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Journal Articles

Investigation of the ground-state spin inversion in the neutron-rich $$^{47,49}$$Cl isotopes

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G$'o$mez-Ramos, M.*; et al.

Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10

no abstracts in English

Journal Articles

Pairing forces govern population of doubly magic $$^{54}$$Ca from direct reactions

Browne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Ogata, Kazuyuki*; Utsuno, Yutaka; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; Calvet, D.*; et al.

Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Direct proton-knockout reactions of $$^{55}$$Sc were studied at the RIKEN Radioactive Isotope Beam Factory. Populated states of $$^{54}$$Ca were investigated through $$gamma$$-ray and invariant-mass spectroscopy. Level energies were calculated from the nuclear shell model employing a phenomenological inter-nucleon interaction. Theoretical cross sections to states were calculated from distorted-wave impulse approximation estimates multiplied by the shell model spectroscopic factors. Despite the calculations showing a significant amplitude of excited neutron configurations in the ground-state of $$^{55}$$Sc, valence proton removals populated predominantly the ground-state of $$^{54}$$Ca. This counter-intuitive result is attributed to pairing effects leading to a dominance of the ground-state spectroscopic factor. Owing to the ubiquity of the pairing interaction, this argument should be generally applicable to direct knockout reactions from odd-even to even-even nuclei.

Journal Articles

Programmable synthesis of silver wheels

Kwon, H.*; Pietrasiak, E.*; Ohara, Takashi; Nakao, Akiko*; Chae, B.*; Hwang, C.-C.*; Jung, D.*; Hwang, I.-C.*; Ko, Y. H.*; Kim, K.*; et al.

Inorganic Chemistry, 60(9), p.6403 - 6409, 2021/05

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

Journal Articles

First spectroscopic study of $$^{51}$$Ar by the ($$p$$,2$$p$$) reaction

Juh$'a$sz, M. M.*; Elekes, Z.*; Sohler, D.*; Utsuno, Yutaka; Yoshida, Kazuki; Otsuka, Takaharu*; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Baba, Hidetada*; et al.

Physics Letters B, 814, p.136108_1 - 136108_8, 2021/03

 Times Cited Count:1 Percentile:74.98(Astronomy & Astrophysics)

The nuclear structure of $$^{51}$$Ar was studied by the ($$p$$,2$$p$$) reaction using $$gamma$$-ray spectroscopy for the bound and unbound states. Comparing the results to our shell-model calculations, two bound and six unbound states were established. The low cross sections populating the two bound states of $$^{51}$$Ar could be interpreted as a clear signature for the presence of significant sub-shell closures at neutron numbers 32 and 34 in argon isotopes.

Journal Articles

Enhancement of fatigue resistance by overload-induced deformation twinning in a CoCrFeMnNi high-entropy alloy

Lam, T.-N.*; Lee, S. Y.*; Tsou, N.-T.*; Chou, H.-S.*; Lai, B.-H.*; Chang, Y.-J.*; Feng, R.*; Kawasaki, Takuro; Harjo, S.; Liaw, P. K.*; et al.

Acta Materialia, 201, p.412 - 424, 2020/12

 Times Cited Count:13 Percentile:92.23(Materials Science, Multidisciplinary)

Journal Articles

Review of Fukushima Daiichi Nuclear Power Station debris endstate location in OECD/NEA preparatory study on analysis of fuel debris (PreADES) project

Nakayoshi, Akira; Rempe, J. L.*; Barrachin, M.*; Bottomley, D.; Jacquemain, D.*; Journeau, C.*; Krasnov, V.; Lind, T.*; Lee, R.*; Marksberry, D.*; et al.

Nuclear Engineering and Design, 369, p.110857_1 - 110857_15, 2020/12

 Times Cited Count:0 Percentile:0.33(Nuclear Science & Technology)

Much is still not known about the end-state of core materials in each of the units at Fukushima Daiichi Nuclear Power Station (Daiichi) that were operating on March 11, 2011. The Nuclear Energy Agency of the Organization for Economic Development has launched the Preparatory Study on Analysis of Fuel Debris (PreADES) project as a first step to reduce some of these uncertainties. As part of the PreADES Task 1, relevant information was reviewed to confirm the accuracy of graphical depictions of the debris endstates at the damaged Daiichi units, which provides a basis for suggesting future debris examinations. Two activities have been completed within the PreADES Task 1. First, relevant knowledge from severe accidents at the Three Mile Island Unit 2 and the Chernobyl Nuclear Power Plant Unit 4 was reviewed, along with results from prototypic tests and hot cell examinations, to glean insights that may inform future decommissioning activities at Daiichi. Second, the current debris endstate diagrams for the damaged reactors at Daiichi were reviewed to confirm that they incorporate relevant knowledge from plant observations and from severe accident code analyses of the BSAF (Benchmark Study of the Accident at Daiichi Nuclear Power Station) 1 and 2 projects. This paper highlights Task 1 insights, which have the potential to not only inform future Decontamination and Decommissioning activities at Daiichi, but also provide important perspectives for severe accident analyses and management, particularly regarding the long term management of a damaged nuclear site following a severe accident.

Journal Articles

$$N$$ = 32 shell closure below calcium; Low-lying structure of $$^{50}$$Ar

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Men$'e$ndez, J.*; Ogata, Kazuyuki*; Schwenk, A.*; Shimizu, Noritaka*; Simonis, J.*; et al.

Physical Review C, 102(6), p.064320_1 - 064320_9, 2020/12

 Times Cited Count:1 Percentile:35.83(Physics, Nuclear)

Low-lying excited states in the $$N$$ = 32 isotope $$^{50}$$Ar were investigated by in-beam $$gamma$$-ray spectroscopy following proton- and neutron-knockout, multinucleon removal, and proton inelastic scattering at the RIKEN Radioactive Isotope Beam Factory. The energies of the two previously reported transitions have been confirmed, and five additional states are presented for the first time, including a candidate for a 3$$^{-}$$ state. The level scheme built using $$gamma$$ $$gamma$$ coincidences was compared to shell-model calculations in the $$sd-pf$$ model space and to ${it ab initio}$ predictions based on chiral two- and three-nucleon interactions. Theoretical proton- and neutron-knockout cross sections suggest that two of the new transitions correspond to 2$$^{+}$$ states, while the previously proposed 4$$^{+}_{1}$$ state could also correspond to a 2$$^{+}$$ state.

Journal Articles

Dosimetric impact of a new computational voxel phantom series for the Japanese atomic bomb survivors; Methodological improvements and organ dose response functions

Sato, Tatsuhiko; Funamoto, Sachiyo*; Paulbeck, C.*; Griffin, K.*; Lee, C.*; Cullings, H.*; Egbert, S. D.*; Endo, Akira; Hertel, N.*; Bolch, W. E.*

Radiation Research, 194(4), p.390 - 402, 2020/10

 Times Cited Count:2 Percentile:0.01(Biology)

Owing to recent advances in computational dosimetry tools, it is desirable to update the dosimetry system for the atomic-bomb survivors as it was established by DS02. In the current study, we have investigated the possible impact of introducing not only the J45 phantom series but also various methodological upgrades to the DS02 dosimetry system. It was found that the anatomical improvement in the J45 phantom series is the most important factor leading to potential changes in survivor organ doses. In addition, this study established a series of response functions which allows for the rapid conversion of the unidirectional quasi-monoenergetic photon and neutron fluences to organ doses within the J45 adult phantoms. This system of response functions can be implemented within a revision to the DS02 dosimetry system and used for future updates to organ doses within the Life Span Study of the atomic-bomb survivors.

Journal Articles

The Joint evaluated fission and fusion nuclear data library, JEFF-3.3

Plompen, A. J. M.*; Cabellos, O.*; De Saint Jean, C.*; Fleming, M.*; Algora, A.*; Angelone, M.*; Archier, P.*; Bauge, E.*; Bersillon, O.*; Blokhin, A.*; et al.

European Physical Journal A, 56(7), p.181_1 - 181_108, 2020/07

 Times Cited Count:73 Percentile:99.41(Physics, Nuclear)

The Joint Evaluated Fission and Fusion nuclear data library 3.3 is described. New evaluations for neutron-induced interactions with the major actinides $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu, on $$^{241}$$Am and $$^{23}$$Na, $$^{59}$$Ni, Cr, Cu, Zr, Cd, Hf, W, Au, Pb and Bi are presented. It includes new fission yileds, prompt fission neutron spectra and average number of neutrons per fission. In addition, new data for radioactive decay, thermal neutron scattering, gamma-ray emission, neutron activation, delayed neutrons and displacement damage are presented. JEFF-3.3 was complemented by files from the TENDL project. The libraries for photon, proton, deuteron, triton, helion and alpha-particle induced reactions are from TENDL-2017. The demands for uncertainty quantification in modeling led to many new covariance data. A comparison between results from model calculations using the JEFF-3.3 library and those from benchmark experiments for criticality, delayed neutron yields, shielding and decay heat, reveals that JEFF-3.3 is excellent for a wide range of nuclear technology applications, in particular nuclear energy.

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri. A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:9 Percentile:88.96(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

Journal Articles

Comparison of dislocation density, twin fault probability, and stacking fault energy between CrCoNi and CrCoNiFe medium entropy alloys deformed at 293 and 140K

Woo, W.*; Naeem, M.*; Jeong, J.-S.*; Lee, C.-M.*; Harjo, S.; Kawasaki, Takuro; He, H.*; Wang, X.-L.*

Materials Science & Engineering A, 781, p.139224_1 - 139224_7, 2020/04

 Times Cited Count:6 Percentile:76.25(Nanoscience & Nanotechnology)

Journal Articles

Shell structure of the neutron-rich isotopes $$^{69,71,73}$$Co

Lokotko, T.*; Leblond, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Poves, A.*; Nowacki, F.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Authelet, G.*; et al.

Physical Review C, 101(3), p.034314_1 - 034314_7, 2020/03

 Times Cited Count:4 Percentile:79.36(Physics, Nuclear)

The structures of the neutron-rich $$^{69,71,73}$$Co isotopes were investigated via ($$p,2p$$) knockout reactions at the Radioactive Isotope Beam Factory, RIKEN. Level schemes were reconstructed using the $$gamma-gamma$$ coincidence technique, with tentative spin-parity assignments based on the measured inclusive and exclusive cross sections. Comparison with shell-model calculations suggests coexistence of spherical and deformed shapes at low excitation energies in the $$^{69,71,73}$$Co isotopes.

Journal Articles

Shell evolution of $$N$$ = 40 isotones towards $$^{60}$$Ca; First spectroscopy of $$^{62}$$Ti

Cort$'e$s, M. L.*; Rodriguez, W.*; Doornenbal, P.*; Obertelli, A.*; Holt, J. D.*; Lenzi, S. M.*; Men$'e$ndez, J.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; et al.

Physics Letters B, 800, p.135071_1 - 135071_7, 2020/01

 Times Cited Count:13 Percentile:97.21(Astronomy & Astrophysics)

Excited states in the $$N$$ = 40 isotone $$^{62}$$Ti were populated via the $$^{63}$$V($$p$$,$$2p$$)$$^{62}$$Ti reaction at $$sim$$200 MeV/nucleon at the Radioactive Isotope Beam Factory and studied using $$gamma$$-ray spectroscopy. The energies of the $$2_1^+ rightarrow 0_{rm gs}^+$$ and $$4_1^+ rightarrow 2_1^+$$ transitions, observed here for the first time, indicate a deformed Ti ground state. These energies are increased compared to the neighboring $$^{64}$$Cr and $$^{66}$$Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings.

Journal Articles

Stacking fault energy analyses of additively manufactured stainless steel 316L and CrCoNi medium entropy alloy using in situ neutron diffraction

Woo, W.*; Jeong, J.-S.*; Kim, D.-K.*; Lee, C. M.*; Choi, S.-H.*; Suh, J.-Y.*; Lee, S. Y.*; Harjo, S.; Kawasaki, Takuro

Scientific Reports (Internet), 10(1), p.1350_1 - 1350_15, 2020/01

 Times Cited Count:10 Percentile:82.97(Multidisciplinary Sciences)

Journal Articles

Quasifree neutron knockout from $$^{54}$$Ca corroborates arising $$N=34$$ neutron magic number

Chen, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Chazono, Yoshiki*; Navr$'a$til, P.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Raimondi, F.*; et al.

Physical Review Letters, 123(14), p.142501_1 - 142501_7, 2019/10


 Times Cited Count:21 Percentile:92.26(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Comparing cyclic tension-compression effects on CoCrFeMnNi high-entropy alloy and Ni-based superalloy

Lam, T.-N.*; Chou, Y.-S.*; Chang, Y.-J.*; Sui, T.-R.*; Yeh, A.-C.*; Harjo, S.; Lee, S. Y.*; Jain, J.*; Lai, B.-H.*; Huang, E.-W.*

Crystals (Internet), 9(8), p.420_1 - 420_8, 2019/08


 Times Cited Count:5 Percentile:69.76(Crystallography)

Journal Articles

Dosimetric impact of a new computational voxel phantom series for the Japanese atomic bomb survivors; Pregnant females

Paulbeck, C.*; Griffin, K.*; Lee, C.*; Cullings, H.*; Egbert, S. D.*; Funamoto, Sachiyo*; Sato, Tatsuhiko; Endo, Akira; Hertel, N.*; Bolch, W. E.*

Radiation Research, 192(5), p.538 - 561, 2019/08

 Times Cited Count:4 Percentile:42.47(Biology)

An important cohort of the atomic bomb survivors are pregnant females exposed to the photon and neutrons fields at both Hiroshima and Nagasaki, as well as their children who were exposed ${it in-utero}$. In the present study, we present a new J45 (Japanese 1945) series of high-resolution phantoms of the adult pregnant female at 8-week, 15-week, 25-week, and 38-week post-conception. As for the maternal organ doses, the use of organ doses in a non-pregnant female were shown, in general, to overestimate the corresponding organ doses in the pregnant female, with greater deviations seen at later stages of pregnancy. These results demonstrate that the J45 pregnant female phantom series offers the opportunity for significant improvements in both fetal and maternal organ dose assessment within this unique cohort of the atomic bomb survivors.

Journal Articles

Dosimetric impact of a new computational voxel phantom series for the Japanese atomic bomb survivors; Children and adults

Griffin, K.*; Paulbeck, C.*; Bolch, W.*; Cullings, H.*; Egbert, S. D.*; Funamoto, Sachiyo*; Sato, Tatsuhiko; Endo, Akira; Hertel, N.*; Lee, C.*

Radiation Research, 191(4), p.369 - 379, 2019/04

 Times Cited Count:9 Percentile:75.27(Biology)

Due to computing limitations of the time, only three stylized phantoms were used in DS86 and DS02 to represent the entire Japanese population: an infant, child, and adult. Our study aimed to evaluate the dosimetric impact that should be expected from using an updated and age-expanded RERF phantom series with the survivor cohort. To this end, we developed a new series of hybrid phantoms, based on the Japanese population of 1945, which has greater anatomical realism and improved age resolution than those previously used by RERF. From the photon portion of the spectra, dose differences of up to nearly 25% are expected between the old and new series, while differences of up to nearly 70% are expected from the neutron portion. Overall, our new series of phantoms has shown to provide significant improvements to survivor organ dosimetry, especially to those survivors who were previously misrepresented in body size by their stylized phantom and to those who experienced a highly-directional irradiation field.

Journal Articles

Pressure-induced Diels-Alder reactions in C$$_{6}$$H$$_{6}$$ - C$$_{6}$$F$$_{6}$$ cocrystal towards graphane structure

Wang, Y.*; Dong, X.*; Tang, X.*; Zheng, H.*; Li, K.*; Lin, X.*; Fang, L.*; Sun, G.*; Chen, X.*; Xie, L.*; et al.

Angewandte Chemie; International Edition, 58(5), p.1468 - 1473, 2019/01

 Times Cited Count:18 Percentile:83.78(Chemistry, Multidisciplinary)

Pressure-induced polymerization (PIP) of aromatics is a novel method to construct sp$$^{3}$$-carbon frameworks, and nanothreads with diamond-like structures were synthesized by compressing benzene and its derivatives. Here by compressing benzene-hexafluorobenzene cocrystal(CHCF), we identified H-F-substituted graphane with a layered structure in the PIP product. Based on the crystal structure determined from the in situ neutron diffraction and the intermediate products identified by the gas chromatography-mass spectrum, we found that at 20 GPa CHCF forms tilted columns with benzene and hexafluorobenzene stacked alternatively, which leads to a [4+2] polymer, and then transfers to short-range ordered hydrogenated-fluorinated graphane. The reaction process contains [4+2] Diels-Alder, retro-Diels-Alder, and 1-1' coupling, and the former is the key reaction in the PIP. Our studies confirmed the elemental reactions of the CHCF for the first time, which provides a novel insight into the PIP of aromatics.

Journal Articles

Nuclear structure of $$^{76}$$Ni from the ($$p$$,$$2p$$) reaction

Elekes, Z.*; Kripk$'o$, $'A$*; Sohler, D.*; Sieja, K.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Doornenbal, P.*; Obertelli, A.*; Authelet, G.*; Baba, Hidetada*; et al.

Physical Review C, 99(1), p.014312_1 - 014312_7, 2019/01

 Times Cited Count:7 Percentile:80.58(Physics, Nuclear)

The nuclear structure of the $$^{76}$$Ni nucleus was investigated by ($$p$$,$$2p$$) reaction using a NaI(Tl) array to detect the deexciting prompt $$gamma$$ rays. A new transition with an energy of 2227 keV was identified by $$gamma gamma$$ and $$gamma gamma gamma$$ coincidences. Our shell-model calculations using the Lenzi, Nowacki, Poves, and Sieja interaction produced good candidates for the experimental proton hole states in the observed energy region, and the theoretical cross sections showed good agreement with the experimental values. Although we could not assign all the experimental states to the theoretical ones unambiguously, the results are consistent with a reasonably large Z = 28 shell gap for nickel isotopes in accordance with previous studies.

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