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Journal Articles

Synthesis of high-entropy hydride from the cantor alloy (fcc-CoCrFeNiMn) at extreme conditions

Glazyrin, K.*; Spektor, K.*; Bykov, M.*; Carvalho, P. H. B.*; Dong, W.*; K$"o$rmann, F.*; Sano, Asami; Hattori, Takanori; Beyer, D. C.*; Sahlberg, M.*; et al.

Nature Communications (Internet), 17, p.2622_1 - 2622_10, 2026/03

 Times Cited Count:3 Percentile:92.69(Multidisciplinary Sciences)

Studies of high entropy materials contribute to various fields of science and reveal ever more exciting properties of applied interest. Here, we perform a study of the resistance of a Cantor alloy (CoCrFeNiMn) to hydrogen through high-pressure experiments at elevated temperatures by X-ray and neutron time-of-flight experiments and ab initio calculations. We report formation of an fcc hydride based on the Cantor alloy composition. We also provide its characterization, including an estimate of hydrogen content. These findings contribute to the growing body of knowledge on the complex chemistry of high-entropy alloys and high-entropy-hydrides.

Journal Articles

L$"u$ders band-assisted high uniform ductility in ultrastrong ferrous medium-entropy alloy via hierarchical microstructure

Kwon, H.*; Lee, J. H.*; Zargaran, A.*; Harjo, S.; Gong, W.; Wang, J.*; Gu, G. H.*; Lee, B.-J.*; Bae, J. W.*; Kim, H. S.*

International Journal of Plasticity, 190, p.104378_1 - 104378_18, 2025/07

 Times Cited Count:19 Percentile:96.51(Engineering, Mechanical)

Journal Articles

Uncertainty quantification for severe-accident reactor modelling; Results and conclusions of the MUSA reactor applications work package

Brumm, S.*; Gabrielli, F.*; Sanchez Espinoza, V.*; Stakhanova, A.*; Groudev, P.*; Petrova, P.*; Vryashkova, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; et al.

Annals of Nuclear Energy, 211, p.110962_1 - 110962_16, 2025/02

 Times Cited Count:17 Percentile:96.20(Nuclear Science & Technology)

Journal Articles

In-situ measurement of radiation driven back-conversion from para to ortho liquid hydrogen state in cold moderators at J-PARC

Teshigawara, Makoto; Lee, Y.*; Tatsumoto, Hideki*; Hartl, M.*; Aso, Tomokazu; Iverson, E. B.*; Ariyoshi, Gen; Ikeda, Yujiro*; Hasegawa, Takumi*

Nuclear Instruments and Methods in Physics Research B, 557, p.165534_1 - 165534_10, 2024/12

 Times Cited Count:1 Percentile:20.23(Instruments & Instrumentation)

At Japanese Spallation Neutron Source in J-PARC, the para-hydrogen fraction was measured by using Raman spectroscopy in-situ for an integrated beam power of 9.4 MW$$cdot$$h at 1 MW operation, to evaluate the functionality of the ferric oxyhydroxide catalyst. This result showed that full functionality of the catalyst was retained up to the 1 MW operation. We attempted to study the effect of neutron scattering driven para to ortho-hydrogen back-conversion rate in the absence of the catalyst effect with a bypass line without catalyst. The measured increase of ortho-hydrogen fraction was 0.44% for an integrated beam power of 2.4 MW$$cdot$$h at 500 kW operation, however, which was considered to be due to not only to neutron collisions in cold moderators but also to the high ortho-hydrogen fraction of initially static liquid hydrogen in the bypass line and passive exudation of quasi-static hydrogen in the catalyst vessel to the main loop.

Journal Articles

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

 Times Cited Count:6 Percentile:74.40(Physics, Nuclear)

no abstracts in English

Journal Articles

Quantum critical behavior of the hyperkagome magnet Mn$$_3$$CoSi

Yamauchi, Hiroki; Sari, D. P.*; Yasui, Yukio*; Sakakura, Terutoshi*; Kimura, Hiroyuki*; Nakao, Akiko*; Ohara, Takashi; Honda, Takashi*; Kodama, Katsuaki; Igawa, Naoki; et al.

Physical Review Research (Internet), 6(1), p.013144_1 - 013144_9, 2024/02

Journal Articles

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

 Times Cited Count:23 Percentile:94.60(Astronomy & Astrophysics)

Gamma decays were observed in $$^{56}$$Ca and $$^{58}$$Ca following quasi-free one-proton knockout reactions from $$^{57,59}$$Sc. For $$^{56}$$Ca, a $$gamma$$ ray transition was measured to be 1456(12) keV, while for $$^{58}$$Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the $$2^{+}_{1} rightarrow 0^{+}_{gs}$$ decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for $$2^{+}_{1}$$ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the $$0_{f5/2}$$ and $$0_{g9/2}$$ orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic $$^{60}$$Ca and potentially drives the dripline of Ca isotopes to $$^{70}$$Ca or even beyond.

Journal Articles

High-density nanoprecipitates and phase reversion via maraging enable ultrastrong yet strain-hardenable medium-entropy alloy

Kwon, H.*; Sathiyamoorthi, P.*; Gangaraju, M. K.*; Zargaran, A.*; Wang, J.*; Heo, Y.-U.*; Harjo, S.; Gong, W.; Lee, B.-J.*; Kim, H. S.*

Acta Materialia, 248, p.118810_1 - 118810_12, 2023/04

 Times Cited Count:71 Percentile:98.84(Materials Science, Multidisciplinary)

Journal Articles

Pressure-modulated magnetism and negative thermal expansion in the Ho$$_2$$Fe$$_{17}$$ intermetallic compound

Cao, Y.*; Zhou, H.*; Khmelevskyi, S.*; Lin, K.*; Avdeev, M.*; Wang, C.-W.*; Wang, B.*; Hu, F.*; Kato, Kenichi*; Hattori, Takanori; et al.

Chemistry of Materials, 35(8), p.3249 - 3255, 2023/04

 Times Cited Count:9 Percentile:46.48(Chemistry, Physical)

Hydrostatic and chemical pressure are efficient stimuli to alter the crystal structure and are commonly used for tuning electronic and magnetic properties in materials science. However, chemical pressure is difficult to quantify and a clear correspondence between these two types of pressure is still lacking. Here, we study intermetallic candidates for a permanent magnet with a negative thermal expansion (NTE). Based on in situ synchrotron X-ray diffraction, negative chemical pressure is revealed in Ho$$_2$$Fe$$_{17}$$ on Al doping and quantitatively evaluated by using temperature and pressure dependence of unit cell volume. A combination of magnetization and neutron diffraction measurements also allowed one to compare the effect of chemical pressure on magnetic ordering with that of hydrostatic pressure. Intriguingly, pressure can be used to control suppression and enhancement of NTE. Electronic structure calculations indicate that pressure affected the top of the majority band with respect to the Fermi level, which has implications for the magnetic stability, which in turn plays a critical role in modulating magnetism and NTE. This work presents a good example of understanding the effect of pressure and utilizing it to control properties of functional materials.

Journal Articles

Multiple mechanisms in proton-induced nucleon removal at $$sim$$100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G$'o$mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

 Times Cited Count:20 Percentile:86.69(Physics, Multidisciplinary)

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient $$^{14}$$O nucleus with large Fermi-surface asymmetry at $$sim$$100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.

Journal Articles

Competitive strengthening between dislocation slip and twinning in cast-wrought and additively manufactured CrCoNi medium entropy alloys

Woo, W.*; Kim, Y. S.*; Chae, H. B.*; Lee, S. Y.*; Jeong, J. S.*; Lee, C. M.*; Won, J. W.*; Na, Y. S.*; Kawasaki, Takuro; Harjo, S.; et al.

Acta Materialia, 246, p.118699_1 - 118699_13, 2023/03

 Times Cited Count:84 Percentile:99.21(Materials Science, Multidisciplinary)

Journal Articles

Si-addition contributes to overcoming the strength-ductility trade-off in high-entropy alloys

Wei, D.*; Gong, W.; Tsuru, Tomohito; Lobzenko, I.; Li, X.*; Harjo, S.; Kawasaki, Takuro; Do, H.-S.*; Bae, J. W.*; Wagner, C.*; et al.

International Journal of Plasticity, 159, p.103443_1 - 103443_18, 2022/12

 Times Cited Count:167 Percentile:99.81(Engineering, Mechanical)

Journal Articles

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; Yoshida, Kazuki; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

 Times Cited Count:6 Percentile:53.58(Physics, Nuclear)

The low-lying level structure of $$^{59}$$V and $$^{61}$$V was investigated for the first time. The neutron knockout reaction and inelastic proton scattering were applied for $$^{61}$$V while the neutron knock-out reaction provided the data for $$^{59}$$V. Four and five new transitions were determined for $$^{59}$$V and $$^{61}$$V, respectively. Based on the comparison to our shell-model calculations using the Lenzi-Nowacki-Poves-Sieja (LNPS) interaction, three of the observed $$gamma$$ rays for each isotope could be placed in the level scheme and assigned to the decay of the first 11/2$$^{-}$$ and 9/2$$^{-}$$ levels. The ($$p$$,$$p'$$) excitation cross sections for $$^{61}$$V were analyzed by the coupled-channels formalism assuming quadrupole plus hexadecapole deformations. Due to the role of the hexadecapole deformation, $$^{61}$$V could not be unambiguously placed on the island of inversion.

Journal Articles

Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

 Times Cited Count:31 Percentile:88.62(Physics, Multidisciplinary)

The one-neutron knockout from $$^{52}$$Ca was performed at $$sim$$230 MeV/nucleon combined with prompt $$gamma$$ spectroscopy. The momentum distributions corresponding to the removal of $$1f_{7/2}$$ and $$2p_{3/2}$$ neutrons were measured. The cross sections are consistent with a shell closure at the neutron number $$N = 32$$, found as strong as at $$N = 28$$ and $$N = 34$$ in Ca isotopes from the same observables. The analysis of the momentum distributions leads to a difference of the root-mean-square radii of the neutron $$1_{f7/2}$$ and $$2p_{3/2}$$ orbitals of 0.61(23) fm, in agreement with the modified-shell-model prediction of 0.7 fm suggesting that the large root-mean-square radius of the $$2p_{3/2}$$ orbital in neutron-rich Ca isotopes is responsible for the unexpected linear increase of the charge radius with the neutron number.

Journal Articles

Urban Working Groups in the IAEA's model testing programmes; Overview from the MODARIA I and MODARIA II programmes

Thiessen, K. M.*; Boznar, M. Z.*; Charnock, T. W.*; Chouhan, S. L.*; Federspiel, L.*; Gra$v{s}$i$v{c}$, B.*; Grsic, Z.*; Helebrant, J.*; Hettrich, S.*; Hulka, J.*; et al.

Journal of Radiological Protection, 42(2), p.020502_1 - 020502_8, 2022/06

 Times Cited Count:5 Percentile:45.73(Environmental Sciences)

Journal Articles

Status of the uncertainty quantification for severe accident sequences of different NPP-designs in the frame of the H-2020 project MUSA

Brumm, S.*; Gabrielli, F.*; Sanchez-Espinoza, V.*; Groudev, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; Bocanegra, R.*; Herranz, L. E.*; Berda$"i$, M.*; et al.

Proceedings of 10th European Review Meeting on Severe Accident Research (ERMSAR 2022) (Internet), 13 Pages, 2022/05

Journal Articles

A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

Koiwai, Takuma*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; Miyagi, Takayuki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

AA2021-0775.pdf:0.62MB

 Times Cited Count:13 Percentile:78.71(Astronomy & Astrophysics)

no abstracts in English

Journal Articles

Delayed gamma-ray spectroscopy for high-radioactivity mixed nuclear material safeguards verification

Rodriguez, D. C.; Abbas, K.*; Koizumi, Mitsuo; Lee, H.-J.; Nonneman, S.*; Oberstedt, S.*; Pedersen, B.*; Rossi, F.; Schillebeeckx, P.*; Takahashi, Tone

Dai-42-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2021/11

Journal Articles

Investigation of the ground-state spin inversion in the neutron-rich $$^{47,49}$$Cl isotopes

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G$'o$mez-Ramos, M.*; et al.

Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10

AA2021-0468.pdf:1.29MB

 Times Cited Count:15 Percentile:74.30(Physics, Nuclear)

no abstracts in English

Journal Articles

Developing delayed gamma-ray spectroscopy for reprocessing plant nuclear safeguards; Fissile nuclide content analysis

Rodriguez, D. C.; Abbas, K.*; Koizumi, Mitsuo; Lee, H.-J.; Nonneman, S.*; Pedersen, B.*; Rossi, F.; Takahashi, Tone

Proceedings of 2021 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC) (Internet), 3 Pages, 2021/10

99 (Records 1-20 displayed on this page)