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Journal Articles

Experimental analysis on dynamics of liquid molecules adjacent to particles in nanofluids

Hashimoto, Shunsuke*; Nakajima, Kenji; Kikuchi, Tatsuya*; Kamazawa, Kazuya*; Shibata, Kaoru; Yamada, Takeshi*

Journal of Molecular Liquids, 342, p.117580_1 - 117580_8, 2021/11

 Times Cited Count:3 Percentile:27(Chemistry, Physical)

Quasi-elastic neutron scattering (QENS) and pulsed-field-gradient nuclear magnetic resonance (PFGNMR) analyses of a nanofluid composed of silicon dioxide (SiO$$_{2}$$) nanoparticles and a base fluid of ethylene glycol aqueous solution were performed. The aim was to elucidate the mechanism increase in the thermal conductivity of the nanofluid above its theoretical value. The obtained experimental results indicate that SiO$$_{2}$$ particles may decrease the self-diffusion coefficient of the liquid molecules in the ethylene glycol aqueous solution because of their highly restricted motion around these nanoparticles. At a constant temperature, the thermal conductivity increases as the self-diffusion coefficient of the liquid molecules decreases in the SiO$$_{2}$$ nanofluids.

Journal Articles

Dimensional reduction by geometrical frustration in a cubic antiferromagnet composed of tetrahedral clusters

Okuma, Ryutaro*; Kofu, Maiko; Asai, Shinichiro*; Avdeev, M.*; Koda, Akihiro*; Okabe, Hirotaka*; Hiraishi, Masatoshi*; Takeshita, Soshi*; Kojima, Kenji*; Kadono, Ryosuke*; et al.

Nature Communications (Internet), 12, p.4382_1 - 4382_7, 2021/07

 Times Cited Count:6 Percentile:61.42(Multidisciplinary Sciences)

Journal Articles

Spin glass behavior and magnetic boson peak in a structural glass of a magnetic ionic liquid

Kofu, Maiko; Watanuki, Ryuta*; Sakakibara, Toshiro*; Kawamura, Seiko; Nakajima, Kenji; Matsuura, Masato*; Ueki, Takeshi*; Akutsu, Kazuhiro*; Yamamuro, Osamu*

Scientific Reports (Internet), 11(1), p.12098_1 - 12098_8, 2021/06

 Times Cited Count:5 Percentile:56.02(Multidisciplinary Sciences)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:56.2(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Colossal barocaloric effects in plastic crystals

Li, B.*; Kawakita, Yukinobu; Kawamura, Seiko; Sugahara, Takeshi*; Wang, H.*; Wang, J.*; Chen, Y.*; Kawaguchi, Saori*; Kawaguchi, Shogo*; Ohara, Koji*; et al.

Nature, 567(7749), p.506 - 510, 2019/03

 Times Cited Count:182 Percentile:99.31(Multidisciplinary Sciences)

Refrigeration is of vital importance for modern society for example, for food storage and air conditioning- and 25 to 30% of the world's electricity is consumed for refrigeration. Current refrigeration technology mostly involves the conventional vapour compression cycle, but the materials used in this technology are of growing environmental concern because of their large global warming potential. As a promising alternative, refrigeration technologies based on solid-state caloric effects have been attracting attention in recent decades. However, their application is restricted by the limited performance of current caloric materials, owing to small isothermal entropy changes and large driving magnetic fields. Here we report colossal barocaloric effects (CBCEs) (barocaloric effects are cooling effects of pressure-induced phase transitions) in a class of disordered solids called plastic crystals. The obtained entropy changes in a representative plastic crystal, neopentylglycol, are about 389 joules per kilogram per kelvin near room temperature. Pressure-dependent neutron scattering measurements reveal that CBCEs in plastic crystals can be attributed to the combination of extensive molecular orientational disorder, giant compressibility and highly anharmonic lattice dynamics of these materials. Our study establishes the microscopic mechanism of CBCEs in plastic crystals and paves the way to next-generation solid-state refrigeration technologies.

Journal Articles

Status report of the chopper spectrometer 4SEASONS

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Iida, Kazuki*; Ishikado, Motoyuki*; Murai, Naoki; Kira, Hiroshi*; Nakatani, Takeshi; et al.

Journal of Physics; Conference Series, 1021(1), p.012030_1 - 012030_6, 2018/06

BB2016-1727.pdf:0.39MB

 Times Cited Count:3 Percentile:88.67(Nuclear Science & Technology)

Journal Articles

Liquid-like thermal conduction in intercalated layered crystalline solids

Li, B.; Wang, H.*; Kawakita, Yukinobu; Zhang, Q.*; Feygenson, M.*; Yu, H. L.*; Wu, D.*; Ohara, Koji*; Kikuchi, Tatsuya*; Shibata, Kaoru; et al.

Nature Materials, 17(3), p.226 - 230, 2018/03

 Times Cited Count:121 Percentile:96.83(Chemistry, Physical)

Journal Articles

Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex, 3; Neutron devices and computational and sample environments

Sakasai, Kaoru; Sato, Setsuo*; Seya, Tomohiro*; Nakamura, Tatsuya; To, Kentaro; Yamagishi, Hideshi*; Soyama, Kazuhiko; Yamazaki, Dai; Maruyama, Ryuji; Oku, Takayuki; et al.

Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09

Neutron devices such as neutron detectors, optical devices including supermirror devices and $$^{3}$$He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.

Journal Articles

Polar rotor scattering as atomic-level origin of low mobility and thermal conductivity of perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$

Li, B.; Kawakita, Yukinobu; Liu, Y.*; Wang, M.*; Matsuura, Masato*; Shibata, Kaoru; Kawamura, Seiko; Yamada, Takeshi*; Lin, S.*; Nakajima, Kenji; et al.

Nature Communications (Internet), 8, p.16086_1 - 16086_9, 2017/06

 Times Cited Count:81 Percentile:91.64(Multidisciplinary Sciences)

Journal Articles

Inelastic and quasi-elastic neutron scattering spectrometers in J-PARC

Seto, Hideki; Ito, Shinichi; Yokoo, Tetsuya*; Endo, Hitoshi*; Nakajima, Kenji; Shibata, Kaoru; Kajimoto, Ryoichi; Kawamura, Seiko; Nakamura, Mitsutaka; Kawakita, Yukinobu; et al.

Biochimica et Biophysica Acta; General Subjects, 1861(1), p.3651 - 3660, 2017/01

 Times Cited Count:32 Percentile:80.67(Biochemistry & Molecular Biology)

J-PARC, Japan Proton Accelerator Research Complex provides short pulse proton beam at a repetition rate 25 Hz and the maximum power is expected to be 1 MW. Materials and Life Science Experimental Facility (MLF) has 23 neutron beam ports and 21 instruments have already been operated or under construction / commissioning. There are 6 inelastic / quasi-elastic neutron scattering spectrometers and the complementary use of these spectrometers will open new insight for life science.

Journal Articles

Recent progress in the chopper spectrometer 4SEASONS at J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Iida, Kazuki*; Ishikado, Motoyuki*; Nakajima, Kenji; Kawamura, Seiko; Nakatani, Takeshi; et al.

JAEA-Conf 2015-002, p.319 - 329, 2016/02

Journal Articles

Precise determination of $$^{12}_{Lambda}$$C level structure by $$gamma$$-ray spectroscopy

Hosomi, Kenji; Ma, Y.*; Ajimura, Shuhei*; Aoki, Kanae*; Dairaku, Seishi*; Fu, Y.*; Fujioka, Hiroyuki*; Futatsukawa, Kenta*; Imoto, Wataru*; Kakiguchi, Yutaka*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2015(8), p.081D01_1 - 081D01_8, 2015/08

 Times Cited Count:14 Percentile:66.59(Physics, Multidisciplinary)

Level structure of the $$^{12}_{Lambda}$$C hypernucleus was precisely determined by means of $$gamma$$-ray spectroscopy. We identified four $$gamma$$-ray transitions via the $$^{12}$$C$$(pi^{+},K^{+}gamma)$$ reaction using a germanium detector array, Hyperball2. The spacing of the ground-state doublet $$(2^{-}, 1^{-}_{1})$$ was measured to be $$161.5pm0.3$$(stat)$$pm0.3$$ (syst)keV from the direct $$M1$$ transition. Excitation energies of the $$1^{-}_{2}$$ and $$1^{-}_{3}$$ states were measured to be $$2832pm3pm4$$, keV and $$6050pm8pm7$$, keV, respectively. The obtained level energies provide definitive references for the reaction spectroscopy of $$Lambda$$ hypernuclei.

Journal Articles

Novel electrothermodynamic power generation

Kim, Y.*; Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Ogawa, Takashi*; Serizawa, Takeshi*; Tanaka, Hirohisa*; Baba, Masaaki*; Fukuda, Tatsuo; Yoshii, Kenji; et al.

Advanced Energy Materials, 5(13), p.1401942_1 - 1401942_6, 2015/07

 Times Cited Count:18 Percentile:60.39(Chemistry, Physical)

An innovative electro-thermodynamic cycle based on temporal temperature variations using pyroelectric effect has been presented. Practical energy is successfully generated in both $textit{in-situ}$ synchrotron X-ray diffraction measurements under controlled conditions and $textit{Operando}$ real engine dynamometer experiments. The main generating origin is revealed as a combination of a crystal structure change and dipole change phenomenon corresponds to the temperature variation. In particular, the electric field induced 180$$^circ$$ domain switching extremely improves generating power, and the true energy breakeven with temperature variation is firstly achieved.

Journal Articles

"Relative rates method" for evaluating the effect of potential geological environmental change due to uplift/erosion to radionuclide migration of high-level radioactive waste

Ebashi, Takeshi; Kawamura, Makoto*; Inagaki, Manabu*; Koo, Shigeru*; Shibata, Masahiro; Itazu, Toru; Nakajima, Kunihiko*; Miyahara, Kaname; Apted, M. J.*

Materials Research Society Symposium Proceedings, Vol.1665, p.39 - 45, 2014/07

In Japan, the likelihood of uplift/erosion on repository performance and waste isolation can be typically greatly reduced or excluded by careful siting, however, the inability to completely exclude the uplift/erosion scenario may require an analysis of the consequences of such a scenario. For this purpose, an assessment approach has been developed to more realistically treat the effect of uplift/erosion for a hypothetical repository located in sedimentary host rock. A key advantage to this approach is the extrapolation of the geohistory of modern analogue sites to develop credible initial inputs for future volunteer sites that may be poorly characterized at the initial stages of site investigation. In addition, the approach provides a systematic basis for bounding the range of possible evolution in thermal-hydrological-mechanical-chemical conditions of a repository experiencing different uplift/ erosion rates.

Journal Articles

Visualization of $$gamma$$H2AX foci caused by heavy ion particle traversal; Distribution between core track versus non-track damage

Nakajima, Nakako*; Brunton, H.*; Watanabe, Ritsuko; Shrikhande, A.*; Hirayama, Ryoichi*; Matsufuji, Naruhiro*; Fujimori, Akira*; Murakami, Takeshi*; Okayasu, Ryuichi*; Jeggo, P.*; et al.

PLOS ONE (Internet), 8(8), p.e70107_1 - e70107_14, 2013/08

 Times Cited Count:63 Percentile:91.05(Multidisciplinary Sciences)

Heavy particle irradiation can produce complex DNA double strand breaks (DSBs) within the particle trajectory. Additionally, secondary electrons, termed delta-electrons, can create low linear energy transfer (LET) damage distant from the track. Using imaging with deconvolution, we show that at 8 hours after exposure to Fe ions, $$gamma$$H2AX foci forming at DSBs within the particle track are large and encompass multiple smaller and closely localised foci, which we designate as clustered $$gamma$$H2AX foci. We also identified simple $$gamma$$H2AX foci distant from the track. They are rapidly repaired. Clustered $$gamma$$H2AX foci induced by heavy particle radiation cause prolonged checkpoint arrest compared to simple $$gamma$$H2AX foci. However, mitotic entry was observed when $$sim$$10 clustered foci remain. Thus, cells can progress into mitosis with multiple clusters of DSBs following the traversal of a heavy particle.

Journal Articles

Recent developments of instruments in a spallation neutron source at J-PARC and those prospects in the future

Arai, Masatoshi; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Nakajima, Kenji; Shibata, Kaoru; Takahashi, Nobuaki; Suzuki, Junichi*; Takata, Shinichi; Yamada, Takeshi*; et al.

Journal of the Physical Society of Japan, 82(Suppl.A), p.SA024_1 - SA024_14, 2013/01

 Times Cited Count:7 Percentile:47.49(Physics, Multidisciplinary)

The paper describes developments of neutron scattering instruments in J-PARC neutron facility, which is a short pulse spallation source operated at a repetition rate 25 Hz and has a proton power 1 MW. New concept has been adopted to utilize high intensity coupled moderator even for a high resolution inelastic scattering instruments by taking a pulse shaping chopper system. Advanced technique has been also realized by taking an ability of event-recording system altogether with an improvement of a chopper system, realizing multi-Ei method. The paper also touches upon a general design concept for diffractometers in accordance with the source characteristics.

Journal Articles

Effects of irradiation-particle energy on critical current density in Co-doped BaFe$$_{2}$$As$$_{2}$$

Taen, Toshihiro*; Yagyuda, Hidenori*; Nakajima, Yasuyuki*; Tamegai, Tsuyoshi*; Okayasu, Satoru; Kitamura, Hisashi*; Murakami, Takeshi*; Laviano, F.*; Ghigo, G.*

Physica C, 484, p.62 - 65, 2013/01

 Times Cited Count:8 Percentile:37.16(Physics, Applied)

We report effects of particle energy on physical properties of Co-doped BaFe$$_{2}$$As$$_{2}$$ in the case of Xe and Au irradiations. The irradiation-induced suppression of $$T$$$$_{rm c}$$ is found to be related with several factors, such as defect structures and the thickness of the crystal. Heavy-ion irradiation induces enhancement of critical current density $$J$$$$_{rm c}$$, and a weak dip in the hysteresis loop. The fish-tail effect is completely suppressed by a modest density of defects. The enhancement of $$J$$$$_{rm c}$$ is closely related to the defect structure. Namely, splayed structure in columnar defects, inevitably introduced at lower energies, results in a strong enhancement of $$J$$$$_{rm c}$$ by forced entanglement of vortices.

Journal Articles

Effects of particle irradiations on vortex states in iron-based superconductors

Tamegai, Tsuyoshi*; Taen, Toshihiro*; Yagyuda, Hidenori*; Tsuchiya, Yuji*; Mohan, S.*; Taniguchi, Tomotaka*; Nakajima, Yasuyuki*; Okayasu, Satoru; Sasase, Masato*; Kitamura, Hisashi*; et al.

Superconductor Science and Technology, 25(8), p.084008_1 - 084008_14, 2012/08

 Times Cited Count:85 Percentile:93.2(Physics, Applied)

Various kinds of energetic particles are irradiated into iron-based superconductors, and their effects on the critical current density $$J$$$$_{rm c}$$ and vortex dynamics have been systematically studied. It is found that $$J$$$$_{rm c}$$ is enhanced and vortex dynamics is strongly suppressed by energetic particles having a sufficient energy deposition rate, similar to the case of high temperature cuprate superconductors. The enhancement of $$J$$$$_{rm c}$$, in general, persists up to much higher irradiation doses than in cuprates. However, details of the effect of irradiation depend on the kind of ion species and their energies. Even with the same ions and energies, the effect is not universal for different kinds of iron-based superconductors. The correlated nature of defects created by heavy-ion irradiation is confirmed by the angular dependence of irreversible magnetization.

JAEA Reports

Design, fabrication and transportation of Si rotating device

Kimura, Nobuaki; Imaizumi, Tomomi; Takemoto, Noriyuki; Tanimoto, Masataka; Saito, Takashi; Hori, Naohiko; Tsuchiya, Kunihiko; Romanova, N. K.*; Gizatulin, S.*; Martyushov, A.*; et al.

JAEA-Technology 2012-012, 34 Pages, 2012/06

JAEA-Technology-2012-012.pdf:12.91MB

Si semiconductor production by Neutron Transmutation Doping (NTD) method using the Japan Materials Testing Reactor (JMTR) has been investigated in Neutron Irradiation and Testing Reactor Center, Japan Atomic Energy Agency (JAEA) in order to expand industry use. As a part of investigations, irradiation test of silicon ingot for development of NTD-Si with high quality was planned using WWR-K in Institute of Nuclear Physics (INP), National Nuclear Center of Republic of Kazakhstan (NNC-RK) based on one of specific topics of cooperation (STC), Irradiation Technology for NTD-Si (STC No.II-4), on the implementing arrangement between NNC-RK and the JAEA for "Nuclear Technology on Testing/Research Reactors" in cooperation in research and development in nuclear energy and technology. As for the irradiation test, Si rotating device was fabricated in JAEA, and the fabricated device was transported with irradiation specimens from JAEA to INP-NNC-RK. This report described the design, the fabrication, the performance test of the Si rotating device and transportation procedures.

Journal Articles

Repetition Rate Multiplication: RRM, an advanced measuring method planed for the backscattering instrument, ${it DNA}$ at the MLF, J-PARC

Takahashi, Nobuaki; Shibata, Kaoru; Kawakita, Yukinobu; Nakajima, Kenji; Inamura, Yasuhiro; Nakatani, Takeshi; Nakagawa, Hiroshi; Fujiwara, Satoru; Sato, Taku*; Tsukushi, Itaru*; et al.

Journal of the Physical Society of Japan, 80(Suppl.B), p.SB007_1 - SB007_4, 2011/12

 Times Cited Count:6 Percentile:43.42(Physics, Multidisciplinary)

136 (Records 1-20 displayed on this page)