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Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count:5 Percentile:92.64(Multidisciplinary Sciences)no abstracts in English
Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.
Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08
Times Cited Count:2 Percentile:68.16(Astronomy & Astrophysics)Detailed -ray spectroscopy of the exotic neon isotope Ne has been performed using the one-neutron removal reaction from Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.
Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.
Physical Review B, 107(18), p.184114_1 - 184114_8, 2023/05
Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)Nakae, Masanori*; Matsuyama, Tsugufumi*; Murakami, Masashi; Yoshida, Yukihiko; Machida, Masahiko; Tsuji, Koichi*
Advances in X-Ray Chemical Analysis, Japan, 54, p.89 - 99, 2023/03
Fundamental research on X-ray absorption imaging for elemental identification was studied. A secondary target was applied to obtain X-ray absorption images above and below the X-ray absorption edge of the target element. X-rays from an X-ray tube were irradiated to the secondary target, where the characteristic X-rays were emitted that were irradiated to the sample. X-ray absorption images were acquired with an exposure time of a few seconds with an X-ray camera. In this technique, it is difficult to change the energy of X-rays as we want, however we can apply this technique for imaging the specific element. Metal foil sample composed of Al, Cu, and Ni was analyzed. To obtain an X-ray elemental image of Ni, two X-ray absorption images were taken using the X-rays above and below the Ni K-edge. X-rays of Cu K and Zn K were prepared by using Cu and Zn plates as the secondary target. Finally, the Ni elemental image was obtained by subtracting two images. Furthermore, the X-ray camera had a function of setting critical energies for imaging, thus it was demonstrated that an X-ray elemental image of Ni was obtained using a single secondary target without changing the secondary target.
Yogo, Akifumi*; Lan, Z.*; Arikawa, Yasunobu*; Abe, Yuki*; Mirfayzi, S. R.*; Wei, T.*; Mori, Takato*; Golovin, D.*; Hayakawa, Takehito*; Iwata, Natsumi*; et al.
Physical Review X, 13(1), p.011011_1 - 011011_12, 2023/01
Times Cited Count:3 Percentile:88.42(Physics, Multidisciplinary)Matsuyama, Tsugufumi*; Nakae, Masanori*; Murakami, Masashi; Yoshida, Yukihiko; Machida, Masahiko; Tsuji, Koichi*
Spectrochimica Acta, Part B, 199, p.106593_1 - 106593_6, 2023/01
Times Cited Count:2 Percentile:45.92(Spectroscopy)Yabe, Takanori; Murakami, Makio; Shiota, Yuki; Isobe, Yuta; Shiohama, Yasutaka; Hamano, Tomoharu; Takagi, Tsuyohiko; Nagaoki, Yoshihiro
JAEA-Technology 2022-002, 66 Pages, 2022/07
In the first stage of "Monju" decommissioning project, "Fuel Unloading Operations" have been carrying out. The operations consists of two processes. The first process is "Fuel Treatment and Storage" is that the fuel assemblies unloaded from the Ex-Vessel fuel Storage Tank are canned after sodium cleaning, and then transferred to the storage pool. The second process is "Fuel Unloading" that the fuel assemblies in the reactor core are replaced with dummy fuel assemblies and stored in the Ex-Vessel fuel Storage Tank. "Fuel Treatment and Storage" and "Fuel Unloading" are performed alternately until 370 fuel assemblies in the core and 160 fuel assemblies in the Ex-Vessel fuel Storage Tank are all transferred to the storage pool. In fiscal 2018, as "Fuel Treatment and Storage", 86 fuel assemblies were transferred to the storage pool. As "Fuel Unloading", 76 dummy fuel assemblies were stored in the Ex-Vessel fuel Storage Tank. In fiscal 2019, as "Fuel Unloading", 60 fuel assemblies and 40 blanket fuel assemblies were unloaded from the core. These assemblies were stored in the Ex-Vessel fuel Storage Tank, and dummy fuel assemblies were loaded into the core instead. During these operations, a total of 38 cases of alarming or equipment malfunctions classified into 24 types occurred. However, no significant events that menaces to safety have occurred. The operations were continued safely by removing the direct factors for the malfunctions in the equipment operation and performance.
Shiota, Yuki; Yabe, Takanori; Murakami, Makio; Isobe, Yuta; Sato, Masami; Hamano, Tomoharu; Takagi, Tsuyohiko; Nagaoki, Yoshihiro
JAEA-Technology 2022-001, 117 Pages, 2022/07
In the first stage of Monju decommissioning project, fuel unload work began to be carried out. There are two tasks in this work. One is fuel treatment and storage work that gets rid of sodium on the fuel assemblies unloaded from Ex-Vessel fuel Storage Tank (EVST) and carries it in the storage pool, and the other is fuel unloading that the fuel assemblies in the reactor core is replaced with dummy fuels and stored in EVST. Fuel treatment and storage work and fuel unloading work are performed alternately, and 370 bodies in the core and 160 pieces in EVST are all carried to the storage pool. 86 fuel assemblies was carried to the storage pool in fuel treatment and storage work in 2018 and 76 dummy fuels were stored in EVST for fuel unloading work. During the work, 86 types and 232 alarms / malfunctions occurred, but there was no impact on safety. There was one equipment's failure at gripper's claw open / close clutch of ex-vessel fuel transfer machine B, but it was repaired and restarted. Also it was eliminated the cause of problem or concession that the equipment failure due to the sticking of the sodium compound and continuous use of the equipment. Some problems related to system control occurred, but the work was done after checking the safety. With estimation of various troubles, reduction of frequency of trouble occurrence and minimization of impacts on schedule performed.
Kato, Atsushi; Kubo, Shigenobu; Chikazawa, Yoshitaka; Miyagawa, Takayuki*; Uchita, Masato*; Suzuno, Tetsuji*; Endo, Junji*; Kubo, Koji*; Murakami, Hisatomo*; Uzawa, Masayuki*; et al.
Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Sustainable Clean Energy for the Future (FR22) (Internet), 11 Pages, 2022/04
The authors are carrying out conceptual design studies for a pool-type sodium-cooled fast reactor. There are main challenges such as measures against severe earthquake in Japan, thermal hydraulic in a reactor vessel (RV), a decay heat removal system design. When the JP-pool SFR of 650 MWe is installed in Japan, it shall be designed against the severe seismic conditions. Additionally, a newly three-dimensional seismic isolation system is under development.
Fuchita, Tomoki*; Urata, Taisei*; Matsuyama, Tsugufumi*; Murakami, Masashi; Yoshida, Yukihiko; Ueda, Akihiko; Machida, Masahiko; Sasaki, Toshiki; Tsuji, Koichi*
Advances in X-Ray Chemical Analysis, Japan, 53, p.77 - 87, 2022/03
X-ray fluorescence (XRF) analysis is an analytical method to obtain elemental information by detecting fluorescence X-rays emitted from a sample irradiated with X-rays. It is possible to obtain two-dimensional elemental distribution images by scanning a sample with micro X-ray beam. In this study, we developed an XRF analytical instrument to rapidly obtain the elemental distributions for moving samples on a belt conveyor by applying the micro XRF technique. X-rays were widely irradiated to the belt conveyor. The elemental distributions were measured by scanning an X-ray detector, crossing above the belt conveyor. A collimator was attached to the top of the detector to limit the analyzing area. Both detection limit and spatial resolutions for moving directions of the detector and the belt conveyor were evaluated. Finally, it was demonstrated that the multi-elemental imaging was possible with the developed XRF instrument.
Kataoka, Takahiro*; Naoe, Shota*; Murakami, Kaito*; Yukimine, Ryohei*; Fujimoto, Yuki*; Kanzaki, Norie; Sakoda, Akihiro; Mitsunobu, Fumihiro*; Yamaoka, Kiyonori*
Journal of Clinical Biochemistry and Nutrition, 70(2), p.154 - 159, 2022/03
Times Cited Count:3 Percentile:57.52(Nutrition & Dietetics)Nakagawa, Akinori; Oyokawa, Atsushi; Murakami, Masashi; Yoshida, Yukihiko; Sasaki, Toshiki; Okada, Shota; Nakata, Hisakazu; Sugaya, Toshikatsu; Sakai, Akihiro; Sakamoto, Yoshiaki
JAEA-Technology 2021-006, 186 Pages, 2021/06
Radioactive wastes generated from R&D activities have been stored in Japan Atomic Energy Agency. In order to reduce the risk of taking long time to process legacy wastes, countermeasures for acceleration of waste processing and disposal were studied. Work analysis of waste processing showed bottleneck processes, such as evaluation of radioactivity concentration, segregation of hazardous and combustibles materials. Concerning evaluation of radioactivity concentration, a radiological characterization method using a scaling factor and a nondestructive gamma-ray measurement should be developed. The number of radionuclides that are to be selected for the safety assessment of the trench type disposal facility can decrease using artificial barriers. Hazardous materials, will be identified using records and nondestructive inspection. The waste identified as hazardous will be unpacked and segregated. Preliminary calculations of waste acceptance criteria of hazardous material concentrations were conducted based on environmental standards in groundwater. The total volume of the combustibles will be evaluated using nondestructive inspection. The waste that does not comply with the waste acceptance criteria should be mixed with low combustible material waste such as dismantling concrete waste in order to satisfy the waste acceptance criteria on a disposal facility average. It was estimated that segregation throughput of compressed waste should be increased about 5 times more than conventional method by applying the countermeasures. Further study and technology development will be conducted to realize the plan.
Tsuchida, Daiki; Haraga, Tomoko; Tobita, Minoru*; Omori, Hiroyuki*; Omori, Takeshi*; Murakami, Hideaki*; Mitsukai, Akina; Aono, Ryuji; Ishimori, Kenichiro; Kameo, Yutaka
JAEA-Data/Code 2020-022, 34 Pages, 2021/03
Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JRR-3 and JPDR. In this report, we summarized the radioactivity concentrations of 22 radionuclides(H, C, Cl, Ca, Co, Ni, Sr, Nb, Ag, Ba, Cs, Eu, Eu, Ho, U, U, Pu, Pu, Am, Am, Cm) which were obtained from radiochemical analysis of the samples.
Ueno, Akio*; Tamazawa, Satoshi*; Tamamura, Shuji*; Murakami, Takuma*; Kiyama, Tamotsu*; Inomata, Hidenori*; Amano, Yuki; Miyakawa, Kazuya; Tamaki, Hideyuki*; Naganuma, Takeshi*; et al.
International Journal of Systematic and Evolutionary Microbiology, 71(2), p.004683_1 - 004683_10, 2021/02
Times Cited Count:8 Percentile:62.07(Microbiology)A novel mesophilic sulfate-reducing bacterium, designated strain HN2, was isolated from groundwater sampled from the subsurface Miocene Wakkanai Formation located in Horonobe, Hokkaido, Japan. The cells were Gram-negative rods, with motility conferred by a single polar flagellum. The isolate expressed desulfoviridin, but no catalase or oxidase activities was detected. Strain HN2 grew in a temperature range of 5-43 C (optimum, 35 C) and in a pH range of 6.5-7.5 (optimum, pH 7.0-7.3). It used sulfate, thiosulfate, dimethyl sulfoxide, anthraquinone-2,6-disulfonate, Fe, and manganese oxide as electron acceptors, but not elemental sulfur, nitrite, or nitrate. The bacterium showed very weak growth with sulfite as the electron acceptor. The strain fermented pyruvate and cysteine in the absence of sulfate, but not malate or succinate. The bacterium did not require NaCl, but tolerated up to 4% NaCl (w/v). Strain HN2 did not require vitamins. The G+C content of the genomic DNA was 56.66 mol%. A 16S rRNA gene sequence analysis showed that the closest recognized relative of strain HN2 is JS1 (97.0% similarity). The average nucleotide identity (ANI) value between strain HN2 and D. JS1 was 79.8%. Based on the phenotypic and molecular genetic evidence, the isolate is assigned to the new species sp. nov. The type strain is HN2 (=DSM 101010 =NBRC 112213).
Do, V. K.; Furuse, Takahiro; Murakami, Erina; Aita, Rena; Ota, Yuki; Sato, Soichi
Journal of Radioanalytical and Nuclear Chemistry, 327(1), p.543 - 553, 2021/01
Times Cited Count:5 Percentile:65.59(Chemistry, Analytical)A new HCl-free chromatographic separation procedure has been developed for sequential separation of Zr and Mo from concrete matrices. Accordingly, Zr and Mo could be sensitively and selectively measured by ICP-MS/MS using ammonia reaction gas. The recoveries of greater than 90% for Zr and Mo from concretes could be achieved. The measurement condition was optimized for complete suppression of interferences from Nb and peak tailing from abundant isotopes of Zr and Mo in concrete matrices. The removal of interferences was verified by measurement of radio-contamination-free concretes used as a sample matrix blank. Method detection limits of 1.7 mBq g and 0.2 Bq g were achieved for Zr and Mo, respectively, in the concrete matrices. The interference removal factor for Nb (equivalent to the decontamination factor in radiochemical separation) was of the order of 10, and the abundance sensitivity was of the order of 10, indicating that the developed method is reliable for verifying the presence of ultralow concentrations of Zr and Mo. The present method is suitable for the rapid assessment of Zr and Mo for radioactivity inventory of concrete rubble.
Tamatsukuri, Hiromu; Murakami, Yoichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Matsuura, Masato*; Kawakita, Yukinobu; Matsuishi, Satoru*; Washio, Yasuhito*; Inoshita, Takeshi*; Hamada, Noriaki*; et al.
Physical Review B, 102(22), p.224406_1 - 224406_5, 2020/12
Times Cited Count:8 Percentile:49.08(Materials Science, Multidisciplinary)Fukuda, Kenji; Watanabe, Yusuke; Murakami, Hiroaki; Amano, Yuki; Aosai, Daisuke*; Hara, Naohiro*
JAEA-Data/Code 2020-012, 80 Pages, 2020/10
Japan Atomic Energy Agency has been investigating groundwater chemistry to understand the influence of excavation and maintenance of underground facilities as part of the Mizunami Underground Research Laboratory (MIU) Project in Mizunami, Gifu, Japan. In this report, we compiled data of groundwater chemistry and microbiology obtained at the MIU in the fiscal year 2019. In terms of ensuring traceability of data, basic information (e.g. sampling location, sampling time, sampling method and analytical method) and methodology for quality control are described.
Seki, Akiyuki; Mayumi, Akie; Wainwright-Murakami, Haruko*; Saito, Kimiaki; Takemiya, Hiroshi; Idomura, Yasuhiro
Proceedings of Joint International Conference on Supercomputing in Nuclear Applications + Monte Carlo 2020 (SNA + MC 2020), p.158 - 164, 2020/10
We developed a method to estimate the temporal change of the air dose rate at the location with sparse (in time) measurements by using the continuous measurement data from the nearby monitoring post. This method determines an observation model from the correlation between sparse data at the target location and dense data at the monitoring post based on a hierarchical Bayesian model. The developed method was validated against the air dose rate measured at the monitoring posts in Fukushima prefecture from 2012 to 2017. The results showed that the developed method can predict the air dose rate at almost all target locations with an error rate of less than 10%.
Sun, D.*; Wainwright-Murakami, Haruko*; Oroza, C. A.*; Seki, Akiyuki; Mikami, Satoshi; Takemiya, Hiroshi; Saito, Kimiaki
Journal of Environmental Radioactivity, 220-221, p.106281_1 - 106281_8, 2020/09
Times Cited Count:9 Percentile:43.42(Environmental Sciences)We have developed a methodology for optimizing the monitoring locations of radiation air dose-rate monitoring. For the method, we use a Gaussian mixture model to identify the representative locations among multiple environmental variables, such as elevation and land-cover types. Next, we use a Gaussian process model to capture and estimate the heterogeneity of air-dose rates across the domain. Our results have shown that this approach allows us to select monitoring locations in a systematic manner such that the heterogeneity of air dose rates is captured by the minimal number of monitoring locations.
Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.
Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08
Times Cited Count:6 Percentile:59.56(Physics, Nuclear)