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論文

Field dispersion and strong coupling of nuclear-electron spin excitation in MnCO$$_3$$

巻内 崇彦*; 吉川 貴史; 今井 正樹; 中堂 博之; 齊藤 英治; 他3名*

Physical Review Research (Internet), 7(3), p.033083_1 - 033083_7, 2025/09

Hybridized nuclear and electron spin excitation in a MnCO$$_3$$ crystal, a weakly anisotropic antiferromagnet, has been investigated. In this material, the hyperfine interaction is strong enough to form a nuclear spin wave. We measure the microwave absorption induced by magnetic resonance in a bulk MnCO$$_3$$ and observe the dispersion representing strong frequency repulsion between electron and nuclear modes due to their hybridization, the signature of nuclear spin wave. Additionally, we observe that the nuclear spin resonance enters a nonlinear regime above a certain excitation power, attributed to the excitation of finite-wavenumber nuclear spin waves.

論文

Tunable sigmoid behavior of a magnon-based parametron using a Y$$_3$$Fe$$_5$$O$$_{12}$$/Pt bilayer disk

Emdi, G.*; 日置 友智*; 巻内 崇彦*; 齊藤 英治

Physical Review Applied (Internet), 22(3), p.L031002_1 - L031002_6, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Applied)

Sigmoidal curve behavior of 0 and n state probability in a magnon parametron, using yttrium iron garnet (Y$$_3$$Fe$$_5$$O$$_{12}$$) thin disk, is systematically investigated. We demonstrate that the probability distribution can be tuned by bias and pump microwave power. Our numerical calculation that considers increasing damping due to four-magnon scattering processes reproduces the results well.

論文

Persistent magnetic coherence in magnets

巻内 崇彦*; 日置 友智*; 清水 祐樹*; 星 幸治郎*; Elyasi, M.*; 山本 慧; 横井 直人*; Serga, A. A.*; Hillebrands, B.*; Bauer, G. E. W.*; et al.

Nature Materials, 23(5), p.627 - 632, 2024/05

 被引用回数:20 パーセンタイル:91.37(Chemistry, Physical)

When excited, a magnetization in a magnet precesses around the field in an anticlockwise manner on a time scale governed by viscous magnetization damping, after which any information carried by the initial actuation seems to be lost. The damping appears to be a fundamental bottleneck for the use of magnets in information processing. Nevertheless, here we demonstrate recall of the magnetization-precession phase after times that far exceed the damping time scale by two orders of magnitude using dedicated two-colour microwave pump-and-probe experiments for a Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ microstructured film. Time- resolved magnetization state tomography confirms the magnetic persistent coherence (MPC) by revealing a double-exponential decay of the magnetization correlation. We attribute MPC to a feedback effect, viz. coherent coupling of the uniform precession with long-lived excitations at the minima of the spin-wave dispersion relation. Our finding liberates magnetic systems from the strong damping in nanostructures tyranny that limits their use in coherent information storage and processing.

論文

Nonlinear enhancement of coherent magnetization dynamics

Elyasi, M.*; 山本 慧; 日置 友智*; 巻内 崇彦*; 清水 祐樹*; 齊藤 英治*; Bauer, G. E. W.*

Physical Review B, 109(18), p.L180402_1 - L180402_7, 2024/05

 被引用回数:4 パーセンタイル:47.83(Materials Science, Multidisciplinary)

Magnets are interesting materials for classical and quantum information technologies. However, the short decoherence and dephasing times that determine the scale and speed of information networks severely limit the appeal of employing the ferromagnetic resonance. Here we show that the lifetime and coherence of the uniform Kittel mode can be enhanced by three-magnon interaction-induced mixing with the long-lived magnons at the minima of the dispersion relation. Analytical and numerical calculations based on this model explain recent experimental results and predict experimental signatures of quantum coherence.

論文

Switching of magnon parametric oscillation by magnetic field direction

堀部 聡平*; 清水 祐樹*; 星 幸治郎*; 巻内 崇彦*; 日置 友智*; 齊藤 英治

Applied Physics Express, 16(7), p.073001_1 - 073001_4, 2023/07

 被引用回数:1 パーセンタイル:6.72(Physics, Applied)

Parametric oscillation occurs when the resonance frequency of an oscillator is periodically modulated. Owing to time-reversal symmetry breaking in magnets, nonreciprocal magnons can be parametrically excited when spatial-inversion symmetry breaking is provided. This means that magnons with opposite propagation directions have different amplitudes. Here we demonstrate switching on and off the magnon parametric oscillation by reversing the external field direction applied to a Y$$_3$$Fe$$_5$$O$$_{12}$$ micro-structured film. The result originates from the nonreciprocity of surface mode magnons, leading to field-direction dependence of the magnon accumulation under nonuniform microwave pumping. Our numericalcalculation well reproduces the experimental result.

論文

Observation of nuclear-spin Seebeck effect

吉川 貴史*; Reitz, D.*; 伊藤 宏陽*; 巻内 崇彦*; 杉本 宜陽*; 恒川 翔*; 大門 俊介*; 大柳 洸一*; Ramos, R.*; 高橋 三郎*; et al.

Nature Communications (Internet), 12, p.4356_1 - 4356_7, 2021/07

 被引用回数:28 パーセンタイル:84.09(Multidisciplinary Sciences)

Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO$$_3$$ having a large nuclear spin $$(I=5/2)$$ of $$^{55}$$Mn nuclei and strong hyperfine coupling, with a Pt contact. In the system, we observe low-temperature thermoelectric signals down to 100 mK due to nuclear-spin excitation. Our theoretical calculation in which interfacial Korringa process is taken into consideration quantitatively reproduces the results. The nuclear thermoelectric effect demonstrated here offers a way for exploring thermoelectric science and technologies at ultralow temperatures.

論文

Observation of quantum interference conductance fluctuations in metal rings with strong spin-orbit coupling

Ramos, R.*; 巻内 崇彦*; 吉川 貴史*; 大門 俊介*; 大柳 洸一*; 齊藤 英治

Applied Physics Letters, 117(24), p.242402_1 - 242402_5, 2020/12

 被引用回数:1 パーセンタイル:3.25(Physics, Applied)

We investigated the magnetotransport properties of mesoscopic platinum nanostructures (wires and rings) with sub-100 nm lateral dimensions at very low temperatures. Despite the strong spin-orbit interaction in platinum, oscillation of the conductance as a function of the external magnetic field due to quantum interference effects was found to appear. The oscillation was decomposed into Aharonov-Bohm periodic oscillations and aperiodic fluctuations of the conductance due to a magnetic flux piercing the loop of the ring and the metal wires forming the nanostructures, respectively. We also investigated the magnetotransport under different bias currents to explore the interplay between electron phase coherence and spin accumulation effects in strong spin-orbit conductors.

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