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Journal Articles

Demonstration of the inherent safety feature of HTGRs through the loss-of-forced-cooling test in the HTTR

Nagasumi, Satoru; Hasegawa, Toshinari; Iigaki, Kazuhiko; Nakagawa, Shigeaki; Kubo, Shinji; Shimazaki, Yosuke; Nakajima, Kunihiro; Sakurai, Yosuke; Shinohara, Masanori; Saito, Kenji; et al.

Nuclear Engineering and Design, 446, p.114542_1 - 114542_14, 2026/01

To demonstrate HTGR's safety features, a loss-of-forced-cooling (LOFC) test was conducted using the HTTR. In this test, the forced cooling in the reactor core was intentionally lost by shutting down all helium gas circulators (HGCs) without reactor scram. During steady-state operation at 100% reactor power (30 MW), after the LOFC, the reactor power spontaneously decreased. This power reduction occurred due to the negative reactivity feedback effect triggered by an increase in core temperature. The power stabilized at a lower value of 1.2% after re-criticality. Additionally, the measured radioactivity concentration in the primary coolant remained nearly unchanged during this LOFC operation and during an immediately subsequent HTTR operation. This indicates no failure of the coated particle fuel, even after the increase in core temperature associated with the LOFC event. These results provide experimental evidence of the safety features of HTGRs.

Journal Articles

Magnetic and quadrupole coupling emerging in NdB$$_4$$ with geometrically frustrated orthogonal antiferromagnetic dimer

Metoki, Naoto; Yamauchi, Hiroki; Hagihara, Masato; Watanuki, Ryuta*; Kawamura, Seiko; Kofu, Maiko*; Nakajima, Kenji; Matsuda, Masaaki*

Physical Review B, 111(10), p.104424_1 - 104424_9, 2025/03

 Times Cited Count:1 Percentile:62.18(Materials Science, Multidisciplinary)

Inelastic neutron scattering experiments were carried out to understand the unusual successive order in NdB$$_4$$ with the frustrated Shatry-Sutherland (SS) lattice. The pseudo-quartet with $$|pm frac{5}{2}rangle$$ and $$|pm frac{7}{2}rangle$$ splits into four levels in the magnetically ordered states. The spectra can be explained with the on-site magnetic interaction $$langle J_x rangle J_x$$, the coupling of $$J_x$$ with quadrupole $$O_{zx}$$, and the uniaxial crystalline electric field. The $$f$$-electron states reproduce the temperature dependences of the in-plane moment $$m_perp=langle J_x rangle$$ which is the primary order parameter, and a weakly induced $$m_c=langle J_z rangle$$ as the secondary order parameter. The magnetic-quadrupole coupling emerges and play essential role under the geometrical frustration, where the Heisenberg interactions are cancelled out.

Journal Articles

Magnetic excitations in the noncentrosymmetric magnet Sr$$_{2}$$MnSi$$_{2}$$O$$_{7}$$

Kawamata, Masahiro*; Pang, X.*; Murakawa, Hiroshi*; Kawamura, Seiko; Nakajima, Kenji; Masuda, Hidetoshi*; Fujita, Masaki*; Hanasaki, Noriaki*; Onose, Yoshinori*; Nambu, Yusuke*

Physical Review Materials (Internet), 9(1), p.014407_1 - 014407_6, 2025/01

 Times Cited Count:1 Percentile:58.55(Materials Science, Multidisciplinary)

Journal Articles

Neutron flux and energy resolution of direct-geometry disk-chopper spectrometer AMATERAS at J-PARC

Nirei, Masami; Kofu, Maiko; Nakajima, Kenji; Kikuchi, Tatsuya*; Kawamura, Seiko; Murai, Naoki; Harada, Masahide; Inamura, Yasuhiro

Journal of Neutron Research, 26(2-3), p.75 - 82, 2024/09

Journal Articles

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

 Times Cited Count:4 Percentile:69.02(Physics, Multidisciplinary)

Journal Articles

Spectral evidence for Dirac spinons in a kagome lattice antiferromagnet

Zeng, Z.*; Zhou, C.*; Zhou, H.*; Han, L.*; Chi, R.*; Li, K.*; Kofu, Maiko; Nakajima, Kenji; Wei, Y.*; Zhang, W.*; et al.

Nature Physics, 20(7), p.1097 - 1102, 2024/07

 Times Cited Count:20 Percentile:96.75(Physics, Multidisciplinary)

Journal Articles

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; Kofu, Maiko; Nakajima, Kenji; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

 Times Cited Count:13 Percentile:91.20(Physics, Applied)

Journal Articles

Overall picture and details of diffusion dynamics for liquid benzene by quasielastic neutron scattering and mode distribution analysis

Kikuchi, Tatsuya*; Kawakita, Yukinobu; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro

Journal of Molecular Liquids, 385, p.121868_1 - 121868_10, 2023/09

Journal Articles

Extreme phonon anharmonicity underpins superionic diffusion and ultralow thermal conductivity in argyrodite Ag$$_{8}$$SnSe$$_{6}$$

Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; Kofu, Maiko; et al.

Nature Materials, 22(8), p.999 - 1006, 2023/08

 Times Cited Count:91 Percentile:99.21(Chemistry, Physical)

Journal Articles

Anomalous behavior of liquid molecules near solid nanoparticles; Novel interpretation on thermal conductivity enhancement in nanofluids

Hashimoto, Shunsuke*; Yamaguchi, Satoshi*; Harada, Masashi*; Nakajima, Kenji; Kikuchi, Tatsuya*; Oishi, Kazuki*

Journal of Colloid and Interface Science, 638, p.475 - 486, 2023/05

 Times Cited Count:11 Percentile:61.91(Chemistry, Physical)

Recently, it has been reported that anomalous improvement in the thermal conductivity of nanofluid composed of base liquids and dispersed solid nanoparticles, compared to the theoretically predicted value calculated from the particle fraction. Generally, the thermal conductivity values of gases and liquids are dominated by the mean free path of the molecules during translational motion. Herein, we present solid evidence showing the possible contribution of the vibrational behavior of liquid molecules around nanoparticles to increasing these thermal conductivities.

Journal Articles

Experimental evidence for the significance of optical phonons in thermal transport of tin monosulfide

Wu, P.*; Murai, Naoki; Li, T.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Kofu, Maiko; Nakajima, Kenji; Xia, K.*; Peng, K.*; Zhang, Y.*; et al.

New Journal of Physics (Internet), 25(1), p.013032_1 - 013032_11, 2023/01

 Times Cited Count:1 Percentile:31.85(Physics, Multidisciplinary)

Journal Articles

Weyl-Kondo semimetal behavior in the chiral structure phase of Ce$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$

Iwasa, Kazuaki*; Suyama, Kazuya*; Kawamura, Seiko; Nakajima, Kenji; Raymond, S.*; Steffens, P.*; Yamada, Akira*; Matsuda, Tatsuma*; Aoki, Yuji*; Kawasaki, Ikuto; et al.

Physical Review Materials (Internet), 7(1), p.014201_1 - 014201_11, 2023/01

 Times Cited Count:5 Percentile:44.41(Materials Science, Multidisciplinary)

Journal Articles

Possible options for efficient wide-band polychromatic measurements using chopper spectrometers at pulsed sources

Nakajima, Kenji; Kikuchi, Tatsuya*; Kawamura, Seiko; Kambara, Wataru*

EPJ Web of Conferences, 272, p.02012_1 - 02012_8, 2022/11

We will present some of attempts on AMATEAS, a cold-neutron chopper spectrometer at a pulsed source, to increase time-windows at a single-measurement condition. One of ways is that, by allowing interveined trajectories on the time-of-flight diagram, the usable width selectable for $$E$$$$_{rm is}$$ is can be increased. Based on our experiences, the conditions of pulse repetition rate multiplication based polychromatic $$E$$$$_{rm i}$$ measurements on chopper spectrometers at pulsed sources will be discussed. Optimization of wide-band polychromatic $$E$$$$_{rm i}$$ measurements and a generalized formulated condition will be proposed. Application of our idea to existing spectrometers and to the criteria design of an optimized chopper spectrometer will be also discussed with suggesting further possibility to improve efficiency by modifying the pulse shaping chopper.

Journal Articles

$$Q$$-dependent collective relaxation dynamics of glass-forming liquid Ca$$_{0.4}$$K$$_{0.6}$$(NO$$_{3}$$)$$_{1.4}$$ investigated by wide-angle neutron spin-echo

Luo, P.*; Zhai, Y.*; Falus, P.*; Garc$'i$a Sakai, V.*; Hartl, M.*; Kofu, Maiko; Nakajima, Kenji; Faraone, A.*; Z, Y.*

Nature Communications (Internet), 13, p.2092_1 - 2092_9, 2022/04

 Times Cited Count:13 Percentile:75.82(Multidisciplinary Sciences)

Journal Articles

Breakdown of linear spin-wave theory and existence of spinon bound states in the frustrated kagome-lattice antiferromagnet

Mattan, K.*; Ono, Toshio*; Kawamura, Seiko; Nakajima, Kenji; Nambu, Yusuke*; Sato, Taku*

Physical Review B, 105(13), p.134403_1 - 134403_8, 2022/04

 Times Cited Count:4 Percentile:28.11(Materials Science, Multidisciplinary)

Spin dynamics of the spin-1/2 kagome-lattice antiferromagnet Cs$$_{2}$$Cu$$_{3}$$SnF$$_{12}$$ was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering.

Journal Articles

Enhanced covalency and nanostructured-phonon scattering lead to high thermoelectric performance in $$n$$-type PbS

Rathore, E.*; Juneja, R.*; Sarkar, D.*; Roychowdhury, S.*; Kofu, Maiko; Nakajima, Kenji; Singh, A. K.*; Biswas, K.*

Materials Today Energy (Internet), 24, p.100953_1 - 100953_9, 2022/03

 Times Cited Count:21 Percentile:79.28(Chemistry, Physical)

Journal Articles

Mictomagnetism and suppressed thermal conduction of the prototype high-entropy alloy CrMnFeCoNi

Yang, J.*; Ren, W.*; Zhao, X.*; Kikuchi, Tatsuya*; Miao, P.*; Nakajima, Kenji; Li, B.*; Zhang, Z.*

Journal of Materials Science & Technology, 99, p.55 - 60, 2022/02

 Times Cited Count:12 Percentile:54.80(Materials Science, Multidisciplinary)

High-entropy alloys are characteristic of extensive atomic occupational disorder on high-symmetric lattices, differing from traditional alloys. Here, we investigate magnetic and thermal transport properties of the prototype face-centered-cubic high-entropy alloy CrMnFeCoNi by combining physical properties measurements and neutron scattering. Direct-current (dc) and alternating-current (ac) magnetizations measurements indicate a mictomagnetic behavior with coexisting antiferromagnetic and ferromagnetic interactions in the entire temperature region and three anomalies are found at about 80, 50, and 20 K, which are related to the paramagnetic to antiferromagnetic transition, the antiferromagnetic to ferromagnetic transition, and the spin freezing, respectively. The electrical and thermal conductivities are significantly reduced compared to Ni and the temperature dependence of lattice thermal conductivity exhibits a glass-like plateau. Inelastic neutron scattering measurements suggest weak anharmonicity so that the thermal transport is expected to be dominated by the defect scattering.

Journal Articles

Magnons and spinons in Ba$$_{2}$$CoTeO$$_{6}$$; A Composite system of isolated spin-$$frac{1}{2}$$ triangular Heisenberg-like and frustrated honeycomb Ising-like antiferromagnets

Kojima, Yuki*; Kurita, Nubuyuki*; Tanaka, Hidekazu*; Nakajima, Kenji

Physical Review B, 105(2), p.L020408_1 - L020408_6, 2022/01

 Times Cited Count:8 Percentile:52.43(Materials Science, Multidisciplinary)

We report the neutron scattering results on magnetic orderings and excitations in Ba$$_{2}$$CoTeO$$_{6}$$ composed of two almost isolated subsystems A and B, which are described as an $${S = 1/2}$$ triangular Heisenberg-like antiferromagnet and a frustrated honeycomb Ising-like antiferromagnet, respectively. It was found that the excitation spectra of both subsystems are well separated and independent of each other. The excitation spectrum of subsystem A is composed of two single-magnon branches with roton-like minima at the M point and a clearly structured intense continuum, as similarly observed in Ba$$_{3}$$CoSb$$_{2}$$O$$_{9}$$, which is strongly indicative of spinon excitations. Dispersion curves for subsystem B can be described by linear spin wave theory within the third-neighbor exchange interaction.

Journal Articles

Experimental analysis on dynamics of liquid molecules adjacent to particles in nanofluids

Hashimoto, Shunsuke*; Nakajima, Kenji; Kikuchi, Tatsuya*; Kamazawa, Kazuya*; Shibata, Kaoru; Yamada, Takeshi*

Journal of Molecular Liquids, 342, p.117580_1 - 117580_8, 2021/11

 Times Cited Count:4 Percentile:20.59(Chemistry, Physical)

Quasi-elastic neutron scattering (QENS) and pulsed-field-gradient nuclear magnetic resonance (PFGNMR) analyses of a nanofluid composed of silicon dioxide (SiO$$_{2}$$) nanoparticles and a base fluid of ethylene glycol aqueous solution were performed. The aim was to elucidate the mechanism increase in the thermal conductivity of the nanofluid above its theoretical value. The obtained experimental results indicate that SiO$$_{2}$$ particles may decrease the self-diffusion coefficient of the liquid molecules in the ethylene glycol aqueous solution because of their highly restricted motion around these nanoparticles. At a constant temperature, the thermal conductivity increases as the self-diffusion coefficient of the liquid molecules decreases in the SiO$$_{2}$$ nanofluids.

Journal Articles

Dimensional reduction by geometrical frustration in a cubic antiferromagnet composed of tetrahedral clusters

Okuma, Ryutaro*; Kofu, Maiko; Asai, Shinichiro*; Avdeev, M.*; Koda, Akihiro*; Okabe, Hirotaka*; Hiraishi, Masatoshi*; Takeshita, Soshi*; Kojima, Kenji*; Kadono, Ryosuke*; et al.

Nature Communications (Internet), 12, p.4382_1 - 4382_7, 2021/07

 Times Cited Count:10 Percentile:61.43(Multidisciplinary Sciences)

429 (Records 1-20 displayed on this page)