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Journal Articles

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and hydrogen production facility, 1; Overview of the HTTR heat application test plan to establish high safety coupling technology

Nomoto, Yasunobu; Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

Journal Articles

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and Hydrogen Production Facility, 2; Development plan for coupling equipment between HTTR and Hydrogen Production Facility

Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; Noguchi, Hiroki; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 6 Pages, 2023/05

Journal Articles

Hybrid process combining solvent extraction / low pressure loss extraction chromatography for a reasonable MA(III) recovery process

Sano, Yuichi; Sakamoto, Atsushi; Miyazaki, Yasunori; Watanabe, So; Morita, Keisuke; Emori, Tatsuya; Ban, Yasutoshi; Arai, Tsuyoshi*; Nakatani, Kiyoharu*; Matsuura, Haruaki*; et al.

Proceedings of International Conference on Nuclear Fuel Cycle; Sustainable Energy Beyond the Pandemic (GLOBAL 2022) (Internet), 4 Pages, 2022/07

We developed a hybrid MA(III) recovery process combining MA(III)+Ln(III) co-recovery flowsheet by solvent extraction with TBP and MA(III)/Ln(III) separation flowsheet by simulated moving bed chromatography using HONTA impregnated adsorbents with large particle size porous silica support.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

https://shop.elsevier.com/books/sodium-cooled-fast-reactors/morishita/978-0-12-824076-2

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Long-term density-dependent groundwater flow analysis and its effect on nuclide migration for safety assessment of high-level radioactive waste disposal with consideration of interaction between fractures and matrix of rock formation in coastal crystalline groundwater systems

Park, Y.-J.*; Sawada, Atsushi; Ozutsumi, Takenori*; Tanaka, Tatsuya*; Hashimoto, Shuji*; Morita, Yutaka*

Proceedings of 3rd International Conference on Discrete Fracture Network Engineering (DFNE 2022) (Internet), 8 Pages, 2022/00

Safety analysis for underground disposal facilities for high-level radioactive waste requires thorough understanding of long-term groundwater flow and nuclide migration processes in geologic media. In the coastal subsurface systems, groundwater flow is defined by the complex interactions between freshwater of meteoric origin and denser saline water from the sea. In addition, sea levels are expected to fluctuate significantly due to a transgression and regression of the sea over the millions of years for safety analysis. This study presents long-term evolution of groundwater environment such as salinity concentration and flow velocity with focus of the interaction between fractures and matrix blocks in regional and near-field scale analysis framework for groundwater flow and nuclide migration for underground disposal facilities in hypothetical fractured crystalline coastal systems.

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

https://doi.org/10.1016/C2018-0-05383-9

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Production of $$^{266}$$Bh in the $$^{248}$$Cm($$^{23}$$Na,5$$n$$)$$^{266}$$Bh reaction and its decay properties

Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.

Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08

https://doi.org/10.1103/PhysRevC.102.024625
 Times Cited Count：6 Percentile：59.56(Physics, Nuclear)

Journal Articles

Determination of fusion barrier distributions from quasielastic scattering cross sections towards superheavy nuclei synthesis

Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.

Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01

https://doi.org/10.7566/JPSJ.87.014201
 Times Cited Count：18 Percentile：74.47(Physics, Multidisciplinary)

Excitation functions of quasielastic scattering cross sections for the $$^{48}$$Ca + $$^{208}$$Pb, $$^{50}$$Ti + $$^{208}$$Pb, and $$^{48}$$Ca + $$^{248}$$Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the $$^{48}$$Ca + $$^{208}$$Pb and $$^{50}$$Ti + $$^{208}$$Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the $$^{48}$$Ca + $$^{248}$$Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.

Journal Articles

Study of the reaction $$^{48}$$Ca + $$^{248}$$Cm $$rightarrow$$ $$^{296}$$Lv$$^{ast}$$ at RIKEN-GARIS

Kaji, Daiya*; Morita, Kosuke*; Morimoto, Koji*; Haba, Hiromitsu*; Asai, Masato; Fujita, Kunihiro*; Gan, Z.*; Geissel, H.*; Hasebe, Hiroo*; Hofmann, S.*; et al.

Journal of the Physical Society of Japan, 86(3), p.034201_1 - 034201_7, 2017/03

https://doi.org/10.7566/JPSJ.86.034201
 Times Cited Count：28 Percentile：81.43(Physics, Multidisciplinary)

The fusion reaction of $$^{48}$$Ca + $$^{248}$$Cm $$rightarrow$$ $$^{296}$$Lv$$^{ast}$$ was studied using the gas-filled recoil-ion separator GARIS at RIKEN. A total of seven $$alpha$$ and spontaneous-fission decay chains were observed, which would originate from the reaction products of the element 116, $$^{292}$$Lv and $$^{293}$$Lv. Decay properties observed in the chains are in good agreement with the previously published ones. However, one of the chains showed a discrepancy, indicating the new spontaneous-fission branch in $$^{285}$$Cn or the production of the new isotope $$^{294}$$Lv.

Journal Articles

Complex chemistry with complex compounds

Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; D$"u$llmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.

EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12

https://doi.org/10.1051/epjconf/201613107005
 Times Cited Count：3 Percentile：72.98(Chemistry, Inorganic & Nuclear)

In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)$$_{6}$$. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO)$$_{6}$$, W(CO)$$_{6}$$, and Sg(CO)$$_{6}$$.

Journal Articles

Decomposition studies of group 6 hexacarbonyl complexes, 1; Production and decomposition of Mo(CO)$$_6$$ and W(CO)$$_6$$

Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; et al.

Radiochimica Acta, 104(3), p.141 - 151, 2016/03

https://doi.org/10.1515/ract-2015-2445
 Times Cited Count：31 Percentile：95.03(Chemistry, Inorganic & Nuclear)

Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO)$$_6$$. A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO)$$_6$$ and W(CO)$$_6$$, indicating that the first bond dissociation energy of Sg(CO)$$_6$$ could be determined with this technique.

Journal Articles

Production of $$^{88}$$Nb and $$^{170}$$Ta for chemical studies of element 105, Db, using the GARIS gas-jet system

Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05

https://doi.org/10.1007/s10967-014-3877-4
 Times Cited Count：3 Percentile：25.85(Chemistry, Analytical)

A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived $$^{88}$$Nb and $$^{170}$$Ta were produced with nuclear reactions using a $$^{19}$$F beam whose energy was the same as that to produce $$^{262}$$Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the $$^{88}$$Nb and $$^{170}$$Ta to a chemistry device for $$^{262}$$Db without changing other experimental conditions.

Journal Articles

In situ synthesis of volatile carbonyl complexes with short-lived nuclides

Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; D$"u$llmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03

https://doi.org/10.1007/s10967-014-3793-7
 Times Cited Count：15 Percentile：77.56(Chemistry, Analytical)

Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.

Journal Articles

Synthesis and detection of a Seaborgium carbonyl complex

Even, J.*; Yakushev, A.*; D$"u$llmann, Ch. E.*; Haba, Hiromitsu*; Asai, Masato; Sato, Tetsuya; Brand, H.*; Di Nitto, A.*; Eichler, R.*; Fan, F. L.*; et al.

Science, 345(6203), p.1491 - 1493, 2014/09

https://doi.org/10.1126/science.1255720
 Times Cited Count：63 Percentile：83.28(Multidisciplinary Sciences)

A new superheavy element complex, a seaborgium carbonyl, has been successfully synthesized, and its adsorption property has been studied using a cryo-thermochromatography and $$alpha$$-detection apparatus COMPACT. Nuclear reaction products of short-lived $$^{265}$$Sg preseparated with a gas-filled recoil ion separator GARIS at RIKEN were directly injected into a gas cell filled with He/CO mixture gas, and chemical reaction products of volatile carbonyl complexes were trasported to COMPACT. The Sg carbonyl complex detected with COMPACT was found to be very volatile with adsorption enthalpy of $$-$$50 kJ/mol, from which we have concluded that this complex should be a Sg hexacarbonyl Sg(CO)$$_{6}$$. This is the first synthesis of organometallic compounds of transactinide elements for which only simple inorganic comounds have been synthesized so far.

Journal Articles

Prepulse and amplified spontaneous emission effects on the interaction of a petawatt class laser with thin solid targets

Esirkepov, T. Z.; Koga, J. K.; Sunahara, Atsushi*; Morita, Toshimasa; Nishikino, Masaharu; Kageyama, Kei*; Nagatomo, Hideo*; Nishihara, Katsunobu; Sagisaka, Akito; Kotaki, Hideyuki; et al.

Nuclear Instruments and Methods in Physics Research A, 745, p.150 - 163, 2014/05

https://doi.org/10.1016/j.nima.2014.01.056
 Times Cited Count：45 Percentile：96.33(Instruments & Instrumentation)

Journal Articles

Production of $$^{262}$$Db in the $$^{248}$$Cm($$^{19}$$F,5$$n$$)$$^{262}$$Db reaction and decay properties of $$^{262}$$Db and $$^{258}$$Lr

Haba, Hiromitsu*; Huang, M.*; Kaji, Daiya*; Kanaya, Jumpei*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Murakami, Masashi*; Ozeki, Kazutaka*; Sakai, Ryutaro*; et al.

Physical Review C, 89(2), p.024618_1 - 024618_11, 2014/02

https://doi.org/10.1103/PhysRevC.89.024618
 Times Cited Count：25 Percentile：82.3(Physics, Nuclear)

Journal Articles

New result in the production and decay of an isotope, $$^{278}$$113 of the 113th element

Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.

Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10

https://doi.org/10.1143/JPSJ.81.103201
 Times Cited Count：167 Percentile：97.27(Physics, Multidisciplinary)

An isotope of the 113th element, $$^{278}$$113, was produced in a nuclear reaction with a $$^{70}$$Zn beam on a $$^{209}$$Bi target. We observed six consecutive $$alpha$$ decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of $$^{262}$$Db and $$^{258}$$Lr both in decay energies and decay times. This indicates that the present decay chain consisted of $$^{278}$$113, $$^{274}$$Rg (Z = 111), $$^{270}$$Mt (Z = 109), $$^{266}$$Bh (Z = 107), $$^{262}$$Db (Z = 105), and $$^{258}$$Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope $$^{278}$$113, of the 113th element.

Journal Articles

Production of $$^{265}$$Sg in the $$^{248}$$Cm($$^{22}$$Ne,5$$n$$)$$^{265}$$Sg reaction and decay properties of two isomeric states in $$^{265}$$Sg

Haba, Hiromitsu*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sakai, Ryutaro*; Sumita, Takayuki*; Yoneda, Akira*; Kasamatsu, Yoshitaka*; et al.

Physical Review C, 85(2), p.024611_1 - 024611_11, 2012/02

https://doi.org/10.1103/PhysRevC.85.024611
 Times Cited Count：52 Percentile：91.35(Physics, Nuclear)

Two isomeric states in $$^{265}$$Sg, i.e, $$^{265}$$Sg$$^{a}$$ and $$^{265}$$Sg$$^{b}$$ were produced in the $$^{248}$$Cm($$^{22}$$Ne,5$$n$$) reaction. Decay properties of $$^{265}$$Sg$$^{a,b}$$ were investigated with a rotating-wheel apparatus for $$alpha$$ and spontaneous fission (SF) spectrometry under low background condition attained by a gas-jet transport system coupled to the RIKEN gas-filled recoil ion separator. Based on genetically correlated $$alpha$$-$$alpha$$ (-$$alpha$$) and $$alpha$$-SF decay chains, 18 and 24 events were assigned to $$^{265}$$Sg$$^{a}$$ and $$^{265}$$Sg$$^{b}$$, respectively. The half-life and $$alpha$$-particle energy of $$^{265}$$Sg$$^{a}$$ were measured to be $$8.5^{+2.6}_{-1.6}$$ s and $$8.84 pm 0.05$$ MeV, respectively, and those of $$^{265}$$Sg$$^{b}$$ were $$14.4^{+3.7}_{-2.5}$$ s and $$8.69 pm 0.05$$ MeV.

Journal Articles

Isolation and characterization of the fragrant cyclamen ${it O}$-methyltransferase involved in flower coloration

Akita, Yusuke; Kitamura, Satoshi; Hase, Yoshihiro; Narumi, Issei; Ishizaka, Hiroshi*; Kondo, Emiko*; Kameari, Naoko*; Nakayama, Masayoshi*; Tanikawa, Natsu*; Morita, Yasumasa*; et al.

Planta, 234(6), p.1127 - 1136, 2011/12

https://doi.org/10.1007/s00425-011-1466-0
 Times Cited Count：41 Percentile：75.95(Plant Sciences)

Journal Articles

Production and decay properties of $$^{264}$$Hs and $$^{265}$$Hs

Sato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sumita, Takayuki*; Yoneda, Akira*; et al.

Journal of the Physical Society of Japan, 80(9), p.094201_1 - 094201_7, 2011/09

https://doi.org/10.1143/JPSJ.80.094201
 Times Cited Count：15 Percentile：65.33(Physics, Multidisciplinary)

Decay properties of $$^{264}$$Hs and $$^{265}$$Hs produced in the $$^{207,208}$$Pb($$^{58}$$Fe, $$xn$$) [$$x$$=1, 2] reactions were studied using a gas-filled recoil ion separator at the linear accelerator facility of RIKEN. A total of 6 decay chains were assigned to $$^{264}$$Hs. Cross sections for the $$^{264}$$Hs production in the $$^{208}$$Pb($$^{58}$$Fe,$$2n$$) and $$^{207}$$Pb($$^{58}$$Fe,$$n$$) reactions were measured to be $$2.8^{+6.5}_{-2.3}$$pb and $$6.9^{+4.4}_{-3.1}$$pb, respectively. The isotope $$^{264}$$Hs decayed with a half-life of $$0.751^{+0.518}_{-0.218}$$ms by $$alpha$$-particle emission and spontaneous fission. The $$alpha$$-particle energy of $$^{264}$$Hs was observed at 10.61$$pm$$0.04 and 10.80$$pm$$0.08 MeV. The spontaneous fission branch of $$^{264}$$Hs was found to be $$17^{+38}_{-14}%$$.

81 (Records 1-20 displayed on this page)