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C-stainless steel composites using the improved MPS methodAhmed, Z.*; Wu, S.*; Sharma, A.*; Kumar, R.*; Yamano, Hidemasa; Pellegrini, M.*; Yokoyama, Ryo*; Okamoto, Koji*
International Journal of Heat and Mass Transfer, 250, p.127343_1 - 127343_17, 2025/11
Aoyama, Takahito; Choudhary, S.*; Pandaleon, A.*; Burns, J. T.*; Kokaly, M.*; Restis, J.*; Ross, J.*; Kelly, R. G.*
Corrosion, 81(6), p.609 - 621, 2025/06
hydridosilicate at high pressures; A Bridge to BaSiH
polyhydrideBeyer, D. C.*; Spektor, K.*; Vekilova, O. Y.*; Grins, J.*; Barros Brant Carvalho, P. H.*; Leinbach, L. J.*; Sannemo-Targama, M.*; Bhat, S.*; Baran, V.*; Etter, M.*; et al.
ACS Omega (Internet), 10(15), p.15029 - 15035, 2025/04
Times Cited Count：0 Percentile：0.00(Chemistry, Multidisciplinary)Hydridosilicates featuring SiH octahedral moieties represent a rather new class of compounds with potential properties relating to hydrogen storage and hydride ion conductivity. Here, we report on the new representative BaSiH obtained from reacting the Zintl phase hydride BaSiH
with H
fluid at pressures above 4 GPa and subsequent decompression to ambient pressure. It consists of complex SiH
ions, which are octahedrally coordinated by Ba
counterions. The arrangement of Ba and Si atoms deviates only slightly from an ideal fcc NaCl structure. IR and Raman spectroscopy showed SiH bending and stretching modes in the ranges 800-1200 and 1400-1800 cm
, respectively. BaSiH is thermally stable up to 95
C above which decomposition into BaH and Si takes place. DFT calculations indicated a direct band gap of 2.5 eV. The discovery of BaSiH consolidates the compound class of hydridosilicates, accessible from hydrogenations of silicides at gigapascal pressures (
10 GPa). The structural properties of BaSiH suggest that it presents an intermediate (or precursor) for further hydrogenation at considerably higher pressures to the predicted superconducting polyhydride BaSiH.
Sakamoto, Masahiro; Okumura, Keisuke; Kanno, Ikuo; Matsumura, Taichi; Terashima, Kenichi; Riyana, E. S.; Mizokami, Masato*; Mizokami, Shinya*
JAEA-Research 2024-017, 14 Pages, 2025/03
JAEA-Research-2024-017.pdf:1.34MB
In the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), a trial retrieval of fuel debris with small-amount from Unit 2 is planned. The retrieved fuel debris will be transported out of 1F to Institutes in Ibaraki prefecture for analysis. The analyzed results will be utilized for the improvement of the processes (retrieval, transportation and storage) in the fuel debris management as feedback, and also for the development of technologies necessary in the future. The weight of fuel debris in the trial retrieval is planned to be a few grams. After the trial, the scale of retrieval will be expanded step by step. In the trial retrieval, a rational transportation container should be considered beforehand, according to the laws and regulations associated with the off-site transportation. The transportation container has a classification and the classification is decided according to the radioactivity of the material in the container. In this report, we evaluated the applicability of the Type A transport container to contribute to the safety assessment of retrieved fuel debris.
Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; Tanaka, Hirohisa*; et al.
Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03
Times Cited Count：0 Percentile：0.00(Physics, Applied)Naeem, M.*; Ma, Y.*; Tian, J.*; Kong, H.*; Romero-Resendiz, L.*; Fan, Z.*; Jiang, F.*; Gong, W.; Harjo, S.; Wu, Z.*; et al.
Materials Science & Engineering A, 924, p.147819_1 - 147819_10, 2025/02
Times Cited Count：0 Percentile：0.00(Nanoscience & Nanotechnology)Song, Y.*; Xu, S.*; Sato, Shunsuke*; Lee, I.*; Xu, X.*; Omori, Toshihiro*; Nagasako, Makoto*; Kawasaki, Takuro; Kiyanagi, Ryoji; Harjo, S.; et al.
Nature, 638, p.965 - 971, 2025/02
Times Cited Count：2 Percentile：88.78(Multidisciplinary Sciences)Matsumura, Taichi; Okumura, Keisuke; Sakamoto, Masahiro; Terashima, Kenichi; Riyana, E. S.; Kondo, Kazuhiro*
Nuclear Engineering and Design, 432, p.113791_1 - 113791_9, 2025/02
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Metcalfe, R.*; Benbow, S. J.*; Kawama, Daisuke*; Tachi, Yukio
Science of the Total Environment, 958, p.177690_1 - 177690_17, 2025/01
Uplifting fractured granitic rocks occur in substantial areas of countries such as Japan. A repository site would be selected in such an area only if it is possible to make a safety case, accounting for the changing conditions during uplift. The safety case must include robust arguments that chemical processes in the rocks around the repository will contribute sufficiently to minimise radiological doses to biosphere receptors. To provide confidence in the safety arguments, numerical models need to be sufficiently realistic, but also parameterised conservatively (pessimistically). However, model development is challenging because uplift involves many complex couplings between groundwater flow, chemical reactions between water and rock, and changing rock properties. The couplings would affect radionuclide mobilisation and retardation, by influencing diffusive radionuclide fluxes between groundwater flowing in fractures and effectively immobile porewater in the rock matrix and radionuclide partitioning between water and solid phases, via: (i) mineral precipitation/dissolution; (ii) mineral alteration; and (iii) sorption/desorption. It is difficult to represent all this complexity in numerical models while showing that they are parameterised conservatively. Here we present a modelling approach, illustrated by simulation cases for some exemplar radioelements, to identify realistically conservative process conceptualisations and model parameterisations.
Sakamoto, Masahiro; Okumura, Keisuke; Kanno, Ikuo; Matsumura, Taichi; Terashima, Kenichi; Riyana, E. S.; Kaneko, Junichi*; Mizokami, Masato*; Mizokami, Shinya*
Journal of Nuclear Science and Technology, 10 Pages, 2025/00
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Ito, Tatsuya; Xu, S.*; Xu, X.*; Omori, Toshihiro*; Kainuma, Ryosuke*
Shape Memory and Superelasticity, 9 Pages, 2025/00
Maekawa, Akihiro*; Sakuma, Kazuyuki; Fan, S.*; Fukuda, Miho*; Nasu, Koki*; Taniguchi, Keisuke*
KEK Proceedings 2024-6, p.7 - 12, 2024/12
no abstracts in English
neutron diffractionNaeem, M.*; Ma, Y.*; Knowles, A. J.*; Gong, W.; Harjo, S.; Wang, X.-L.*; Romero Resendiz, L.*; 6 of others*
Materials Science & Engineering A, 916, p.147374_1 - 147374_8, 2024/11
Times Cited Count：2 Percentile：63.37(Nanoscience & Nanotechnology)Matsuba, Kenichi; Kato, Shinya; Kamiyama, Kenji; Akaev, A. S.*; Vurim, A. D.*; Baklanov, V. V.*
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 7 Pages, 2024/11
During a severe accident in sodium-cooled fast reactors, molten core materials could be discharged from the core region toward the lower sodium region of the reactor vessel through coolant channels, such as control rod guide tubes. Typical SFRs have a sodium plenum with limited depth and volume, such as the core inlet plenum located under the core region. Therefore, it is important to evaluate the coolability of molten core materials discharged into a depth- and volume-limited sodium plenum. In the present study, to deepen the understanding on the coolability of molten core materials discharged into such a sodium plenum, conditions under which molten core materials form solidified fragments were discussed based on an experiment discharging a molten fuel simulant (molten Al2O3) into a test vessel filled with liquid sodium.
Kato, Hiroyuki S.*; Muroyama, Mizuho*; Kobayakawa, Nano*; Muneyasu, Riku*; Tsuda, Yasutaka; Murase, Natsumi*; Watanabe, Seiya*; Yamada, Takashi*; Kanematsu, Yusuke*; Tachikawa, Masanori*; et al.
Journal of Physical Chemistry Letters (Internet), 15(43), p.10769 - 10776, 2024/10
Times Cited Count：1 Percentile：42.16(Chemistry, Physical)Sogabe, Joji; Ishida, Shinya; Tagami, Hirotaka; Okano, Yasushi; Kamiyama, Kenji; Onoda, Yuichi; Matsuba, Kenichi; Yamano, Hidemasa; Kubo, Shigenobu; Kubota, Ryuzaburo*; et al.
Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10
In the frame of France-Japan collaboration, the calculational methodologies were defined and assessed, and the phenomenology and the severe accident consequences were investigated in a pool-type sodium-cooled fast reactor.
Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*
Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09
Times Cited Count：1 Percentile：48.32(Physics, Multidisciplinary)C-stainless steel using the Moving Particle Semi-Implicit (MPS) MethodAhmed, Z.*; Wu, S.*; Pellegrini, M.*; Okamoto, Koji*; Sharma, A.*; Yamano, Hidemasa
Proceedings of 14th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation, and Safety (NTHOS-14) (Internet), 14 Pages, 2024/08
The analysis show that once eutectic reaction occurs, the boron diffuses into the stainless steel (SS) wall. Melting initiates at the BC and SS interface, with melt flow following SS cladding penetration. Also, we observed that as temperature rises, a proportional increase in the boron concentration within the melt. The updated MPS method indicated a computational capability of the eutectic reaction model used to effectively analyze control rod eutectic reactions, simulating severe accidents, and its subsequent relocation to understand the effect of BC ingress into the core.
Lan, Z.*; Arikawa, Yasunobu*; Mirfayzi, S. R.*; Morace, A.*; Hayakawa, Takehito*; Sato, Hirotaka*; Kamiyama, Takashi*; Wei, T.*; Tatsumi, Yuta*; Koizumi, Mitsuo; et al.
Nature Communications (Internet), 15, p.5365_1 - 5365_7, 2024/07
Times Cited Count：3 Percentile：79.20(Multidisciplinary Sciences)Zeng, Z.*; Zhou, C.*; Zhou, H.*; Han, L.*; Chi, R.*; Li, K.*; Kofu, Maiko; Nakajima, Kenji; Wei, Y.*; Zhang, W.*; et al.
Nature Physics, 20(7), p.1097 - 1102, 2024/07
Times Cited Count：10 Percentile：94.36(Physics, Multidisciplinary)