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Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; Nishio, Katsuhisa; et al.
JAEA-Conf 2022-001, p.129 - 133, 2022/11
For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors composed of the NE213 liquid organic scintillators and photomultiplier tubes, which were connected to a multi-channel digitizer mounted with a field-programmable gate array (FPGA), for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination applying the gate integration method to the FPGA. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics.
Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.
Journal of Nuclear Science and Technology, 15 Pages, 2022/00
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)Double-differential thick target neutron yields (TTNYs) for Fe, Pb, and Bi targets induced by 107-MeV protons were measured using the fixed-field alternating gradient accelerator at Kyoto University for research and development of accelerator-driven systems (ADSs) and fundamental ADS reactor physics research at the Kyoto University Critical Assembly (KUCA). Note that TTNYs were obtained with the time-of-flight method using a neutron detector system comprising eight neutron detectors; each detector has a small NE213 liquid organic scintillator and photomultiplier tube. The TTNYs obtained were compared with calculation results using Monte Carlo-based spallation models (i.e., INCL4.6/GEM, Bertini/GEM, JQMD/GEM, and JQMD/SMM/GEM) and the evaluated high-energy nuclear data library, i.e., JENDL-4.0/HE, implemented in the particle and heavy iontransport code system (PHITS). All models, including JENDL-4.0/HE, failed to predict high-energy peaks at a detector angle of 5
. Comparing the energy- and angle-integrated spallation neutron yields at energies of 
20 MeV estimated using the measured TTNYs and the PHITS indicated that INCL4.6/GEM would be suitable for the Monte Carlo transport simulation of ADS reactor physics experiments at the KUCA.
Tamura, Jun; Kondo, Yasuhiro; Yee-Rendon, B.; Meigo, Shinichiro; Maekawa, Fujio; Hasegawa, Kazuo; Kako, Eiji*; Umemori, Kensei*; Sakai, Hiroshi*; Konomi, Taro*
JPS Conference Proceedings (Internet), 33, p.011049_1 - 011049_6, 2021/03
Tamura, Jun; Kondo, Yasuhiro; Yee-Rendon, B.; Meigo, Shinichiro; Maekawa, Fujio; Hasegawa, Kazuo; Kako, Eiji*; Umemori, Kensei*; Sakai, Hiroshi*; Konomi, Taro*
Proceedings of 19th International Conference on RF Superconductivity (SRF 2019) (Internet), p.399 - 402, 2019/11
Kobayashi, Nobukiyo*; Masumoto, Hiroshi*; Takahashi, Saburo*; Maekawa, Sadamichi
Scientific Reports (Internet), 6, p.34227_1 - 34227_7, 2016/09
Times Cited Count：28 Percentile：76.25(Multidisciplinary Sciences)
-tetrafluoroethylene) films using different mediaNuryanthi, N.*; Yamaki, Tetsuya; Kitamura, Akane; Koshikawa, Hiroshi; Yoshimura, Kimio; Sawada, Shinichi; Hasegawa, Shin; Asano, Masaharu; Maekawa, Yasunari; Suzuki, Akihiro*; et al.
Transactions of the Materials Research Society of Japan, 40(4), p.359 - 362, 2015/12
The ion-track grafting of a vinylbenzyl chloride (VBC) into a poly(ethylene-co-tetrafluoroethylene) (ETFE) film is necessary for preparing nanostructured hydroxide-ion-conductive electrolyte membranes. A key for success here is to obtain as high graft levels as possible (for higher conductivity) in a smaller number of tracks (for improving the other membrane properties). To this end, therefore, the effect of the medium for the VBC grafting was investigated as part of our continuing effort to optimize the experimental conditions. A 25 
m-thick ETFE film was irradiated in a vacuum chamber with 560 MeV 
Xe at different fluences, and then the grafting was performed by immersing the irradiated films in a 20vol% VBC monomer at 60C. A medium was a mixture of water (H
O) and isopropyl alcohol (iPrOH) at different volume ratios. The degree of grafting increased as the HO content became higher, and reached a maximum in pure HO. These results can be explained by considering the well-known Trommsdorff effect, in which poor solubility of the grafted polymer in polar media leads to an increased polymerization rate probably due to a lower termination rate.
Hamada, Takashi; Hasegawa, Shin; Fukasawa, Hideyuki*; Sawada, Shinichi; Koshikawa, Hiroshi; Miyashita, Atsumi; Maekawa, Yasunari
Journal of Materials Chemistry A, 3(42), p.20983 - 20991, 2015/11
Times Cited Count：31 Percentile：71.09(Chemistry, Physical)no abstracts in English
Amemiya, Kuniaki*; Koshikawa, Hiroshi; Yamaki, Tetsuya; Maekawa, Yasunari; Shitomi, Hiroshi*; Numata, Takayuki*; Kinoshita, Kenichi*; Tanabe, Minoru*; Fukuda, Daiji*
Nuclear Instruments and Methods in Physics Research B, 356-357, p.154 - 159, 2015/08
Times Cited Count：9 Percentile：64.36(Instruments & Instrumentation)Broadband low reflectance materials have various applications in the field of optical energy management; however, materials with ultra-low reflectance (below 0.1%) have been considered as mechanically delicate. We have developed a novel hard-surface optical absorber with microstructured, diamond-like carbon coated ion tracks on CR-39 plastic substrate. The spectral reflectance of the first prototype was below 2% for wavelengths ranging from 400 nm to 1400 nm; moreover, the optical absorber had mechanically hard surface and exhibited temporal durability. Choosing the appropriate design of the surface structure and coating layer is likely to reduce the reflectance to the order of 0.1%. This technique yields easy-to-handle broadband ultra-low reflectance absorbers.
Ooka, Makoto; Maekawa, Yasunari; Tomizuka, Chiaki; Murakami, Tomoyuki*; Katagiri, Genichi*; Ozaki, Hiroshi*; Kawamura, Hiroshi
JAEA-Technology 2015-003, 31 Pages, 2015/03
JAEA-Technology-2015-003.pdf:3.95MB
An action for the decommissioning of the Fukushima Daiichi Nuclear Power Station (Tokyo Electric Power Company) is pushed forward now. For fuel debris Remove, it is necessary to fill the Primary Containment Vessel (PCV) with water. Because a coolant leaks out from the PCV, it becomes the most important problem to seal leak the coolant. Nuclear Plant Decommissioning Safety Research Establishment has examined the method of seal leak using the photocoagulation resin. However, originally the photocoagulation resin is used as coating or the painting, and the applicability to seal leak water is unknown. This report describes the result that examined the applicability to seal leak using photocoagulation resin.
Harada, Masahide; Teshigawara, Makoto; Maekawa, Fujio; Oi, Motoki; Kasugai, Yoshimi; Takada, Hiroshi
Journal of Nuclear Materials, 450(1-3), p.104 - 109, 2014/07
Times Cited Count：1 Percentile：9.57(Materials Science, Multidisciplinary)Japan Spallation Neutron Source (JSNS) in Japan Proton Accelerator Research Complex (J-PARC) has three super-critical hydrogen moderators. The moderator piping has a multilayer structure; a cryogenic layer, a vacuum layer, a helium layer and a cooling water layer. Through the fabrication of the current (1st) moderators, we learned that thermal shrinkage between room temperature (R.T.) and cryogenic temperature at the cryogenic layer made the fabrication process very difficult. Therefore, for the spare (2nd) moderators, we proposed to use a low thermal shrinkage material, Invar, as a piping material. However, there were items to be solved for realizing the Invar duct inview of the fabrication. In this presentation, we report results of (1) Bending test, (2) Welding test and (3) Dissimilar joint test on the Invar duct. (1) In the bending test, the Invar ducts of 22 mm in diameter and 1.5 mm in thickness were tried to be bent into an elbow with 40 mm in radius. By pre-cooling the duct in the liquid nitrogen followed by the bending with slow speed (1 minute), the duct could be bent without any cracks. (2) Through some welding testes by TIG-welding, the proper groove geometry was determined. (3) For the dissimilar joint test, tensile specimens including a bonding region having size of 4 or 6 mm in diameter at the smallest part and 60 mm in length were cut from three rods made by Invar-A6061 and Invar-SS316L, respectively. Those rods were bonded by the friction welding. All specimens were examined at two temperatures, R.T. and 77 K (liquid nitrogen temperature), resulting that 0.2% proof stresses corresponding to the bonding strengths were larger than those of base materials for both the Invar-A6061 and the Invar-SS316L cases. The present result indicates that the Invar duct is available for the 2nd moderators.
Kobayashi, Nobukiyo*; Masumoto, Hiroshi*; Takahashi, Saburo*; Maekawa, Sadamichi
Nature Communications (Internet), 5, p.4417_1 - 4417_6, 2014/07
Times Cited Count：49 Percentile：87.44(Multidisciplinary Sciences)The electric and magnetic properties of matter are of great interest for materials science and their use in electronic applications. Large dielectric and magnetoelectric responses of materials at room temperature are a great advantage for electromagnetic device applications. Here we present a study of FeCo-MgF nanogranular films exhibiting giant dielectric and magnetoelectric responses at room temperature; with dielectric constant 
'=490 and magnetoelectric response 
'/'
=3%. In these films, Fe-Co alloy-based nanometer-sized magnetic granules are dispersed in a Mg-fluoride-based insulator matrix. Insulating nanogranular films are a new class of multifunctional materials. The giant responses are caused by spin-dependent charge oscillation between magnetic granules via quantum-mechanical tunnelling. A possible application of such insulating nanogranular materials with giant response is in the construction of a tunable device, in which impedance components such as capacitance and inductance are tunable at room temperature.
Chudo, Hiroyuki; Ono, Masao; Harii, Kazuya; Matsuo, Mamoru; Ieda, Junichi; Haruki, Rie*; Okayasu, Satoru; Maekawa, Sadamichi; Yasuoka, Hiroshi; Saito, Eiji
Applied Physics Express, 7(6), p.063004_1 - 063004_4, 2014/06
Times Cited Count：43 Percentile：84.64(Physics, Applied)A magnetic field is predicted to emerge on a particle in a rotating body even if the body is electrically neutral. This emergent field is called a Barnett field. We show that nuclear magnetic resonance (NMR) enables direct measurement of the Barnett field in solids. We rotated both a sample and an NMR coil synchronously at high speed and found an NMR shift whose sing reflects that of the nuclear magnetic moments. This result provides direct evidence of the Barnett field. The use of NMR for Barnett field measurement enables the unknown signs of nuclear magnetic moments in solids to be determined.
Yoshimura, Kimio; Koshikawa, Hiroshi; Yamaki, Tetsuya; Shishitani, Hideyuki*; Yamamoto, Kazuya*; Yamaguchi, Susumu*; Tanaka, Hirohisa*; Maekawa, Yasunari
Journal of the Electrochemical Society, 161(9), p.F889 - F893, 2014/06
Times Cited Count：20 Percentile：63.13(Electrochemistry)Graft-type anion-conducting electrolyte membranes (AEMs) with imidazolium cations on graft polymers were synthesized through radiation-induced graft polymerization of 
-vinylimidazole (NVIm) on poly(ethylene-co-tetrafluoroethylene) (ETFE) films, followed by -propylation and ion-exchange reactions. The -propylation proceeded quantitatively, whereas the ion-exchange reactions in 1 M KOH at 60C were accompanied by partial 
-elimination of the imidazolium cations(AEM2), which exhibited an ion-exchange capacity (IEC) of 0.85 mmol g
and ionic conductivity of 10 mS cm. AEM2 showed alkaline stability at 60C but it gradually degraded at 80C for ca. 150 h. The copolymer-type AEM (AEM3) with an IEC of 1.20 mmol g was prepared through the copolymerization of NVIm with styrene on ETFE films, followed by the same -propylation and ion-exchange reactions. AEM3 was shown higher alkaline durability in 1 M KOH at 80C. As a result, it exhibited higher conductivity (
10 mS cm) for 250 h. Therefore, alkylimidazolium cations in copolymer grafts are a promising anion conducting group for alkaline-durable AEMs. A maximum power density of 75 mW cm
is obtained for AEM3 in a direct hydrazine hydrate fuel cell.
Izuchi, Hiroshi*; Fukuma, Yasuhiro*; Takahashi, Saburo*; Maekawa, Sadamichi; Otani, Yoshichika*
Physical Review B, 89(8), p.081308_1 - 081308_5, 2014/02
Times Cited Count：25 Percentile：72.72(Materials Science, Multidisciplinary)Yamaki, Tetsuya; Nuryanthi, N.*; Koshikawa, Hiroshi; Asano, Masaharu; Sawada, Shinichi; Hakoda, Teruyuki; Maekawa, Yasunari; Voss, K.-O.*; Severin, D.*; Seidl, T.*; et al.
Nuclear Instruments and Methods in Physics Research B, 314, p.77 - 81, 2013/11
Times Cited Count：3 Percentile：27.9(Instruments & Instrumentation)Ion-track membranes of poly(vinylidene fluoride) (PVDF), a type of fluoropolymer, could find wide applications due to its superior chemical and mechanical properties. In order to produce track-etched pores in PVDF films, we have independently employed much milder etching conditions without any oxidant additives in the alkaline etching solution. The goal of this work is to pursue the possibility of varying beam parameters and applying the effect of the etching pretreatment to control the pore size and shape. Ongoing in-situ/on-line analyses at the M-branch of the UNILAC would shed light on the detailed chemistry of not only ion-induced degradation but also the post-irradiation reactivity.
Nuryanthi, N.*; Yamaki, Tetsuya; Koshikawa, Hiroshi; Asano, Masaharu; Sawada, Shinichi; Hasegawa, Shin; Maekawa, Yasunari; Katsumura, Yosuke*
Nuclear Instruments and Methods in Physics Research B, 314, p.95 - 98, 2013/11
Times Cited Count：3 Percentile：27.9(Instruments & Instrumentation)Our efforts have been focused on ion-track etched membranes of poly(vinylidene fluoride) (PVDF). This study deals with the effect of the transmembrane potential applied during the conductometry in order to offer a higher degree of freedom to control the pore size. We can say that higher voltage application during the conductometry would accelerate the etching in the tracks. The electrophoretic migration of dissolved products occurring out of each pore might be one of the reasons for this enhanced pore evolution and growth.
Koshikawa, Hiroshi; Yoshimura, Kimio; Sinnananchi, W.; Yamaki, Tetsuya; Asano, Masaharu; Yamamoto, Kazuya*; Yamaguchi, Susumu*; Tanaka, Hirohisa*; Maekawa, Yasunari
Macromolecular Chemistry and Physics, 214(15), p.1756 - 1762, 2013/08
Times Cited Count：13 Percentile：43.36(Polymer Science)Graft-type anion-conducting polymer electrolyte membranes were prepared by the radiation-induced graft polymerization of chloromethylstyrene into poly(ethylene-co-tetrafluoroethylene) (ETFE) films and subsequent quaternization with trimethylamine to evaluate the counter anion effects on fuel cell properties. The hydroxide form was maintained in -saturated water to prevent the bicarbonate formation. The hydroxide form showed conductivity and water uptake four and two times higher than the chloride and bicarbonate forms. The hydroxide form is thermally and chemically less stable, resulting in the tendency to absorb water and to convert to the bicarbonate form.
Nuryanthi, N.*; Yamaki, Tetsuya; Koshikawa, Hiroshi; Asano, Masaharu; Sawada, Shinichi; Hasegawa, Shin; Maekawa, Yasunari; Katsumura, Yosuke*
Transactions of the Materials Research Society of Japan, 38(1), p.105 - 108, 2013/03
We report here how conditions of the conductometric analysis affected the etching characteristics of 25 m-thick poly(vinylidene fluoride) film irradiated with 450 MeV Xe ions. The etching was performed in a 9 mol dm
aqueous potassium hydroxide solution at 80C in a conductometric cell. According to the scanning electron microscope observations, the ion-track membrane obtained with an applied AC voltage of 1.0 V had the surface pores of 168
20 nm in diameter. On the other hand, the etching without an applied voltage gave the approximately two-thirds smaller pores. The conductomeric etching would provide a higher degree of freedom for controlling the pore diameter.
Satoh, Daiki; Maeda, Yoshikazu*; Tameshige, Yuji*; Nakashima, Hiroshi; Shibata, Tokushi*; Endo, Akira; Tsuda, Shuichi; Sasaki, Makoto*; Maekawa, Motokazu*; Shimizu, Yasuhiro*; et al.
Journal of Nuclear Science and Technology, 49(11), p.1097 - 1109, 2012/11
Times Cited Count：12 Percentile：68.7(Nuclear Science & Technology)At the Fukui Prefectural Hospital Proton Therapy Center, neutron doses behind concrete shields and at maze have been measured by using radiation monitors, DARWIN, Wendi-2, a rem meter, and solid state nuclear track detectors. The measured data were compared with the estimations by analytical models and Monte Carlo code PHITS. The analytical model with the parameters employed in shielding design of the facility gave considerably larger estimates than the measured data. This means that the facility was designed with an enough safety margin. The calculation results of PHITS were less than those of the analytical model, and were about 3 times larger than the measured data. From the view point of a safety policy with conservative estimation for shielding design, Monte Carlo simulation is a better tool for estimating radiation safety at accelerator-based proton treatment facilities.
Yoshimura, Kimio; Koshikawa, Hiroshi; Yamaki, Tetsuya; Maekawa, Yasunari; Yamamoto, Kazuya*; Shishitani, Hideyuki*; Asazawa, Koichiro*; Yamaguchi, Susumu*; Tanaka, Hirohisa*
ECS Transactions, 50(2), p.2075 - 2081, 2012/10
no abstracts in English
