Magnetic and quadrupole coupling emerging in NdB with geometrically frustrated orthogonal antiferromagnetic dimer

Metoki, Naoto; Yamauchi, Hiroki; Hagihara, Masato; Watanuki, Ryuta*; Kawamura, Seiko; Kofu, Maiko*; Nakajima, Kenji; Matsuda, Masaaki*

Physical Review B, 111(10), p.104424_1 - 104424_9, 2025/03

https://doi.org/10.1103/PhysRevB.111.104424

Inelastic neutron scattering experiments were carried out to understand the unusual successive order in NdB with the frustrated Shatry-Sutherland (SS) lattice. The pseudo-quartet with and splits into four levels in the magnetically ordered states. The spectra can be explained with the on-site magnetic interaction , the coupling of with quadrupole , and the uniaxial crystalline electric field. The -electron states reproduce the temperature dependences of the in-plane moment which is the primary order parameter, and a weakly induced as the secondary order parameter. The magnetic-quadrupole coupling emerges and play essential role under the geometrical frustration, where the Heisenberg interactions are cancelled out.

Measurement of displacement cross-sections of Nb irradiated by protons with kinetic energy range between 0.4 and 3 GeV

Meigo, Shinichiro; Nakano, Keita*; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*

EPJ Web of Conferences, 284, p.05001_1 - 05001_4, 2023/05

https://doi.org/10.1051/epjconf/202328405001

In high-intensity proton accelerator facilities such as Accelerator Driven System (ADS) and the spallation neutron source, it is crucial to evaluate the damage of beam-interception materials and accelerator components, such as a magnet coil. The displacement per atom (dpa) is used as a damage index, which is derived by integrating the particle flux and the displacement cross section based on the NRT model. Although the dpa is employed as the standard, the experimental data of displacement cross section are scarce for a proton in the energy region above 20 MeV. To obtain the data for superconducting materials for high-intensity accelerators and magnets, the displacement cross section of Nb for proton irradiation with a kinetic energy range between 0.4 and 3 GeV was measured. For sustaining damage in the sample, the Nb sample was cooled at a cryogenic temperature (8 K), where the recombination of Frenkel pairs due to thermal motion was well suppressed with maintaining the normal conductivity to maintain Matthiessen's rule. The displacement cross section of Nb was calculated using the PHITS code, and was compared with the present experimental results. It was found that the widely utilized NRT model overestimates the cross section by a factor of 2, as suggested by the previous works. It was also found that the calculation with a recently proposed athermal recombination corrected (arc) model based on Molecular Dynamics (MD) shows good agreement with the present data.

Measurement of nuclide production cross sections for proton-induced reactions on Ni and Zr at 0.4, 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 527, p.17 - 27, 2022/09

https://doi.org/10.1016/j.nimb.2022.07.002

To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems and so on, nuclide production cross sections on Ni and Zr were measured for GeV energy protons. The measured results were compared with PHITS calculations, JENDL/HE-2007 and so on.

Measurement of nuclide production cross-sections in high-energy proton-induced spallation reactions at J-PARC

Nakano, Keita; Matsuda, Hiroki*; Meigo, Shinichiro; Iwamoto, Hiroki; Takeshita, Hayato*; Maekawa, Fujio

JAEA-Research 2021-014, 25 Pages, 2022/03

JAEA-Research-2021-014.pdf:2.1MB

For the development of accelerator-driven transmutation system (ADS), measurement of nuclide production cross-sections in proton-induced reactions on Be, C, Al, Sc, and V have been performed. The measured data are compared with the calculations by the latest nuclear reaction models and with the nuclear data library to investigate the reproducibilities.

Measurement of nuclide production cross sections for proton-induced reactions on Mn and Co at 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 511, p.30 - 41, 2022/01

https://doi.org/10.1016/j.nimb.2021.10.016

Nuclide production cross sections for proton-induced reactions on Mn and Co at incident energies of 1.3, 2.2, and 3.0 GeV were measured by the activation method at the J-PARC. In total, 143 production cross sections of reaction products were obtained. Among them, the cross sections of Mn(p,X)S and Mn(p,X)Ar were measured for the first time. The stable proton beam and well established beam monitoring system contributed to the reduction of the systematic uncertainties to typically less than 5%, which was better than those of the previous data. To examine the prediction capabilities of spallation reaction models and evaluated data library, the measured data were compared with the spallation reaction models in PHITS (INCL4.6/GEM, etc.), INCL++/ABLA07, and the JENDL/HE-2007 library. The comparison of the mean square deviation factors indicated that both INCL4.6/GEM and JENDL/HE-2007 showed better agreement with the measured data than the others.

Measurement of nuclide production cross-sections of Fe for 0.4-3.0 GeV protons in J-PARC

Matsuda, Hiroki; Takeshita, Hayato*; Meigo, Shinichiro; Maekawa, Fujio; Iwamoto, Hiroki

JPS Conference Proceedings (Internet), 33, p.011047_1 - 011047_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011047

Accurate nuclide production cross-section data are required for the design of Accelerator-Driven nuclear transmutation System (ADS) such as the design of radioactive waste disposal, design of remote-handling procedure of highly activated components, and evaluation of exposure doses of rad-workers. Although much efforts have been devoted to nuclide production cross-section measurements so far, uncertainties of the measured data are sometimes large as several tens percentage, and there is no experimental data in the GeV energy region even for some of important nuclides. In this study, proton induced nuclide production cross-section of iron, which is the most important constituent element of steel, was measured. The present experiment was compared with calculations by the PHITS code with several physics models including Bertini and INCL4.6 and evaluated nuclear data JENDL-HE/2007. The most significant discrepancy found in this study was the production cross sections via the (p,xn) reaction. It was suggested that further improvements, such as the in-medium effect on the nucleon-nucleon scattering and the Pauli blocking, were required in the intra-nuclear cascade models used in this study.

Measurement of displacement cross section for proton in the kinetic energy range from 0.4 GeV to 3 GeV

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

JPS Conference Proceedings (Internet), 33, p.011050_1 - 011050_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011050

R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and aluminum and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.

Measurement of thick target neutron yield at 180 for a mercury target induced by 3-GeV protons

Matsuda, Hiroki; Iwamoto, Hiroki; Meigo, Shinichiro; Takeshita, Hayato*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 483, p.33 - 40, 2020/11

https://doi.org/10.1016/j.nimb.2020.09.012

A thick target neutron yield for a mercury target at an angle of 180 from the incident beam direction is measured with the time-of-flight method using a 3-GeV proton beam at the Japan Proton Accelerator Research Complex (J-PARC). Comparing the experimental result with a Monte Carlo particle transport simulation by the Particle and Heavy Ion Transport code System (PHITS) shows that there are apparent discrepancies. We find that this trend is consistent with an experimental result of neutron-induced re- action rates obtained using indium and niobium activation foils. Comparing proton-induced neutron-production double-differential cross-sections for a lead target at backward directions between the PHITS calculation and experimental data suggests that the dis- crepancies for our experiments would be linked to the neutron production calculation around 3 GeV by the PHITS spallation model and/or the calculation of nonelastic cross-sections around 3 GeV in the particle transport simulation.

A Comprehensive study of spallation models for proton-induced spallation product yields utilized in transport calculation

Iwamoto, Hiroki; Meigo, Shinichiro; Matsuda, Hiroki

EPJ Web of Conferences, 239, p.06001_1 - 06001_6, 2020/09

https://doi.org/10.1051/epjconf/202023906001

no abstracts in English

Measurement of displacement cross section of structural materials utilized in the proton accelerator facilities with the kinematic energy above 400 MeV

Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*

EPJ Web of Conferences, 239, p.06006_1 - 06006_4, 2020/09

https://doi.org/10.1051/epjconf/202023906006

R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.