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JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2023)

Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Fujita, Natsuko; Yokoyama, Tatsunori; Ogita, Yasuhiro; Fukuda, Shoma; Nakajima, Toru; Kagami, Saya; Ogata, Manabu; et al.

JAEA-Review 2023-017, 27 Pages, 2023/10

JAEA-Review-2023-017.pdf:0.94MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2023. The objectives and contents in fiscal year 2023 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Quantitative micro-X-ray fluorescence scanning spectroscopy of wet sediment based on the X-ray absorption and emission theories; Its application to freshwater lake sedimentary sequences

Katsuta, Nagayoshi*; Takano, Masao*; Sano, Naomi; Tani, Yukinori*; Ochiai, Shinya*; Naito, Sayuri*; Murakami, Takuma*; Niwa, Masakazu; Kawakami, Shinichi*

Sedimentology, 66(6), p.2490 - 2510, 2019/10

 Times Cited Count:7 Percentile:49.6(Geology)

Micro-X-ray fluorescence (XRF) scanning spectroscopy of marine and lake sedimentary sequences can provide detailed paleoenvironmental records available through element intensities proxy data. However, problems for effects of interstitial pore water on the micro-XRF intensities have been pointed out so far because of direct measurement on the split wet sediment surfaces. In this study, new methods for the XRF corrections were developed by being considered with the micro-X-ray scanning spectroscopy.

Journal Articles

Development of function-graded proton exchange membrane for PEFC using heavy ion beam irradiation

Shiraki, Fumiya*; Yoshikawa, Taeko*; Oshima, Akihiro*; Oshima, Yuji*; Takasawa, Yuya*; Fukutake, Naoyuki*; Oyama, Tomoko*; Urakawa, Tatsuya*; Fujita, Hajime*; Takahashi, Tomohiro*; et al.

Nuclear Instruments and Methods in Physics Research B, 269(15), p.1777 - 1781, 2011/08

 Times Cited Count:8 Percentile:53.37(Instruments & Instrumentation)

The graded energy deposition of heavy ion beam irradiation to polymeric materials was utilized to synthesize a novel proton exchange membrane (PEM) with the graded density of sulfonic acid groups toward the thickness direction. Stacked Poly(tetrafluoroethylene-co-hexafluoropropylene) (FEP) films were irradiated by Xe$$^{54+}$$ ion beam with the energy of 6 MeV/u under a vacuum condition. Irradiated films were grafted with styrene monomer and then sulfonated. The membrane electrode assembly (MEA) fabricated by the function graded PEM showed improved fuel cell performance in terms of voltage stability. It was expected that the function-graded PEM could control the graded concentration of sulfonic acid groups in PEM.

Journal Articles

Study on depth profile of heavy ion irradiation effects in poly(tetrafluoroethylene-co-ethylene)

Gowa, Tomoko*; Shiotsu, Tomoyuki*; Urakawa, Tatsuya*; Oka, Toshitaka; Murakami, Takeshi*; Oshima, Akihiro*; Hama, Yoshimasa*; Washio, Masakazu*

Radiation Physics and Chemistry, 80(2), p.264 - 267, 2011/02

 Times Cited Count:8 Percentile:53.37(Chemistry, Physical)

High linear energy transfer (LET) heavy ion beams were irradiated to poly(tetrafluoroethylene-co-ethylene) (ETFE) under vacuum and in air. The irradiation effects in ETFE as a function of the depth was precisely evaluated by analyzing each one of the films of the irradiation samples which were made of stacked ETFE films. It was indicated that conjugated double bonds would be generated by heavy ion beam irradiation, and their amounts should show the Bragg-curve-like distributions. Also, it was suggested that higher LET beams would induce radical formation in high density and longer conjugated C=C double bonds could be generated by the second-order reactions. Moreover, for irradiation samples in air, C=O was produced correlating to the yield of oxygen molecules diffusing from the sample surface.

Journal Articles

Changes to the chemical structure of isotactic-polypropylene induced by ion-beam irradiation

Oka, Toshitaka; Oshima, Akihiro*; Motohashi, Ryota*; Seto, Naoto*; Watanabe, Yuji*; Kobayashi, Ryoji*; Saito, Koki*; Kudo, Hisaaki*; Murakami, Takeshi*; Washio, Masakazu*; et al.

Radiation Physics and Chemistry, 80(2), p.278 - 280, 2011/02

 Times Cited Count:7 Percentile:48.91(Chemistry, Physical)

The chemical structures of various ion-beam irradiated isotactic-polypropylene samples were studied. Results of micro-Fourier transform infrared spectroscopy and ultraviolet-visible spectroscopy suggest not only the linear energy transfer, but also the fluence is effective in local transformation of the isotactic-polypropylene.

Journal Articles

Ion beam irradiation effects on resist materials

Gowa, Tomoko*; Takahashi, Tomohiro*; Oka, Toshitaka; Murakami, Takeshi*; Oshima, Akihiro*; Tagawa, Seiichi*; Washio, Masakazu*

Journal of Photopolymer Science and Technology, 23(3), p.399 - 404, 2010/08

JAEA Reports

Long-term outlook of energy demand and supply in Japan; Estimation of energy demand and supply for "Nuclear Energy Vision 2100" of JAEA

Tatematsu, Kenji; Kawasaki, Hirotsugu; Nemoto, Masahiro; Murakami, Masakazu

JAEA-Research 2009-007, 46 Pages, 2009/06

JAEA-Research-2009-007.pdf:3.96MB

In this study, we showed an energy demand and supply scenario toward the year 2100 in Japan, which underlies JAEA's "Nuclear Energy Vision 2100" published in October 2008. This energy demand and supply scenario aims at the coexistence of the reduction of the carbon dioxide emission and the energy security through reduction of the fossil fuel usage, positive electrification and the nuclear energy usage. We reduce the ratio of the fossil fuel in the primary energy supply to about 1/3 and extend the share of renewable and nuclear energy to 70% from current 15%. As a result, the carbon dioxide emission is reduced to current 10%, and it developed that the half was the contribution of the nuclear energy.

Oral presentation

Analysis of radiation-induced cell death in vivo by in-air micro-PIXE

Hasegawa, Masatoshi*; Sakurai, Hideyuki*; Shin, Masako*; Okamoto, Masahiko*; Ishiuchi, Shogo*; Asakawa, Isao*; Tamamoto, Tetsuo*; Ono, Tatsuya*; Oikawa, Masakazu*; Kamiya, Tomihiro; et al.

no journal, , 

no abstracts in English

Oral presentation

Nuclear energy vision 2100; Toward a low carbon society

Murakami, Masakazu

no journal, , 

JAEA works to show the public easy-to-understand basic information on future energy supply and demand hoping to encourage vigorous discussion. In this study, a variety of technological options are quantitatively examined on their effectiveness in reducing emissions and stabilizing energy supplies and shown as a simple supply and demand scenario toward the year 2100.

Oral presentation

Nuclear energy vision 2100; Toward a low carbon society

Murakami, Masakazu

no journal, , 

Outline of "the Nuclear Energy Vision 2100", which JAEA published in October 2008 will be reported along with some reactions received.

Oral presentation

Changes of the chemical structures of isotactic-polypropylene induced by ion-beam irradiation

Oka, Toshitaka; Oshima, Akihiro*; Motohashi, Ryota*; Seto, Naoto*; Watanabe, Yuji*; Kobayashi, Ryoji*; Kudo, Hisaaki*; Murakami, Takeshi*; Washio, Masakazu*; Hama, Yoshimasa*

no journal, , 

Oral presentation

Study on depth profile of heavy ion irradiation effects in poly(tetrafluoroethylene-co-ethylene)

Gowa, Tomoko*; Shiotsu, Tomoyuki*; Urakawa, Tatsuya*; Oka, Toshitaka; Murakami, Takeshi*; Oshima, Akihiro*; Hama, Yoshimasa*; Washio, Masakazu*

no journal, , 

Oral presentation

Study on direct etching of fluoropolymers by heavy ion beam irradiation

Takasawa, Yuya*; Fukutake, Naoyuki*; Takahashi, Tomohiro*; Urakawa, Tatsuya*; Oshima, Yuji*; Gowa, Tomoko*; Shiraki, Fumiya*; Fujita, Hajime*; Oka, Toshitaka; Murakami, Takeshi*; et al.

no journal, , 

Oral presentation

Oral presentation

Development of functionally-graded materials using high energy heavy ion beam

Oshima, Akihiro*; Shiraki, Fumiya*; Takasawa, Yuya*; Fujita, Hajime*; Yoshikawa, Taeko*; Tatsumi, Takahiro*; Tsubokura, Hidehiro*; Takahashi, Tomohiro*; Gowa, Tomoko*; Sakaue, Kazuyuki*; et al.

no journal, , 

no abstracts in English

Oral presentation

Post-irradiation effects on the chemical structure of the ion-beam irradiated isotactic-polypropylene

Oka, Toshitaka; Oshima, Akihiro*; Kudo, Hisaaki*; Murakami, Takeshi*; Washio, Masakazu*; Hama, Yoshimasa*

no journal, , 

Oral presentation

Fabrication of functionally gradient PEM using heavy ion beams grafting

Washio, Masakazu*; Shiraki, Fumiya*; Oshima, Yuji*; Takasawa, Yuya*; Fujita, Hajime*; Gowa, Tomoko*; Kudo, Hisaaki*; Oka, Toshitaka; Hama, Yoshimasa*; Murakami, Takeshi*; et al.

no journal, , 

no abstracts in English

Oral presentation

Modification of STACY for study of criticality characteristics of fuel debris, 6; Progress on manufacture and construction of the modified STACY

Maekawa, Tomoyuki; Seki, Masakazu; Sumiya, Masato; Araki, Shohei; Murakami, Takahiko; Hasegawa, Kenta; Yoshikawa, Tomoki; Mori, Takashi*; Ishii, Junichi; Kobayashi, Fuyumi; et al.

no journal, , 

As previously reported, to clarify critical characteristics of fuel debris, the Static Experiment Critical Facility (STACY) is being converted to the heterogenous thermal system using fuel rods and light water moderator from the homogenous system using solution fuel. Seismic reinforcement of the support structure of the core tank started in 2022. This report presents progress on manufacture and construction of the modified STACY in 2021 and 2022.

Oral presentation

Paleoenvironment variations in southern Lake Baikal during the 150 kyrs using the lake sediment cores

Itayama, Yui*; Hayano, Asuka*; Kamegai, Yushi*; Yasuda, Shiori*; Murakami, Takuma*; Ochiai, Shinya*; Niwa, Masakazu; Katsuta, Nagayoshi*

no journal, , 

In this presentation, we report paleo-environmental changes in the southern region of Lake Baikal by chemical and grain-size analyses for the lake sediment cores.

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