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and CrUOAkiyama, Daisuke*; Kusaka, Ryoji; Kumagai, Yuta; Nakada, Masami; Watanabe, Masayuki; Okamoto, Yoshihiro; Nagai, Takayuki; Sato, Nobuaki*; Kirishima, Akira*
Journal of Nuclear Materials, 568, p.153847_1 - 153847_10, 2022/09
Times Cited Count：3 Percentile：68.71(Materials Science, Multidisciplinary)FeUO, CrUO, and Fe
Cr
UO are monouranates containing pentavalent U. Even though these compounds have similar crystal structures, their formation conditions and thermal stability are significantly different. To determine the factors causing the difference in thermal stability between FeUO and CrUO, their crystal structures were evaluated in detail. A Raman band was observed at 700 cm
in all the samples. This Raman band was derived from the stretching vibration of the O-U-O axis band, indicating that FeCrUO was composed of a uranyl-like structure in its lattice regardless of its "x"' value. M
ssbauer measurements indicated that the Fe in FeUO and FeCrUO were trivalent. Furthermore, FeCrUO lost its symmetry around Fe
with increasing electron densities around Fe, as the abundance of Cr increased. These results suggested no significant structural differences between FeUO and CrUO. Thermogravimetric measurements for UO
, FeUO, and CrUO showed that the temperature at which FeUO decomposed under an oxidizing condition (approximately 800 
C) was significantly lower than the temperature at which the decomposition of CrUO started (approximately 1250 C). Based on these results, we concluded that the decomposition of FeUO was triggered by an "in-crystal" redox reaction, i.e., Fe 
U
Fe
U
, which would not occur in the CrUO lattice because Cr could never be reduced under the investigated condition. Finally, the existence of Cr in FexCrUO effectively suppressed the decomposition of the FeCrUO crystal, even at a very low Cr content.
Nishimori, Nobuyuki; Hajima, Ryoichi; Nagai, Ryoji; Sawamura, Masaru
Proceedings of 56th ICFA Advanced Beam Dynamics Workshop on Energy Recovery Linacs (ERL 2015) (Internet), p.100 - 102, 2015/12
Nishimori, Nobuyuki; Nagai, Ryoji; Sawamura, Masaru; Hajima, Ryoichi
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.508 - 510, 2015/09
no abstracts in English
Nishimori, Nobuyuki; Nagai, Ryoji; Mori, Michiaki; Hajima, Ryoichi; Yamamoto, Masahiro*; Honda, Yosuke*; Miyajima, Tsukasa*; Uchiyama, Takashi*; Jin, X.*; Obina, Takashi*; et al.
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.511 - 515, 2015/09
no abstracts in English
-ray beamsHajima, Ryoichi; Sawamura, Masaru; Nagai, Ryoji; Nishimori, Nobuyuki; Hayakawa, Takehito; Shizuma, Toshiyuki; Angell, C.
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.79 - 83, 2015/09
Generation of energy-tunable narrow-bandwidth -rays via Laser Compton Scattering (LCS) is of great interest for scientific studies and applications of MeV photons which interact with nuclei. We are developing technologies relevant to generation of high-brightness LCS -ray beams. One of the promising applications of such -rays is the nondestructive detection and assay of nuclides which are necessary for nuclear security and safeguards. We summarize R-and-D status of LCS -ray sources and overview future applications.
Nagai, Ryoji; Hajima, Ryoichi; Shizuma, Toshiyuki; Mori, Michiaki; Akagi, Tomoya*; Kosuge, Atsushi*; Honda, Yosuke*; Araki, Sakae*; Terunuma, Nobuhiro*; Urakawa, Junji*
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1328 - 1330, 2015/09
Accelerator and laser technologies required for laser Compton scattering (LCS) photon source based on an energy-recovery linac (ERL) have been developed at the Compact ERL (cERL) facility. A high-flux, energy tunable, and monochromatic photon source such as the ERL-based LCS photon source is necessary for nondestructive assay of nuclear materials. For the demonstration of the ERL-based LCS photon generation, a laser enhancement cavity was installed at the recirculation loop of the cERL. The electron beam energy, the laser wavelength, and the collision angle are 20 MeV, 1064 nm, and 18 , respectively. The calculated maximum energy of the LCS photons is about 7 keV. A silicon drift detector (SDD) with active area of 17 mm
placed 16.6 m from the collision point was used for observation of the LCS photons. As a result of the measurement, the flux on the detector, central energy, and energy width of the LCS photons were obtained as 1200/s, 6.91 keV, and 81 eV, respectively.
Sawamura, Masaru; Hajima, Ryoichi; Nishimori, Nobuyuki; Nagai, Ryoji; Iwashita, Yoshihisa*; Tongu, Hiromu*; Kubo, Takayuki*; Saeki, Takayuki*
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.583 - 586, 2015/09
no abstracts in English
Nagai, Ryoji; Hajima, Ryoichi; Mori, Michiaki; Shizuma, Toshiyuki; Akagi, Tomoya*; Araki, Sakae*; Honda, Yosuke*; Kosuge, Atsushi*; Terunuma, Nobuhiro*; Urakawa, Junji*
Proceedings of 6th International Particle Accelerator Conference (IPAC '15) (Internet), p.1607 - 1609, 2015/06
Accelerator and laser technologies required for laser Compton scattering (LCS) photon source based on an energy-recovery linac (ERL) have been developed at the Compact ERL (cERL) facility. A high-flux, energy tunable, and monochromatic photon source such as the ERL-based LCS photon source is necessary for nondestructive assay of nuclear materials. For the demonstration of the ERL-based LCS photon generation, a laser enhancement cavity was installed at the recirculation loop of the cERL. The electron beam energy, the laser wavelength, and the collision angle are 20 MeV, 1064 nm, and 18 deg., respectively. The calculated maximum energy of the LCS photons is about 7 keV. A silicon drift detector (SDD) with active area of 17 mm placed 16.6 m from the collision point was used for observation of the LCS photons. As a result of the measurement, the flux on the detector, central energy, and energy width of the LCS photons were obtained as 1200 /s, 6.91 keV, and 81 eV, respectively.
-rays with energies of 1.17 and 1.33 MeV by a flat Si crystalMatsuba, Shunya*; Hayakawa, Takehito; Shizuma, Toshiyuki; Nishimori, Nobuyuki; Nagai, Ryoji; Sawamura, Masaru; Angell, C.; Fujiwara, Mamoru; Hajima, Ryoichi
Japanese Journal of Applied Physics, 54(5), p.052203_1 - 052203_5, 2015/05
Times Cited Count：3 Percentile：13.89(Physics, Applied)-ray nondestructive assay by laser Compton scattered sourceHajima, Ryoichi; Shizuma, Toshiyuki; Nagai, Ryoji; Mori, Michiaki; Hayakawa, Takehito; Angell, C.; Seya, Michio
Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-35-Kai Nenji Taikai Rombunshu (Internet), 7 Pages, 2015/01
no abstracts in English
-ray generationNishimori, Nobuyuki; Nagai, Ryoji; Matsuba, Shunya; Hajima, Ryoichi; Yamamoto, Masahiro*; Honda, Yosuke*; Miyajima, Tsukasa*; Uchiyama, Takashi*; Kuriki, Masao*
Nuclear Physics and -ray sources for Nuclear Security and Nonproliferation, p.321 - 326, 2014/12
Nishimori, Nobuyuki; Nagai, Ryoji; Matsuba, Shunya; Sawamura, Masaru; Hajima, Ryoichi
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1031 - 1033, 2014/10
no abstracts in English
Nishimori, Nobuyuki; Nagai, Ryoji; Yamamoto, Masahiro*
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.165 - 170, 2014/10
no abstracts in English
Sawamura, Masaru; Nagai, Ryoji; Nishimori, Nobuyuki; Hajima, Ryoichi; Iwashita, Yoshihisa*; Fujisawa, Hiroshi*; Tongu, Hiromu*; Kubo, Takayuki*; Saeki, Takayuki*
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.618 - 620, 2014/10
no abstracts in English
Nagai, Ryoji; Hajima, Ryoichi; Mori, Michiaki; Shizuma, Toshiyuki; Akagi, Tomoya*; Kosuge, Atsushi*; Honda, Yosuke*; Urakawa, Junji*
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1328 - 1331, 2014/10
A high intensity -ray source from the laser Compton scattering (LCS) by an electron beam in an energy-recovery linac (ERL) is a key technology for a nondestructive assay system to identify nuclear materials. In order to demonstrate accelerator and laser technologies required for a LCS photon generation, a LCS photon source is under construction at the Compact ERL (cERL). The LCS photon source consists of a mode-locked fiber laser and a laser enhancement cavity. A beamline and an experimental hatch are also under construction. The commissioning of the LCS photon source will be started in February 2015 and LCS photon generation is scheduled in March 2015.
Nagai, Ryoji; Hajima, Ryoichi; Mori, Michiaki; Shizuma, Toshiyuki; Akagi, Tomoya*; Kosuge, Atsushi*; Honda, Yosuke*; Urakawa, Junji*
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.839 - 842, 2014/10
In order to demonstrate accelerator and laser technologies required for a laser Compton scattering (LCS) photon generation, a LCS photon source is under construction at the Compact ERL (cERL). We considered the flux monitors for the adjustment LCS photon source. A thin scintillator detector and a silicon drift detector are employed as flux monitors and are installed at the upstream part of the LCS beamline. The background signal level due to the bremsstrahlung of the electron beam was measured by a CsI(pure) scintillator. In the result of the measurement, the background signal is acceptable level for the flux monitors.
Nagai, Ryoji; Sawamura, Masaru; Nishimori, Nobuyuki; Hajima, Ryoichi
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1016 - 1018, 2014/10
In order to realize a high-brightness and monochromatic light source based on accelerator technologies, increasing of the cathode surface field of an electron gun is mandatory. Dust-free technique is a key technology to realize a high-field electron gun. We propose a new style dust-free technique. In this paper, R&D status and result of the preliminary test of the dust-free technique are reported.
Hwang, J.-G.*; Kim, E.-S.*; Miyajima, Tsukasa*; Honda, Yosuke*; Harada, Kentaro*; Shimada, Miho*; Takai, Ryota*; Kume, Tatsuya*; Nagahashi, Shinya*; Obina, Takashi*; et al.
Nuclear Instruments and Methods in Physics Research A, 753, p.97 - 104, 2014/07
Times Cited Count：7 Percentile：48.36(Instruments & Instrumentation)Nagai, Ryoji; Hajima, Ryoichi; Mori, Michiaki; Shizuma, Toshiyuki; Akagi, Tomoya*; Honda, Yosuke*; Kosuge, Atsushi*; Urakawa, Junji*
Proceedings of 5th International Particle Accelerator Conference (IPAC '14) (Internet), p.1940 - 1942, 2014/07
In order to demonstrate required accelerator and laser technologies for a high intensity -ray source from the laser Compton scattering (LCS), an LCS photon source and the peripheral equipment are under construction at the Compact ERL (cERL) at High Energy Accelerator Research Organization (KEK). The LCS photon source by an electron beam in the energy-recovery linac (ERL) is a key technology for a nondestructive assay system to identify nuclear species. The LCS photon source and the peripheral equipment consist of a mode-locked fiber laser, laser enhancement cavity, beamline, and experimental hatch. The commissioning of the LCS photon source will be started in February 2015.
Sawamura, Masaru; Hajima, Ryoichi; Nagai, Ryoji; Kubo, Takayuki*; Fujisawa, Hiroshi*; Iwashita, Yoshihisa*; Tongu, Hiromu*
Proceedings of 5th International Particle Accelerator Conference (IPAC '14) (Internet), p.1946 - 1948, 2014/07
We have launched a 5-year research program to develop superconducting spoke cavity for laser Compton scattered (LCS) photon sources. For realizing a wide use of LCS X-ray and -ray sources in academic and industrial applications, we adopt 325-MHz super-conducting spoke cavity to electron beam drivers. The spoke cavity, originally invented for ion and proton acceleration, can be used for electron accelerators, in which we can make best use of features of spoke cavity: relative compactness in comparison with a TM cavity of the same frequency, robustness with respect to manufacturing inaccuracy due to its strong cell-to-cell coupling, couplers on outer conductor for the better packing in a linac, and so on. In this paper, we present our research plan and results of cavity shape optimization.
