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Journal Articles

Occupation sites and valence states of Co dopants in (La, Co)-codoped M-type Sr ferrite; $$^{57}$$Fe and $$^{59}$$Co nuclear magnetic resonance studies

Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ueda, Hiroaki*; Tanioku, Yasuaki*; Michioka, Chishiro*; Yoshimura, Kazuyoshi*; Takao, Kenta*; Shimoda, Aiko*; et al.

Physical Review B, 98(6), p.064403_1 - 064403_10, 2018/08

 Times Cited Count:10 Percentile:46.45(Materials Science, Multidisciplinary)

To specify preferential occupation sites of Co substituents and to clarify charge and spin states of Co ions in (La, Co)-cosubstituted hexagonal magnetoplumbite-type (M-type) Sr ferrite, $$^{57}$$Fe and $$^{59}$$Co nuclear magnetic resonance (NMR) spectra are measured under zero and external magnetic fields using powdered and single crystalline specimens. To a considerable degree, the charge compensation between La$$^{3+}$$ and Co$$^{2+}$$ works in the equal (La, Co)-codoped case, where more than half of the Co ions are considered to be present in the minority spin $$4f_1$$ sites at the center of the oxygen tetrahedra, with the $$S$$ = 3/2 state carrying a small orbital moment owing to spin-orbit interaction. The remaining small number of high-spin Co$$^{2+}$$ ($$S$$ = 3/2, $$L$$ = 1) ions with unquenched orbital moments would be distributed to the other octahedral $$12k$$, $$2a$$, and $$4f_2$$ sites.

Journal Articles

NMR investigation of spin fluctuations in the itinerant-electron magnetic compound $${rm Sr}_{1-x}{rm Ca}_x{rm Co}_2{rm P}_2$$

Imai, Masaki; Michioka, Chishiro*; Ueda, Hiroaki*; Yoshimura, Kazuyoshi*

Physical Review B, 95(5), p.054417_1 - 054414_7, 2017/02

 Times Cited Count:2 Percentile:11.64(Materials Science, Multidisciplinary)

We took $$^{31}$$P NMR measurements of mainly paramagnetic phase $${rm Sr}_{1-x}{rm Ca}_x{rm Co}_2{rm P}_2$$ to reveal the itinerant-electron metamagnetic transition, and of its magnetically ordered phase, and characterized their spin fluctuations by estimating the spin fluctuation parameter $$T_{0}$$ corresponding to the width of the spin fluctuation in the spectrum in frequency space. As $$x$$ increases from 0 to 0.5, the in-plane component of $$T_{0}$$ decreases proportionally with the metamagnetic transition field. In the antiferromagnetic cT phase, $$T_{0}$$ is constant and spin fluctuations show an isotropic character in contrast to their behavior in the paramagnetic ucT phase. These results indicate that the in-plane spin fluctuations due to the quasi-two-dimensional crystal structure play a significant role in the metamagnetic transition of this system.

Journal Articles

Observation of the partial Fermi surface quenching in the noncentrosymmetric superconductor Mo$$_3$$Al$$_2$$C

Koyama, Takehide*; Ozaki, Yuzuru*; Ueda, Koichi*; Mito, Takeshi*; Kohara, Takao*; Waki, Takeshi*; Tabata, Yoshikazu*; Michioka, Chishiro*; Yoshimura, Kazuyoshi*; Suzuki, Michito; et al.

Journal of the Physical Society of Japan, 81(Suppl.B), p.SB008_1 - SB008_5, 2012/12

 Times Cited Count:1 Percentile:10.83(Physics, Multidisciplinary)

The normal state properties of a noncentrosymmetric superconductor Mo$$_3$$Al$$_2$$C are studied by means of the nuclear magnetic resonance (NMR) experiment. The change of NMR line shape and the peak of the nuclear spin-echo decay rate at $$simeq$$ 130 K indicate that the Mo$$_3$$Al$$_2$$C exhibits the phase transition prior to the emergence of superconductivity. The reduction in the conduction electron density is inferred from the decrease in the nuclear spin-lattice relaxation rate. The nature of the newly found phase transition is discussed by considering the result of the first principle calculations, indicating a good nesting property of the Fermi surfaces.

Journal Articles

Partial gap opening on the Fermi surface of the noncentrosymmetric superconductor Mo$$_3$$Al$$_2$$C

Koyama, Takehide*; Ozaki, Yuzuru*; Ueda, Koichi*; Mito, Takeshi*; Kohara, Takao*; Waki, Tsuyoshi*; Tabata, Yoshikazu*; Michioka, Chishiro*; Yoshimura, Kazuyoshi*; Suzuki, Michito; et al.

Physical Review B, 84(21), p.212501_1 - 212501_4, 2011/12

 Times Cited Count:11 Percentile:44.74(Materials Science, Multidisciplinary)

The results of $$^{27}$$Al nuclear magnetic resonance and specific-heat measurements of the noncentrosymmetric superconductor Mo$$_3$$Al$$_2$$C are reported. The phase transition around 130 K is inferred from a distinct change in the NMR spectrum, a clear peak in the spin-echo decay rate, and an anomaly in the specific heat. Possibility of charge-density wave ordering around 130 K is discussed by calculating the Fermi surfaces in the normal states and considering the partial quenching of the Fermi surfaces with the decrease in 1/$$T$$$$_1$$ below the superconducting transition temperature.

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