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論文

Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co$$_{1/3}$$TaS$$_{2}$$

Park, P.*; Cho, W.*; Kim, C.*; An, Y.*; Kang, Y.-G.*; Avdeev, M.*; Sibille, R.*; 飯田 一樹*; 梶本 亮一; Lee, K. H.*; et al.

Nature Communications (Internet), 14, p.8346_1 - 8346_9, 2023/12

The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120$$^{circ}$$ structure. However, a new triple-$$mathbf{Q}$$ chiral ordering can emerge in metallic TLAFs, representing the short wavelength limit of magnetic skyrmion crystals. We report the metallic TLAF Co$$_{1/3}$$TaS$$_{2}$$ as the first example of tetrahedral triple-$$mathbf{Q}$$ magnetic ordering with the associated topological Hall effect (non-zero $$sigma_{xy}(mathbf{H}=0)$$). We also present a theoretical framework that describes the emergence of this magnetic ground state, which is further supported by the electronic structure measured by angle-resolved photoemission spectroscopy. Additionally, our measurements of the inelastic neutron scattering cross section are consistent with the calculated dynamical structure factor of the tetrahedral triple-$$mathbf{Q}$$ state.

論文

Fetal and maternal atomic bomb survivor dosimetry using the J45 pregnant female phantom series; Considerations of the kneeling and lying posture with comparisons to the DS02 system

Domal, S. J.*; Correa-Alfonso, C. M.*; Paulbeck, C. J.*; Griffin, K. T.*; 佐藤 達彦; 船本 幸代*; Cullings, H. M.*; Egbert, S. D.*; 遠藤 章; Hertel, N. E.*; et al.

Health Physics, 125(4), p.245 - 259, 2023/10

原爆被爆者に対する線量評価は、大人・小児・幼児の3体の単純な数学ファントムに基づいて構築されたDS02システムが利用されており、妊婦や胎児に対する詳細な線量評価は行われていかなった。そこで、放射線影響研究所を中心とする日米共同研究チームは、最新の計算科学に基づいて1945年の日本人体型を再現した様々な人体模型(J45シリーズ)を開発し、より精度の高い線量評価を実施してきた。本研究では、様々な週齢の胎児・妊婦人体模型を用いて、その姿勢が被ばく線量に与える影響を検討した。その結果、妊婦の姿勢は、特に胎児の被ばく線量に大きな影響を与えることが分かった。

論文

Spiral spin cluster in the hyperkagome antiferromagnet Mn$$_{3}$$RhSi

社本 真一; 山内 宏樹; 飯田 一樹*; 池内 和彦*; Hall, A. E.*; Chen, Y.-S.*; Lee, M. K.*; Balakrishnan, G.*; Chang, L.-J.*

Communications Physics (Internet), 6, p.248_1 - 248_6, 2023/09

Mn$$_{3}$$RhSi単結晶の中性子散乱測定により、局所スピン相関秩序がらせん構造を持つことがわかった。磁気クラスター形成の起源の可能性を、リフシッツ不変量とグリフィス相の観点から議論し、Co$$_{7}$$Zn$$_{7}$$Mn$$_{6}$$の室温スキルミオン相とMnの非フェルミ液体挙動と比較した。

論文

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

$$^{57,59}$$Scからの1陽子ノックアウト反応を用いて、$$^{56}$$Caと$$^{58}$$Caのガンマ崩壊を観測した。$$^{56}$$Caでは1456(12)keVの$$gamma$$線遷移が、$$^{58}$$Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に$$2^{+}_{1} rightarrow 0^{+}_{gs}$$と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、$$2^{+}_{1}$$準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である$$0_{f5/2}$$$$0_{g9/2}$$軌道はほぼ縮退しており、これは$$^{60}$$Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを$$^{70}$$Caあるいはそれ以上にまで広げる可能性がある。

論文

OECD/NEA ARC-F Project; Summary of fission product transport

Lind, T.*; Kalilainen, J.*; Marchetto, C.*; Beck, S.*; 中村 康一*; 木野 千晶*; 丸山 結; 城戸 健太朗; Kim, S. I.*; Lee, Y.*; et al.

Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.4796 - 4809, 2023/08

The OECD/NEA ARC-F project was established to investigate the accidents at Fukushima Daiichi nuclear power station with the aim of consolidating the observations for deeper understanding of the severe accident progression and the status of reactors and containment vessels. Additionally, the project formed an information sharing framework in reactor safety between Japan and international experts. In order to achieve these objectives, the project focused on three tasks: i) to refine analysis for accident scenarios and associated fission-product transport and dispersion, ii) to compile and manage data on the Fukushima Daiichi NPS accident, and iii) to discuss future long-term projects relevant to the Fukushima Daiichi NPS accident. The work was carried out by 22 partners from 12 countries. In the fission product group, ten organizations worked on five topics which were ranked with a high significance as open issues based on the BSAF project and were thereby selected for further investigations. The five fission product related topics were: i) fission product speciation, ii) iodine chemistry, iii) pool scrubbing, iv) fission product transport and behavior in the buildings, and v) uncertainty analysis and variant calculations. In this paper, the work carried out to investigate these five fission product release and transport topics of special interest in the ARC-F project will be described and summarized.

論文

Fetal atomic bomb survivor dosimetry using the J45 series of pregnant female phantoms with realistic survivor exposure scenarios; Comparisons to dose estimates in the DS02 system

Paulbeck, C. J.*; 佐藤 達彦; 船本 幸代*; Lee, C.*; Griffin, K. T.*; Cullings, H. M.*; Egbert, S. D.*; 遠藤 章; Hertel, N. E.*; Bolch, W. E.*

Radiation and Environmental Biophysics, 62(3), p.317 - 329, 2023/08

 被引用回数:0 パーセンタイル:0.01(Biology)

胎児被ばくした原爆生存者に対する線量評価は、放射線被ばくリスクを評価する上で極めて重要となる。原子力機構、放射線影響研究所、フロリダ大学、米国がんセンターらで構成する研究チームは、これまで、1945年の日本人体型を反映した成人、小児及び胎児を含む妊婦の人体模型を作成し、前方照射や等方照射など理想的な照射条件に対してその被ばく線量を評価してきた。本研究では、原爆線量評価システムDS02に含まれる現実的な照射条件に対して、胎児及び母体の被ばく線量を評価した。その結果、現実的な照射条件においては、胎児の臓器線量は、胎児内での臓器の位置や週齢に大きく依存することが分かった。このような胎児に対する詳細被ばく線量解析結果は、将来の胎児被ばくリスク評価モデルの改訂に役立つと考えられる。

論文

Tensile overload-induced texture effects on the fatigue resistance of a CoCrFeMnNi high-entropy alloy

Lam, T.-N.*; Chin, H.-H.*; Zhang, X.*; Feng, R.*; Wang, H.*; Chiang, C.-Y.*; Lee, S. Y.*; 川崎 卓郎; Harjo, S.; Liaw, P. K.*; et al.

Acta Materialia, 245, p.118585_1 - 118585_9, 2023/02

 被引用回数:2 パーセンタイル:62.4(Materials Science, Multidisciplinary)

The present study investigates the crystallographic-texture effects on the improved fatigue resistance in the CoCrFeMnNi high-entropy alloys (HEAs) with the full-size geometry of the ASTM Standards E647-99. We exploited X-ray nano-diffraction mapping to characterize the crystal-deformation levels ahead of the crack tip after stress unloading under both constant- and tensile overloaded-fatigue conditions. The crack-tip blunting-induced much higher deformation level was concentrated surrounding the crack-tip which delays the fatigue-crack growth immediately after a tensile overload. The predominant deformation texture orientation in the Paris regime was investigated, using electron backscatter diffraction and orientation distribution function analyses. The twinning formation-driven shear deformation gave rise to the development of the Goss-type texture within the plastic deformation regime under a tensile-overloaded-fatigue condition, which was attributed to enhance the crack deflection and thus the tensile induced crack-growth-retardation period in the CoCrFeMnNi HEA.

論文

Nonlinear magnon polaritons

Lee, O.*; 山本 慧; 埋田 真樹; Zollitsch, C. W.*; Elyasi, M.*; 吉川 貴史*; 齊藤 英治; Bauer, G. E. W.*; 紅林 秀和*

Physical Review Letters, 130(4), p.046703_1 - 046703_6, 2023/01

 被引用回数:0 パーセンタイル:69.97(Physics, Multidisciplinary)

We experimentally and theoretically demonstrate that nonlinear spin-wave interactions suppress the hybrid magnon-photon quasiparticle or "magnon polariton" in microwave spectra of an yttrium iron garnet film detected by an on-chip split-ring resonator. We observe a strong coupling between the Kittel and microwave cavity modes in terms of an avoided crossing as a function of magnetic fields at low microwave input powers, but a complete closing of the gap at high powers. The experimental results are well explained by a theoretical model including the three-magnon decay of the Kittel magnon into spin waves. The gap closure originates from the saturation of the ferromagnetic resonance above the Suhl instability threshold by a coherent back reaction from the spin waves.

論文

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

 被引用回数:0 パーセンタイル:0.02(Physics, Nuclear)

$$^{59}$$Vと$$^{61}$$Vの低励起準位構造を初めて探索した。$$^{61}$$Vについては中性子ノックアウト反応と陽子非弾性散乱が、$$^{59}$$Vについては中性子ノックアウト反応データが得られた。$$^{59}$$Vについては4つ、$$^{61}$$Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2$$^{-}$$状態とfirst 9/2$$^{-}$$状態からの崩壊と決定された。$$^{61}$$Vについては、($$p$$,$$p'$$)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。

論文

Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; 緒方 一介*; Poves, A.*; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

 被引用回数:0 パーセンタイル:31.68(Physics, Multidisciplinary)

$$sim$$230MeV/nucleonでの$$^{52}$$Caからの中性子ノックアウト反応が$$gamma$$線分光と行われ、$$1f_{7/2}$$$$2p_{3/2}$$軌道からの中性子ノックアウト反応の運動量分布が測定された。断面積は$$N=32$$の閉殻と整合し、Ca同位体での$$N=28$$$$N=34$$閉殻と同程度に強い閉殻であることが確認された。運動量分布の分析から$$1_{f7/2}$$$$2p_{3/2}$$軌道の平均二乗根半径の差は0.61(23)fmと決定され、これはmodified-shell-modelによる予言の0.7fmと整合した。これは、中性子過剰なCa同位体での$$2p_{3/2}$$軌道半径が大きいことが、中性子数にしたがって線形的に荷電半径が増える意外な現象の原因であることを示唆している。

論文

Estimating fine melt pool, coarse melt pool, and heat affected zone effects on the strengths of additive manufactured AlSi10Mg alloys

Lam, T.-N.*; Lee, A.*; Chiu, Y.-R.*; Kuo, H.-F.*; 川崎 卓郎; Harjo, S.; Jain, J.*; Lee, S. Y.*; Huang, E.-W.*

Materials Science & Engineering A, 856, p.143961_1 - 143961_9, 2022/10

 被引用回数:2 パーセンタイル:51.7(Nanoscience & Nanotechnology)

Fine melt pool (FMP), coarse melt pool (CMP), and heat affected zone (HAZ) are generally observed in the additive manufactured AlSi10Mg alloys. In this study, we demonstrated that the yield strength can be estimated by the combination of the sizes and volume fractions of FMP, CMP, HAZ together with the second-phase hardening. Two different AlSi10Mg alloys fabricated via powder bed fusion (PBF) process were prepared to examine the lattice strain evolution of constituent phases during uniaxial tensile loading via in-situ neutron diffraction measurements. The horizontally-built (Hz-built) exhibited a much better yield and tensile strength as well as elongation compared to the vertically-built (Vt-built) AlSi10Mg alloy. We reported empirical strength quantification based on the sizes and ratios of fine melt pool (FMP), coarse melt pool (CMP), and heat affected zone (HAZ) together with the possible failure mode to prevent early fracture in the additive manufactured alloys.

論文

Status of the uncertainty quantification for severe accident sequences of different NPP-designs in the frame of the H-2020 project MUSA

Brumm, S.*; Gabrielli, F.*; Sanchez-Espinoza, V.*; Groudev, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; Bocanegra, R.*; Herranz, L. E.*; Berda$"i$, M.*; et al.

Proceedings of 10th European Review Meeting on Severe Accident Research (ERMSAR 2022) (Internet), 13 Pages, 2022/05

The current HORIZON-2020 project on "Management and Uncertainties of Severe Accidents (MUSA)" aims at applying Uncertainty Quantification (UQ) in the modeling of Severe Accidents (SA), particularly in predicting the radiological source term of mitigated and unmitigated accident scenarios. Within its application part, the project is devoted to the uncertainty quantification of different severe accident codes when predicting the radiological source term of selected severe accident sequences of different nuclear power plant designs, e.g. PWR, VVER, and BWR. Key steps for this investigation are, (a) the selection of severe accident sequences for each reactor design, (b) the development of a reference input model for the specific design and SA-code, (c) the selection of a list of uncertain model parameters to be investigated, (d) the choice of an UQ-tool e.g. DAKOTA, SUSA, URANIE, etc., (e) the definition of the figures of merit for the UA-analysis, (f) the performance of the simulations with the SA-codes, and, (g) the statistical evaluation of the results using the capabilities, i.e. methods and tools offered by the UQ-tools. This paper describes the project status of the UQ of different SA codes for the selected SA sequences, and the technical challenges and lessons learnt from the preparatory and exploratory investigations performed.

論文

A First glimpse at the shell structure beyond $$^{54}$$Ca; Spectroscopy of $$^{55}$$K, $$^{55}$$Ca, and $$^{57}$$Ca

小岩井 拓真*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; 宮城 宇志*; Navr$'a$til, P.*; 緒方 一介*; et al.

Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04

 被引用回数:2 パーセンタイル:55.85(Astronomy & Astrophysics)

中性子過剰核$$^{54}$$Caでは、新魔法数34が発見されて以来、その構造を知るために多くの実験がなされてきたが、それを超える中性子過剰核の情報は全く知られてこなかった。本論文では、理化学研究所RIBFにて$$^{55}$$K, $$^{55}$$Ca, $$^{57}$$Caの励起状態から脱励起するガンマ線を初めて観測した結果を報告した。それぞれ1つのガンマ線しか得られなかったものの、$$^{55}$$Kおよび$$^{55}$$Caのデータは、それぞれ、陽子の$$d_{3/2}$$$$s_{1/2}$$軌道間のエネルギー差、中性子の$$p_{1/2}$$$$f_{5/2}$$軌道間のエネルギー差を敏感に反映し、両方とも最新の殻模型計算によって200keV程度の精度で再現できることがわかった。また、1粒子状態の程度を特徴づける分光学的因子を実験データと歪曲波インパルス近似による反応計算から求め、その値も殻模型計算の値と矛盾しないことがわかった。

論文

Overview and main outcomes of the pool scrubbing lumped-parameter code benchmark on hydrodynamic aspects in IPRESCA project

Marchetto, C.*; Ha, K. S*; Herranz, L. E.*; 廣瀬 意育; Jankowski, T.*; Lee, Y.*; Nowack, H.*; Pellegrini, M.*; Sun, X.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 17 Pages, 2022/03

After the Fukushima Daiichi accident of March 2011, one of the main concerns of the nuclear industry has been the research works for improving atmospheric radioactive release mitigation systems. Pool scrubbing is an important process in reactors that mitigates radioactive release. It is based on the injection of gases containing fission products through a water pool. Bubble hydrodynamics, as a result of gas injection and the associated water pool thermal-hydraulics, is an important aspect of the process since the bubble size, shape, velocity, etc. influence the fission product trapping at the bubble interface with the water. Computer codes dedicated to the pool scrubbing have been mainly developed in the 90's last century and modelling drawbacks have been identified in particular for bubble hydrodynamics. One of IPRESCA project objectives is to improve the pool scrubbing modelling. In order to highlight the main modelling issues, a benchmark exercise has been performed focusing on the bubble hydrodynamics. This benchmark, performed by nine organisations coming from six countries, aims at simulating a basic configuration, a single upward injector in ambient conditions, experimentally characterized in the RSE tests carried out in the European PASSAM project. In this paper, a short description of the code modelling and a comparison between the code results and the experimental data are presented and discussed. Then, outcomes from the benchmark result analysis and proposals of improvements are emphasized.

論文

Grain-size-dependent microstructure effects on cyclic deformation mechanisms in CoCrFeMnNi high-entropy-alloys

Luo, M.-Y.*; Lam, T.-N.*; Wang, P.-T.*; Tsou, N.-T.*; Chang, Y.-J.*; Feng, R.*; 川崎 卓郎; Harjo, S.; Liaw, P. K.*; Yeh, A.-C.*; et al.

Scripta Materialia, 210, p.114459_1 - 114459_7, 2022/03

 被引用回数:7 パーセンタイル:92.76(Nanoscience & Nanotechnology)

The effect of grain size on strain-controlled low-cycle fatigue (LCF) properties in the CoCrFeMnNi high-entropy alloys (HEAs) was investigated towards the distinct microstructural developments during cyclic loading at a strain amplitude of $$pm$$ 1.0%. A much more prominent secondary cyclic hardening (SCH) behavior at the final deformation stage was observed in the fine-grained (FG) than in the coarse-grained (CG) CoCrFeMnNi. In-situ neutron-diffraction and microscopic examination, strongly corroborated by molecular dynamic (MD) simulations, indicated that dislocation activities from planar slip to wavy slip-driven subgrain structures within the grains acted as the primary cyclic-deformation behaviors in the FG CoCrFeMnNi. Differently observed in the cyclic behavior of the CG CoCrFeMnNi was due to a transition from the planar dislocation slip to twinning.

論文

Tensile response of as-cast CoCrFeNi and CoCrFeMnNi high-entropy alloys

Lam, T.-N.*; Luo, M.-Y.*; 川崎 卓郎; Harjo, S.; Jain, J.*; Lee, S.-Y.*; Yeh, A.-C.*; Huang, E.-W.*

Crystals (Internet), 12(2), p.157_1 - 157_9, 2022/02

 被引用回数:3 パーセンタイル:86.54(Crystallography)

In this research, we systematically investigated equiatomic CoCrFeNi and CoCrFeMnNi high-entropy alloys (HEAs). Both of these HEA systems are single-phase, face-centered-cubic (FCC) structures. Specifically, we examined the tensile response in as-cast quaternary CoCrFeNi and quinary CoCrFeMnNi HEAs at room temperature. Compared to CoCrFeNi HEA, the elongation of CoCrFeMnNi HEA was 14% lower, but the yield strength and ultimate tensile strength were increased by 17% and 6%, respectively. The direct real-time evolution of structural defects during uniaxial straining was acquired via in situ neutron-diffraction measurements. The dominant microstructures underlying plastic deformation mechanisms at each deformation stage in as-cast CoCrFeNi and CoCrFeMnNi HEAs were revealed using the Convolutional Multiple Whole Profile (CMWP) software for peak-profile fitting. The possible mechanisms are reported.

論文

Microstructural evolution and mechanical properties of non-equiatomic (CoNi)$$_{74.66}$$Cr$$_{17}$$Fe$$_{8}$$C$$_{0.34}$$ high-entropy alloy

Kim, Y. S.*; Chae, H.*; Huang, E.-W.*; Jain, J.*; Harjo, S.; 川崎 卓郎; Hong, S. I.*; Lee, S. Y.*

Materials, 15(4), p.1312_1 - 1312_11, 2022/02

 被引用回数:0 パーセンタイル:0(Chemistry, Physical)

In this study, we manufactured a non-equiatomic (CoNi)$$_{74.66}$$Cr$$_{17}$$Fe$$_{8}$$C$$_{0.34}$$ high-entropy alloy (HEA) consisting of a single-phase face-centered-cubic structure. The non-equiatomic (CoNi)$$_{74.66}$$Cr$$_{17}$$Fe$$_{8}$$C$$_{0.34}$$ HEA revealed a good combination of strength and ductility in mechanical properties compared to the equiatomic CoNiCrFe HEA, due to both stable solid solution and precipitation-strengthened effects. The non-equiatomic stoichiometry resulted in not only a lower electronegativity mismatch, indicating a more stable state of solid solution, but also a higher stacking fault energy (SFE, $$sim$$50 mJ/m$$^{2}$$) due to the higher amount of Ni and the lower amount of Cr. This higher SFE led to a more active motion of dislocations relative to mechanical twinning, resulting in severe lattice distortion near the grain boundaries and dislocation entanglement near the twin boundaries.

論文

Investigation of the ground-state spin inversion in the neutron-rich $$^{47,49}$$Cl isotopes

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G$'o$mez-Ramos, M.*; et al.

Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10

AA2021-0468.pdf:1.29MB

 被引用回数:3 パーセンタイル:49.55(Physics, Nuclear)

理化学研究所のRIビームファクトリーにて中性子過剰$$^{47,49}$$Clの励起状態を$$^{50}$$Arからのノックアウト反応によって生成し、脱励起ガンマ線からそのエネルギー準位を測定した。また、陽子ノックアウトの運動量分布から$$^{49}$$Clの基底状態が$$3/2^+$$であることがわかった。その結果を大規模殻模型計算およびいくつかの第一原理計算と比較した。$$^{47,49}$$Cl同位体の基底状態および第一励起状態は、計算で用いた相互作用に敏感であることがわかった。それは、陽子の一粒子エネルギーと四重極集団運動との複雑な結合によるためであると考えられる。

論文

Pairing forces govern population of doubly magic $$^{54}$$Ca from direct reactions

Browne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; 緒方 一介*; 宇都野 穣; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; Calvet, D.*; et al.

Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06

 被引用回数:8 パーセンタイル:71.69(Physics, Multidisciplinary)

理化学研究所RIビームファクトリーにて、中性子過剰核$$^{55}$$Scからの1陽子ノックアウト反応によって$$^{54}$$Caを生成し、そのエネルギー準位と反応断面積をガンマ線分光および不変質量分光によって得た。その結果を歪曲波インパルス近似による核反応計算と大規模殻模型による核構造計算を組み合わせた理論値と比較した。実験の準位と断面積は理論計算によってよく再現された。$$^{54}$$Caの正パリティ状態については、基底状態の生成断面積が励起状態のものに比べて圧倒的に大きいという結果が得られた。これは、$$^{55}$$Scでは中性子魔法数34が消滅し$$^{54}$$Caではその魔法数が存在するというこれまでの知見と一見矛盾するが、対相関による分光学的因子のコヒーレンスから理解することができる。

論文

Programmable synthesis of silver wheels

Kwon, H.*; Pietrasiak, E.*; 大原 高志; 中尾 朗子*; Chae, B.*; Hwang, C.-C.*; Jung, D.*; Hwang, I.-C.*; Ko, Y. H.*; Kim, K.*; et al.

Inorganic Chemistry, 60(9), p.6403 - 6409, 2021/05

 被引用回数:0 パーセンタイル:0.01(Chemistry, Inorganic & Nuclear)

The synthesis of sandwich-shaped multinuclear silver complexes with planar penta- and tetranuclear wheel-shaped silver units and a central anion is reported, along with complete spectroscopic and structural characterization. An NMR mechanistic study reveals that silver complexes were formed in the following order: 2Ag $$rightarrow$$ 3Ag$$^{rm H2O}$$ $$rightarrow$$ 5Ag$$^{rm OH}$$ $$rightarrow$$ 4Ag$$^{rm OH}$$. The central hydroxides in 4Ag$$^{rm OH}$$ and 5Ag$$^{rm OH}$$ exhibit exotic physical properties due to the confined environment inside the complex. The size of these silver wheels can be tuned by changing the central anion or extracting/adding one silver atom. This study provides the facile way to synthesize discrete wheel-shaped multinuclear silver complexes and provides valuable insights into the dynamics of the self-assembly process.

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