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論文

A Systematic approach for the adequacy analysis of a set of experimental databases: Application in the framework of the ATRIUM activity

Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.

Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05

https://doi.org/10.1016/j.nucengdes.2024.113035

In the Best-Estimate Plus Uncertainty (BEPU) framework, the use of best-estimate code requires to go through a Verification, Validation and Uncertainty Quantification process (VVUQ). The relevance of the experimental data in relation to the physical phenomena of interest in the VVUQ process is crucial. Adequacy analysis of selected experimental databases addresses this problem. The outcomes of the analysis can be used to select a subset of relevant experimental data, to encourage designing new experiments or to drop some experiments from a database because of their substantial lack of adequacy. The development of a specific transparent and reproducible approach to analyze the relevance of experimental data for VVUQ still remains open and is the topic of this contribution. In this paper, the concept of adequacy initially introduced in the OECD/NEA SAPIUM (Systematic APproach for model Input Uncertainty quantification Methodology) activity is formalized. It is defined through two key properties, called representativeness and completeness, that allows considering the multifactorial dimension of the adequacy problem. A new systematic approach is then proposed to analyze the adequacy of a set of experimental databases. It relies on the introduction of two sets of criteria to characterize representativeness and completeness and on the use of multi-criteria decision analysis method to perform the analysis. Finally, the approach is applied in the framework of the new OECD/NEA ATRIUM activity which includes a set of practical IUQ exercises in thermal-hydraulics to test the SAPIUM guideline in determining input uncertainties and forward propagating them on an application case. It allows evaluating the adequacy of eight experimental databases coming from the Super Moby-dick, Sozzi-Sutherland and Marviken experiments and identifying the most adequate ones.

論文

Chiral Dirac fermion in a collinear antiferromagnet

Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.

Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12

https://doi.org/10.1088/0256-307X/40/12/126101
 被引用回数：1 パーセンタイル：0(Physics, Multidisciplinary)

In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.

論文

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

https://doi.org/10.1016/j.physletb.2023.138025
 被引用回数：1 パーセンタイル：0.02(Astronomy & Astrophysics)

$$^{57,59}$$Scからの1陽子ノックアウト反応を用いて、$$^{56}$$Caと$$^{58}$$Caのガンマ崩壊を観測した。$$^{56}$$Caでは1456(12)keVの$$gamma$$線遷移が、$$^{58}$$Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に$$2^{+}_{1} rightarrow 0^{+}_{gs}$$と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、$$2^{+}_{1}$$準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である$$0_{f5/2}$$と$$0_{g9/2}$$軌道はほぼ縮退しており、これは$$^{60}$$Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを$$^{70}$$Caあるいはそれ以上にまで広げる可能性がある。

論文

Deformation mechanism of a strong and ductile maraging steel investigated using ${it in situ}$ X-ray synchrotron diffraction

Li, H.*; Liu, Y.*; Zhao, W.*; Liu, B.*; 冨永 亜希; 菖蒲 敬久; Wei, D.*

International Journal of Plasticity, 165, p.103612_1 - 103612_20, 2023/06

https://doi.org/10.1016/j.ijplas.2023.103612
 被引用回数：2 パーセンタイル：78.7(Engineering, Mechanical)

コバルトフリーのマルエージング鋼の強度特性を明らかにするために、高エネルギー放射光X線回折法を利用したその場引張試験を行った。マルテンサイト相とオーステナイト相からの回折プロファイルが得られ、それらの強度及び幅が負荷に伴い変化している様子が観察された。回折プロファイルを解析した結果、時効(as-aged)材では、低応力レベルにてマルテンサイトの含有量が緩やかに減少し、高応力レベルでは急激に減少した。一方、熱処理(as-solution)材では、応力の増加とともにオーステナイト相がマルテンサイト相に著しく転移変態している結果が得られた。これらのことがそれぞれの強度特性に起因していることを明らかにした。

論文

Multiple mechanisms in proton-induced nucleon removal at $$sim$$100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G$'o$mez-Ramos, M.*; 緒方 一介*; 吉田 数貴; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

https://doi.org/10.1103/PhysRevLett.130.172501
 被引用回数：5 パーセンタイル：92.42(Physics, Multidisciplinary)

大きなフェルミ面非対称性を持つ陽子過剰な$$^{14}$$O原子核からの100MeV/nucleonでの陽子による陽子・中性子除去反応について報告した。この結果は、quasi-freeノックアウト反応、非弾性散乱、核子移行反応を含む複数の反応機構の定量的寄与を初めて示すものである。このようなエネルギー領域では通常無視される非弾性散乱と核子移行の寄与が、弱束縛陽子と強束縛中性子の除去反応断面積にそれぞれ約50%と30%寄与していることが示された。

論文

Corrosion fatigue crack growth behavior of a structurally gradient steel for high-speed railway axles

Ao, N.*; Zhang, H.*; Xu, H. H.*; Wu, S. C.*; Liu, D.*; 徐 平光; Su, Y. H.; Kang, Q. H.*; Kang, G. Z.*

Engineering Fracture Mechanics, 281, p.109166_1 - 109166_14, 2023/03

https://doi.org/10.1016/j.engfracmech.2023.109166
 被引用回数：4 パーセンタイル：85.05(Mechanics)

Considering the complex service environments that high-speed railway axles are subjected to, the fatigue crack growth (FCG) behavior of a structurally gradient axle steel with different pre-crack depths both in air and corrosive medium was investigated at a frequency of 5 Hz. The results indicated that in the high $$Delta$$$$K$$ region, FCG rate was dramatically accelerated by corrosion, but the gap narrows as $$Delta$$$$K$$ decreased. The accelerated corrosion FCG rate was a comprehensive result of the acceleration effect of the anodic dissolution, hydrogen-enhanced localized plasticity and the retardation effect of corrosion-induced crack-tip blunting. Despite the fact that the corrosion resistance gradually decreased as the pre-crack depth increased, the FCG rate in the corrosive medium gradually decreased. This was because fatigue loading played a more important role than corrosion in accelerating the corrosion FCG rate.

論文

Hybridized propagation of spin waves and surface acoustic waves in a multiferroic-ferromagnetic heterostructure

Chen, J.*; 山本 慧; Zhang, J.*; Ma, J.*; Wang, H.*; Sun, Y.*; Chen, M.*; Ma, J.*; Liu, S.*; Gao, P.*; et al.

Physical Review Applied (Internet), 19(2), p.024046_1 - 024046_9, 2023/02

https://doi.org/10.1103/PhysRevApplied.19.024046
 被引用回数：4 パーセンタイル：90.23(Physics, Applied)

Coherent coupling in magnon based hybrid system has many potential applications in quantum information processing. Magnons can propagate in magnetically ordered materials without any motion of electrons, offering a unique method to build low-power-consumption devices and information channels free of heat dissipation. In this article, we demonstrate the coherent propagation of hybridized modes between spin waves and Love surface acoustic waves in a multiferroic BiFeO$$_{3}$$ and ferromagnetic La$$_{0.67}$$Sr$$_{0.33}$$MnO$$_{3}$$ based heterostructure. The magneto-elastic coupling enables a giant enhancement of strength of the hybridized mode by a factor of 26 compared to that of the pure spin waves. A short wavelength down to 250 nm is demonstrated for the hybridized mode, which is desirable for nanoscale acousto-magnonic applications. Our combined experimental and theoretical analyses represent an important step towards the coherent control in hybrid magnonics, which may inspire the study of magnon-phonon hybrid systems for coherent information processing and manipulation.

論文

Soft, environmentally degradable microfluidic devices for measurement of sweat rate and total sweat loss and for colorimetric analysis of sweat biomarkers

Liu, S.*; Yang, D. S.*; Wang, S.*; Luan, H.*; 関根 由莉奈; Model, J. B.*; Aranyosi, A. J.*; Ghaffari, R.*; Rogers, J. A.*

EcoMat (Internet), 5(1), p.e12270_1 - e12270_18, 2023/01

https://doi.org/10.1002/eom2.12270
 被引用回数：17 パーセンタイル：91.64(Chemistry, Physical)

発汗量やバイオマーカーの非侵襲的でin situモニタリング技術は、人間の生理学的状態,健康、およびパフォーマンスに関するリアルタイムの洞察を取得するために重要である。最近、様々なウェアラブル型のマイクロ流体システムが開発されているが、ほとんどは使い捨てとして設計されおり、廃棄物問題への懸念がある。本研究では、発汗量の測定、バイオマーカーの比色分析など、あらゆる機能を備えた生分解性マイクロ流体システムを通じて、廃棄物問題を解決する材料と成形技術を確立した。本技術で利用する材料は、自然の土壌環境または産業用堆肥施設での微生物の酵素作用によって完全に分解した。構成材料、製造手順、組み立てプロセス、および完成したデバイスの詳細な特性評価により、従来のデバイスに匹敵する、またはそれよりも優れた性能パラメータが明らかになった。実際の利用試験により、これらのデバイスが身体活動および熱曝露中の発汗速度、発汗量、pH、および塩化物濃度の正確な測定値を取得可能であることが明らかとなった。

論文

Study of the $$N=32$$ and $$N=34$$ shell gap for Ti and V by the first high-precision multireflection time-of-flight mass measurements at BigRIPS-SLOWRI

飯村 俊*; Rosenbusch, M.*; 高峰 愛子*; 角田 佑介*; 和田 道治*; Chen, S.*; Hou, D. S.*; Xian, W.*; 石山 博恒*; Yan, S.*; et al.

Physical Review Letters, 130(1), p.012501_1 - 012501_6, 2023/01

https://doi.org/10.1103/PhysRevLett.130.012501
 被引用回数：5 パーセンタイル：94.66(Physics, Multidisciplinary)

The atomic masses of $$^{55}$$Sc, $$^{56,58}$$Ti, and $$^{56-59}$$V have been determined using the high-precision multireflection time-of-flight technique. The radioisotopes have been produced at RIKEN's Radioactive Isotope Beam Factory (RIBF) and delivered to the novel designed gas cell and multireflection system, which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $$^{56,58}$$Ti and $$^{56-59}$$V, the mass uncertainties have been reduced down to the order of 10 keV, shedding new light on the $$N=34$$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $$^{58}$$Ti and $$^{59}$$V. With the new precision achieved, we reveal the nonexistence of the $$N=34$$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $$nu$$p$$_{3/2}$$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $$nu$$d$$_{5/2}$$ and $$nu$$g$$_{9/2}$$ orbits and compare the results with conventional shell model calculations, which exclude the $$nu$$g$$_{9/2}$$ and the $$nu$$d$$_{5/2}$$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $$N = 34$$.

論文

Heat-induced structural changes in magnesium alloys AZ91 and AZ31 investigated by in situ synchrotron high-energy X-ray diffraction

Liu, X. J.*; 徐 平光; 城 鮎美*; Zhang, S. Y.*; 菖蒲 敬久; 行武 栄太郎*; 秋田 貢一*; Zolotoyabko, E.*; Liss, K.-D.*

Journal of Materials Science, 57(46), p.21446 - 21459, 2022/12

https://doi.org/10.1007/s10853-022-07917-y
 被引用回数：3 パーセンタイル：41.53(Materials Science, Multidisciplinary)

In situ time/temperature-resolved synchrotron high-energy X-ray diffraction is applied to study heat-mediated structural changes and phase transformations in rolled sheets of AZ91 and AZ31 magnesium alloys. Azimuthal diffraction intensities along the Debye-Scherrer rings (AT-plots) are used to obtain information on grain recovery and recrystallization temperatures as well as temperature-assisted grain rotations. The azimuthally integrated diffraction intensities, plotted as functions of the scattering vector (QT-plots), provide vital data on the temperature-dependent lattice parameters of the Mg/Al matrix and intermetallic precipitates, as well as on the evolution of the precipitates' volume fraction. It was found that in AZ31, the main precipitates are of the AlMn type, which is rather stable in the investigated temperature range (up to 773 K). In contrast, in AZ91, the major intermetallic precipitates, Al$$_{12}$$Mg$$_{17}$$, undergo complete dissolution above 600 K. It is caused by the enhanced diffusion of Al into the Mg/Al matrix, which according to the Al-Mg phase diagram, can adopt more Al at elevated temperatures. This diffusion is revealed by the proportional diminishing of the matrix lattice parameter (chemical strain), allowing us to quantify the Al content in the matrix. Fast temperature-dependent manipulation with intermetallic content in the Mg/Al alloy can, in principle, be used for controlling its mechanical properties.

論文

"Southwestern" boundary of the $$N = 40$$ island of inversion; First study of low-lying bound excited states in $$^{59}$$V and $$^{61}$$V

Elekes, Z.*; Juh$'a$sz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12

https://doi.org/10.1103/PhysRevC.106.064321
 被引用回数：2 パーセンタイル：0.02(Physics, Nuclear)

$$^{59}$$Vと$$^{61}$$Vの低励起準位構造を初めて探索した。$$^{61}$$Vについては中性子ノックアウト反応と陽子非弾性散乱が、$$^{59}$$Vについては中性子ノックアウト反応データが得られた。$$^{59}$$Vについては4つ、$$^{61}$$Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2$$^{-}$$状態とfirst 9/2$$^{-}$$状態からの崩壊と決定された。$$^{61}$$Vについては、($$p$$,$$p'$$)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。

論文

Extended $$p_{3/2}$$ neutron orbital and the $$N = 32$$ shell closure in $$^{52}$$Ca

Enciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; 緒方 一介*; Poves, A.*; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; et al.

Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12

https://doi.org/10.1103/PhysRevLett.129.262501
 被引用回数：4 パーセンタイル：46.35(Physics, Multidisciplinary)

$$sim$$230MeV/nucleonでの$$^{52}$$Caからの中性子ノックアウト反応が$$gamma$$線分光と行われ、$$1f_{7/2}$$と$$2p_{3/2}$$軌道からの中性子ノックアウト反応の運動量分布が測定された。断面積は$$N=32$$の閉殻と整合し、Ca同位体での$$N=28$$と$$N=34$$閉殻と同程度に強い閉殻であることが確認された。運動量分布の分析から$$1_{f7/2}$$と$$2p_{3/2}$$軌道の平均二乗根半径の差は0.61(23)fmと決定され、これはmodified-shell-modelによる予言の0.7fmと整合した。これは、中性子過剰なCa同位体での$$2p_{3/2}$$軌道半径が大きいことが、中性子数にしたがって線形的に荷電半径が増える意外な現象の原因であることを示唆している。

論文

Ten years of warming increased plant-derived carbon accumulation in an East Asian monsoon forest

Zhang, J.*; Kuang, L.*; Mou, Z.*; 近藤 俊明*; 小嵐 淳; 安藤 麻里子; Li, Y.*; Tang, X.*; Wang, Y.-P.*; Pe$~n$uelas, J.*; et al.

Plant and Soil, 481(1-2), p.349 - 365, 2022/12

https://doi.org/10.1007/s11104-022-05642-8
 被引用回数：3 パーセンタイル：22.98(Agronomy)

Soil warming effects on soil organic carbon (SOC) decomposition and stabilization are highly variable, and the underlying mechanisms are poorly understood. In this study, concentration, stability (dissolved, particle and mineral-associated SOC), and source (plant-derived and microbial-derived) of SOC, soil microbial community composition, and enzyme activities were studied in a 10-year soil warming field experiment in an East Asian monsoon forest. The results showed that 10-year soil warming significantly enhanced SOC in the top 0-10 cm soil. The increased SOC induced by warming was mainly derived from plants with lignin markers, accompanied by a decrease in microbial-derived SOC. This highlights an urgent need for a better understanding of how the contrasting effects of plant- and microbial-derived C mediate the response of the SOC pool to warming across different biomes.

論文

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$

Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12

https://doi.org/10.1073/pnas.2211193119
 被引用回数：3 パーセンタイル：28(Multidisciplinary Sciences)

Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$ provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.

論文

First observation of the decay of the 13/2$$^+$$ isomer in $$^{183}$$Hg and $$B$$(${it M}$2) systematics of neutron transitions across the nuclear chart

Huang, H.*; Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Li, Z. H.*; Guo, C. Y.*; Barzakh, A. E.*; Van Duppen, P.*; Andel, B.*; et al.

Physics Letters B, 833, p.137345_1 - 137345_8, 2022/10

https://doi.org/10.1016/j.physletb.2022.137345
 被引用回数：0 パーセンタイル：0.02(Astronomy & Astrophysics)

The decay of the 13/2$$^+$$ isomeric state in $$^{183}$$Hg was observed for the first time following the $$alpha$$ decay of the 13/2$$^+$$ isomer in $$^{187}$$Pb produced in the $$^{142}$$Nd$$(^{50}$$Cr$$, 2p3n)$$ reaction. Using $$alpha$$-$$gamma$$ delayed coincidence measurements, the half-life of this isomer was measured to be 290(30) $$mu$$s. This isomer is proposed to deexcite by an unobserved low-energy $$M$$2 transition to the known 9/2$$^-$$ member of a strongly prolate-deformed 7/2$$^-$$[514] band, followed by a 105-keV $$M$$1 transition to the bandhead. A lower limit of B($$M$$2)$$geq$$0.018 W.u. was deduced for the unobserved transition. The presumed retardation is proposed to be due to the notable shape change between the initial, nearly spherical, and the final, strongly deformed, states. A similar scenario is also considered for the 13/2$$^+$$ isomer in $$^{181}$$Hg, suggesting both are cases of shape isomers. The B($$M$$2) systematics of neutron transitions across the nuclear chart is discussed.

論文

Synergistic hybrid electrocatalysts of platinum alloy and single-atom platinum for an efficient and durable oxygen reduction reaction

Liu, B.*; Feng, R.*; Busch, M.*; Wang, S.*; Wu, H.*; Liu, P.*; Gu, J.*; Bahadoran, A.*; 松村 大樹; 辻 卓也; et al.

ACS Nano, 16(9), p.14121 - 14133, 2022/09

https://doi.org/10.1021/acsnano.2c04077
 被引用回数：49 パーセンタイル：98.33(Chemistry, Multidisciplinary)

Pt single-atom materials possess an ideal atom economy but suffer from limited intrinsic activity and side reaction of producing H$$_{2}$$O$$_{2}$$ in catalyzing the oxygen reduction reaction (ORR). Here, we demonstrate that anchoring platinum alloys on single-atom Pt-decorated carbon (Pt- SAC) surmounts their inherent deficiencies, thereby enabling a complete four-electron ORR pathway catalysis with high efficiency and durability. Pt$$_{3}$$Co@Pt-SAC demonstrates an exceptional mass and specific activities 1 order of magnitude higher than those of commercial Pt/C. They are durable throughout 50000 cycles, showing only a 10 mV decay in halfwave potential. The superior durability is attributed to the shielding effect of the Pt-SAC coating, which significantly mitigates the dissolution of Pt$$_{3}$$Co cores.

論文

Identification of excited states in $$^{188}$$Bi and $$^{188}$$Po

Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Huang, H.*; 他37名*

Physical Review C, 106(2), p.024317_1 - 024317_11, 2022/08

https://doi.org/10.1103/PhysRevC.106.024317
 被引用回数：1 パーセンタイル：33.4(Physics, Nuclear)

The neutron-deficient $$^{188}$$Bi and $$^{188}$$Po isotopes have been studied by $$gamma$$-ray spectroscopy using the recoil-decay tagging technique with the Argonne Gas-Filled Analyzer. A new 0.25(5)-micro second isomeric state and a prompt cascade formed by 319-, 366-, and 462-keV $$gamma$$ rays have been established on top of the (10$$^{-}$$) $$alpha$$-decaying isomer in $$^{188}$$Bi. The first excited (2$$^{+}$$) state in $$^{188}$$Po was identified, its excitation energy of 242(2) keV continues the nearly constant trend for the first 2$$^{+}$$ states in $$^{190,192,194}$$Po. The state is most likely a member of a prolate rotational band built on the ground state, albeit mixing with other coexisting configurations cannot be excluded. The new results obtained in the present work provide new information to shape coexistence in bismuth and polonium isotopes near the neutron midshell at $$N$$ = 104. In this mass region, a reduction in the prompt $$gamma$$-ray yield obtained with recoil decay tagging was observed for a few nuclides, and the possible reasons are presented.

論文

Modelling of the LTDE-SD radionuclide diffusion experiment in crystalline rock at the $"A$sp$"o$ Hard Rock Laboratory (Sweden)

Soler, J. M.*; Meng, S.*; Moreno, L.*; Neretnieks, I.*; Liu, L.*; Kek$"a$l$"a$inen, P.*; Hokr, M.*; $v{R}$$'i$ha, J.*; Vete$v{s}$n$'i$k, A.*; Reimitz, D.*; et al.

Geologica Acta, 20(7), 32 Pages, 2022/07

https://doi.org/10.1344/GeologicaActa2022.20.7
 被引用回数：3 パーセンタイル：57.97(Geology)

亀裂性岩石中の地下水流動と物質移行のモデル化に関するSKBタスクフォースにおけるTask 9Bは、スウェーデンのエスポ岩盤研究所で実施された原位置長期収着・拡散試験(LTDE-SD)の試験結果のモデル化に焦点をあてたものである。10のモデリングチームによって、異なるモデル概念やコードを用いたモデル化が実施された。モデル化のアプローチは、(1)拡散方程式の解析解、(2)連続多孔質媒体中の数値計算モデル、(3)微細な不均質性(鉱物粒界,微細亀裂の分布等)を考慮した微細構造モデルの大きく3種に分類できる。異なるチームによるモデル化結果から、岩石や亀裂の表面の擾乱影響を含む岩石特性の不均質な分布、微細な亀裂の効果など、様々な異なるモデル概念の比較・評価がなされた。

論文

Predictive modeling of a simple field matrix diffusion experiment addressing radionuclide transport in fractured rock. Is it so straightforward?

Soler, J. M.*; Neretnieks, I.*; Moreno, L.*; Liu, L.*; Meng, S.*; Svensson, U.*; Iraola, A.*; Ebrahimi, K.*; Trinchero, P.*; Molinero, J.*; et al.

Nuclear Technology, 208(6), p.1059 - 1073, 2022/06

https://doi.org/10.1080/00295450.2021.1988822
 被引用回数：4 パーセンタイル：45.99(Nuclear Science & Technology)

SKBタスクフォースは、亀裂性岩石中の地下水流動と物質移行のモデル化に関する国際フォーラムである。WPDE試験はフィンランドのオンカロ地下施設において実施された片麻岩中のマトリクス拡散試験である。複数の非収着性及び収着性のトレーサーを含む模擬地下水が試錐孔の試験区間に沿って注入された。タスク9Aは、WPDE試験で得られたトレーサー破過曲線に対する予測モデリングを行うことを目的とした。複数のチームが本タスクに参加し、異なるモデル化手法とコードを用いた予測解析を行った。この予測解析の重要な結論は、試錐孔の開口部における地下水流動に関連する分散パラメータにモデル化結果が大きく影響されることである。マトリクス拡散及び収着に関連する破過曲線のテール部に着目すると、異なるチーム間の解析結果の差異は相対的に小さい結果となった。

論文

First observation of a shape isomer and a low-lying strongly-coupled prolate band in neutron-deficient semi-magic $$^{187}$$Pb

Zhang, W. Q.*; Andreyev, A. N.; Liu, Z.*; Seweryniak, D.*; Huang, H.*; Li, Z. H.*; Li, J. G.*; Guo, C. Y.*; 他34名*

Physics Letters B, 829, p.137129_1 - 137129_7, 2022/06

https://doi.org/10.1016/j.physletb.2022.137129
 被引用回数：4 パーセンタイル：76.34(Astronomy & Astrophysics)

Prompt and delayed $$gamma$$-ray spectroscopy of the neutron-deficient, semi-magic isotope $$^{187}$$Pb has been performed at the Argonne Gas-Filled Analyzer. A new 5.15(15)-$$mu$$s isomeric state at only 308 keV above the spherical 3/2$$^{-}$$ ground state is identified and classified as a shape isomer. A strongly-coupled band is observed on top of the isomer, which is nearly identical to the one built on the prolate 7/2$$^{-}$$[514] Nilsson state in the isotone $$^{185}$$Hg. Based on this similarity and on the result of the potential-energy surface calculations, the new isomer in $$^{187}$$Pb is proposed to originate from the same configuration. The retarded character of the 308-keV transition can be well explained by the significant difference between the prolate parent and spherical daughter configurations, leading to the shape isomerism. The combined results of the present work and the previous $$alpha$$-decay and laser spectroscopy studies present evidence for triple shape coexistence at low energy in the negative-parity configurations of $$^{187}$$Pb, which is well reproduced by the potential-energy surface calculations.

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