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JAEA Reports

Horonobe Underground Research Laboratory Project Investigation report for the 2024 fiscal year

Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Fukatsu, Yuta; Mochizuki, Akihito; Ozaki, Yusuke; et al.

JAEA-Review 2025-042, 136 Pages, 2025/12

JAEA-Review-2025-042.pdf:12.95MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe-cho in Hokkaido, north Japan. In the fiscal year 2024, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on near-field system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100$$^{circ}$$C" were addressed for "Demonstration of repository design options". The validation of a method for assessing permeability using the Ductility Index and a method for estimating the state of in-situ ground pressure from hydraulic perturbation tests were investigated as part of the study "Understanding of buffering behaviour of sedimentary rock to natural perturbations". In FY2024, we continued construction of the East Access Shaft and the Ventilation Shaft, and construction of these shafts were completed to a depth of 500 m. After the completion of the East Access Shaft, excavation of the West Access Shaft and 500 m gallery has began. As of the end of FY2024, excavation progress is as follows, the East Access Shaft and the Ventilation Shaft were 500 m depth, the West Access Shaft was 472 m depth, 500 m gallery was 112.9 m, respectively. In the Horonobe International Project (HIP), Management Board and Joint Task Meeting was held at the Horonobe URL in June 2024 to review the progress of construction of galleries and preparations of experiments. Task Meetings to review the implementation plan for in-situ testing and analysis were also held. HIP will be implemented in two phases: Phase 1 (from FY2022 to FY2024) and Phase 2 (from FY2025 to FY2028), the research results of Phase 1 were compiled in FY2024.

JAEA Reports

Horonobe Underground Research Laboratory Project Investigation Program for the Fiscal Year 2025

Nakayama, Masashi; Ishii, Eiichi; Hayano, Akira; Aoyagi, Kazuhei; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Mochizuki, Akihito; Ozaki, Yusuke; Kimura, Shun; et al.

JAEA-Review 2025-027, 80 Pages, 2025/09

JAEA-Review-2025-027.pdf:6.22MB

The Horonobe Underground Research Laboratory Project is being pursued by the Japan Atomic Energy Agency to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2025, we continue R&D on "Study on near-field system performance in geological environment" and "Demonstration of repository design options". These are identified as key R&D challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. In the "Study on near-field system performance in geological environment", we continue to obtain data from the full-scale engineered barrier system performance experiment, and work on the specifics of the full-scale engineered barrier system dismantling experiment. As for "Demonstration of repository design options", the investigation, design, and evaluation techniques are to be systemized at various scales, from the tunnel to the pit, by means of an organized set of evaluation methodologies for confinement performance at these respective scales. Preliminary borehole investigations will be conducted within a 500 m gallery, with the objectives of obtaining rock strength and rock permeability data, as well as surveying the extent of the excavation damaged zone surrounding the test tunnel via tomographic analysis. A planning study for the in-situ construction test will be conducted to investigate the construction of backfill material and watertight plugs. The volume of water inflow associated with the excavation of the 500 m gallery will be observed, and its magnitude will be compared with the range of water inflow predicted in the analysis. The test plan to determine the extent of the excavation damaged zone around the pit, which is planned to be constructed in the 500 m gallery, will be studied to determine the in-situ excavation damaged zone. In addition, the investigation and evaluation methods for the amount of water inflow from fractures and the extent of the excavation damaged zone around the pit will be organized. Concerning the construction and maintenance of the subsurface facilities, excavation of the West Access Shaft and the 500 m gallery will continue. It is anticipated that the construction of the facilities will be completed by the end of the fiscal year 2025. In addition, we continue R&D on the following three tasks in the Horonobe International Project; Task A: Solute transport experiment with model testing, Task B: Systematic integration of repository technology options, and Task C: Full-scale engineered barrier system dismantling experiment.

Journal Articles

Discrimination of disposal-restricted materials in waste containers by nondestructive testing and image analysis with high-energy X-ray computed tomography

Murakami, Masashi; Yoshida, Yukihiko; Nango, Nobuhito*; Kubota, Shogo*; Kurosawa, Takuya*; Sasaki, Toshiki

Journal of Nuclear Science and Technology, 62(7), p.650 - 661, 2025/07

 Times Cited Count:1 Percentile:68.76(Nuclear Science & Technology)

Journal Articles

Development of the buckling evaluation method for thick cylindrical vessels with a conical section in fast reactors made of austenitic stainless steel

Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Watakabe, Tomoyoshi; Ando, Masanori; Miyazaki, Masashi

Proceedings of the ASME 2025 Pressure Vessels & Piping Conference (PVP2025) (Internet), 8 Pages, 2025/07

Journal Articles

Development of radiological characterization method for research reactor decommissioning in JAEA

Kochiyama, Mami; Murakami, Masashi; Kubota, Shintaro; Sakai, Akihiro

Proceedings of International Conference on Nuclear Decommissioning; Addressing the Past and Ensuring the Future 2023 (Internet), 5 Pages, 2025/00

Japan Atomic Energy Agency has been studied radioactivity evaluation methods with activation calculations as part of those for radioactive waste generated by the decommissioning of research reactors. As part of the study, calculation tools and libraries have been evaluated. Activation calculations were performed using the ORIGEN or ORIGEN-S codes and the cross-section library attached to the SCALE system or JENDL/AD-2017 library, and the results were compared.

Journal Articles

Development of the buckling evaluation method for large scale vessels in fast reactors made of grade 91 steel and austenitic stainless steel with large initial imperfections

Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Watakabe, Tomoyoshi; Ando, Masanori; Miyazaki, Masashi

Proceedings of the ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 8 Pages, 2024/07

We have developed the buckling strength equations of vessels for fast reactors with seismic isolation system. The applicability of the buckling equations was confirmed by a series of buckling tests and analyses under monotonic or cyclic axial compressive load accompanied with constant horizontal load in the previous reports. In this report, we proposed a correction factor to reduce the buckling strength calculated by the buckling equations for large initial imperfections. A series of elastic-plastic buckling analyses considering large displacement and large strain theories was conducted to Grade 91 steel and austenitic stainless steel vessels which has a wide range of dimensions, initial imperfection amplitude, and vertical/horizontal load ratio. The simulation results showed that the correction factor generally shows a reduction tendency of buckling strength corresponding to initial imperfection amplitude, and the modified buckling equations are applicable to the vessels in fast reactors even for large initial imperfection amplitude which exceeds half the wall thickness.

Journal Articles

Application of Bayesian estimation to X-ray fluorescent image

Matsuyama, Tsugufumi*; Igarashi, Momo*; Yasuda, Sora*; Murakami, Masashi; Yoshida, Yukihiko; Hayashi, Kazunori*; Machida, Masahiko; Tsuji, Koichi*

Analytical Chemistry, 9 Pages, 2024/01

Journal Articles

Lattice parameters of fluorite-structured uranium-americium mixed oxides

Vauchy, R.; Hirooka, Shun; Watanabe, Masashi; Yokoyama, Keisuke; Murakami, Tatsutoshi

Journal of Nuclear Materials, 584, p.154576_1 - 154576_11, 2023/10

 Times Cited Count:8 Percentile:82.99(Materials Science, Multidisciplinary)

JAEA Reports

Strategic roadmap for back-end technology development

Nakazawa, Osamu; Takiya, Hiroaki; Murakami, Masashi; Donomae, Yasushi; Meguro, Yoshihiro

JAEA-Review 2023-012, 6 Pages, 2023/08

JAEA-Review-2023-012.pdf:0.93MB

The selection of back-end technology development issues to be prioritized and their schedule of the Japan Atomic Energy Agency (JAEA) have been put together as the "Strategic Roadmap for Back-end Technology Development." The results of questionnaires on development technologies (seeds) and technical issues (needs) within JAEA conducted in FY2022 were reflected in the selection. The issues were extracted from among those that match the seeds and needs, from the perspective of early implementation in the work front and the perspective of common issues, and nine themes were selected. We will build a cross-organizational implementation framework within JAEA and aim to implement the development results in the work front as well as social implementation.

Journal Articles

Machine learning sintering density prediction model for MOX fuel pellet

Kato, Masato; Nakamichi, Shinya; Hirooka, Shun; Watanabe, Masashi; Murakami, Tatsutoshi; Ishii, Katsunori

Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 22(2), p.51 - 58, 2023/04

Uranium and Plutonium mixed oxide (MOX) pellets used as fast reactor fuels have been produced from several raw materials by mechanical blending method through processes of ball milling, additive blending, granulation, pressing, sintering and so on. It is essential to control the pellet density which is one of the important fuel specifications, but it is difficult to understand relationships among many parameters in the production. Database for MOX production was prepared from production results in Japan, and input data of eighteen types were chosen from production process and made a data set. Machine learning model to predict sintered density of MOX pellet was derived by gradient boosting regressor, and represented the measured sintered density with coefficient of determination of R$$^{2}$$=0.996

Journal Articles

Fundamental research of X-ray absorption imaging for elemental identification using a secondary target

Nakae, Masanori*; Matsuyama, Tsugufumi*; Murakami, Masashi; Yoshida, Yukihiko; Machida, Masahiko; Tsuji, Koichi*

Advances in X-Ray Chemical Analysis, Japan, 54, p.89 - 99, 2023/03

Fundamental research on X-ray absorption imaging for elemental identification was studied. A secondary target was applied to obtain X-ray absorption images above and below the X-ray absorption edge of the target element. X-rays from an X-ray tube were irradiated to the secondary target, where the characteristic X-rays were emitted that were irradiated to the sample. X-ray absorption images were acquired with an exposure time of a few seconds with an X-ray camera. In this technique, it is difficult to change the energy of X-rays as we want, however we can apply this technique for imaging the specific element. Metal foil sample composed of Al, Cu, and Ni was analyzed. To obtain an X-ray elemental image of Ni, two X-ray absorption images were taken using the X-rays above and below the Ni K-edge. X-rays of Cu K$$alpha$$ and Zn K$$alpha$$ were prepared by using Cu and Zn plates as the secondary target. Finally, the Ni elemental image was obtained by subtracting two images. Furthermore, the X-ray camera had a function of setting critical energies for imaging, thus it was demonstrated that an X-ray elemental image of Ni was obtained using a single secondary target without changing the secondary target.

Journal Articles

Liquid phase sintering of alumina-silica co-doped cerium dioxide CeO$$_{2}$$ ceramics

Vauchy, R.; Hirooka, Shun; Watanabe, Masashi; Yokoyama, Keisuke; Sunaoshi, Takeo*; Yamada, Tadahisa*; Nakamichi, Shinya; Murakami, Tatsutoshi

Ceramics International, 49(2), p.3058 - 3065, 2023/01

 Times Cited Count:11 Percentile:54.21(Materials Science, Ceramics)

Journal Articles

Spectrum prediction in X-ray fluorescence analysis using Bayesian estimation

Matsuyama, Tsugufumi*; Nakae, Masanori*; Murakami, Masashi; Yoshida, Yukihiko; Machida, Masahiko; Tsuji, Koichi*

Spectrochimica Acta, Part B, 199, p.106593_1 - 106593_6, 2023/01

 Times Cited Count:3 Percentile:28.49(Spectroscopy)

JAEA Reports

Common evaluation procedure radioactivity concentration by theoretical calculation for radioactive waste generated from the decommissioning of research reactors

Okada, Shota; Murakami, Masashi; Kochiyama, Mami; Izumo, Sari; Sakai, Akihiro

JAEA-Testing 2022-002, 66 Pages, 2022/08

JAEA-Testing-2022-002.pdf:2.46MB

Japan Atomic Energy Agency is an implementing organization of burial disposal for low-level radioactive waste generated from research, industrial and medical facilities in Japan. Radioactivity concentrations of the waste are essential information for design of the disposal facility and for licensing process. A lot of the waste subjected to the burial disposal is arising from dismantling of nuclear facilities. Radioactive Wastes Disposal enter has therefore discussed a procedure to evaluate the radioactivity concentrations by theoretical calculation for waste arising from the dismantling of the research reactors facilities and summarized the common procedure. The procedure includes evaluation of radioactive inventory by activation calculation, validation of the calculation results, and determination of the disposal classification as well as organization of the data on total radioactivity and maximum radioactivity concentration for each classification. For the evaluation of radioactive inventory, neutron flux and energy spectra are calculated at each region in the reactor facility using two- or three-dimensional neutron transport code. The activation calculation is then conducted for 140 nuclides using the results of neutron transport calculation and an activation calculation code. The recommended codes in this report for neutron transport calculation are two-dimensional discrete ordinate code DORT, three-dimensional discrete ordinate code TORT, or Monte Carlo codes MCNP and PHITS, and for activation calculation is ORIGEN-S. Other recommendation of cross-section libraries and calculation conditions are also indicated in this report. In the course of the establishment of the procedure, Radioactive Wastes Disposal Center has discussed the commonly available procedure at meetings. It has periodically held to exchange information with external operators which have research reactor facilities. The procedure will properly be reviewed and be revised by reflecting future situ

JAEA Reports

Survey on the planning process for waste characterization with statistical methods; Data quality objectives process

Murakami, Masashi; Sasaki, Toshiki

JAEA-Review 2022-004, 106 Pages, 2022/06

JAEA-Review-2022-004.pdf:3.95MB

A numerous analytical data will be required for the characterization of the radioactive waste stored in Japan Atomic Energy Agency toward their processing and disposal. A "Data Quality Objectives (DQO) Process" is widely applied as a tool for the development of a cost-effective characterization plan in the overseas nuclear sites. The DQO Process is a multi-step planning process developed by the United States Environmental Protection Agency (EPA), and can be used for the planning of a scientifically rigorous and cost-effective data collection program for the various projects involving the collection of the environmental data. We have considered to reduce the cost required for the future characterization of the stored waste by applying the statistical methods and have performed a literature survey on the DQO Process. The survey effort was focused on the guidance documents of the DQO Process published by the EPA and was also spent for the related matters such as a quality system of the EPA and the activities beyond the DQO Process as well as the examples of the application at the nuclear sites. In this report, the details on the planning procedure using the DQO Process are reviewed together with the background information such as why DQO Process was developed, what kind of transition was occurred, and how it is currently used in the EPA. The examples on the application for various objects at Hanford Site in the United States, where has the various legacy waste generated in the past activities and has the big environmental problems, are also reviewed. This report summarizes the important matters and methodology on the planning with the statistical sampling methods. It also provides the examples of the approaches for the complex objects, and will therefore be helpful in the future planning for the various kind of the waste characterization.

Journal Articles

Development and evaluation of XRF imaging instrument for moving objects

Fuchita, Tomoki*; Urata, Taisei*; Matsuyama, Tsugufumi*; Murakami, Masashi; Yoshida, Yukihiko; Ueda, Akihiko; Machida, Masahiko; Sasaki, Toshiki; Tsuji, Koichi*

Advances in X-Ray Chemical Analysis, Japan, 53, p.77 - 87, 2022/03

X-ray fluorescence (XRF) analysis is an analytical method to obtain elemental information by detecting fluorescence X-rays emitted from a sample irradiated with X-rays. It is possible to obtain two-dimensional elemental distribution images by scanning a sample with micro X-ray beam. In this study, we developed an XRF analytical instrument to rapidly obtain the elemental distributions for moving samples on a belt conveyor by applying the micro XRF technique. X-rays were widely irradiated to the belt conveyor. The elemental distributions were measured by scanning an X-ray detector, crossing above the belt conveyor. A collimator was attached to the top of the detector to limit the analyzing area. Both detection limit and spatial resolutions for moving directions of the detector and the belt conveyor were evaluated. Finally, it was demonstrated that the multi-elemental imaging was possible with the developed XRF instrument.

Journal Articles

Development of the buckling evaluation method for large scale vessel by the testing of Gr.91 vessel subjected to horizontal and cyclic vertical loading

Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Ando, Masanori; Miyazaki, Masashi

Proceedings of ASME 2021 Pressure Vessels and Piping Conference (PVP 2021) (Internet), 9 Pages, 2021/07

Buckling evaluation methods capable of evaluating elasto-plastic buckling under axial compression, bending, and shear loads are required for cylindrical vessels of fast reactors to cope with thinning due to increasing diameter and application to the seismic isolation design against huge seismic ground motion. In this study, in order to confirm the applicability of the proposal evaluation method, several buckling tests and FE analyses were carried out using the specimens made of Modified 9Cr-1Mo steel. The buckling modes and strength data in the load region where the interaction of cyclic axial compression, bending and shear buckling could occur were examined. As a result, it was confirmed that the proposal evaluation method estimated the buckling load in the tests conservatively. Moreover, a series of finite element analyzes using a model with residual stress due to welding revealed that the effect of residual stress on buckling strength is negligible in the evaluation method.

JAEA Reports

Basic policy for rational measures of radioactive waste processing and disposal; Results of studies for acceleration of waste processing

Nakagawa, Akinori; Oyokawa, Atsushi; Murakami, Masashi; Yoshida, Yukihiko; Sasaki, Toshiki; Okada, Shota; Nakata, Hisakazu; Sugaya, Toshikatsu; Sakai, Akihiro; Sakamoto, Yoshiaki

JAEA-Technology 2021-006, 186 Pages, 2021/06

JAEA-Technology-2021-006.pdf:54.45MB

Radioactive wastes generated from R&D activities have been stored in Japan Atomic Energy Agency. In order to reduce the risk of taking long time to process legacy wastes, countermeasures for acceleration of waste processing and disposal were studied. Work analysis of waste processing showed bottleneck processes, such as evaluation of radioactivity concentration, segregation of hazardous and combustibles materials. Concerning evaluation of radioactivity concentration, a radiological characterization method using a scaling factor and a nondestructive gamma-ray measurement should be developed. The number of radionuclides that are to be selected for the safety assessment of the trench type disposal facility can decrease using artificial barriers. Hazardous materials, will be identified using records and nondestructive inspection. The waste identified as hazardous will be unpacked and segregated. Preliminary calculations of waste acceptance criteria of hazardous material concentrations were conducted based on environmental standards in groundwater. The total volume of the combustibles will be evaluated using nondestructive inspection. The waste that does not comply with the waste acceptance criteria should be mixed with low combustible material waste such as dismantling concrete waste in order to satisfy the waste acceptance criteria on a disposal facility average. It was estimated that segregation throughput of compressed waste should be increased about 5 times more than conventional method by applying the countermeasures. Further study and technology development will be conducted to realize the plan.

Journal Articles

Production of $$^{266}$$Bh in the $$^{248}$$Cm($$^{23}$$Na,5$$n$$)$$^{266}$$Bh reaction and its decay properties

Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.

Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08

 Times Cited Count:8 Percentile:56.07(Physics, Nuclear)

Journal Articles

Development of the buckling evaluation method for large scale vessel by the testing of Gr.91 vessel subjected to vertical and horizontal loading

Okafuji, Takashi*; Miura, Kazuhiro*; Sago, Hiromi*; Murakami, Hisatomo*; Ando, Masanori; Miyazaki, Masashi

Proceedings of ASME 2020 Pressure Vessels and Piping Conference (PVP 2020) (Internet), 9 Pages, 2020/08

Buckling evaluation methods capable of evaluating elasto-plastic buckling under axial compression, bending, and shear loads are required for cylindrical vessels of fast reactors to cope with thinning due to increasing diameter and application to the seismic isolation design against huge seismic ground motion. In this study, in order to confirm the applicability of the proposal evaluation method, several buckling tests and FE analyses were carried out using the specimens made of Modified 9Cr-1Mo steel. The buckling modes and strength data in the load region where the interaction of axial compression, bending and shear buckling could occur were examined. As a result, it was confirmed that the proposal evaluation method estimated the buckling load in the tests conservatively. In addition, buckling strength evaluated by elasto-plastic buckling analysis had good accuracy compared to each test result by considering the stress-strain relationship and imperfection of test specimen.

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