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Kikuchi, Tatsuya*; Mashita, Ryo*; Masui, Tomomi*; Kanaya, Toshiji*; Kishimoto, Hiroyuki*; Nakajima, Kenji
Physical Review E, 113(6), p.065418_1 - 064518_10, 2026/06
We investigated the local dynamics of polybutadiene over a wide temperature range, using quasielastic neutron scattering combined in the modified mode distribution analysis. Among these processes, the subpicosecond fast process was analyzed using a local diffusion model, which characterizes the dynamics via two physically meaningful parameters: the local diffusion coefficient and the harmonic potential stiffness. Temperature-dependent analysis revealed a distinct dynamic transition near the glass transition, which is interpreted as the disappearance of cooperative diffusion involving multiple segments. Furthermore, an additional relaxation mode, termed the extra-fast process, was identified and interpreted as a higher-order mode within the local diffusion model. These findings suggest a unified physical framework for the evolution of local motions across the glass transition and establish a robust methodology for quantifying polymer dynamics at subnanometer and subpicosecond scales.
SbO
Piyakulworawat, C.*; Morita, Katsuhiro*; Fukumoto, Yoshiyuki*; Hsieh, W.-Y.*; Chen, W.-T.*; Nakajima, Kenji; Kawamura, Seiko; Zhao, Y.*; Wannapaiboon, S.*; Piyawongwatthana, P.; et al.
Physical Review Research (Internet), 8(1), p.013247_1 - 013247_16, 2026/03
We analyze powder-averaged inelastic neutron scattering and magnetization data for the distorted honeycomb compound CuSbO using a first-order dimer expansion calculation and quantum Monte Carlo simulations. We show that, in contrast to the previously proposed honeycomb lattice model, CuSbO accommodates interacting dimerized spin chains with alternating ferromagnetic-antiferromagnetic couplings along the chain. Moreover, unlike the typical couplings observed in other Cu
-based distorted honeycomb magnets, the spin chains in CuSbO primarily couple through an antiferromagnetic coupling that arises between the honeycomb layers, rather than the expected interchain coupling in the layers. This finding reveals a different magnetic coupling scheme for CuSbO. In addition, utilizing X-ray spectroscopy and transmission electron microscopy, we also refine the crystal structure and stacking-fault model of the compound.
Nagasumi, Satoru; Hasegawa, Toshinari; Iigaki, Kazuhiko; Nakagawa, Shigeaki; Kubo, Shinji; Shimazaki, Yosuke; Nakajima, Kunihiro; Sakurai, Yosuke; Shinohara, Masanori; Saito, Kenji; et al.
Nuclear Engineering and Design, 446(Part A), p.114542_1 - 114542_14, 2026/01
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)To demonstrate HTGR's safety features, a loss-of-forced-cooling (LOFC) test was conducted using the HTTR. In this test, the forced cooling in the reactor core was intentionally lost by shutting down all helium gas circulators (HGCs) without reactor scram. During steady-state operation at 100% reactor power (30 MW), after the LOFC, the reactor power spontaneously decreased. This power reduction occurred due to the negative reactivity feedback effect triggered by an increase in core temperature. The power stabilized at a lower value of 1.2% after re-criticality. Additionally, the measured radioactivity concentration in the primary coolant remained nearly unchanged during this LOFC operation and during an immediately subsequent HTTR operation. This indicates no failure of the coated particle fuel, even after the increase in core temperature associated with the LOFC event. These results provide experimental evidence of the safety features of HTGRs.
with geometrically frustrated orthogonal antiferromagnetic dimerMetoki, Naoto; Yamauchi, Hiroki; Hagihara, Masato; Watanuki, Ryuta*; Kawamura, Seiko; Kofu, Maiko*; Nakajima, Kenji; Matsuda, Masaaki*
Physical Review B, 111(10), p.104424_1 - 104424_9, 2025/03
Times Cited Count：2 Percentile：53.44(Materials Science, Multidisciplinary)Inelastic neutron scattering experiments were carried out to understand the unusual successive order in NdB with the frustrated Shatry-Sutherland (SS) lattice. The pseudo-quartet with 
and 
splits into four levels in the magnetically ordered states. The spectra can be explained with the on-site magnetic interaction 
, the coupling of 
with quadrupole 
, and the uniaxial crystalline electric field. The 
-electron states reproduce the temperature dependences of the in-plane moment 
which is the primary order parameter, and a weakly induced 
as the secondary order parameter. The magnetic-quadrupole coupling emerges and play essential role under the geometrical frustration, where the Heisenberg interactions are cancelled out.
MnSiO
Kawamata, Masahiro*; Pang, X.*; Murakawa, Hiroshi*; Kawamura, Seiko; Nakajima, Kenji; Masuda, Hidetoshi*; Fujita, Masaki*; Hanasaki, Noriaki*; Onose, Yoshinori*; Nambu, Yusuke*
Physical Review Materials (Internet), 9(1), p.014407_1 - 014407_6, 2025/01
Times Cited Count：1 Percentile：27.06(Materials Science, Multidisciplinary)Li, S.*; Meng, Z. Y.*; Nakajima, Kenji
Neutron News, 35(3-4), p.26 - 28, 2024/10
Nirei, Masami; Kofu, Maiko; Nakajima, Kenji; Kikuchi, Tatsuya*; Kawamura, Seiko; Murai, Naoki; Harada, Masahide; Inamura, Yasuhiro
Journal of Neutron Research, 26(2-3), p.75 - 82, 2024/09
Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*
Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09
Times Cited Count：11 Percentile：80.20(Physics, Multidisciplinary)Zeng, Z.*; Zhou, C.*; Zhou, H.*; Han, L.*; Chi, R.*; Li, K.*; Kofu, Maiko; Nakajima, Kenji; Wei, Y.*; Zhang, W.*; et al.
Nature Physics, 20(7), p.1097 - 1102, 2024/07
Times Cited Count：30 Percentile：96.04(Physics, Multidisciplinary)
-MgAgSbLi, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; Kofu, Maiko; Nakajima, Kenji; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.
Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03
Times Cited Count：18 Percentile：87.02(Physics, Applied)Kikuchi, Tatsuya*; Kawakita, Yukinobu; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro
Journal of Molecular Liquids, 385, p.121868_1 - 121868_10, 2023/09
Times Cited Count：3 Percentile：23.65(Chemistry, Physical)
SnSeRen, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; Kofu, Maiko; et al.
Nature Materials, 22(8), p.999 - 1006, 2023/08
Times Cited Count：135 Percentile：99.25(Chemistry, Physical)Hashimoto, Shunsuke*; Yamaguchi, Satoshi*; Harada, Masashi*; Nakajima, Kenji; Kikuchi, Tatsuya*; Oishi, Kazuki*
Journal of Colloid and Interface Science, 638, p.475 - 486, 2023/05
Times Cited Count：13 Percentile：55.81(Chemistry, Physical)Recently, it has been reported that anomalous improvement in the thermal conductivity of nanofluid composed of base liquids and dispersed solid nanoparticles, compared to the theoretically predicted value calculated from the particle fraction. Generally, the thermal conductivity values of gases and liquids are dominated by the mean free path of the molecules during translational motion. Herein, we present solid evidence showing the possible contribution of the vibrational behavior of liquid molecules around nanoparticles to increasing these thermal conductivities.
Wu, P.*; Murai, Naoki; Li, T.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Kofu, Maiko; Nakajima, Kenji; Xia, K.*; Peng, K.*; Zhang, Y.*; et al.
New Journal of Physics (Internet), 25(1), p.013032_1 - 013032_11, 2023/01
Times Cited Count：3 Percentile：26.91(Physics, Multidisciplinary)
Rh
Sn
Iwasa, Kazuaki*; Suyama, Kazuya*; Kawamura, Seiko; Nakajima, Kenji; Raymond, S.*; Steffens, P.*; Yamada, Akira*; Matsuda, Tatsuma*; Aoki, Yuji*; Kawasaki, Ikuto; et al.
Physical Review Materials (Internet), 7(1), p.014201_1 - 014201_11, 2023/01
Times Cited Count：7 Percentile：40.89(Materials Science, Multidisciplinary)Nakajima, Kenji; Kikuchi, Tatsuya*; Kawamura, Seiko; Kambara, Wataru*
EPJ Web of Conferences, 272, p.02012_1 - 02012_8, 2022/11
We will present some of attempts on AMATEAS, a cold-neutron chopper spectrometer at a pulsed source, to increase time-windows at a single-measurement condition. One of ways is that, by allowing interveined trajectories on the time-of-flight diagram, the usable width selectable for 
is can be increased. Based on our experiences, the conditions of pulse repetition rate multiplication based polychromatic 
measurements on chopper spectrometers at pulsed sources will be discussed. Optimization of wide-band polychromatic measurements and a generalized formulated condition will be proposed. Application of our idea to existing spectrometers and to the criteria design of an optimized chopper spectrometer will be also discussed with suggesting further possibility to improve efficiency by modifying the pulse shaping chopper.
-dependent collective relaxation dynamics of glass-forming liquid Ca
K
(NO)
investigated by wide-angle neutron spin-echoLuo, P.*; Zhai, Y.*; Falus, P.*; Garc
a Sakai, V.*; Hartl, M.*; Kofu, Maiko; Nakajima, Kenji; Faraone, A.*; Z, Y.*
Nature Communications (Internet), 13, p.2092_1 - 2092_9, 2022/04
Times Cited Count：15 Percentile：75.79(Multidisciplinary Sciences)Matan, K.*; Ono, Toshio*; Kawamura, Seiko; Nakajima, Kenji; Nambu, Yusuke*; Sato, Taku*
Physical Review B, 105(13), p.134403_1 - 134403_8, 2022/04
Times Cited Count：4 Percentile：23.74(Materials Science, Multidisciplinary)Spin dynamics of the spin-1/2 kagome-lattice antiferromagnet CsCuSnF
was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering.
-type PbSRathore, E.*; Juneja, R.*; Sarkar, D.*; Roychowdhury, S.*; Kofu, Maiko; Nakajima, Kenji; Singh, A. K.*; Biswas, K.*
Materials Today Energy (Internet), 24, p.100953_1 - 100953_9, 2022/03
Times Cited Count：26 Percentile：78.15(Chemistry, Physical)Yang, J.*; Ren, W.*; Zhao, X.*; Kikuchi, Tatsuya*; Miao, P.*; Nakajima, Kenji; Li, B.*; Zhang, Z.*
Journal of Materials Science & Technology, 99, p.55 - 60, 2022/02
Times Cited Count：14 Percentile：52.84(Materials Science, Multidisciplinary)High-entropy alloys are characteristic of extensive atomic occupational disorder on high-symmetric lattices, differing from traditional alloys. Here, we investigate magnetic and thermal transport properties of the prototype face-centered-cubic high-entropy alloy CrMnFeCoNi by combining physical properties measurements and neutron scattering. Direct-current (dc) and alternating-current (ac) magnetizations measurements indicate a mictomagnetic behavior with coexisting antiferromagnetic and ferromagnetic interactions in the entire temperature region and three anomalies are found at about 80, 50, and 20 K, which are related to the paramagnetic to antiferromagnetic transition, the antiferromagnetic to ferromagnetic transition, and the spin freezing, respectively. The electrical and thermal conductivities are significantly reduced compared to Ni and the temperature dependence of lattice thermal conductivity exhibits a glass-like plateau. Inelastic neutron scattering measurements suggest weak anharmonicity so that the thermal transport is expected to be dominated by the defect scattering.
