Pulsed muon facility of J-PARC MUSE

Shimomura, Koichiro*; Koda, Akihiro*; Pant, A. D.*; Sunagawa, Hikaru*; Fujimori, Hiroshi*; Umegaki, Izumi*; Nakamura, Jumpei*; Fujihara, Masayoshi; Tampo, Motonobu*; Kawamura, Naritoshi*; et al.

Interactions (Internet), 245(1), p.31_1 - 31_6, 2024/12

https://doi.org/10.1007/s10751-024-01863-8

Uranium-plutonium-americium cation interdiffusion in polycrystalline (U,Pu,Am)O mixed oxides

Vauchy, R.; Matsumoto, Taku; Hirooka, Shun; Uno, Hiroki*; Tamura, Tetsuya*; Arima, Tatsumi*; Inagaki, Yaohiro*; Idemitsu, Kazuya*; Nakamura, Hiroki; Machida, Masahiko; et al.

Journal of Nuclear Materials, 588, p.154786_1 - 154786_13, 2024/01

https://doi.org/10.1016/j.jnucmat.2023.154786

Measurements of capture cross-section of Nb by activation method and half-life of Nb by mass analysis

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Kimura, Atsushi

Journal of Nuclear Science and Technology, 60(11), p.1361 - 1371, 2023/11

https://doi.org/10.1080/00223131.2023.2198526

The thermal-neutron capture cross section () and resonance integral (I) for Nb among nuclides for decommissioning were measured by an activation method and the half-life of Nb by mass analysis. Niobium-93 samples were irradiated with a hydraulic conveyer installed in the research reactor in Institute for Integral Radiation and Nuclear Science, Kyoto University. Gold-aluminum, cobalt-aluminum alloy wires were used to monitor thermal-neutron fluxes and epi-thermal Westcott's indexes at an irradiation position. A 25-m-thick gadolinium foil was used to sort out reactions ascribe to thermal-and epi-thermal neutrons. Its thickness provided a cut-off energy of 0.133 eV. In order to attenuate radioactivity of Ta due to impurities, the Nb samples were cooled for nearly 2 years. The induced radio activity in the monitors and Nb samples were measured by -ray spectroscopy. In analysis based on Westcott's convention, the and I values were derived as 1.110.04 barn and 10.50.6 barn, respectively. After the -ray measurements, mass analysis was applied to the Nb sample to obtain the reaction rate. By combining data obtained by both -ray spectroscopy and mass analysis, the half-life of Nb was derived as (2.000.15)10 years.

Neutron capture cross-section measurement by mass spectrometry for Pb-204 irradiated in JRR-3

Nakamura, Shoji; Shibahara, Yuji*; Kimura, Atsushi; Endo, Shunsuke; Shizuma, Toshiyuki*

Journal of Nuclear Science and Technology, 60(9), p.1133 - 1142, 2023/09

https://doi.org/10.1080/00223131.2023.2172088

In recent years, research has been advanced on lead-cooled fast reactors and accelerator drive systems, and it is required to improve the accuracy of the neutron capture cross section of Pb isotopes. Although Pb has a small natural abundance, it is of importance because it produces the long-lived radionuclide Pb (17.3 million years) by neutron capture reaction. However, it is difficult to measure its cross section by a conventional activation method using a nuclear reactor because the induced radioactivity of Pb is weak. Hence, the cross-section measurement was performed by applying mass spectrometry. This presentation gives the details of the experiment and the results obtained in the neutron capture cross-section measurement of Pb using mass spectroscopy.

First observation of O

Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.

Nature, 620(7976), p.965 - 970, 2023/08

https://doi.org/10.1038/s41586-023-06352-6

no abstracts in English

Neutron capture cross-section measurements with TC-Pn in KUR for some nuclides targeted for decommissioning

Nakamura, Shoji; Endo, Shunsuke; Kimura, Atsushi; Shibahara, Yuji*

KURNS Progress Report 2022, P. 73, 2023/07

The present study is concerned with the neutron capture cross-sections that contribute to the evaluation of the amount of radionuclides possessing problems in decommissioning. In this study, Sc, Cu, Zn, Ag, In and W were selected among the objective nuclides, and their thermal-neutron capture cross-sections were measured using TC-Pn equipment of the KUR of the Institute for Integrated Radiation and Nuclear Science, Kyoto University. High purity metal samples were prepared. A gold-aluminum ally wire, cobalt and molybdenum foils were used to monitor the neutron flux at the irradiation position of TC-Pn. The flux monitors and metal samples were irradiated for 1 hour at 1-MW operation of the KUR. After irradiation, the irradiation capsule was opened, samples and flux monitors were enclosed in a vinyl bag one by one, and then rays emitted from the samples and monitors were measured with a high-purity Ge detector. The thermal-neutron flux component was derived with the reaction rates of flux monitors (Au, Co and Mo) on the basis of Westcott's convention, and found to be (5.920.10)10 n/cm/sec at the irradiation position. The measured reaction rate for each metal sample divided by the evaluated thermal-neutron capture cross-section should give the same value of the thermal-neutron flux component if the cross section is suitable. This time, we found that the cross sections of Sc and Zn were consistent with the evaluated one, but those of other nuclides were inconsistent with their evaluated ones; that is, it turned out that their thermal-neutron capture cross-sections should be modified.

Single crystal growths and magnetic properties of hexagonal polar semimetals AuGe ( = Y, Gd-Tm, and Lu)

Kurumaji, Takashi*; Gen, Masaki*; Kito, Shunsuke*; Ikeuchi, Kazuhiko*; Nakamura, Mitsutaka; Ikeda, Akihiko*; Arima, Takahisa*

Journal of Alloys and Compounds, 947, p.169475_1 - 169475_8, 2023/06

https://doi.org/10.1016/j.jallcom.2023.169475

General-purpose nuclear data library JENDL-5 and to the next

Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Nagaya, Yasunobu; Tada, Kenichi; et al.

EPJ Web of Conferences, 284, p.14001_1 - 14001_7, 2023/05

https://doi.org/10.1051/epjconf/202328414001

Low-temperature magnetic fluctuations investigated by Te-NMR on the uranium-based superconductor UTe

Fujibayashi, Hiroki*; Kinjo, Katsuki*; Nakamine, Genki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; et al.

Journal of the Physical Society of Japan, 92(5), p.053702_1 - 053702_5, 2023/05

https://doi.org/10.7566/JPSJ.92.053702

Development of nondestructive elemental analysis system for Hayabusa2 samples using muonic X-rays

Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.

ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04

https://doi.org/10.1021/acsearthspacechem.2c00303

The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.