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報告書

セメント固化におけるペーストの流動性に影響する化学物質についての調査

谷口 拓海; 松本 早織; 平木 義久; 佐藤 淳也; 藤田 英樹*; 金田 由久*; 黒木 亮一郎; 大杉 武史

JAEA-Review 2024-059, 20 Pages, 2025/03

JAEA-Review-2024-059.pdf:1.0MB

廃棄物のセメント固化で求められる基本的な性能である硬化前の流動性および硬化後の強度特性は、廃棄物に含まれる物質や成分などの化学的作用の影響を受けることが予想される。硬化前の流動性および硬化後の強度特性はセメントの硬化速度に大きく影響されることから、セメントの硬化速度に影響を与える化学物質を対象に着目して既往の知見を調査し、取りまとめを行った。本報告書ではセメントの流動性に影響を及ぼす化学物質を大きく分類し、無機物質として(1)陰イオン種、(2)重金属等金属元素、(3)セメント混和剤として用いられる無機物質および(4)セメント混和剤として用いられる有機物質の4つに整理した。調査の結果、化学物質によって硬化を促進する効果と遅延する効果に大きく分類されることが分かったが、一部の化学物質ではその添加量によって硬化に与える影響が逆転するものも見られたことから、実際に化学物質を添加し、凝結時間測定を実施した。その結果、硬化促進に寄与するメカニズムが複数あることが分かった。セメントの硬化反応を阻害する化学物質を調査し、セメント固化における混入禁忌成分を検討するための情報を整理することができた。

報告書

軽水炉実機水環境模擬照射装置の整備と試験運転

佐谷戸 夏紀; 大塚 薫; 冬島 拓実; 遠藤 泰一; 大塚 紀彰; 北岸 茂; 飛田 正浩*; 磯崎 太*; 松本 聡*; 竹本 紀之

JAEA-Technology 2024-016, 247 Pages, 2025/02

JAEA-Technology-2024-016.pdf:28.43MB

文部科学省が行う最先端研究基盤事業の補助対象事業として、材料試験炉JMTR(Japan Materials Testing Reactor, 50MW)では「世界最先端研究用原子炉の高度利用による国際的研究開発拠点の整備」が採択された。本事業の一環として、JMTRでは平成22年度から「軽水炉実機水環境模擬照射装置」を整備した。本装置は、温度、圧力、水質(溶存酸素、溶存水素等)を制御し、軽水炉(BWR及びPWR)条件の水環境を模擬しながら、炉内構造材等の中性子照射が行える照射装置である。さらにPWR条件用の照射装置には、ホウ素やリチウムを添加するための薬液注入機能を追加した。本装置の整備後は試験運転を実施し、本装置の性能を確認した。本報告書は、軽水炉実機水環境模擬照射装置の整備及び整備後に実施した本装置の試験運転についてまとめたものである。

論文

Integration of multiple dense point clouds based on estimated parameters in photogrammetry with QR code for reducing computation time

中村 啓太*; 馬場 啓多*; 渡部 有隆*; 羽成 敏秀; 松本 拓*; 今渕 貴志; 川端 邦明

Artificial Life and Robotics, 29(4), p.546 - 556, 2024/09

This paper describes a method for integrating multiple dense point clouds using a shared landmark to generate a single real-scale integrated result for photogrammetry. It is difficult to integrate high-density point clouds reconstructed by photogrammetry because the scale differs with each photogrammetry. To solve this problem, this study places a QR code of known sizes, which is a shared landmark, in the reconstruction target environment and divides the reconstruction target environment based on the position of the QR code that is placed. Then, photogrammetry is performed for each divided environment to obtain each high-density point cloud. Finally, we propose a method of scaling each high-density point cloud based on the size of the QR code and aligning each high-density point cloud as a single high-point cloud by partial-to-partial registration. To verify the effectiveness of the method, this paper compares the results obtained by applying all images to photogrammetry with those obtained by the proposed method in terms of accuracy and computation time. In this verification, ideal images generated by simulation and images obtained in real environments are applied to photogrammetry. We clarify the relationship between the number of divided environments, the accuracy of the reconstruction result, and the computation time required for the reconstruction.

論文

Enthalpy measurement on (U$$_{1-x}$$Pu$$_{x}$$)O$$_{2}$$ (x = 0, 0.18, 0.45, and 1) and analysis of heat capacity

廣岡 瞬; 森本 恭一; 松本 卓; 小笠原 誠洋*; 加藤 正人; 村上 龍敏

Journal of Nuclear Materials, 598, p.155188_1 - 155188_9, 2024/09

 被引用回数:0 パーセンタイル:0.00(Materials Science, Multidisciplinary)

酸化物燃料の温度解析において重要な役割を持つ比熱は、特に高温領域において文献間でばらつきが大きい。さらに、UO$$_{2}$$のデータと比べてPuO$$_{2}$$やMOXのデータは報告例が少ないため、比熱においてPu含有率の依存性の評価が困難である。本研究では、UO$$_{2}$$、PuO$$_{2}$$、MOX (Pu=0.18, 0.45)を対象に、ドロップカロリメータを用いて最高2200Kのエンタルピーのデータを取得した。取得したエンタルピーの温度依存性を評価することで比熱を算出した。エンタルピー、比熱ともに、2000Kまでは温度とともにほぼ線形に上昇し、2000Kを超えると急激に上昇する結果が得られた。2000K以下のデータは文献値とよく一致し、2000K以上のデータは文献値と大きく異なる結果となった。この結果について、酸素及び電子正孔対の欠陥の観点で考察を行った。

論文

High temperature nanoindentation of (U,Ce)O$$_{2}$$ compounds

Frazer, D.*; Saleh, T. A.*; 松本 卓; 廣岡 瞬; 加藤 正人; McClellan, K.*; White, J. T.*

Nuclear Engineering and Design, 423, p.113136_1 - 113136_7, 2024/07

 被引用回数:0 パーセンタイル:0.00(Nuclear Science & Technology)

ナノインデンテーション法では、微小な試験片を用いてヤング率,硬度及びクリープ強度といった機械物性を評価することが可能である。本研究ではMOX燃料の代替物質として(U,Ce)O$$_{2}$$を用いて、高温ナノインデンテーション試験を実施した。試料のCe含有率は0.1、0.2及び0.3mol%とし、温度は800$$^{circ}$$Cまでの測定を行い、ヤング率、硬度及びクリープ強度の評価を行った。温度の上昇に伴い、ヤング率は線形的に低下し、硬度は指数関数的に低下する結果が得られた。また、800$$^{circ}$$Cにおいては、応力指数n=4.7$$sim$$6.9のクリープ変形が得られた。

論文

Monte Carlo simulation study on the dose and dose-averaged linear energy transfer distributions in carbon ion radiotherapy

石川 諒尚; 古場 裕介*; 古田 琢哉; Chang, W.*; 米内 俊祐*; 松本 真之介*; 橋本 慎太郎; 平井 悠大*; 佐藤 達彦

Radiological Physics and Technology, 17(2), p.553 - 560, 2024/06

At the Heavy Ion Medical Accelerator in Chiba (HIMAC), a series of retrospective studies are ongoing in patients treated with carbon ion radiotherapy (CIRT) to obtain the knowledge to improve tumor control and reveal the mechanism of the low risk of secondary cancer after CIRT. Dose-averaged linear energy transfer (LET$$_{rm d}$$) is generally used as a measure of treatment effectiveness or biological effects in such retrospective studies; however, it is conventionally evaluated from the relative biological effectiveness (RBE)-LET$$_{rm d}$$ fitted function used in the treatment planning system. In this study, we calculated the physical doses and their linear energy transfer (LET) distributions for a series of treatment plans for a homogeneous rectangular phantom and a human body phantom with typical CIRT beams using Monte Carlo (MC) simulation. The LET$$_{rm d}$$ was then deduced from the MC simulation and compared with the corresponding data obtained using the conventional method. The comparison suggested that the two types of LET$$_{rm d}$$ agreed well with each other, except around the distal end of the spread-out Bragg peak, where the MC simulation yielded significantly higher LET$$_{rm d}$$ values than that of the conventional method. This is because the RBE-LET$$_{rm d}$$ fitted function adopted in the conventional method ignores the contribution of the high-LET components, causing an overkill effect. Furthermore, an MC simulation was conducted to determine the material composition of water and realistic materials from the CT number in the planned image. The profiles of physical dose and LET$$_{rm d}$$ were in good agreement for both techniques. These results indicate the possibility of enhancing the efficiency of retrospective studies of CIRT using MC simulations in the future.

論文

Estimated camera trajectory-based integration among local 3D models sequentially generated from image sequences by SfM-MVS

松本 拓; 羽成 敏秀; 川端 邦明; 中村 啓太*; 八代 大*

Artificial Life and Robotics, 29(2), p.358 - 371, 2024/05

This paper describes a three-dimensional (3D) modeling method for sequentially and spatially understanding situations in unknown environments from an image sequence acquired from a camera. The proposed method chronologically divides the image sequence into sub-image sequences by the number of images, generates local 3D models from the sub-image sequences by the Structure from Motion and Multi-View Stereo (SfM-MVS), and integrates the models. Images in each sub-image sequence partially overlap with previous and subsequent sub-image sequences. The local 3D models are integrated into a 3D model using transformation parameters computed from a camera trajectory estimated by the SfM-MVS. In our experiment, we quantitatively compared the quality of integrated models with a 3D model generated from all images in a batch and the computational time to obtain these models using three real data sets acquired from a camera. Consequently, the proposed method can generate a quality integrated model that is compared with a 3D model using all images in a batch by the SfM-MVS and reduce the computational time.

論文

A Study on the effects of photogrammetry by the camera angle of view using computer simulation

中村 啓太; 羽成 敏秀; 松本 拓; 川端 邦明; 八代 大*

Journal of Robotics and Mechatronics, 36(1), p.115 - 124, 2024/02

During the decommissioning activities, a movie was shot inside the reactor building during the investigation of the primary containment vessel by applying photogrammetry, which is one of the methods for three-dimensional (3D) reconstruction from images, to the images from this movie, it is feasible to perform 3D reconstruction of the environment around the primary containment vessel. However, the images from this movie may not be suitable for 3D reconstruction because they were shot remotely by robots owing to limited illumination, high-dose environments, etc. Moreover, photogrammetry has the disadvantage of easily changing 3D reconstruction results by simply changing the shooting conditions. Therefore, this study investigated the accuracy of the 3D reconstruction results obtained by photogrammetry with changes in the camera angle of view under shooting conditions. In particular, we adopted 3D computer graphics software to simulate shooting target objects for 3D reconstruction in a dark environment while illuminating them with light for application in decommissioning activities. The experimental results obtained by applying artificial images generated by simulation to the photogrammetry method showed that more accurate 3D reconstruction results can be obtained when the camera angle of view is neither too wide nor too narrow when the target objects are shot and surrounded. However, the results showed that the accuracy of the obtained results is low during linear trajectory shooting when the camera angle of view is wide.

論文

Uranium-plutonium-americium cation interdiffusion in polycrystalline (U,Pu,Am)O$$_{2 pm x}$$ mixed oxides

Vauchy, R.; 松本 卓; 廣岡 瞬; 宇野 弘樹*; 田村 哲也*; 有馬 立身*; 稲垣 八穂広*; 出光 一哉*; 中村 博樹; 町田 昌彦; et al.

Journal of Nuclear Materials, 588, p.154786_1 - 154786_13, 2024/01

 被引用回数:6 パーセンタイル:87.16(Materials Science, Multidisciplinary)

Diffusion couples made of dense polycrystalline (U,Pu,Am)O$$_{2 pm x}$$ oxides were annealed in various thermodynamic conditions (temperature, oxygen partial pressure), and for different durations. The associated actinide redistribution was quantified using Electron Probe Micro-Analysis (EPMA). Average diffusion profiles were obtained from elemental U, Pu, and Am X-ray maps and the resulting interdiffusion coefficients were calculated, then analyzed at the light of our model of point defect chemistry.

論文

Integration of multiple partial point clouds based on estimated parameters in photogrammetry with QR codes

馬場 啓多*; 渡部 有隆*; 中村 啓太*; 松本 拓; 羽成 敏秀; 川端 邦明

Proceedings of 29th International Symposium on Artificial Life and Robotics (AROB 29th 2024) (Internet), p.751 - 756, 2024/01

This study proposes a partial-to-partial point cloud registration method based on estimated parameters in photogrammetry and QR code. Some research and development on Generating a 3D map of the workspace by photogrammetric methods have been proposed for the decommissioning work at the Fukushima Daiichi Nuclear Power Plant. Photogrammetry is a method for 3D reconstruction of the location and shape of target objects from many images, and the processing time depends on the number of images. Considering the reconstruction of a large area, the number of images increases, and processing time also increases significantly. To reduce such computational time, this study considers applying SfM-MVS (Structure from Motion and Multi-View Stereo), which is one of the photogrammetry methods, to each segmented image group, aligning each obtained result, integrating them, and creating a model of the entire space. This alignment is called partial-to-partial registration and it is difficult to find the correspondence points for registration. Therefore, we place markers such as QR codes in the target reconstruction space to make it easy to find the correspondence points. We adopt the QR code as a 2D code because it is easy to reconstruct by photogrammetry. In this paper, we discuss the validity of this approach by comparing it with the integrated model using all images applying SfM-MVS. We verify the validation of the proposed method by simulation due to the large number of images and the ease of modifying the environment. The experiment about varying the number of image divisions shows that the reconstruction result from all images is more accurate than the integrated result. However, all of these models have high reconstruction accuracy. Moreover, the accuracy of the integrated model does not depend on the number of divisions.

論文

Automatic system for sequential reconstruction from image sequences acquired from a camera by SfM-MVS

松本 拓; 羽成 敏秀; 川端 邦明; 八代 大*; 中村 啓太*

Proceedings of 2023 IEEE International Conference on Robotics and Biomimetics (IEEE ROBIO 2023) (Internet), 7 Pages, 2023/12

This paper describes an automatic system that performs three-dimensional (3D) modeling from image sequences acquired from a camera during a survey to understand the state of the environment sequentially. The developed system sequentially generates local 3D models from image sequences acquired from a camera by the Structure from Motion and Multi-View Stereo (SfM-MVS) and integrates the models. This system, consisting of a camera, a computer, and storage, handles streaming, image acquisition, 3D modeling, and integration processes. The system is designed to perform each process in parallel while performing image acquisition. Local 3D models are integrated based on the similarity of camera trajectories, which correspond to overlapped images in each sequence, estimated from SfM. Our experiments verified the operation of the developed system from the image acquisition to the integration of local 3D models in two cases. Consequently, we confirmed that an integrated model could be generated by automatically executing each process in the system through experiments.

論文

Compact moving particle semi-implicit method for incompressible free-surface flow

Wang, Z.; 松本 俊慶; Duan, G.*; 松永 拓也*

Computer Methods in Applied Mechanics and Engineering, 414, p.116168_1 - 116168_49, 2023/09

 被引用回数:12 パーセンタイル:85.89(Engineering, Multidisciplinary)

Recently, consistent meshfree particle methods have been intensively studied. It has been pointed out that numerical inaccuracy or instability could easily occur with incomplete or biased neighbor support. This study proposes a new meshfree particle method called the compact moving particle semi-implicit (CMPS) method to decrease the condition number. In the proposed CMPS, the first-order and second-order derivatives are discretized separately, enhancing the numerical stability significantly. By adopting a small dilation parameter of the compact support, the CMPS can remarkably improve accuracy and reduce computational costs. Formulations for zeroth-order, first-order, and second-order derivatives are derived, and various boundary conditions, e.g., Dirichlet and Neumann, are discussed. In order to better deal with complex free-surface flows using the CMPS, some new numerical techniques, i.e., optimized regularization and reconstructed particle shifting schemes, are also developed. Furthermore, the surface fitting method is extended to address the surface tension. A convergence study is conducted in complex geometry to verify the stability, accuracy, and efficiency of the CMPS. Then, second-order accuracy is confirmed using the Taylor-Green vortex problem. After that, numerical examples concerning various free-surface flows, including square patch, hydrostatic pressure, dam break, droplet oscillation, and droplet coalescence, are calculated to demonstrate the potential of the CMPS.

論文

Integration of 3D environment models generated from the sections of the image sequence based on the consistency of the estimated camera trajectories

松本 拓; 羽成 敏秀; 川端 邦明; 八代 大*; 中村 啓太*

Proceedings of 22nd World Congress of the International Federation of Automatic Control (IFAC 2023) (Internet), p.12107 - 12112, 2023/07

This paper describes a method that integrates Three-Dimensional (3D) environment models reconstructed from image sequences to reduce the computation time of 3D environment modeling that estimates camera poses and simultaneously reconstructs a 3D environment model from images based on photogrammetry. However, 3D environment modeling is time-consuming when using many images because it finds correspondence points between them by feature matching. Therefore, we assume that the computation time is reduced by reconstructing 3D environment models from image sequences divided from an image sequence because the number of images used in 3D environment modeling becomes less. However, it is difficult to integrate the 3D environment models because the scale between them may not be the same, and overlapping regions between 3D environment models are small for integrating the models. In this paper, we propose a method that integrates 3D environment models based on camera trajectories corresponding to overlapped images between image sequences used in 3D environment modeling. To integrate them, transformation parameters are calculated from poses of camera trajectories between 3D environment models. After that, the transformed camera trajectory is aligned using coarse and fine registration. Consequently, compared with 3D environment modeling that processes an image sequence in batch, the proposed method could reduce the computation time and reconstruct a comparable integrated model.

論文

Toward long-term storage of nuclear materials in MOX fuels fabrication facility

廣岡 瞬; 中道 晋哉; 松本 卓; 土持 亮太; 村上 龍敏

Frontiers in Nuclear Engineering (Internet), 2, p.1119567_1 - 1119567_7, 2023/03

プルトニウム(Pu)を含む核燃料物質の保管は安全や計量管理等の観点から慎重な配慮が必要であるが、保管に関する技術的な情報に関しては、イギリスやアメリカからの報告例が僅かに存在するのみである。日本も多量のPuをウラン-プルトニウム混合酸化物(MOX)燃料の形態で所有しており、その形状や性質、含まれる不純物等に応じて適切な保管管理を行うことが重要である。本報告では、日本原子力研究開発機構のプルトニウム燃料技術開発センターが所有する様々なMOX燃料とその保管方法、また、保管中に起こった問題や今後の長期保管における対策について報告する。

論文

Implication of E3 ligase RAD18 in UV-induced mutagenesis in human induced pluripotent stem cells and neuronal progenitor cells

島田 幹男*; 徳宮 巧実*; 三宅 智子*; 塚田 海馬*; 神崎 訓枝; 柳原 啓見*; 小林 純也*; 松本 義久*

Journal of Radiation Research (Internet), 64(2), p.345 - 351, 2023/03

 被引用回数:3 パーセンタイル:55.17(Biology)

Pluripotent stem cells (PSCs) have the potential to differentiate to any of the other organs. The genome DNA integrity of PSCs is maintained by a high level of transcription for a number of genes involved in DNA repair, cell cycle and apoptosis. However, it remains unclear how high the frequency of genetic mutation is and how these DNA repair factors function in PSCs. In this study, we employed Sup F assay for the measurement of mutation frequency after UV-C irradiation in induced pluripotent stem cells (iPSCs) as PSC models and neural progenitor cells (NPCs) were derived from iPSCs as differentiated cells. iPSCs and NPCs exhibited a lower mutation frequency compared with the original skin fibroblasts. In RNA-seq analysis, iPSCs and NPCs showed a high expression of RAD18, which is involved in trans-lesion synthesis (TLS) for the emergency tolerance system during the replication process of DNA. Although RAD18 is involved in both error free and error prone TLS in somatic cells, it still remains unknown the function of RAD18 in PSCs. In this study we depleted of the RAD18 by siRNA knockdown resulted in decreased frequency of mutation in iPSCs and NPCs. Our results will provide information on the genome maintenance machinery in PSCs.

論文

Automatic process for 3D environment modeling from acquired image sequences

松本 拓; 羽成 敏秀; 川端 邦明; 八代 大*; 中村 啓太*

Proceedings of 28th International Symposium on Artificial Life and Robotics (AROB 28th 2023) (Internet), p.768 - 773, 2023/01

This paper reports on an automatic process for 3D environmental modeling from acquired image sequences. We have studied methods of 3D environment modeling to understand unknown environments. However, 3D environment modeling using acquired image sequences is a time-consuming task. When 3D environment modeling is performed using image sequences acquired in an unknown environment, the generated models do not always produce the expected result. Therefore, we consider that the quality of the generated 3D environment models could be quickly verified by realizing the sequential presentation of the generated models. To verify the effectiveness of the automatic process, we implemented it under different execution environments. Consequently, the automatic process could generate a 3D environment model from acquired image sequences.

論文

Cation interdiffusion in uranium-plutonium mixed oxide fuels; Where are we now?

Vauchy, R.; 廣岡 瞬; 松本 卓; 加藤 正人

Frontiers in Nuclear Engineering (Internet), 1, p.1060218_1 - 1060218_18, 2022/12

Diffusion phenomena in uranium-plutonium mixed oxides U$$_{1-y}$$PuyO$$_{2}$$ dictate the physicochemical properties of MOX nuclear fuel throughout manufacturing, irradiation and storage. More precisely, estimating the cation interdiffusion is paramount insofar as it dovetails with the actinide redistribution during sintering and under irradiation. In this paper, we propose a critical review of the existing experimental data of U and Pu interdiffusion coefficients in MOX fuel.

論文

Materials science and fuel technologies of uranium and plutonium mixed oxide

加藤 正人; 町田 昌彦; 廣岡 瞬; 中道 晋哉; 生澤 佳久; 中村 博樹; 小林 恵太; 小澤 隆之; 前田 宏治; 佐々木 新治; et al.

Materials Science and Fuel Technologies of Uranium and Plutonium mixed Oxide, 171 Pages, 2022/10

プルトニウム燃料を使用した革新的で先進的な原子炉が各国で開発されている。新しい核燃料を開発するためには、照射試験が不可欠であり、核燃料の性能と安全性を実証する必要がある。照射試験を補完する技術として、照射挙動を正確にシミュレートする技術を開発できれば、核燃料の研究開発にかかるコスト,時間,労力を大幅に削減でき、核燃料の照射挙動をシミュレーションすることで、安全性と信頼性を大幅に向上させることができる。核燃料の性能を評価するためには、高温での燃料の物理的および化学的性質を知る必要がある。そして、照射中に発生するさまざまな現象を記述した行動モデルの開発が不可欠である。以前の研究開発では、モデル開発の多くの部分で、フィッティングパラメータを使用した経験的手法が使用されてきた。経験的手法では、データがない領域では非常に異なる結果が得られる可能性がある。したがって、この研究では、燃料の基本的な特性を組成と温度に外挿できる科学的記述モデルを構築し、モデルが適用される照射挙動分析コードの開発を行った。

論文

Development of the DICOM-based Monte Carlo dose reconstruction system for a retrospective study on the secondary cancer risk in carbon ion radiotherapy

古田 琢哉; 古場 裕介*; 橋本 慎太郎; Chang, W.*; 米内 俊祐*; 松本 真之介*; 石川 諒尚*; 佐藤 達彦

Physics in Medicine & Biology, 67(14), p.145002_1 - 145002_15, 2022/07

 被引用回数:7 パーセンタイル:61.41(Engineering, Biomedical)

炭素線治療は従来の放射線治療よりも腫瘍部への線量集中性に関する優位性を持つが、二次的ながんの発生原因となり得る正常組織への照射を完全に無くすことは困難である。そのため、発がんリスクを照射炭素ビームの核反応によって生成される二次粒子による線量まで含めて評価するには、計算シミュレーション解析が有効となる。本研究では、PHITSコードを中核とした炭素線治療の線量再構築システムを開発した。このシステムでは、治療計画を記録したDICOMデータから自動でPHITSの入力ファイルを作成し、PHITSシミュレーションの実行によって腫瘍および周辺正常組織での線量分布を計算する。PHITSの様々な機能を利用することで、粒子毎の線量寄与や二次粒子の発生場所の特定など、詳細な解析が実施可能である。開発したシステムの妥当性は、水中での線量分布の実験結果や人体等価ファントムへの治療計画との比較により確認した。今後、本システムは量子科学技術研究開発機構において、過去の治療データを用いたシミュレーション解析による遡及的研究に利用される予定である。

論文

Relative oxygen potential measurements of (U,Pu)O$$_{2}$$ with Pu = 0.45 and 0.68 and related defect formation energy

廣岡 瞬; 松本 卓; 砂押 剛雄*; 日野 哲士*

Journal of Nuclear Materials, 558, p.153375_1 - 153375_8, 2022/01

 被引用回数:5 パーセンタイル:50.16(Materials Science, Multidisciplinary)

日立GEニュークリアエナジーでは、商用炉として実績のあるBWRをベースとして、高速中性子によりTRU元素を燃料として燃やすことができる資源再利用型BWR(RBWR)の開発が進められている。RBWRでは燃料設計上PuやMAの含有率が高くなる傾向があることから、本研究ではPu含有率が45at%及び68at%と、これまでの高速炉用MOXで研究されてきたものよりも高いPu含有率のMOXを対象に、酸素ポテンシャルの測定、評価を行った。還元しやすいPuの含有率が高くなると酸素ポテンシャルは高くなることが分かっているが、本研究の結果、Pu含有率68at%のMOXとPuO$$_{2}$$では大きな違いがないことが確認された。得られたデータから、MOXの酸素/金属原子数比(O/M),温度,Pu含有率,雰囲気の酸素分圧の関係式を導出し、さらに、解析の過程で得られる欠陥生成エネルギーから、電気伝導率や比熱の考察を行った。

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