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ceramicsVauchy, R.; Hirooka, Shun; Watanabe, Masashi; Yokoyama, Keisuke; Sunaoshi, Takeo*; Yamada, Tadahisa*; Nakamichi, Shinya; Murakami, Tatsutoshi
Ceramics International, 49(2), p.3058 - 3065, 2023/01
Times Cited Count：1 Percentile：0.01(Materials Science, Ceramics)Matsuyama, Tsugufumi*; Nakae, Masanori*; Murakami, Masashi; Yoshida, Yukihiko; Machida, Masahiko; Tsuji, Koichi*
Spectrochimica Acta, Part B, 199, p.106593_1 - 106593_6, 2023/01
Times Cited Count：0 Percentile：0.09(Spectroscopy)Kato, Masato; Nakamichi, Shinya; Hirooka, Shun; Watanabe, Masashi; Murakami, Tatsutoshi; Ishii, Katsunori
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 8 Pages, 2023/00
Uranium and Plutonium mixed oxide (MOX) pellets used as fast reactor fuels have been produced from several raw materials by mechanical blending method through processes of ball milling, additive blending, granulation, pressing, sintering and so on. It is essential to control the pellet density which is one of the important fuel specifications, but it is difficult to understand relationships among many parameters in the production. Database for MOX production was prepared from production results in Japan, and input data of eighteen types were chosen from production process and made a data set. Machine learning model to predict sintered density of MOX pellet was derived by gradient boosting regressor, and represented the measured sintered density with coefficient of determination of R
=0.996
Okada, Shota; Murakami, Masashi; Kochiyama, Mami; Izumo, Sari; Sakai, Akihiro
JAEA-Testing 2022-002, 66 Pages, 2022/08
JAEA-Testing-2022-002.pdf:2.46MB
Japan Atomic Energy Agency is an implementing organization of burial disposal for low-level radioactive waste generated from research, industrial and medical facilities in Japan. Radioactivity concentrations of the waste are essential information for design of the disposal facility and for licensing process. A lot of the waste subjected to the burial disposal is arising from dismantling of nuclear facilities. Radioactive Wastes Disposal enter has therefore discussed a procedure to evaluate the radioactivity concentrations by theoretical calculation for waste arising from the dismantling of the research reactors facilities and summarized the common procedure. The procedure includes evaluation of radioactive inventory by activation calculation, validation of the calculation results, and determination of the disposal classification as well as organization of the data on total radioactivity and maximum radioactivity concentration for each classification. For the evaluation of radioactive inventory, neutron flux and energy spectra are calculated at each region in the reactor facility using two- or three-dimensional neutron transport code. The activation calculation is then conducted for 140 nuclides using the results of neutron transport calculation and an activation calculation code. The recommended codes in this report for neutron transport calculation are two-dimensional discrete ordinate code DORT, three-dimensional discrete ordinate code TORT, or Monte Carlo codes MCNP and PHITS, and for activation calculation is ORIGEN-S. Other recommendation of cross-section libraries and calculation conditions are also indicated in this report. In the course of the establishment of the procedure, Radioactive Wastes Disposal Center has discussed the commonly available procedure at meetings. It has periodically held to exchange information with external operators which have research reactor facilities. The procedure will properly be reviewed and be revised by reflecting future situ
Murakami, Masashi; Sasaki, Toshiki
JAEA-Review 2022-004, 106 Pages, 2022/06
JAEA-Review-2022-004.pdf:3.95MB
A numerous analytical data will be required for the characterization of the radioactive waste stored in Japan Atomic Energy Agency toward their processing and disposal. A "Data Quality Objectives (DQO) Process" is widely applied as a tool for the development of a cost-effective characterization plan in the overseas nuclear sites. The DQO Process is a multi-step planning process developed by the United States Environmental Protection Agency (EPA), and can be used for the planning of a scientifically rigorous and cost-effective data collection program for the various projects involving the collection of the environmental data. We have considered to reduce the cost required for the future characterization of the stored waste by applying the statistical methods and have performed a literature survey on the DQO Process. The survey effort was focused on the guidance documents of the DQO Process published by the EPA and was also spent for the related matters such as a quality system of the EPA and the activities beyond the DQO Process as well as the examples of the application at the nuclear sites. In this report, the details on the planning procedure using the DQO Process are reviewed together with the background information such as why DQO Process was developed, what kind of transition was occurred, and how it is currently used in the EPA. The examples on the application for various objects at Hanford Site in the United States, where has the various legacy waste generated in the past activities and has the big environmental problems, are also reviewed. This report summarizes the important matters and methodology on the planning with the statistical sampling methods. It also provides the examples of the approaches for the complex objects, and will therefore be helpful in the future planning for the various kind of the waste characterization.
Fuchita, Tomoki*; Urata, Taisei*; Matsuyama, Tsugufumi*; Murakami, Masashi; Yoshida, Yukihiko; Ueda, Akihiko; Machida, Masahiko; Sasaki, Toshiki; Tsuji, Koichi*
X-sen Bunseki No Shimpo, 53, p.77 - 87, 2022/03
X-ray fluorescence (XRF) analysis is an analytical method to obtain elemental information by detecting fluorescence X-rays emitted from a sample irradiated with X-rays. It is possible to obtain two-dimensional elemental distribution images by scanning a sample with micro X-ray beam. In this study, we developed an XRF analytical instrument to rapidly obtain the elemental distributions for moving samples on a belt conveyor by applying the micro XRF technique. X-rays were widely irradiated to the belt conveyor. The elemental distributions were measured by scanning an X-ray detector, crossing above the belt conveyor. A collimator was attached to the top of the detector to limit the analyzing area. Both detection limit and spatial resolutions for moving directions of the detector and the belt conveyor were evaluated. Finally, it was demonstrated that the multi-elemental imaging was possible with the developed XRF instrument.
Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Ando, Masanori; Miyazaki, Masashi
Proceedings of ASME 2021 Pressure Vessels and Piping Conference (PVP 2021) (Internet), 9 Pages, 2021/07
Buckling evaluation methods capable of evaluating elasto-plastic buckling under axial compression, bending, and shear loads are required for cylindrical vessels of fast reactors to cope with thinning due to increasing diameter and application to the seismic isolation design against huge seismic ground motion. In this study, in order to confirm the applicability of the proposal evaluation method, several buckling tests and FE analyses were carried out using the specimens made of Modified 9Cr-1Mo steel. The buckling modes and strength data in the load region where the interaction of cyclic axial compression, bending and shear buckling could occur were examined. As a result, it was confirmed that the proposal evaluation method estimated the buckling load in the tests conservatively. Moreover, a series of finite element analyzes using a model with residual stress due to welding revealed that the effect of residual stress on buckling strength is negligible in the evaluation method.
Nakagawa, Akinori; Oyokawa, Atsushi; Murakami, Masashi; Yoshida, Yukihiko; Sasaki, Toshiki; Okada, Shota; Nakata, Hisakazu; Sugaya, Toshikatsu; Sakai, Akihiro; Sakamoto, Yoshiaki
JAEA-Technology 2021-006, 186 Pages, 2021/06
JAEA-Technology-2021-006.pdf:54.45MB
Radioactive wastes generated from R&D activities have been stored in Japan Atomic Energy Agency. In order to reduce the risk of taking long time to process legacy wastes, countermeasures for acceleration of waste processing and disposal were studied. Work analysis of waste processing showed bottleneck processes, such as evaluation of radioactivity concentration, segregation of hazardous and combustibles materials. Concerning evaluation of radioactivity concentration, a radiological characterization method using a scaling factor and a nondestructive gamma-ray measurement should be developed. The number of radionuclides that are to be selected for the safety assessment of the trench type disposal facility can decrease using artificial barriers. Hazardous materials, will be identified using records and nondestructive inspection. The waste identified as hazardous will be unpacked and segregated. Preliminary calculations of waste acceptance criteria of hazardous material concentrations were conducted based on environmental standards in groundwater. The total volume of the combustibles will be evaluated using nondestructive inspection. The waste that does not comply with the waste acceptance criteria should be mixed with low combustible material waste such as dismantling concrete waste in order to satisfy the waste acceptance criteria on a disposal facility average. It was estimated that segregation throughput of compressed waste should be increased about 5 times more than conventional method by applying the countermeasures. Further study and technology development will be conducted to realize the plan.
Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Ando, Masanori; Miyazaki, Masashi
Proceedings of ASME 2020 Pressure Vessels and Piping Conference (PVP 2020) (Internet), 9 Pages, 2020/08
Buckling evaluation methods capable of evaluating elasto-plastic buckling under axial compression, bending, and shear loads are required for cylindrical vessels of fast reactors to cope with thinning due to increasing diameter and application to the seismic isolation design against huge seismic ground motion. In this study, in order to confirm the applicability of the proposal evaluation method, several buckling tests and FE analyses were carried out using the specimens made of Modified 9Cr-1Mo steel. The buckling modes and strength data in the load region where the interaction of axial compression, bending and shear buckling could occur were examined. As a result, it was confirmed that the proposal evaluation method estimated the buckling load in the tests conservatively. In addition, buckling strength evaluated by elasto-plastic buckling analysis had good accuracy compared to each test result by considering the stress-strain relationship and imperfection of test specimen.
Murakami, Masashi; Hoshino, Yuzuru; Nakatani, Takayoshi; Sugaya, Toshikatsu; Fukumura, Nobuo*; Sanda, Toshio*; Sakai, Akihiro
JAEA-Technology 2019-003, 50 Pages, 2019/06
JAEA-Technology-2019-003.pdf:4.42MB
Toward the establishment of a common approach to determine the radioactivity concentrations in dismantling wastes arising from research reactors, radionuclide concentrations in the reactor structure materials of aluminum, carbon steel, shield concrete, and graphite of TRIGA Mark II reactor at Rikkyo University, Japan, were evaluated with both radiochemical analysis and theoretical calculation. The measured nuclides by the radiochemical analysis were 
H, 
Co, and 
Ni in aluminum, H, Co, Ni, and 
Eu in carbon steel, H, Co, and Eu in shield concrete, and H, 
C, Co, Ni, and Eu in graphite. Neutron-flux distributions and neutron-induced activities were computed with DORT and ORIGEN-ARP codes, respectively. Using the results of material composition analysis, radioactivity concentrations were conservatively predicted with good accuracy except for graphite material.
acidic solutionsYokoyama, Akihiko*; Kitayama, Yuta*; Fukuda, Yoshiki*; Kikunaga, Hidetoshi*; Murakami, Masashi*; Komori, Yukiko*; Yano, Shinya*; Haba, Hiromitsu*; Tsukada, Kazuaki; Toyoshima, Atsushi*
Radiochimica Acta, 107(1), p.27 - 32, 2019/01
Times Cited Count：1 Percentile：13.66(Chemistry, Inorganic & Nuclear)Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.
Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01
Times Cited Count：14 Percentile：71.95(Physics, Multidisciplinary)Excitation functions of quasielastic scattering cross sections for the 
Ca + 
Pb, 
Ti + Pb, and Ca + 
Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the Ca + Pb and Ti + Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the Ca + Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.
-delayed fission of 
AmWilson, G. L.*; Takeyama, Mirei*; Andreyev, A. N.; Andel, B.*; Antalic, S.*; Catford, W. N.*; Ghys, L.*; Haba, Hiromitsu*; He
berger, F. P.*; Huang, M.*; et al.
Physical Review C, 96(4), p.044315_1 - 044315_7, 2017/10
Times Cited Count：5 Percentile：45.02(Physics, Nuclear)Ca + Cm 
Lv
at RIKEN-GARISKaji, Daiya*; Morita, Kosuke*; Morimoto, Koji*; Haba, Hiromitsu*; Asai, Masato; Fujita, Kunihiro*; Gan, Z.*; Geissel, H.*; Hasebe, Hiroo*; Hofmann, S.*; et al.
Journal of the Physical Society of Japan, 86(3), p.034201_1 - 034201_7, 2017/03
Times Cited Count：23 Percentile：81.4(Physics, Multidisciplinary)The fusion reaction of Ca + Cm Lv was studied using the gas-filled recoil-ion separator GARIS at RIKEN. A total of seven 
and spontaneous-fission decay chains were observed, which would originate from the reaction products of the element 116, 
Lv and 
Lv. Decay properties observed in the chains are in good agreement with the previously published ones. However, one of the chains showed a discrepancy, indicating the new spontaneous-fission branch in 
Cn or the production of the new isotope 
Lv.
Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; D
llmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.
EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12
Times Cited Count：2 Percentile：63.24In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)
. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO), W(CO), and Sg(CO).
and W(CO)Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; et al.
Radiochimica Acta, 104(3), p.141 - 151, 2016/03
Times Cited Count：30 Percentile：95.82(Chemistry, Inorganic & Nuclear)Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO). A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO) and W(CO), indicating that the first bond dissociation energy of Sg(CO) could be determined with this technique.
Kaji, Daiya*; Morimoto, Koji*; Wakabayashi, Yasuo*; Takeyama, Mirei*; Yamaki, Sayaka*; Tanaka, Kengo*; Haba, Hiromitsu*; Huang, M.*; Murakami, Masashi*; Kanaya, Jumpei*; et al.
JPS Conference Proceedings (Internet), 6, p.030107_1 - 030107_4, 2015/06
Performance of the new gas-filled recoil ion separator GARIS-II was investigated using asymmetric 
Ne-induced fusion reactions. The use of He-H mixture gas for the gas-filled magnet significantly reduced background scattered particles detected at the focal-plane Si detector, and increased a transmission of the asymmetric reaction products. A target-identification system was newly installed for efficient measurements of excitation functions without changing beam energy nor target.
Nb and 
Ta for chemical studies of element 105, Db, using the GARIS gas-jet systemHuang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05
Times Cited Count：3 Percentile：27.78(Chemistry, Analytical)A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived Nb and Ta were produced with nuclear reactions using a 
F beam whose energy was the same as that to produce 
Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the Nb and Ta to a chemistry device for Db without changing other experimental conditions.
Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03
Times Cited Count：14 Percentile：78(Chemistry, Analytical)Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.
Watanabe, Hitoshi; Nakano, Masanao; Fujita, Hiroki; Takeyasu, Masanori; Mizutani, Tomoko; Isozaki, Tokuju; Morisawa, Masato; Nagaoka, Mika; Hokama, Tomonori; Yokoyama, Hiroya; et al.
JAEA-Review 2014-042, 175 Pages, 2015/01
JAEA-Review-2014-042.pdf:10.89MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2013 to March 2014. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Co. in March 2011.
