Local structure analysis of BiFeO-BaTiO solid solutions

Yoneda, Yasuhiro; Kim, S.*; Mori, Shigeo*; Wada, Satoshi*

Japanese Journal of Applied Physics, 61(SN), p.SN1022_1 - SN1022_10, 2022/11

https://doi.org/10.35848/1347-4065/ac835d

Local structural analysis of the (1-) BiFeO-BaTiO solid solution was performed by PDF analysis of the data obtained in the synchrotron radiation high-energy X-ray diffraction experiment. First, when XAFS experiments were performed and sample screening was performed, it was found that structural fluctuations were large in the BiFeO-rich composition. Therefore, PDF analysis of a sample with BiFeO-rich composition was performed. As a result, it was found that although the average structure is a cubic structure, the local structure can be reproduced with a rhombohedral crystal structure, and there is a displacement that breaks the symmetry of the rhombohedral structure in a composition with a large fluctuation.

Development of numerical analysis codes for multi-level and multi-physics approaches in an advanced reactor design study

Tanaka, Masaaki; Doda, Norihiro; Mori, Takero; Yokoyama, Kenji; Uwaba, Tomoyuki; Okajima, Satoshi; Matsushita, Kentaro; Hashidate, Ryuta; Yada, Hiroki

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Japan Atomic Energy Agency is developing an innovative design system named ARKADIA to achieve the design of an advanced nuclear reactor as a safe, economic, and sustainable carbon-free energy source. In the first phase of its development, ARKADIA-Design for design study and ARKADIA-Safety for safety assessment will be developed individually. In this paper, focusing on the ARKADIA-Design, the concept of the system is described and numerical analysis codes to be used for the multi-level and multi-physics analyses are introduced. Descriptions of the practical functions composed by the analysis codes and the representative problems in application studies for validation are introduced.

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

https://doi.org/10.1038/s41550-020-01271-2

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Study of quasielastic barrier distributions as a step towards the synthesis of superheavy elements with hot fusion reactions

Tanaka, Taiki*; Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Boll, R. A.*; Brewer, N. T.*; Van Cleve, S.*; Dean, D. J.*; Ishizawa, Satoshi*; et al.

Physical Review Letters, 124(5), p.052502_1 - 052502_6, 2020/02

https://doi.org/10.1103/PhysRevLett.124.052502

Treatment technology of highly radioactive solid waste generated by experimental tests and sample analysis in reprocessing facilities

Goto, Yuichi; Inada, Satoshi; Kuno, Takehiko; Mori, Eito*

Nihon Hozen Gakkai Dai-16-Kai Gakujutsu Koenkai Yoshishu, p.221 - 224, 2019/07

Test equipment, containers, and analytical wastes, generated by experiments using spent fuel pieces in hot cell of Operation Testing Laboratory and by analysis of highly active liquid wastes in hot analytical cell line of Tokai Reprocessing Plant, are treated as highly radioactive solid wastes. These wastes are stored in specific shielded containers called waste cask and then transport to the storage facility. The treatment of these highly radioactive solid wastes have been carried out for 40 years with upgrading waste taking out system and transportation device. As a results, automation of several procedures have been achieved utilizing conventional equipment, and work efficiency and safety have been improved.

Determination of fusion barrier distributions from quasielastic scattering cross sections towards superheavy nuclei synthesis

Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.

Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01

https://doi.org/10.7566/JPSJ.87.014201

Excitation functions of quasielastic scattering cross sections for the Ca + Pb, Ti + Pb, and Ca + Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the Ca + Pb and Ti + Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the Ca + Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.

Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

Frandsen, B. A.*; Liu, L.*; Cheung, S. C.*; Guguchia, Z.*; Khasanov, R.*; Morenzoni, E.*; Munsie, T. J. S.*; Hallas, A. M.*; Wilson, M. N.*; Cai, Y.*; et al.

Nature Communications (Internet), 7, p.12519_1 - 12519_8, 2016/08

https://doi.org/10.1038/ncomms12519

Radiation monitoring using manned helicopter around the Fukushima Daiichi Nuclear Power Station in the fiscal year 2014 (Contract research)

Sanada, Yukihisa; Mori, Airi; Ishizaki, Azusa; Munakata, Masahiro; Nakayama, Shinichi; Nishizawa, Yukiyasu; Urabe, Yoshimi; Nakanishi, Chika; Yamada, Tsutomu; Ishida, Mutsushi; et al.

JAEA-Research 2015-006, 81 Pages, 2015/07

JAEA-Research-2015-006.pdf:22.96MB

By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (NPS), Tokyo Electric Power Company (TEPCO), caused by the East Japan earthquake and the following tsunami occurred on March 11, 2011, a large amount of radioactive materials was released from the NPP. These results of the aerial radiation monitoring using the manned helicopter in the fiscal 2014 were summarized in the report.

Radionuclide release to stagnant water in the Fukushima-1 Nuclear Power Plant

Nishihara, Kenji; Yamagishi, Isao; Yasuda, Kenichiro; Ishimori, Kenichiro; Tanaka, Kiwamu; Kuno, Takehiko; Inada, Satoshi; Goto, Yuichi

Journal of Nuclear Science and Technology, 52(3), p.301 - 307, 2015/03

https://doi.org/10.1080/00223131.2014.946455

After the severe accident at the Fukushima-1 nuclear power plant, large amounts of contaminated stagnant water have accumulated in turbine buildings and their surroundings. This rapid communication reports calculation of the radionuclide inventory in the core, collection of measured inventory in the stagnant water, and estimation of radionuclide release ratios from the core to the stagnant water. This evaluation is based on data obtained before June 3, 2011. The release ratios of tritium, iodine, and cesium were several tens of percent, whereas those of strontium and barium were smaller by one or two orders of magnitude. The release ratios in the Fukushima accident were equivalent to those in the TMI-2 accident.

Probing strongly correlated 4-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission

Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12

https://doi.org/10.7566/JPSJ.83.123702

We show that the strongly correlated 4-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRhSi and YbCuSi. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4 symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.