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Nagasumi, Satoru; Hasegawa, Toshinari; Iigaki, Kazuhiko; Nakagawa, Shigeaki; Kubo, Shinji; Shimazaki, Yosuke; Nakajima, Kunihiro; Sakurai, Yosuke; Shinohara, Masanori; Saito, Kenji; et al.
Nuclear Engineering and Design, 446, p.114542_1 - 114542_14, 2026/01
To demonstrate HTGR's safety features, a loss-of-forced-cooling (LOFC) test was conducted using the HTTR. In this test, the forced cooling in the reactor core was intentionally lost by shutting down all helium gas circulators (HGCs) without reactor scram. During steady-state operation at 100% reactor power (30 MW), after the LOFC, the reactor power spontaneously decreased. This power reduction occurred due to the negative reactivity feedback effect triggered by an increase in core temperature. The power stabilized at a lower value of 1.2% after re-criticality. Additionally, the measured radioactivity concentration in the primary coolant remained nearly unchanged during this LOFC operation and during an immediately subsequent HTTR operation. This indicates no failure of the coated particle fuel, even after the increase in core temperature associated with the LOFC event. These results provide experimental evidence of the safety features of HTGRs.
Nagasumi, Satoru; Hasegawa, Toshinari; Nakagawa, Shigeaki; Kubo, Shinji; Iigaki, Kazuhiko; Shinohara, Masanori; Saikusa, Akio; Nojiri, Naoki; Saito, Kenji; Furusawa, Takayuki; et al.
JAEA-Research 2025-005, 23 Pages, 2025/07
A safety demonstration test under abnormal operating conditions using the HTTR (High Temperature Engineering Test Reactor) was conducted to demonstrate safety features of the HTGRs (High Temperature Gas-cooled Reactors). Under a simulation of a control rod shutdown failure, all primary helium gas circulators were intentionally stopped during a steady-state operation at 100% reactor thermal power (30 MW), temporal changes of the reactor power and temperatures around the reactor pressure vessel (RPV) were obtained after the complete loss of forced heat removal from the reactor core. After the event (primary coolant flow stopped), the reactor power quickly decreased due to the negative reactivity feedback associated with the core temperature rise, and then the reactor power spontaneously shifted to a stable state of low power (about 1.2%) even after a recriticality. Heat dissipation from RPV surface to a surrounding vessel cooling system (water-cooled panels) ensured the amount of heat removal required to maintain the reactor temperature constant in the low power state. In this way, the transition from the event occurrence to the stable and safety state, i.e., inherent safety features of HTGRs, were demonstrated in the case of core forced cooling loss without active shutdown operations.
-nonyl N,N-dimethylammonio)-propyl sulfate, present in isotropic solutions above its upper critical solution temperatureTanji, Tamao*; Kusunoki, Yuto*; Nakagawa, Taichi; Takase, Tsugiko*; Ueda, Yuki; Motokawa, Ryuhei; Hinze, W. L.*; Takagai, Yoshitaka*
Langmuir, 41(21), p.13184 - 13191, 2025/06
Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)Hirata, Yoshinobu*; Nakagawa, Hiroshi; Yamauchi, Hiroki; Kaneko, Koji; Hagihara, Masato; Yamaguchi, Hideyuki*; Imaizumi, Teppei*; Nishizu, Takahisa*
International Journal of Biological Macromolecules, 306, p.141668_1 - 141668_7, 2025/03
Times Cited Count:1 Percentile:64.84(Biochemistry & Molecular Biology)We used quasi-elastic neutron scattering (QENS) to investigate the effect of the ratio of water to rice on the molecular dynamics of cooked rice starch during retrogradation. X-ray diffraction and differential scanning calorimetric measurements revealed that the degree of recrystallization and change in enthalpy were smaller with an increase in the amount of water added for cooking rice, whereas little difference in the crystallinity of the gelatinized rice starch was detected. The QENS measurements determined that the elastic incoherent structure factor (EISF) values of gelatinized samples were smaller with an increase in the amount of water added for cooking rice, indicating that the molecular dynamics of gelatinized rice starch with higher added water content were spatially more extended.
Inoue, Rintaro*; Oda, Takashi; Nakagawa, Hiroshi; Tominaga, Taiki*; Ikegami, Takahisa*; Konuma, Tsuyoshi*; Iwase, Hiroki*; Kawakita, Yukinobu; Sato, Mamoru*; Sugiyama, Masaaki*
Biophysical Journal, 124(3), p.540 - 548, 2025/02
Times Cited Count:2 Percentile:87.10(Biophysics)Hirata, Yoshinobu*; Kaneko, Fumitoshi*; Radulescu, A.*; Nishizu, Takahisa*; Katsuno, Nakako*; Imaizumi, Teppei*; Motokawa, Ryuhei; Kumada, Takayuki; Nakagawa, Hiroshi
Journal of Applied Glycoscience, 72(1), p.7201102_1 - 7201102_9, 2025/02
A simultaneous measurement system of SANS/FTIR-ATR was applied to record multiple structural changes in potato starch during retrogradation. In the SANS patterns, the shoulder-like peak becomes more pronounced with time. The peak intensity, Imax, which represents the amount of orderly arranged double helical structures, increased over time, showing that starch reassembled orderly on the nanoscale upon retrogradation. In the FTIR-ATR spectra, the increase of the ratio of absorptions at 1042 cm
and 1016 cm
, indicating the amount of short-range ordered structure in starch increased during retrogradation. The time to obtain half of the equilibrium value for
was larger than that for Imax. Changes in the short-range ordered structure of starch were observed to converge prior to changes in the nanostructure. These results indicate that the double-helix structures are initially formed by amylopectin side chains, and then these double-helical structures are arranged orderly.
Kumada, Takayuki; Nakagawa, Hiroshi; Miura, Daisuke; Sekine, Yurina; Motokawa, Ryuhei; Hiroi, Kosuke; Inamura, Yasuhiro; Oku, Takayuki; Oishi, Kazuki*; Morikawa, Toshiaki*; et al.
Hamon, 34(2), p.50 - 53, 2024/05
Spin-contrast-variation (SCV) small-angle neutron scattering (SANS) enabled us to determine structure of nano-ice crystals that were generated in rapidly frozen sugar solution. In the frozen glucose solution, we found that the nano-ice crystals formed a planar structure with a radius larger than several tens of nanometers and a thickness of 2-3 nm, which was close to the critical nucleation size of ice crystals in supercooled water. This result suggests that the glucose molecules were preferentially bound to a specific face of nano-ice crystals, and then blocked the crystal growth perpendicular to that face.
Murakami, Kenta*; Arai, Taku*; Yamada, Koji*; Momma, Kensuke*; Tsuji, Takashi*; Nakagawa, Nobuyuki*; Onizawa, Kunio
Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 3 Pages, 2024/03
This paper studied the future vision of codes and standards in Japan by systematically comparing Japanese regulatory rules, standards, and industry guides related to long term operation with international safety standards, and confirmed that the Japanese standard system generally meets their recommendations. The recommendation for the future improvements of Japanese codes and standards were summarized into five items.
Kumada, Takayuki; Motokawa, Ryuhei; Oba, Yojiro; Nakagawa, Hiroshi; Sekine, Yurina; Micheau, C.; Ueda, Yuki; Sugita, Tsuyoshi; Birumachi, Atsushi; Sasaki, Miki; et al.
Journal of Applied Crystallography, 56(6), p.1776 - 1783, 2023/12
Times Cited Count:21 Percentile:98.10(Chemistry, Multidisciplinary)The combination of the existing position-sensitive photomultiplier and the
He main detector with focusing devices, and the newly installed front detectors in SANS-J at JRR-3 covers small-angle neutron scattering signals in the range of the magnitude of the scattering vector Q from 0.002 to 6 nm-1 gaplessly with three standard device layouts. The installation of the front detector and a graphical user interface system largely improved the usability of SANS-J.
Hirata, Yoshinobu*; Nakagawa, Hiroshi; Yamauchi, Hiroki; Kaneko, Koji; Hagihara, Masato; Yamaguchi, Hideyuki*; Omoto, Chie*; Katsuno, Nakako*; Imaizumi, Teppei*; Nishizu, Takahisa*
Food Hydrocolloids, 141, p.108728_1 - 108728_7, 2023/08
Times Cited Count:14 Percentile:76.01(Chemistry, Applied)Crystallinity is reflected in the mechanical properties of foods and materials. Crystallinity should be related to the structural dynamics of starch. In this study, we used quasi-elastic neutron scattering (QENS) to investigate changes in the molecular dynamics of cooked rice starch during retrogradation. The width of the measured QENS narrowed with retrogradation. The elastic incoherent structure factor (EISF) increased, which indicated that the molecular dynamics are spatially suppressed upon retrogradation. Analysis of EISF with a bimodal continuous diffusion model, where low and high mobilities are assumed to correspond to crystalline and amorphous phases, respectively, showed that the fraction of the low-mobility component increases with retrogradation.
Kumada, Takayuki; Nakagawa, Hiroshi; Miura, Daisuke; Sekine, Yurina; Motokawa, Ryuhei; Hiroi, Kosuke; Inamura, Yasuhiro; Oku, Takayuki; Oishi, Kazuki*; Morikawa, Toshiaki*; et al.
Journal of Physical Chemistry Letters (Internet), 14(34), p.7638 - 7643, 2023/08
Times Cited Count:0 Percentile:0.00(Chemistry, Physical)The structure of nano-ice crystals in rapidly frozen glucose solution was elucidated by using spin-contrast-variation small-angle neutron scattering, which distinguishes the nano-ice crystal signal from the frozen amorphous solution signal by the polarization-dependent neutron scattering. The analysis revealed that the nano-ice crystals form a planar structure with a diameter exceeding tens of nanometers and a thickness of 1 nm, which is close to the critical nucleation size. This result suggests that the glucose molecules are preferentially bound to a specific face of nano-ice crystals, and then block the crystal growth perpendicular to that face.
Kitamura, Akihisa*; Okazaki, Sota*; Kondo, Mitsuru*; Watanabe, Takahiro; Nakanishi, Toshimichi*; Hori, Rie*; Ikeda, Masayuki*; Ichimura, Koji*; Nakagawa, Yuki*; Mori, Hideki*
Shizuoka Daigaku Chikyu Kagaku Kenkyu Hokoku, (49), p.73 - 86, 2022/07
On July 3 2021, a debris flow caused by a landslide from a landfill occurred along the Aizome River in the Izusan area of Atami City, Shizuoka. In this study, debris flow deposits and soil samples were characterized in terms of their sedimentology and geochemically analyzed.
continuous air monitor for the measurement of highly radioactive alpha-emitting particulates (
-aerosols) under high humidity environmentTsubota, Yoichi; Honda, Fumiya; Tokonami, Shinji*; Tamakuma, Yuki*; Nakagawa, Takahiro; Ikeda, Atsushi
Nuclear Instruments and Methods in Physics Research A, 1030, p.166475_1 - 166475_7, 2022/05
Times Cited Count:4 Percentile:55.72(Instruments & Instrumentation)In the long-lasting decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), the dismantling of nuclear fuel debris (NFD) remaining in the damaged reactors is an unavoidable but significant issue with many technical difficulties. The dismantling is presumed to involve mechanical cutting, generating significant concentrations of particulates containing
-radionuclides (
-aerosols) that pose significant health risk upon inhalation. In order to minimize the radiation exposure of workers with
-aerosols during the dismantling/decommissioning process at 1F, it is essential to monitor the concentration of
-aerosols at the point of initial generation, i.e. inside the primary containment vessels (PCV) of the damaged reactors. Toward this end, an
monitoring system for
-aerosols (
alpha air monitor: IAAM) was developed and its technical performance was investigated under the conditions expected for the actual environments at 1F. IAAM was confirmed to fulfill four technical requirements: (1) steady operation under high humidity, (2) operation without using filters, (3) capability of measuring a high counting rate of
-radiation, and (4) selective measurement of
-radiation even under high radiation background with
/
-rays. IAAM is capable of selectively measuring
-aerosols with a concentration of 3.3
10
Bq/cm
or higher without saturation under a high humid environment (100%-relative humidity) and under high background with
/
-radiation (up to 100 mSv/h of
-radiation). These results demonstrate promising potential of IAAM to be utilized as a reliable monitoring system for
-aerosols during the dismantling of NFD, as well as the whole long-lasting decommissioning of 1F.
Barucci, M. A.*; Reess, J.-M.*; Bernardi, P.*; Doressoundiram, A.*; Fornasier, S.*; Le Du, M.*; Iwata, Takahiro*; Nakagawa, Hiromu*; Nakamura, Tomoki*; Andr
, Y.*; et al.
Earth, Planets and Space (Internet), 73(1), p.211_1 - 211_28, 2021/12
Times Cited Count:30 Percentile:86.73(Geosciences, Multidisciplinary)The MMX InfraRed Spectrometer (MIRS) is an imaging spectrometer on board of MMX JAXA mission. MIRS is built at LESIA-Paris Observatory in collaboration with four other French laboratories, collaboration and financial support of CNES and close collaboration with JAXA and MELCO. The instrument is designed to fully accomplish MMX's scientific and measurement objectives. MIRS will remotely provide near-infrared spectral maps of Phobos and Deimos containing compositional diagnostic spectral features that will be used to analyze the surface composition and to support the sampling site selection. MIRS will also study Mars atmosphere, in particular to spatial and temporal changes such as clouds, dust and water vapor.
Tominaga, Taiki*; Sahara, Masae*; Kawakita, Yukinobu; Nakagawa, Hiroshi; Yamada, Takeshi*
Journal of Applied Crystallography, 54(6), p.1631 - 1640, 2021/12
Times Cited Count:6 Percentile:54.42(Chemistry, Multidisciplinary)Nakagawa, Hiroshi; Saio, Tomohide*; Nagao, Michihiro*; Inoue, Rintaro*; Sugiyama, Masaaki*; Ajito, Satoshi; Tominaga, Taiki*; Kawakita, Yukinobu
Biophysical Journal, 120(16), p.3341 - 3354, 2021/08
Times Cited Count:7 Percentile:49.86(Biophysics)A multi-domain protein can have various conformations in solution. Interactions with other molecules result in the stabilization of one of the conformations and change in the domain dynamics. SAXS, a well-established experimental technique, can be employed to elucidate the conformation of a multi-domain protein in solution. NSE spectroscopy is a promising technique for recording the domain dynamics in nanosecond and nanometer scale. Despite the great efforts, there are still under development. Thus, we quantitatively removed the contribution of diffusion dynamics and hydrodynamic interactions from the NSE data via incoherent scattering, revealing the differences in the domain dynamics of the three functional states of a multi-domain protein, MurD. The differences among the three states can be explained by two domain modes.
electron paramagnetic resonanceSaio, Tomohide*; Hiramatsu, Soya*; Asada, Mizue*; Nakagawa, Hiroshi; Shimizu, Kazumi*; Kumeta, Hiroyuki*; Nakamura, Toshikazu*; Ishimori, Koichiro*
Biophysical Journal, 120(15), p.2943 - 2951, 2021/08
Times Cited Count:1 Percentile:9.37(Biophysics)A rigid double-arm lanthanide tag was utilized in electron paramagnetic resonance spectroscopy to measure the distance between two specific points on a protein, and conformational states and distribution of a multi-domain protein enzyme MurD was investigated. Although the previous crystallographic and NMR studies have reported the three distinct conformational states of MurD, our data unveiled that the protein exists in much more variety of conformational states in the absence of the ligand. Given the fact that MurD is one of the potent drug target for infectious diseases, the finding in this study will provide important structural basis for drug development.
Nakagawa, Akinori; Oyokawa, Atsushi; Murakami, Masashi; Yoshida, Yukihiko; Sasaki, Toshiki; Okada, Shota; Nakata, Hisakazu; Sugaya, Toshikatsu; Sakai, Akihiro; Sakamoto, Yoshiaki
JAEA-Technology 2021-006, 186 Pages, 2021/06
Radioactive wastes generated from R&D activities have been stored in Japan Atomic Energy Agency. In order to reduce the risk of taking long time to process legacy wastes, countermeasures for acceleration of waste processing and disposal were studied. Work analysis of waste processing showed bottleneck processes, such as evaluation of radioactivity concentration, segregation of hazardous and combustibles materials. Concerning evaluation of radioactivity concentration, a radiological characterization method using a scaling factor and a nondestructive gamma-ray measurement should be developed. The number of radionuclides that are to be selected for the safety assessment of the trench type disposal facility can decrease using artificial barriers. Hazardous materials, will be identified using records and nondestructive inspection. The waste identified as hazardous will be unpacked and segregated. Preliminary calculations of waste acceptance criteria of hazardous material concentrations were conducted based on environmental standards in groundwater. The total volume of the combustibles will be evaluated using nondestructive inspection. The waste that does not comply with the waste acceptance criteria should be mixed with low combustible material waste such as dismantling concrete waste in order to satisfy the waste acceptance criteria on a disposal facility average. It was estimated that segregation throughput of compressed waste should be increased about 5 times more than conventional method by applying the countermeasures. Further study and technology development will be conducted to realize the plan.
Cs in water and phyto- and zooplankton in a reservoir affected by the Fukushima Daiichi Nuclear Power Plant AccidentTsuji, Hideki*; Nakagawa, Megumi*; Iijima, Kazuki; Funaki, Hironori; Yoshimura, Kazuya; Sakuma, Kazuyuki; Hayashi, Seiji*
Global Environmental Research (Internet), 24(2), p.115 - 127, 2021/06
Lake water, phytoplankton and zooplankton were sampled by a total of 12 quarterly surveys from August 2014 to May 2017 at a dam lake in the Fukushima nuclear disaster area, and variations of dissolved form of
Cs and planktonic
Cs were observed. Seasonal variations in dissolved
Cs concentration with high in summer and low in winter were observed in the upstream, midstream and downstream areas of the lake, but no seasonal or site specific differences in planktonic
Cs concentrations and dominant species were found. The amount of planktonic form of
Cs in the water was less than 1.4% of the total
Cs in the lake water, therefore the effect of plankton on the dynamics of
Cs in the lake was minimal.
Miura, Daisuke*; Kumada, Takayuki; Sekine, Yurina; Motokawa, Ryuhei; Nakagawa, Hiroshi; Oba, Yojiro; Ohara, Takashi; Takata, Shinichi; Hiroi, Kosuke; Morikawa, Toshiaki*; et al.
Journal of Applied Crystallography, 54(2), p.454 - 460, 2021/04
Times Cited Count:1 Percentile:12.21(Chemistry, Multidisciplinary)We developed a spin-contrast-variation neutron powder diffractometry technique that extracts the structure factor of hydrogen atoms, namely, the contribution of hydrogen atoms to a crystal structure factor. Crystals of L-glutamic acid were dispersed in a dpolystyrene matrix containing 4-methacryloyloxy-2,2,6,6,-tetramethyl-1-piperidinyloxy (TEMPO methacrylate) to polarize their proton spins dynamically. The intensities of the diffraction peaks of the sample changed according to the proton polarization, and the structure factor of the hydrogen atoms was extracted from the proton-polarization dependent intensities. This technique is expected to enable analyses of the structures of hydrogen-containing materials that are difficult to determine with conventional powder diffractometry.