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Journal Articles

Development of the ReaxFF methodology for electrolyte-water systems

Fedkin, M. V.*; Shin, Y. K.*; Dasgupta, N.*; Yeon, J.*; Zhang, W.*; van Duin, D.*; Van Duin, A. C. T.*; Mori, Kento*; Fujiwara, Atsushi*; Machida, Masahiko; et al.

Journal of Physical Chemistry A, 123(10), p.2125 - 2141, 2019/03

 Percentile:100(Chemistry, Physical)

no abstracts in English

Journal Articles

Investigation for dust behavior of cutting in air and cutting underwater by thermal cutting methods

Soejima, Goro; Iwai, Hiroki; Nakamura, Yasuyuki; Tsuzuki, Satoshi*; Yasunaga, Kazushi*; Kume, Kyo*

Heisei-29-Nendo Koeki Zaidan Hojin Wakasawan Enerugi Kenkyu Senta kenkyu Nempo, 20, P. 80, 2018/11

We investigated the behavior of the dust generated by Laser and Plasma-arc cutting underwater and in air aimed at the simulant material of reactor components (SUS304) and the pressure and calandria tube (Zr-2.5%Nb, Zry-2) of the prototype reactor "FUGEN".

Journal Articles

New antiferromagnetic order with pressure-induced superconductivity in EuFe$$_2$$As$$_2$$

Ikeda, Shugo*; Tsuchiya, Yu*; Zhang, X.-W.*; Kishimoto, Shunji*; Kikegawa, Takumi*; Yoda, Yoshitaka*; Nakamura, Hiroki; Machida, Masahiko; Glasbrenner, J.*; Kobayashi, Hisao*

Physical Review B, 98(10), p.100502_1 - 100502_6, 2018/09

 Percentile:100(Materials Science, Multidisciplinary)

The interplay between magnetism and superconductivity is one of important subjects to investigate the pairing mechanism in novel superconductors. We have found new coexistence between an antiferromagnetic order in the Fe sublattice and superconductivity of the FeAs-based EuFe$$_2$$As$$_2$$ superconductor in the pressure range from 2.4 to 3.0 GPa by $$^{57}$$Fe nuclear forward scattering (NFS) using a single crystal sample. The magnetic state in the Fe sublattice changes to a new antiferromagnetic one with superconductivity from a stripe-type antiferromagnetic one observed in normal conducting state at 2.7 GPa. Below the superconducting transition temperature, the temperature dependence of $$^{57}$$Fe NFS spectra reveals that the new antiferromagnetic order develops with the superconductivity. This non-trivial coupling of two ordered states in EuFe$$_2$$As$$_2$$ under pressure demonstrates a new and intriguing relationship between magnetism and superconductivity in Fe-based superconductors.

Journal Articles

Neutron inelastic scattering study of the $$f$$-electron states in NdPd$$_5$$Al$$_2$$

Metoki, Naoto; Yamauchi, Hiroki; Suzuki, Hiroyuki*; Kitazawa, Hideaki*; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro

Journal of the Physical Society of Japan, 87(8), p.084708_1 - 084708_7, 2018/08

 Times Cited Count:3 Percentile:20.01(Physics, Multidisciplinary)

Inelastic neutron scattering experiments were carried out in order to study the $$f$$-electron states of NdPd$$_5$$Al$$_2$$The CEF levels at 0K, 35.4K, 88.3K, 101.5K, and 198.8K were clarified from the excitation spectra. The $$Gamma_6$$ ground state contains the orbital with $$J_z=pm9/2$$ as a main component due to a large negative B$$_{20}=-1.4$$K, which is the origin of the strong uniaxial anisotropy. The estimated magnetic moment, the calculated susceptibility, magnetization curve, and specific heat are in good agreement with the experimental data. The existence of a common charge distribution with CePd$$_5$$Al$$_2$$ and PrPd$$_5$$Al$$_2$$. Indicates that a localized character is important even in actinide-based iso-structural compounds as actually observed in UPd$$_5$$Al$$_2$$ and also NpPd$$_5$$Al$$_2$$, in which the valence crossover plays important role for the heavy fermion superconductivity.

Journal Articles

Neutron scattering study of yttrium iron garnet

Shamoto, Shinichi; Ito, Takashi; Onishi, Hiroaki; Yamauchi, Hiroki; Inamura, Yasuhiro; Matsuura, Masato*; Akatsu, Mitsuhiro*; Kodama, Katsuaki; Nakao, Akiko*; Moyoshi, Taketo*; et al.

Physical Review B, 97(5), p.054429_1 - 054429_9, 2018/02

 Times Cited Count:1 Percentile:100(Materials Science, Multidisciplinary)

Nuclear and magnetic structure and full magnon dispersions of yttrium iron garnet Y$$_3$$Fe$$_5$$O$$_{12}$$ have been studied by neutron scattering. The lowest-energy dispersion below 14 meV exhibits a quadratic dispersion as expected from ferromagnetic magnons. The imaginary part of $$q$$-integrated dynamical spin susceptibility $$chi$$"($$E$$) exhibits a square-root energy-dependence in the low energies. The magnon density of state is estimated from the $$chi$$"($$E$$) obtained on an absolute scale. The value is consistent with a single chirality mode for the magnon branch expected theoretically.

Journal Articles

Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12

The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.

Journal Articles

Study of the dust behavior on the laser and plasma cutting

Soejima, Goro; Iwai, Hiroki; Kadowaki, Haruhiko; Nakamura, Yasuyuki; Tsuzuki, Satoshi*; Yasunaga, Kazushi*; Nakata, Yoshinori*; Kume, Kyo*

Heisei-28-Nendo Koeki Zaidan Hojin Wakasawan Enerugi Kenkyu Senta kenkyu Nempo, 19, P. 9, 2017/10

no abstracts in English

Journal Articles

Technology development on reactor dismantling and investigation of contamination in FUGEN

Soejima, Goro; Iwai, Hiroki; Nakamura, Yasuyuki; Hayashi, Hirokazu; Kadowaki, Haruhiko; Mizui, Hiroyuki; Sano, Kazuya

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 5 Pages, 2017/07

no abstracts in English

Journal Articles

NIRS3; The Near Infrared Spectrometer on Hayabusa2

Iwata, Takahiro*; Kitazato, Kohei*; Abe, Masanao*; Otake, Makiko*; Arai, Takehiko*; Arai, Tomoko*; Hirata, Naru*; Hiroi, Takahiro*; Honda, Chikatoshi*; Imae, Naoya*; et al.

Space Science Reviews, 208(1-4), p.317 - 337, 2017/07

NIRS3: The Near Infrared Spectrometer is installed on the Hayabusa2 spacecraft to observe the target C-type asteroid 162173 Ryugu at near infrared wavelengths of 1.8 to 3.2 micrometer. It aims to obtain reflectance spectra in order to detect absorption bands of hydrated and hydroxide minerals in the 3 micrometer-band. We adopted a linear-image sensor with indium arsenide (InAs) photo diodes and a cooling system with a passive radiator to achieve an optics temperature of 188 K, which enables to retaining sufficient sensitivity and noise level in the 3 micrometer wavelength region. We conducted ground performance tests for the NIRS3 flight model (FM) to confirm its baseline specifications. The results imply that the properties such as the signal-to-noise ratio (SNR) conform to scientific requirements to determine the degree of aqueous alteration, such as CM or CI chondrite, and the stage of thermal metamorphism on the asteroid surface.

Journal Articles

Defect chemistry and basic properties of non-stoichiometric PuO$$_{2}$$

Kato, Masato; Nakamura, Hiroki; Watanabe, Masashi; Matsumoto, Taku; Machida, Masahiko

Defect and Diffusion Forum, 375, p.57 - 70, 2017/05

The basic properties of PuO$$_{2-x}$$ were reviewed, and the equilibrium defects in PuO$$_{2-x}$$ were evaluated from the experimental data of the oxygen potential and electrical conductivity as well as the Ab-initio calculation results. Consistency among various properties was confirmed, and the mechanistic models for thermal property representations were derived.

Journal Articles

High-temperature properties of thorium dioxide; A First-principles molecular dynamics study

Nakamura, Hiroki; Machida, Masahiko

Journal of Nuclear Materials, 478, p.56 - 60, 2016/09

 Times Cited Count:1 Percentile:76.09(Materials Science, Multidisciplinary)

Thorium has been considered a potential nuclear fuel for decades. To develop evaluation method for high-temperature properties of thorium dioxide as a candidate nuclear fuel, we perform first-principles molecular dynamics. The calculated enthalpy and thermal expansion agree well with the observed data. The Bredig transition temperature also coincides with experiments. Our results indicate that this method can provide reliable data of thermal properties of nuclear fuels.

Journal Articles

Effects of Mn substitution on the thermoelectric properties and thermal excitations of the electron-doped perovskite Sr$$_{1-x}$$La$$_{x}$$TiO$$_{3}$$

Okuda, Tetsuji*; Hata, Hiroto*; Eto, Takahiro*; Sobaru, Shogo*; Oda, Ryosuke*; Kaji, Hiroki*; Nishina, Kosuke*; Kuwahara, Hideki*; Nakamura, Mitsutaka; Kajimoto, Ryoichi

Journal of the Physical Society of Japan, 85(9), p.094717_1 - 094717_6, 2016/09

 Times Cited Count:4 Percentile:44.55(Physics, Multidisciplinary)

Journal Articles

Multi-band Eilenberger theory of superconductivity; Systematic low-energy projection

Nagai, Yuki; Nakamura, Hiroki

Journal of the Physical Society of Japan, 85(7), p.074707_1 - 074707_18, 2016/07

 Percentile:100(Physics, Multidisciplinary)

no abstracts in English

JAEA Reports

Applicability test of abrasive water jet cutting technology for dismantling of the core internals of Fukushima Daiichi NPS

Nakamura, Yasuyuki; Iwai, Hiroki; Tezuka, Masashi; Sano, Kazuya

JAEA-Technology 2015-055, 89 Pages, 2016/03

JAEA-Technology-2015-055.pdf:17.54MB

It was reported that Fukushima Daiichi Nuclear Power Station (1F) had lost the cooling function of the reactor by the Tohoku Earthquake. It is assumed that the core internals became narrow and complicated debris structure mixed with the molten fuel. In consideration of the above situations, the AWJ cutting method, which has features of the long work distance and little heat effect for a material, has been developed for the removal of the molten core internals through cutting tests for 3 years since FY 2012. And it was confirmed that AWJ cutting method is useful for the removal of the core internals etc. The results in FY 2012 were reported in "R&D of the fuel debris removal technologies by abrasive water jet cutting technology (JAEA-Technology 2013-041)" and this report summarizes the results of FY 2012, 2013 and 2014 in this report. It was confirmed the possibility to apply the removal work of the fuel debris and the core internals.

JAEA Reports

Applicability test of plasma cutting technology for dismantling of the core internals of Fukushima Daiichi NPS

Tezuka, Masashi; Nakamura, Yasuyuki; Iwai, Hiroki; Sano, Kazuya

JAEA-Technology 2015-047, 114 Pages, 2016/03

JAEA-Technology-2015-047.pdf:46.17MB

It was reported that Fukushima Daiichi Nuclear Power Plant had been lost the function of cooling the reactor by the Tohoku Earthquake. It is assumed that the original shapes of the internal core are not kept and the inside of the reactor makes so narrow in the space, however the fuel debris and the molten internal core will have to be removed for the decommissioning of 1F. We concerned the suppression of dross by optimization of cutting conditions, in using some moderated test pieces. And we can improve the cutting capability by heating the objects in advance. Moreover, it's possible that plasma arc cutting can cut off the mixed material the fuel debris and the molten internal core by using the cooperation cutting technique both the plasma arc and the plasma jet cutting. From these results, we have got the prospect that plasma cutting method can apply the removal of the fuel debris and the molten internal core.

JAEA Reports

The Development of the basic dismantling procedure of the reactor of FUGEN

Iwai, Hiroki; Nakamura, Yasuyuki; Mizui, Hiroyuki; Sano, Kazuya

JAEA-Technology 2015-046, 110 Pages, 2016/03

JAEA-Technology-2015-046.pdf:85.22MB

Advanced Thermal Reactor (ATR) FUGEN is a proto-type heavy water moderated, boiling light water cooled, pressure tube-type reactor with the thermal power of 557 MW and the electrical power of 165 MW. The reactor of FUGEN is classified into the core region and the shielding region. The core region is highly activated owing to the long term operation, and characterized by its tube-cluster construction that contains 224 fuel channels arranging both the pressure and the calandria tubes coaxially in each channel closely. And the shielding region surrounding the core region has the laminated structure composed of up to 150 mm thickness of carbon steel. The reactor is planning to be dismantled under water remotely in order to shield the radiation around the core and prevent airborne dust generated by the cutting, and firing of zirconium material. This paper reports on the result of development of the basic dismantling procedure of the reactor of FUGEN.

JAEA Reports

The Selection of the cutting technologies for dismantling the FUGEN reactor

Nakamura, Yasuyuki; Iwai, Hiroki; Mizui, Hiroyuki; Sano, Kazuya

JAEA-Technology 2015-045, 137 Pages, 2016/03

JAEA-Technology-2015-045.pdf:27.77MB

FUGEN is 9 m outer-diameter and 7m height, and characterized by its tube-cluster construction that contains 224 fuel channels arranging both the pressure and the calandria tubes coaxially in each channel. And the periphery part of the core has the laminated structure composed of up to 150 mm thickness of carbon steel for radiation shielding. The structure of the reactor, which is made of various materials such as stainless steel, carbon steel, zirconium alloy and aluminum. The reactor is planning to be dismantled under water in order to shield the radiation ray around the core and prevent airborne dust generated by the cutting, the temporary pool structure and the remote-operated dismantling machines needs to be installed on the top of reactor. In consideration of above the structure of Fugen reactor, the cutting method was selected for dismantling the reactor core in order to shorten the dismantling term and reduce the secondary waste.

Journal Articles

Effect of magnetism on lattice dynamics in SrFe$$_2$$As$$_2$$ using high-resolution inelastic X-ray scattering

Murai, Naoki*; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.

Physical Review B, 93(2), p.020301_1 - 020301_5, 2016/01

 Times Cited Count:4 Percentile:57.78(Materials Science, Multidisciplinary)

Journal Articles

Phonons of Fe-based superconductor Ca$$_{10}$$Pt$$_4$$As$$_8$$(Fe$$_{1-x}$$Pt$$_x$$As)$$_{10}$$

Ikeuchi, Kazuhiko*; Kobayashi, Yoshiaki*; Suzukia, Kazunori*; Ito, Masayuki*; Kajimoto, Ryoichi; Bourges, P.*; Christianson, A. D.*; Nakamura, Hiroki; Machida, Masahiko; Sato, Masatoshi*

Journal of Physics; Condensed Matter, 27(46), p.465701_1 - 465701_7, 2015/11

 Times Cited Count:1 Percentile:90.95(Physics, Condensed Matter)

We report the results of inelastic neutron scattering measurements on particular phonons of a superconducting (SC) Ca$$_{10}$$Pt$$_4$$As$$_8$$(Fe$$_{1-x}$$Pt$$_x$$As)$$_{10}$$ with the onset transition temperature $$T_c sim 33$$ K to investigate mainly what roles orbital fluctuation plays in Cooper pairing, where we observed a slight softening of the in-plane transverse acoustic mode corresponding to the elastic constant $$C_{66}$$. This softening starts at temperature $$T$$ well above the SC $$T_c$$, as $$T$$ decreases. An anomalously strong change of the scattering intensity of in-plane optical modes was observed at the M point of the pseudo tetragonal reciprocal space in the range of 35 $$< omega <$$ 40 meV with decreasing $$T$$ from far above $$T_c$$. Because this $$omega$$ region mainly corresponds to the motion of Fe and As atoms in the FeAs planes, the finding presents information on the coupling between the orbital fluctuation of Fe $$3d$$ electrons and the lattice system, useful for studying the possible roles of orbital fluctuation in the pairing mechanism and/or the appearance of the so-called nematic phase.

Journal Articles

First-principles study of antimony doping effects on the iron-based superconductor CaFe(Sb$$_{x}$$As$$_{1-x}$$)$$_{2}$$

Nagai, Yuki; Nakamura, Hiroki; Machida, Masahiko; Kuroki, Kazuhiko*

Journal of the Physical Society of Japan, 84(9), p.093702_1 - 093702_4, 2015/09

 Times Cited Count:4 Percentile:50.01(Physics, Multidisciplinary)

no abstracts in English

320 (Records 1-20 displayed on this page)