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Journal Articles

Unveiling the local effects of PTL passivation in PEM Electrolyzers through gas and current mapping using operando neutron radiography and polarized neutron imaging

Karimi, V.*; Qvistgaard, C. H.*; Schmidt, S.*; Wolfertz, A.*; Parker, J. D.*; Kai, Tetsuya; Hayashida, Hirotoshi*; Shinohara, Takenao; Angelis, S. D.*; Tengattini, A.*; et al.

ACS Applied Materials & Interfaces, 17(36), p.50742 - 50752, 2025/08

 Times Cited Count:0 Percentile:0.00

Journal Articles

VQE-generated quantum circuit dataset for machine learning

Nakayama, Akimoto*; Mitarai, Kosuke*; Placidi, L.*; Sugimoto, Takanori*; Fujii, Keisuke*

Physical Review Research (Internet), 7(3), p.033048_1 - 033048_9, 2025/07

Journal Articles

Synthesis of BaSiH$$_6$$ hydridosilicate at high pressures; A Bridge to BaSiH$$_8$$ polyhydride

Beyer, D. C.*; Spektor, K.*; Vekilova, O. Y.*; Grins, J.*; Barros Brant Carvalho, P. H.*; Leinbach, L. J.*; Sannemo-Targama, M.*; Bhat, S.*; Baran, V.*; Etter, M.*; et al.

ACS Omega (Internet), 10(15), p.15029 - 15035, 2025/04

 Times Cited Count:0 Percentile:61.98(Chemistry, Multidisciplinary)

Hydridosilicates featuring SiH$$_6$$ octahedral moieties represent a rather new class of compounds with potential properties relating to hydrogen storage and hydride ion conductivity. Here, we report on the new representative BaSiH$$_6$$ obtained from reacting the Zintl phase hydride BaSiH$$_{sim 1.8}$$ with H$$_2$$ fluid at pressures above 4 GPa and subsequent decompression to ambient pressure. It consists of complex SiH$$_{6}^{2-}$$ ions, which are octahedrally coordinated by Ba$$^{2+}$$ counterions. The arrangement of Ba and Si atoms deviates only slightly from an ideal fcc NaCl structure. IR and Raman spectroscopy showed SiH$$_{6}^{2-}$$ bending and stretching modes in the ranges 800-1200 and 1400-1800 cm$$^{-1}$$, respectively. BaSiH$$_6$$ is thermally stable up to 95$$^circ$$C above which decomposition into BaH$$_2$$ and Si takes place. DFT calculations indicated a direct band gap of 2.5 eV. The discovery of BaSiH$$_6$$ consolidates the compound class of hydridosilicates, accessible from hydrogenations of silicides at gigapascal pressures ($$textless$$10 GPa). The structural properties of BaSiH$$_6$$ suggest that it presents an intermediate (or precursor) for further hydrogenation at considerably higher pressures to the predicted superconducting polyhydride BaSiH$$_8$$.

Journal Articles

Characterization of the thorium-229 defect structure in CaF$$_{2}$$ crystals

Takatori, Sayuri*; Pimon, M.*; Pollitt, S.*; Bartokos, M.*; Beeks, K.*; Gr$"u$neis, A.*; Hiraki, Takahiro*; Homma, Tetsuo*; Hosseini, N.*; Leitner, A.*; et al.

New Journal of Physics (Internet), 27(4), p.043024_1 - 043024_10, 2025/04

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Recent reports on laser excitation of the low-energy thorium-229 ($$^{229}$$Th) nuclear isomeric state in calcium fluoride single crystals render this system a promising candidate for a solid-state nuclear clock. However, experimental characterization of the microscopic ion arrangement around the doped $$^{229}$$Th and its electronic charge state, crucial for the precise control of the clock transition and assessing the solid-state clock's performance, remains an unresolved task. This study uses X-ray absorption fine structure spectroscopy of $$^{229}$$Th:CaF$$_{2}$$ to investigate the charge state and coordination environment of doped $$^{229}$$Th. The results indicate that $$^{229}$$Th is doped with a 4+ valence at the substitutional site of the Ca$$^{2+}$$ ion, with charge compensated provided by two F$$^{-}$$ ions located at interstitial sites adjacent to $$^{229}$$Th.

Journal Articles

Competition between mass-symmetric and asymmetric fission modes in $$^{258}$$Md produced in the $$^{4}$$He + $$^{254}$$Es reaction

Nishio, Katsuhisa; Hirose, Kentaro; Makii, Hiroyuki; Orlandi, R.; Kean, K. R.*; Tsukada, Kazuaki; Toyoshima, Atsushi*; Asai, Masato; Sato, Tetsuya; Chiera, N. M.*; et al.

Physical Review C, 111(4), p.044609_1 - 044609_12, 2025/04

 Times Cited Count:0 Percentile:0.00(Physics, Nuclear)

Journal Articles

Unusual low-temperature ductility increase mediated by dislocations alone

Naeem, M.*; Ma, Y.*; Tian, J.*; Kong, H.*; Romero-Resendiz, L.*; Fan, Z.*; Jiang, F.*; Gong, W.; Harjo, S.; Wu, Z.*; et al.

Materials Science & Engineering A, 924, p.147819_1 - 147819_10, 2025/02

 Times Cited Count:1 Percentile:63.96(Nanoscience & Nanotechnology)

Journal Articles

Configuration and dynamics of hydride ions in the nitride-hydride catalyst Ca$$_{3}$$CrN$$_{3}$$H

Fine, L.*; Lav$'{e}$n, R.*; Wei, Z.*; Tsumori, Tatsuya*; Kageyama, Hiroshi*; Kajimoto, Ryoichi; Jimen$'{e}$z-Ruiz, M.*; Koza, M. M.*; Karlsson, M.*

Chemistry of Materials, 37(1), p.489 - 496, 2024/12

 Times Cited Count:0 Percentile:15.31(Chemistry, Physical)

Journal Articles

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; Kofu, Maiko*; Nirei, Masami; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

 Times Cited Count:16 Percentile:91.80(Multidisciplinary Sciences)

Journal Articles

Meeting report on the EPRBioDose2024, Hirosaki

Fujishima, Yohei*; Anderson, D.*; Abe, Yu*; Alkebsi, L.*; Oka, Toshitaka; Tani, Atsushi*; Kranrod, C.*; Toyoda, Shin*; Hamasaki, Kanya*; Hirota, Seiko*; et al.

Nihon Hoshasen Jiko, Saigai Igakkai Zasshi, 7(1), p.21 - 26, 2024/12

no abstracts in English

Journal Articles

Enhanced cryogenic mechanical properties of heterostructured CrCoNi multicomponent alloy; Insights from ${it in situ}$ neutron diffraction

Naeem, M.*; Ma, Y.*; Knowles, A. J.*; Gong, W.; Harjo, S.; Wang, X.-L.*; Romero Resendiz, L.*; 6 of others*

Materials Science & Engineering A, 916, p.147374_1 - 147374_8, 2024/11

 Times Cited Count:4 Percentile:61.30(Nanoscience & Nanotechnology)

Journal Articles

Development of a strip-shaped X-ray mapping system for 9-cell superconducting cavities

Kuriyama, Yasutoshi*; Iwashita, Yoshihisa*; Fuwa, Yasuhiro; Tongu, Hiromu*; Hayano, Hitoshi*; Geng, R. L.*

Journal of Instrumentation (Internet), 19(9), p.P09037_1 - P09037_15, 2024/09

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Journal Articles

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

 Times Cited Count:4 Percentile:70.50(Physics, Multidisciplinary)

Journal Articles

Progress of material characterization techniques based on neutron Bragg-edge transmission imaging

Wang, Y. W.*; Xu, P. G.; Su, Y. H.; Ma, Y. L.*; Wang, H. H.*

Physics Examination and Testing, 42(4), p.32 - 41, 2024/08

Journal Articles

Spectral evidence for Dirac spinons in a kagome lattice antiferromagnet

Zeng, Z.*; Zhou, C.*; Zhou, H.*; Han, L.*; Chi, R.*; Li, K.*; Kofu, Maiko; Nakajima, Kenji; Wei, Y.*; Zhang, W.*; et al.

Nature Physics, 20(7), p.1097 - 1102, 2024/07

 Times Cited Count:20 Percentile:96.79(Physics, Multidisciplinary)

Journal Articles

New isomeric transition in $$^{36}$$Mg; Bridging the $$N = 20$$ and $$N = 28$$ islands of inversion

Madurga, M.*; Christie, J. M.*; Xu, Z.*; Grzywacz, R.*; Poves, A.*; King, T.*; Allmond, J. M.*; Chester, A.*; Cox, I.*; Farr, J.*; et al.

Physical Review C, 109(6), p.L061301_1 - L061301_6, 2024/06

 Times Cited Count:2 Percentile:58.98(Physics, Nuclear)

no abstracts in English

Journal Articles

Microscopic insights of the extraordinary work-hardening due to phase transformation

Ma, Y.*; Naeem, M.*; Zhu, L.*; He, H.*; Sun, X.*; Yang, Z.*; He, F.*; Harjo, S.; Kawasaki, Takuro; Wang, X.-L.*

Acta Materialia, 270, p.119822_1 - 119822_13, 2024/05

 Times Cited Count:11 Percentile:91.62(Materials Science, Multidisciplinary)

Journal Articles

DNA damage response in a 2D-culture model by diffusing alpha-emitters radiation therapy (Alpha-DaRT)

Nojima, Hitomi*; Kaida, Atsushi*; Matsuya, Yusuke; Uo, Motohiro*; Yoshimura, Ryoichi*; Arazi, L.*; Miura, Masahiko*

Scientific Reports (Internet), 14, p.11468_1 - 11468_13, 2024/05

 Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)

Diffusing alpha-emitters radiation therapy (Alpha-DaRT) is a unique radiotherapy that uses seeds emitting alpha particles placed in solid tumors to kill cancer cells surrounding the seeds. Although the DNA damage response is an important cellular response that determines cell death after radiation; however, how DNA damage response occurs during Alpha-DaRT treatment has not yet been explored. In this study, we measured the spatiotemporal characteristics of the DNA damage response, including the number of DNA double-strand breaks and G2 arrest, during Alpha-DaRT treatment by cell experiments using HeLa cells expressing the Fucci cell cycle visualization system. As a result, we found a strong correlation between the number of alpha particles detected by solid-state track detector CR-39 and $$gamma$$-H2AX staining, a marker for detecting DNA damage, and that the area of G2-arrested cells spread over a wider area up to 24 hours. In addition, time-lapse observations revealed that cell cycle dynamics change depending on the distance from the seed. The experimental model in this study revealed for the first time the spatiotemporal information of the DNA damage response around the seed during Alpha-DaRT treatment.

Journal Articles

Observation of high-pressure polymorphs in bulk silicon formed at relativistic laser intensities

Rapp, L.*; Matsuoka, Takeshi*; Firestein, K. L.*; Sagae, Daisuke*; Habara, Hideaki*; Mukai, Keiichiro*; Tanaka, Kazuo*; Gamaly, E. G.*; Kodama, Ryosuke*; Seto, Yusuke*; et al.

Physical Review Research (Internet), 6(2), p.023101_1 - 023101_18, 2024/04

It is generally known that irradiating a solid surface with a laser pulse of ultra-relativistic intensity generates a plasma on the surface, which in turn creates an ultrahigh pressure inside. In this study, the crystal structure analysis of high-pressure phases generated inside silicon single-crystals irradiated by this laser was performed using the diffraction system at the Stress and Imaging apparatus of BL22XU, which is a JAEA-BL. The results obtained confirm the existence of high-pressure phases that silicon is said to possess: body-centered, rhombohedral, hexagonal, and tetragonal phases in the interior. We can get the results that the crystal structure of silicon polymorphs of being include body-centered, rhombohedral, hexagonal-diamond, tetragonal exists. In the future, we will accumulate data and apply them to control the internal structure, strength, and functionality of materials.

Journal Articles

ALTEMIS: Using integrated hydrology and reactive transport modeling to support resilience at the Savannah River Site

Xu, Z.*; Litzinger, A.*; Sakuma, Kazuyuki; Arora, B.*; Hazenberg, P.*; Wang, L.*; Gonzalez Raymat, H.*; Fabricatore, E.*; Wainwright, Haruko*; Eddy-Dilek, C.*

Proceedings of Waste Management Symposia 2024 (WM2024) (Internet), 14 Pages, 2024/03

Journal Articles

System of radiological protection; Towards a consistent framework on earth and in space

R$"u$hm, W.*; Ban, Nobuhiko*; Chen, J.*; Li, C.*; Dobynde, M.*; Durante, M.*; El-Jaby, S.*; Komiyama, Tatsuto*; Ozasa, Kotaro*; Sato, Tatsuhiko; et al.

Journal of Medical Physics - Zeitschrift f$"u$r medizinische Physik -, 34(1), p.4 - 13, 2024/02

 Times Cited Count:0 Percentile:0.00(Radiology, Nuclear Medicine & Medical Imaging)

The International Commission on Radiological Protection (ICRP) provides independent recommendations on radiological protection for the public benefit. For more than 90 years, the ICRP System of Radiological Protection has been guiding the development and implementation of national and international standards and regulations on radiological protection. In 2019, ICRP established Task Group (TG) 115 to address a broader range of topics related to dose and risk assessment for radiological protection of astronauts. This paper gives an overview of the System of Radiological Protection and a brief summary of ICRP's work on radiological protection of astronauts.

619 (Records 1-20 displayed on this page)