Yoshida, Hisao*; Yamamoto, Akira*; Hosokawa, Saburo*; Yamazoe, Seiji*; Kikkawa, Soichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tanaka, Tsunehiro*
Topics in Catalysis, 64(9-12), p.660 - 671, 2021/08
Matsukawa, Takeshi*; Iida, Kazuki*; Nakamura, Mitsutaka; Ishigaki, Toru*
CrystEngComm (Internet), 23(12), p.2355 - 2359, 2021/03
Kawakita, Yukinobu; Kikuchi, Tatsuya*; Tahara, Shuta*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Maruyama, Kenji*; Yamauchi, Yasuhiro*; Kawamura, Seiko; Nakajima, Kenji
JPS Conference Proceedings (Internet), 33, p.011071_1 - 011071_6, 2021/03
CuI is a well-known superionic conductor in a high temperature solid phase where the mobile cations migrate between interstitial sites in the f.c.c. sublattice formed by iodine ions. Even in the molten state, it shows several features suggesting collective or cooperative ionic motion. MD results show that Cu diffuses much faster than I. The Cu-Cu partial structure factor have a FSDP which indicates a medium-range ordering of Cu ions. Moreover the Cu-Cu partial pair distribution deeply penetrates into the nearest neighboring Cu-I shell. To reveal origin such anomalous behaviors of molten CuI, we performed quaiselastic neutron scattering (QENS) by the disk-chopper spectrometer AMATERAS at MLF, J-PARC. To interpret the total dynamic structure factor obtained from coherent QENS, the mode distribution analysis was applied. It is found that the motion of iodine is a kind of fluctuating within an almost local area while Cu ions diffuse much faster than iodine ions.
Fujita, Masaki*; Ikeuchi, Kazuhiko*; Kajimoto, Ryoichi; Nakamura, Mitsutaka
Journal of the Physical Society of Japan, 90(2), p.025001_1 - 025001_2, 2021/02
Yamazoe, Seiji*; Yamamoto, Akira*; Hosokawa, Saburo*; Fukuda, Ryoichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tsukuda, Tatsuya*; Yoshida, Hisao*; Tanaka, Tsunehiro*
Catalysis Science & Technology, 11(1), p.116 - 123, 2021/01
Zhang, D.*; Hu, X.*; Chen, T.*; Abernathy, D. L.*; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Kofu, Maiko; Foley, B. J.*; Yoon, M.*; Choi, J. J.*; et al.
Physical Review B, 102(22), p.224310_1 - 224310_10, 2020/12
Kajimoto, Ryoichi; Nakamura, Mitsutaka; Iida, Kazuki*; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Inamura, Yasuhiro; Ishikado, Motoyuki*
Journal of Neutron Research, 22(2-3), p.99 - 107, 2020/10
Cai, Z.*; Bao, S.*; Wang, W.*; Ma, Z.*; Dong, Z.-Y.*; Shangguan, Y.*; Wang, J.*; Ran, K.*; Li, S.*; Kamazawa, Kazuya*; et al.
Physical Review B, 101(13), p.134408_1 - 134408_10, 2020/04
Dirac matters provide a platform for exploring the interplay of their carriers with other quantum phenomena. SrMnSb has been proposed to be a magnetic Weyl semimetal and provides an excellent platform to study the coupling between Weyl fermions and magnons. We performed inelastic neutron scattering measurements on single crystals of SrMnSb, and found The dispersion in the magnetic Mn layer extends up to about 76 meV, while that between the layers has a narrow band width of 6 meV. Despite the coexistence of Weyl fermions and magnons, we find no clear evidence that the magnetic dynamics are influenced by the Weyl fermions in SrMnSb, possibly because that the Weyl fermions and magnons reside in the Sb and Mn layers separately, and the interlayer coupling is weak due to the quasi-two-dimensional nature of the material.
Ueda, Hiroshi*; Onoda, Shigeki*; Yamaguchi, Yasuhiro*; Kimura, Tsuyoshi*; Yoshizawa, Daichi*; Morioka, Toshiaki*; Hagiwara, Masayuki*; Hagiwara, Masato*; Soda, Minoru*; Masuda, Takatsugu*; et al.
Physical Review B, 101(14), p.140408_1 - 140408_6, 2020/04
Metoki, Naoto; Aczel, A. A.*; Aoki, Dai*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; Hagiwara, Masato*; Hong, T.*; Haga, Yoshinori; Ikeuchi, Kazuhiko*; et al.
JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03
Rare earths (4) and actinides (5) provide variety of interesting states realized with competing interactions between the increasing number of electrons. Since crystal field splitting of many-body electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the electron states of heavy electron compounds NpPdAl and actinide and rare earth based iso-structural family.
Ishikado, Motoyuki*; Kodama, Katsuaki; Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Ikeuchi, Kazuhiko*; Ji, S.*; Arai, Masatoshi*; Shamoto, Shinichi
Condensed Matter (Internet), 4(3), p.69_1 - 69_10, 2019/09
The enhancement magnetic resonance mode of FeTeSe is limited around Q = (, 0). Q dependence is found to be consistent with a theoretical simulation of the magnetic resonance mode with the sign-reversing order parameter of swave.
Nakamura, Mitsutaka; Kikuchi, Tatsuya*; Kawakita, Yukinobu
Physica B; Condensed Matter, 567, p.61 - 64, 2019/08
Recently, we reported the phonon dynamical study of a polycrystalline NaI by using the dynamical structure factor in real-space transformed from the inelastic neutron scattering (INS) data. Our study has shown that the INS experiments under the conventional condition Q 5 can provide us a meaningful information on the phonon dynamics at around the first nearest neighbor distance on accepting the worse real-space resolution. These results suggest the possibility that a large amount of data which were previously obtained can be effectively reused. In this study, we will examine both the applicability and limitations of analysis for various types of materials whose INS data were obtained at the Fermi chopper spectrometer 4SEASONS in J-PARC.
Kikuchi, Tatsuya*; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Nakamura, Mitsutaka; Wakai, Daisuke*; Aoyama, Kazuhiro*; Iwahashi, Takaaki*; Kambara, Wataru*
Physica B; Condensed Matter, 564, p.45 - 53, 2019/07
Details of the background, that is, unwanted signals accumulated by the data acquisition system of neutron instruments, observed by the cold-neutron chopper spectrometer AMATERAS installed at the Materials and Life Science Experimental Facility at J-PARC are reported. In the design phase of AMATERAS, we carefully considered the achievement of high signal-to-noise ratio, and possible countermeasures were implemented. Actually, recent scientific outputs from AMATERAS indicates that the spectrometer is one of excellent neutron instruments with low background. In spite of that, in nine years of AMATERAS operation, we have encountered unwanted signals due to various reasons, including gamma-rays emitted at materials on or near the beam line including the sample itself, scattered neutrons from the beam line devices, air scattering, electronic noise in data acquisition system, cosmic rays, T0 burst, and other unknown sources. In this report, we discuss the background observed by AMATERAS, especially in the conditions of without samples, comprehensively. The possible sources of these signals and the countermeasures considered against the above sources are discussed, which may be helpful to those who are engaged in other existing or planned neutron-scattering instruments.
Kajimoto, Ryoichi; Yokoo, Tetsuya*; Nakamura, Mitsutaka; Kawakita, Yukinobu; Matsuura, Masato*; Endo, Hitoshi*; Seto, Hideki*; Ito, Shinichi*; Nakajima, Kenji; Kawamura, Seiko
Physica B; Condensed Matter, 562, p.148 - 154, 2019/06
Yamaura, Junichi*; Hiraka, Haruhiro*; Iimura, Soshi*; Muraba, Yoshinori*; Bang, J.*; Ikeuchi, Kazuhiko*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Honda, Takashi*; Hiraishi, Masatoshi*; et al.
Physical Review B, 99(22), p.220505_1 - 220505_6, 2019/06
Inelastic neutron scattering was performed for an iron-based superconductor, where most of D (deuterium) replaces oxygen, while a tiny amount goes into interstitial sites. By first-principle calculation, we characterize the interstitial sites for D (and for H slightly mixed) with four equivalent potential minima. Below the superconducting transition temperature Tc = 26 K, new excitations emerge in the range 5-15 meV, while they are absent in the reference system LaFeAsOF. The strong excitations at 14.5 meV and 11.1 meV broaden rapidly around 15 K and 20 K, respectively, where each energy becomes comparable to twice of the superconducting gap. The strong excitations are ascribed to a quantum rattling, or a band motion of hydrogen, which arises only if the number of potential minima is larger than two.
Kajimoto, Ryoichi; Ishikado, Motoyuki*; Kira, Hiroshi*; Kaneko, Koji; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Inamura, Yasuhiro; Ikeuchi, Kazuhiko*; Iida, Kazuki*; Murai, Naoki; et al.
Physica B; Condensed Matter, 556, p.26 - 30, 2019/03
Nakamura, Mitsutaka; Kambara, Wataru*; Iida, Kazuki*; Kajimoto, Ryoichi; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Ishikado, Motoyuki*; Aoyama, Kazuhiro*
Physica B; Condensed Matter, 551, p.480 - 483, 2018/12
Recently there has been an increasing need for inelastic neutron scattering experiments under some special environments such as magnetic fields, pressure and high temperatures. In order to obtain high quality data, the unnecessary scattering caused by sample environmental apparatus should be suppressed as much as possible. We have developed an oscillating radial collimator with a view to satisfying users' needs, which is specialized for the Fermi chopper spectrometer 4SEASONS at J-PARC.4SEASONS provides relatively high incident energies, and thus we chose hydrogen free metal sheets as the collimator blades. The control system of this oscillating radial collimator enables us to flexibly tune the oscillating pattern, such as the oscillating speed and oscillating angle. In this presentation, we report the performances and remaining issues of the newly developed oscillating radial collimator for 4SEASONS.
Nakamura, Mitsutaka; Kikuchi, Tatsuya*; Kamazawa, Kazuya*; Kawakita, Yukinobu
Physica B; Condensed Matter, 551, p.351 - 354, 2018/12
The dynamic structure function in real space G() is deduced from the dynamical structure factor S() which can be obtained from inelastic neutron scattering measurement. In this study, we applied the G() analysis to NaI which is a typical alkali halide crystal. The optic and acoustic phonons of NaI are widely separated in energy because the difference in mass between the constituent atoms is large. These characteristic properties certainly help us to evaluate the G() features associated with the phonon modes. We measured the S() for NaI powder using the Fermi chopper spectrometer 4SEASONS at J-PARC, and converted S() into G() by newly developed software which utilizes the maximum entropy method. Our analysis clearly demonstrated the G() of TO mode oscillates out of phase with that of LA mode, which is physically reasonable. Further analyses will be given in the presentation.
Kawakita, Yukinobu; Kikuchi, Tatsuya*; Inamura, Yasuhiro; Tahara, Shuta*; Maruyama, Kenji*; Hanashima, Takayasu*; Nakamura, Mitsutaka; Kiyanagi, Ryoji; Yamauchi, Yasuhiro*; Chiba, Kaori*; et al.
Physica B; Condensed Matter, 551, p.291 - 296, 2018/12
There are elemental liquid metals with complex structures far from the hard sphere (HS) packing model. Liquid Bi has an asymmetric first peak in the structure factors S(Q). The pair distribution function g(r) exhibits strange distance ratio of 1:2 between the first and the second peaks. Since a HS model with two kinds of radius produces asymmetry of the main peak in S(Q), existence of short-lived covalent bonds was discussed. Contrarily, modulation of the atomic distribution by the Friedel oscillations of shielding electrons around metallic ions was discussed. To examine its bonding nature from viewpoints of dynamic correlation functions, we have measured neutron quasielastic scattering of liquid Bi by using cold disk chopper spectrometer installed at MLF of J-PARC. The van Hove function revealed that the shoulder structure located at a longer side of the first peak in g(r) exhibits a longer relaxation time than the main structures such as the first and second peaks.
Tamatsukuri, Hiromu*; Hiraka, Haruhiro*; Ikeuchi, Kazuhiko*; Iimura, Soshi*; Muraba, Yoshinori*; Nakamura, Mitsutaka; Sagayama, Hajime*; Yamaura, Junichi*; Murakami, Yoichi*; Kuramoto, Yoshio*; et al.
Physical Review B, 98(17), p.174415_1 - 174415_6, 2018/11
Magnetic excitations in a heavily electron-doped antiferromagnet, LaFeAsOD, have been investigated using powder inelastic neutron scattering. Unlike other parent compounds of the iron-based superconductors, the magnetic excitation gap in LaFeAsOD was not detected down to the lowest measured temperature of 4 K. This result can be understood as a result of quasi-isotropy within the ab plane, which is consistent with the band calculation result that the orbital plays the dominant role in the magnetism of LaFeAsOH. In addition, the intensities of the magnetic excitations in this phase are much stronger than those in nondoped LaFeAsO. Even in the paramagnetic phase, the magnetic excitation in LaFeAsOD persists. These results corroborate recent studies showing that the electron doping enhances the localized nature in this system.