excitations in an optimally P-doped BaFe$$_2$$(As$$_{0.7}$$P$$_{0.3}$$)$$_2$$ superconductor (T$$_c$$ = 30 K) were studied by using inelastic neutron scattering. Experimental results are consistent with calculations from a combined density functional theory and dynamical mean field theory, and suggest that the decreased average pnictogen height in BaFe$$_2$$(As$$_{0.7}$$P$$_{0.3}$$)$$_2$$ reduces the strength of electron correlations and increases the effective bandwidth of magnetic excitation.

Journal Articles

$$beta$$-delayed fission and $$alpha$$ decay of $$^{196}$$At

Truesdale, V. L.*; Andreyev, A. N.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.

Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09

 Times Cited Count:9 Percentile:65.08(Physics, Nuclear)

Journal Articles

A New view of the tree of life

Hug, L. A.*; Baker, B. J.*; Anantharaman, K.*; Brown, C. T.*; Probst, A. J.*; Castelle, C. J.*; Butterfield, C. N.*; Hernsdorf, A. W.*; Amano, Yuki; Ise, Kotaro; et al.

Nature Microbiology (Internet), 1(5), p.16048_1 - 16048_6, 2016/05

 Times Cited Count:842 Percentile:99.98(Microbiology)

The tree of life is one of the most important organizing principles in biology. Gene surveys suggest the existence of an enormous number of branches, but even an approximation of the full scale of The Tree has remained elusive. Here, we use newly available information from genomes of uncultivated organisms, along with other published sequences, to present a new version of the Tree of life, with Bacteria, Archaea and Eukaryotes included. The depiction is both a global overview and a snapshot of the diversity within each major lineage. The results imply the predominance of bacterial diversification and underline the importance of organisms lacking isolated representatives, with substantial evolution concentrated in a major radiation of such organisms.

Journal Articles

Fast-timing study of the $$l$$-forbidden 1/2$$^+$$ $$rightarrow$$ 3/2$$^+$$ $$M1$$ transition in $$^{129}$$Sn

Lic$u{a}$, R.*; Mach, H.*; Fraile, L. M.*; Gargano, A.*; Borge, M. J. G.*; M$u{a}$rginean, N.*; Sotty, C. O.*; Vedia, V.*; Andreyev, A. N.; Benzoni, G.*; et al.

Physical Review C, 93(4), p.044303_1 - 044303_7, 2016/04

 Times Cited Count:5 Percentile:46.38(Physics, Nuclear)

Journal Articles

Montane ecosystem productivity responds more to global circulation patterns than climatic trends

Desai, A. R.*; Wohlfahrt, G.*; Zeeman, M. J.*; Katata, Genki; Eugster, W.*; Montagnani, L.*; Gianelle, D.*; Mauder, M.*; Schmid, H. P.*

Environmental Research Letters, 11(2), p.024013_1 - 024013_9, 2016/02

AA2015-0882.pdf:2.25MB

 Times Cited Count:16 Percentile:62.07(Environmental Sciences)

Regional ecosystem productivity is highly sensitive to inter-annual climate variability, both within and outside the primary carbon uptake period. However, Earth system models lack sufficient spatial scales and ecosystem processes to resolve how these processes may change in a warming climate. Here, we show, how for the European Alps, mid-latitude Atlantic ocean winter circulation anomalies drive high-altitude summer forest and grassland productivity, through feedbacks among orographic wind circulation patterns, snowfall, winter and spring temperatures, and vegetation activity. Therefore, to understand future global climate change influence to regional ecosystem productivity, Earth systems models need to focus on improvements towards topographic downscaling of changes in regional atmospheric circulation patterns and to lagged responses in vegetation dynamics to non-growing season climate anomalies.

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