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JAEA Reports

Elemental composition analysis of main structural materials of JMTR

Nagata, Hiroshi; Kochiyama, Mami; Chinone, Marina; Sugaya, Naoto; Nishimura, Arashi; Ishikawa, Joji; Sakai, Akihiro; Ide, Hiroshi

JAEA-Data/Code 2024-016, 44 Pages, 2025/03

JAEA-Data-Code-2024-016.pdf:3.54MB

The elemental composition of the structural materials of nuclear reactor facilities is used as one of the important parameters in activation calculations that are evaluated when formulating decommissioning plans. Regarding the elemental composition of aluminum alloys and other materials used as structural materials for test and research reactors, sufficient data is not available regarding elements other than the major elements. For this reason, samples were collected from aluminum alloy, beryllium, hafnium, and other materials that have been used as the main structural materials of JMTR (Japan Materials Testing Reactor), and their elemental compositions were analyzed. This report summarizes the elemental composition data of 78 elements obtained in FY2023.

Journal Articles

Bayesian estimation analysis of X-ray photoelectron spectra; Application to Si 2p spectrum analysis of oxidized silicon surfaces

Shinotsuka, Hiroshi*; Nagata, Kenji*; Yoshikawa, Hideki*; Ogawa, Shuichi*; Yoshigoe, Akitaka

Applied Surface Science, 685, p.162001_1 - 162001_11, 2025/03

 Times Cited Count:1 Percentile:0.00(Chemistry, Physical)

Silicon (Si) 2p photoelectron spectra of thermally oxidized Si(001) surfaces were analyzed using Bayesian estimation, a type of mathematical statistical processing, considering spin-orbit interactions. The accuracy of the estimation of fitting parameters and the model selection of the number of peaks were discussed. The spectral analysis was performed without any prior information on the positions of other Si peaks, except for the prominent bulk Si peak, and without using chemical-state assumptions. Our method completely verified previous findings on the surface species and the changes in peaks due to oxidation-induced strain as oxidation progressed.

JAEA Reports

Accident consequence analysis for JMTR as a decommission facilities

Nagata, Hiroshi; Omori, Takazumi; Maeda, Eita; Otsuka, Kaoru; Nakano, Hiroko; Hanakawa, Hiroki; Ide, Hiroshi

JAEA-Review 2023-033, 40 Pages, 2024/01

JAEA-Review-2023-033.pdf:1.39MB

Japan Materials Testing Reactor (JMTR) was decided as a one of decommission facilities in April 2017. In order to submit the decommissioning plan to the Nuclear Regulation Authority, the type of accident assumed in the first stage of the decommissioning plan was selected, and the public exposure dose was evaluated. A fuel handling accident and a fire accident during storage of waste were selected as assumed accidents in the first stage of the decommissioning plan. An evaluation of the public exposure dose from the radioactive materials released into the atmosphere due to these accidents was estimated to be a maximum of 0.019 mSv (due to a fire accident during storage of waste). This estimated value was found to be sufficiently smaller than the judging criteria (5 mSv), and not to pose a significant risk of radiation exposure to the general public.

Journal Articles

None

Nagata, Shuhei*; Ogawa, Yusuke*; Suzuki, Satoru*; Inoue, Hiroyuki*; Watanabe, Yutaka*; Yamamoto, Masahiro*; Abe, Hiroshi*; Mitsui, Seiichiro

NUMO-TR-22-02, p.21 - 22, 2023/03

no abstracts in English

JAEA Reports

Evaluation on secondary radioactive contamination remaining in JMTR Reactor Facility

Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi

JAEA-Technology 2022-029, 55 Pages, 2023/02

JAEA-Technology-2022-029.pdf:2.77MB

Japan Materials Testing Reactor (JMTR) was decided as a one of decommission facilities in April 2017. The activation activity of secondary radioactive contamination remaining in the reactor facility was evaluated in order to submit the decommissioning plan to the Nuclear Regulation Authority. Total activation activity was 2.73$$times$$10$$^{12}$$Bq after 12 years, 1.46$$times$$10$$^{12}$$Bq after 21 years, respectively. The system with high activation activity was the primary cooling system in JMTR. The relatively large radionuclide was H-3, Fe-55, Co-60, Ni-63, Sr-90 and Cs-137. The radioactivity level was classified based on the values of the obtained radioactivity concentration. As a result, the primary cooling system and the drain system was classified as L2, and others was classified as L3. The nuclide that affected classification result was only Co-60 in irradiation facility of HR-1 and OSF-1. H-3, Co-60, Sr-90, Cs-137 and so on were affected classification in other system. When treating and disposing of radioactive waste, evaluation will be carried out based on appropriate methods.

JAEA Reports

On-site training using JMTR and related facilities in FY2019

Nakano, Hiroko; Nishikata, Kaori; Nagata, Hiroshi; Ide, Hiroshi; Hanakawa, Hiroki; Kusunoki, Tsuyoshi

JAEA-Review 2022-073, 23 Pages, 2023/01

JAEA-Review-2022-073.pdf:2.02MB

A practical training course using the JMTR (Japan Materials Testing Reactor) and other research infrastructures was held from July 24th to July 31st in 2019 for Asian young researchers and engineers. This course was adopted as Japan-Asia Youth Exchange Program in Science (SAKURA Exchange Program in Science) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, 12 young researchers and engineers joined the course from 6 countries. This course consists of lectures, which are related to irradiation test research, safety management of nuclear reactors, nuclear characteristics of the nuclear reactors, etc., practical training such as practice of research reactor operation using simulator and technical tour of nuclear facilities on nuclear energy. The content of this course in FY 2019 is reported in this paper.

JAEA Reports

Evaluation on activation activity of radioactive materials remaining in JMTR Reactor Facility

Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Ide, Hiroshi

JAEA-Technology 2022-017, 113 Pages, 2022/08

JAEA-Technology-2022-017.pdf:6.17MB

Japan Materials Testing Reactor (JMTR) was decided as a one of decommission facilities in April 2017. The activation activity of radioactive materials remaining in the reactor facility was evaluated in order to submit the decommissioning plan to the Nuclear Regulation Authority. Total activation activity was 9.3$$times$$10$$^{18}$$ Bq after the permanent shutdown of reactor, 2.7$$times$$10$$^{16}$$ Bq after 21 years, 1.0$$times$$10$$^{16}$$ Bq after 40 years and 2.4$$times$$10$$^{15}$$ Bq after 100 years. The structure with high activation activity was the core structural materials in JMTR such as beryllium frame, aluminum reflector, etc., and the material was stainless steel, beryllium, etc. The ratio of nuclides to the total amount of activated radioactivity was highest in H-3 until about 40 years after the reactor shutdown, and then in Ni-63. For reference, the radioactivity level was classified based on the results of the obtained radioactivity concentration. The ratio of the weight of each radioactivity level to the total weight was 0.3-0.4% (10-13t) for L1, 0.0-0.4% (0-14t) for L2, 1.0-1.2% (32-39t) for L3 and 98.0-98.7% (about 3200t) for CL until 100 years after the reactor shutdown. It was found that those classified as CL account for more than 90% of the total. When treating and disposing of radioactive waste, evaluation will be carried out based on appropriate methods, including evaluation results of secondary pollutants.

Journal Articles

Development of stabilization treatment technology for radioactive aluminum waste

Seki, Misaki; Fujita, Yoshitaka; Fujihara, Yasuyuki*; Zhang, J.*; Yoshinaga, Hisao*; Sano, Tadafumi*; Hori, Junichi*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; et al.

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 29(1), p.2 - 9, 2022/06

no abstracts in English

JAEA Reports

Study on the evaluation method to determine the radioactivity concentration in radioactive waste on Oarai Research and Development Institute (FY2020)

Asakura, Kazuki; Shimomura, Yusuke; Donomae, Yasushi; Abe, Kazuyuki; Kitamura, Ryoichi; Miyakoshi, Hiroyuki; Takamatsu, Misao; Sakamoto, Naoki; Isozaki, Ryosuke; Onishi, Takashi; et al.

JAEA-Review 2021-020, 42 Pages, 2021/10

JAEA-Review-2021-020.pdf:2.95MB

The disposal of radioactive waste from the research facility need to calculate from the radioactivity concentration that based on variously nuclear fuels and materials. In Japan Atomic Energy Agency Oarai Research and Development Institute, the study on considering disposal is being advanced among the facilities which generate radioactive waste as well as the facilities which process radioactive waste. This report summarizes a study result in FY2020 about the evaluation method to determine the radioactivity concentration in radioactive waste on Oarai Research and Development Institute.

Journal Articles

U-Pb ages of zircons from metamorphic rocks in the upper sequence of the Hidaka metamorphic belt, Hokkaido, Japan; Identification of two metamorphic events and implications for regional tectonics

Takahashi, Hiroshi*; Mikoshiba, Masumi*; Shimura, Toshiaki*; Nagata, Mitsuhiro; Iwano, Hideki*; Danhara, Toru*; Hirata, Takafumi*

Island Arc, 30(1), p.e12393_1 - e12393_15, 2021/01

 Times Cited Count:3 Percentile:15.93(Geosciences, Multidisciplinary)

The Hidaka metamorphic belt is an excellent example of island-arc-type crust, and in this belt the metamorphic grade increases westwards from unmetamorphosed sediment up to the granulite facies. The metamorphic age of the belt had previously been considered to be ca. 55 Ma. However, zircons from the granulites in the lower sequence have given U-Pb ages of ca. 21-19 Ma and a preliminary report on zircons from pelitic gneiss in the upper sequence gave a U-Pb age of ca. 40 Ma. In this paper we provide new U-Pb ages for zircons from the pelitic gneisses in the upper sequence in order to assess the metamorphic age and also the maximum depositional age of the sedimentary protolith. The weighted mean $$^{206}$$Pb/$$^{238}$$U ages and 2 sigma errors for zircons from biotite gneiss in the central area of the belt are 39.6 $$pm$$ 0.9 Ma for metamorphic overgrowth rims and 53.1 $$pm$$ 0.9 Ma for the youngest inherited detrital cores. The ages of zircons from cordierite-biotite gneiss in the southern area are 35.9 $$pm$$ 0.7 Ma for overgrowth rims and 46.5 $$pm$$ 2.8 Ma for the youngest detrital cores. These results indicate that the metamorphism of the upper sequence took place at ca. 40-36 Ma, and that the sedimentary protolith was deposited after ca. 53-47 Ma. These metamorphic ages are consistent with the reported ages of ca. 37-36 Ma plutonic rocks in the upper sequence, but contrast with the ca. 21-19 Ma ages of metamorphic and plutonic rocks in the lower sequence. Therefore, we conclude, that the upper and lower metamorphic sequences developed independently but became coupled before ca. 19 Ma as a result of dextral reverse tectonic movements, as indicated by the intrusion of ca. 19-18 Ma magmas, possibly generated in the lower sequence, into the upper sequence.

Journal Articles

Development of the treatment method for difficult wastes aimed at decommissioning of JMTR; Structural materials of reactor and used ion-exchange resins

Seki, Misaki; Nakano, Hiroko; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Takeuchi, Tomoaki; Ide, Hiroshi; Tsuchiya, Kunihiko

Dekomisshoningu Giho, (62), p.9 - 19, 2020/09

Japan Materials Testing Reactor (JMTR) has been contributing to various research and development activities such as the fundamental research of nuclear materials/fuels, safety research and development of power reactors, and radioisotope production since the beginning of the operation in 1968. JMTR, however, was decided as a one of decommission facilities in April 2017 and it is taken an inspection of a plan concerning decommissioning because the performance of JMTR does not confirm with the stipulated earthquake resistance. As aluminum and beryllium are used for the core structural materials in JMTR, it is necessary to establish treatment methods of these materials for the fabrication of stable wastes. In addition, a treatment method for the accumulated spent ion-exchange resins needs to be examined. This report describes the overview of these examination situations.

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning, 2

Seki, Misaki; Ishikawa, Koji*; Sano, Tadafumi*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2019, P. 279, 2020/08

no abstracts in English

JAEA Reports

On-site training using JMTR and related facilities in FY2018

Eguchi, Shohei; Nakano, Hiroko; Otsuka, Noriaki; Nishikata, Kaori; Nagata, Hiroshi; Ide, Hiroshi; Kusunoki, Tsuyoshi

JAEA-Review 2019-012, 22 Pages, 2019/10

JAEA-Review-2019-012.pdf:3.37MB

A practical training course using the JMTR and other research infrastructures was held from July 31st to August 7th in 2018 for Asian young researchers and engineers. This course was adopted as Japan-Asia Youth Exchange Program in Science (SAKURA Exchange Program in Science) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, 11 young researchers and engineers joined the course from 6 countries. This course consists of lectures, which are related to irradiation test research, safety management of nuclear reactors, nuclear characteristics of the nuclear reactors, etc., practical training such as practice of research reactor operation using simulator and technical tour of nuclear facilities on nuclear energy. The content of this course in FY 2018 is reported in this paper.

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning

Seki, Misaki; Ishikawa, Koji*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 257, 2019/08

no abstracts in English

Journal Articles

Status of JMTR decommissioning plan formulation, 2

Otsuka, Kaoru; Ide, Hiroshi; Nagata, Hiroshi; Omori, Takazumi; Seki, Misaki; Hanakawa, Hiroki; Nemoto, Hiroyoshi; Watanabe, Masao; Iimura, Koichi; Tsuchiya, Kunihiko; et al.

UTNL-R-0499, p.12_1 - 12_8, 2019/03

no abstracts in English

Journal Articles

Status of JMTR decommissioning plan formulation

Otsuka, Kaoru; Hanakawa, Hiroki; Nagata, Hiroshi; Omori, Takazumi; Takeuchi, Tomoaki; Tsuchiya, Kunihiko

UTNL-R-0496, p.13_1 - 13_11, 2018/03

no abstracts in English

JAEA Reports

On-site training using JMTR and related facilities in FY2017

Eguchi, Shohei; Shibata, Hiroshi; Imaizumi, Tomomi; Nagata, Hiroshi; Tanimoto, Masataka; Kusunoki, Tsuyoshi

JAEA-Review 2017-032, 26 Pages, 2018/02

JAEA-Review-2017-032.pdf:2.44MB

A practical training course using the JMTR and other research infrastructures was held from July 24th to August 4th in 2017 for Asian young researchers and engineers. This course was adopted as Japan-Asia Youth Exchange Program in Science (SAKURA Exchange Program in Science) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, 10 young researchers and engineers joined the course from 6 countries. This course consists of lectures, which are related to irradiation test research, safety management of nuclear reactors, nuclear characteristics of the nuclear reactors, etc., practical training such as practice of research reactor operation using simulator and technical tour of nuclear facilities on nuclear energy. The content of this course in FY 2017 is reported in this paper.

Journal Articles

Investigation of main radiation source above shield plug of Unit 3 at Fukushima Daiichi Nuclear Power Station

Hirayama, Hideo*; Kondo, Kenjiro*; Suzuki, Seishiro*; Tanimura, Yoshihiko; Iwanaga, Kohei*; Nagata, Hiroshi*

EPJ Web of Conferences, 153, p.08010_1 - 08010_3, 2017/09

 Times Cited Count:3 Percentile:83.66(Nuclear Science & Technology)

Pulse height distributions were measured using a CdZnTe detector inside a lead collimator to investigate main source producing high dose rates above the shield plugs of Unit 3 at Fukushima Daiichi Nuclear Power Station. It was confirmed that low energy photons are dominant. Concentrations of Cs-137 under 60 cm concrete of the shield plug were estimated to be between 8.1$$times$$10$$^9$$ and 5.7$$times$$10$$^{10}$$ Bq/cm$$^2$$ from the measured peak count rate of 0.662 MeV photons. If Cs-137 was distributed on the surfaces of the gaps of the shied plugs with radius 6 m and with the averaged concentration of 5 points, 2.6$$times$$10$$^{10}$$ Bq/cm$$^2$$, total amount of Cs-137 is estimated to be 30 PBq.

Journal Articles

Development of radiation detectors for in-pile measurement

Takeuchi, Tomoaki; Otsuka, Noriaki; Shibata, Hiroshi; Nagata, Hiroshi; Endo, Yasuichi; Matsui, Yoshinori; Tsuchiya, Kunihiko

KAERI/GP-418/2015, p.110 - 112, 2015/00

$$gamma$$ irradiation experiments with a $$^{60}$$Co source were carried out for developing Self-Powered Gamma Detectors (SPGDs) with lead (Pb) emitter and Self-Powered Neutron Detectors (SPNDs) with Pt-40%Rh emitter prior to in-core irradiation experiments. The results showed the output currents of the SPGDs were proportional to the $$gamma$$ dose rate in the range from about 200-6000 Gy/h with about 10% accuracy. In the case of SPNDs, the output currents flowed in inverse direction and were an order of magnitude lower compared with that of the SPGDs. These different behaviors of the output currents are considered to be caused by the difference in the emitter sizes and the current component originated at the MI cables.

Journal Articles

Development of instrumentation systems for safety measure at LWR's severe accident

Takeuchi, Tomoaki; Shibata, Akira; Nagata, Hiroshi; Kimura, Nobuaki; Otsuka, Noriaki; Saito, Takashi; Nakamura, Jinichi; Matsui, Yoshinori; Tsuchiya, Kunihiko

Proceedings of 3rd Asian Symposium on Material Testing Reactors (ASMTR 2013), p.52 - 58, 2013/11

In-pile instrumentation systems in present LWR's are indispensable to monitor all situations during reactor operation and reactor shut down. However, those systems did not work sufficiently under the conditions like as the severe accident at the Fukushima Dai-Ichi Nuclear Power Station. Therefore, based on the irradiation measurement technique of experiences accumulated in JMTR, the developments of reactor instrumentation systems to prevent severe core damage accident in advance have been started. The development objects are four instrumentation systems, which are a solid electrolysis type hydrogen concentration sensor, a water gauge of thermocouple type equipped with the heater, a $$gamma$$-ray detector of self-powered type SPGD, and an image analysis system of Cherenkov light for quantification of in-reactor information by CCD cameras. After the developments, the in-pile verification tests of four instrumentation systems are planned at the JMTR.

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