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Battulga, B.; Nakanishi, Takahiro; Atarashi-Andoh, Mariko; Otosaka, Shigeyoshi*; Koarashi, Jun
Environmental Science and Pollution Research, 31, p.60080 - 60092, 2024/10
A ubiquitous distribution of plastic debris has been reported in aquatic and terrestrial environments; however, the interactions between plastics and radionuclides and the radioactivity of environmental plastics remain largely unknown. Here, we characterize biofilms developing on the surface of plastic debris to explore the role of plastic-associated biofilms as an interaction medium between plastics and radiocesium (Cs) in the environment. Biofilm samples were extracted from plastics (1-50 mm in size) collected from two contrasting coastal areas in Japan. The radioactivity of plastics was estimated based on the
Cs activity concentration of the biofilms and compared seasonally with surrounding environmental samples (i.e., sediment and sand).
Cs traces were detected in biofilms with activity concentrations of 21-1300 Bq kg
biofilm (dry weight), corresponding to 0.04-4.5 Bq kg
plastic (dry weight). Our results reveal the interaction between
Cs and plastics and provide evidence that organic and mineral components in biofilms are essential in
Cs retention in environmental plastics.
Tanaka, Takuro*; Fukuoka, Masafumi*; Toda, Kanako*; Nakanishi, Takahiro; Terashima, Motoki; Fujiwara, Kenso; Niwano, Yuma*; Kato, Hiroaki*; Kobayashi, Natsuko*; Tanoi, Keitaro*; et al.
ACS ES&T Water (Internet), 4(8), p.3579 - 3586, 2024/08
Nakanishi, Takahiro; Sakuma, Kazuyuki; Oyama, Takuya; Hagiwara, Hiroki; Suzuki, Takashi
Environmental Pollution, 355, p.124213_1 - 124213_7, 2024/08
Times Cited Count:2 Percentile:63.70(Environmental Sciences)This study investigated the transport behavior of I by riverbank surveys conducted from 2013 to 2015 in a watershed where the
I/
Cs activity ratio is low in the mountainous area and high in the plain as of 2011. Until 2015, the
I/
Cs activity ratio of the levee crown in the studied watershed was similar to that of the surrounding area in 2011. However, the
I/
Cs ratios of the surface riverbank sediments were all low, indicating that radionuclides transported from the mountainous area were deposited on the riverbank in the plain. The vertical distribution of the
I/
Cs ratio in the riverbank sediments indicated that some
I and
Cs deposited during the accident remained in the lower layers, but most were eroded immediately after the accident. Based on the
I/
Cs ratios of sediments deposited on the riverbank, which remained constant until 2015 after the accident, the amount of
I discharged to the ocean was determined from the previously evaluated
Cs discharge. It was calculated that 1.8
10
Bq and 1.2
10
Bq of
I were discharged with sediment from the studied watershed and the contaminated river watersheds (Abukuma River and Fukushima coastal rivers, including the study river), respectively. The results of this study indicate that the continuous
I discharge from the river contribute little to their amount in the seafloor sediments along the Fukushima coast.
Tamura, Koji; Nakanishi, Ryuzo; Oba, Hironori; Karino, Takahiro; Shibata, Takuya; Taira, Takunori*; Wakaida, Ikuo
Journal of Nuclear Science and Technology, 61(8), p.1109 - 1116, 2024/08
Times Cited Count:1 Percentile:27.70(Nuclear Science & Technology)Ikenoue, Tsubasa; Nakanishi, Takahiro; Shimadera, Hikari*; Kawamura, Hideyuki; Kondo, Akira*
E3S Web of Conferences (Internet), 530, p.02005_1 - 02005_10, 2024/05
The accident at the Fukushima Daiichi Nuclear Power Plant (FDNPP) caused a radioactive contamination in seabed sediment. The Cs supply from rivers could be an important process for the long-term behavior of
Cs in seabed sediment. In this study, a ten-year simulation of the
Cs behavior in seabed sediment was conducted using an oceanic dispersion model combined with a prediction model of
Cs behavior in land and river. In the waters north of FDNPP, the simulation results suggested that the
Cs supply from rivers had a great impact on the concentrations in coastal sediment due to the initial low concentrations in seabed sediment and the large supply of
Cs from rivers. In the waters near FDNPP and south of FDNPP, the simulation results suggested that the impact of the
Cs supply on the temporal variation of
Cs concentration in coastal sediment was relatively small due to the large initial adsorption from seawater. Overall, these results indicated that
Cs supply from rivers had an impact on the spatiotemporal distribution of
Cs concentrations in seabed sediment on a decadal time scale and the impact was especially great in the waters north of FDNPP.
Takata, Hyoe*; Wakiyama, Yoshifumi*; Wada, Toshihiro*; Hirao, Shigekazu*; Aono, Tatsuo*; Nakanishi, Takahiro; Misono, Toshiharu; Shiribiki, Takehiko; Aoyama, Michio*
Marine Chemistry, 262, p.104384_1 - 104384_6, 2024/05
Times Cited Count:1 Percentile:50.38(Chemistry, Multidisciplinary)Nakanishi, Takahiro; Tsuruta, Tadahiko; Misono, Toshiharu; Shiribiki, Takehiko; Urabe, Yoshimi*; Sanada, Yukihisa
Journal of Coastal Research, 116(SI), p.161 - 165, 2024/01
Continuous data of Cs-137 concentration in surface seabed sediment around the Fukushima Daiichi Nuclear Power Plant (FDNPP) from 2012 to 2022 was compiled and its temporal change was fitted by exponential function. In general, Cs-137 concentrations were gradually declining with time. However, at some monitoring points in shallow region, long half-lives and/or large deviations of Cs-137 concentrations were noticed. To gain insight into cesium dynamics in shallow seafloor, long sediment cores were collected at shallow region near the FDNPP, and the vertical profiles of Cs-137 concentration and particle size distribution were determined. At the beach, Cs-137 concentration and particle size distribution were very homogenized from several tens of cm to more than 1 m deep, probably due to strong vertical mixing by wind waves and tides. Therefore, beach sediments have significant Cs-137 reserves in deeper layers at present. It was suggested that the Cs-137 supply from deep layers as well as the land area might suppress the decline of surface Cs-137 concentration in this area. At sampling points located at the bases of cliffs and depressions at the offshore zone, the vertical distributions of Cs-137 concentration were highly heterogeneous, showing the particle size dependency. Moreover, Cs-137 profiles obtained at the same point for several years were quite different. Therefore, it might cause the large fluctuation of Cs-137 concentration at surface sediment over time.
Koyama, Shinichi; Ikeuchi, Hirotomo; Mitsugi, Takeshi; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Tsai, T.-H.; Takano, Masahide; Fukaya, Hiroyuki; Nakamura, Satoshi; et al.
Hairo, Osensui, Shorisui Taisaku Jigyo Jimukyoku Homu Peji (Internet), 216 Pages, 2023/11
In FY 2021 and 2022, JAEA perfomed the subsidy program for "the Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy, Thermal Bahavior Estimation, and Simplified Analysis of Fuel Debris)" started in FY 2021. This presentation material summarized the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning, Contaminated Water and Treated Water Management.
Ikenoue, Tsubasa; Shimadera, Hikari*; Nakanishi, Takahiro; Kondo, Akira*
Water (Internet), 15(15), p.2734_1 - 2734_18, 2023/08
Times Cited Count:0 Percentile:0.00(Environmental Sciences)The Fukushima Daiichi Nuclear Power Plant accident caused an accumulation of Cs in coastal sediment. The
Cs supply from rivers to the ocean can affect the long-term fate of
Cs in coastal sediment. Since the Fukushima coastal river basins include large decontaminated and evacuation order areas, considering the decontamination work and resumption of agriculture is important for predicting the
Cs supply. We conducted a 30-year prediction of the
Cs supply from the Fukushima coastal rivers to the ocean using a distributed radiocesium prediction model, considering the effects of human activities. In river basins with decontaminated and evacuation order areas, human activities reduced the total
Cs outflow from agricultural lands, urban lands, and forest areas to the rivers and the
Cs supply to the ocean by 5.0% and 6.0%, respectively. These results indicated that human activities slightly impacted the
Cs outflow and supply. The
Cs supply from rivers impacted by the accident to the coastal sediment was estimated to correspond to 11-36% of the total
Cs in the coastal sediment in the early phase of the accident. Therefore, the
Cs supply from rivers to the ocean is important for the long-term behavior of
Cs in coastal sediment.
Sato, Yuhi*; Otosaka, Shigeyoshi*; Suzuki, Takashi; Nakanishi, Takahiro
Limnology and Oceanography, 68(7), p.1580 - 1594, 2023/07
Times Cited Count:4 Percentile:63.68(Limnology)To investigate the factors regulating the concentration of particulate iodine (PI) in seawater, it was measured in two Pacific coastal areas adjacent to Japan in two seasons along with parameters such as particulate organic carbon (POC) and nitrogen (PON), dissolved iodine (DI), and phytoplankton pigments. The dataset was divided in three groups namely, lower (Group A), average (Group B), and higher (Group C) atomic ratios of PI to POC (I/C). The three groups were characterized by phytoplanktonic physiological states as highly productive, steady, and senescent states, respectively. Based on the finding that PI production is associated with the phytoplankton physiological state, the seasonal and regional differences in PI concentration and I/C in the observation areas were consistently explained. Finally, we suggest that the phytoplanktonic physiological state is one of the vital factors regulating the PI concentration in seawater.
Sakuma, Kazuyuki; Yamada, Susumu; Machida, Masahiko; Kurikami, Hiroshi; Misono, Toshiharu; Nakanishi, Takahiro; Iijima, Kazuki
Marine Pollution Bulletin, 192, p.115054_1 - 115054_10, 2023/07
Times Cited Count:4 Percentile:53.08(Environmental Sciences)Ikenoue, Tsubasa; Shimadera, Hikari*; Nakanishi, Takahiro; Kondo, Akira*
Science of the Total Environment, 876, p.162846_1 - 162846_12, 2023/06
Times Cited Count:4 Percentile:46.73(Environmental Sciences)We conducted 30 years simulation of environmental fate of Cs in the Abukuma River basin considering the characteristics of the
Cs behavior in land uses. Overall, in the Abukuma River basin, the
Cs transported into the ocean for 30 years was estimated to correspond to 4.6% of the initial deposition in the basin, and the effective half-life of
Cs deposited in the basin was estimated to be 3.7 years shorter (by 11.6%) than its physical half-life. These results suggested that
Cs deposited from the accident could still remain for decades. Based on the analysis of the
Cs behavior in land use, in 2011, the contribution of
Cs export to the ocean from urban lands was estimated to correspond to 70% of the total
Cs export. Meanwhile, from 2012 to 2040, the contribution of
Cs export from agricultural lands was estimated to correspond to 75% of the total
Cs export. The reduction ratios excluding radioactive decay of
Cs remained in areas with and without human activities for 30 years after the accident, defined as the ratios of the total outflow to the initial deposition, were estimated to be 11.5%-17.7% and 0.4%-1.4%, respectively. These results suggested that human activities enhance the reduction of
Cs remaining in land in the past and future.
Tatsuno, Takahiro*; Waki, Hiromichi*; Kakuma, Minato*; Nihei, Naoto*; Takase, Tsugiko*; Wada, Toshihiro*; Yoshimura, Kazuya; Nakanishi, Takahiro; Ote, Nobuhito*
Journal of Environmental Management, 329, p.116983_1 - 116983_13, 2023/03
Times Cited Count:2 Percentile:13.07(Environmental Sciences)Misono, Toshiharu; Nakanishi, Takahiro; Sanada, Yukihisa; Shiribiki, Takehiko; Urabe, Yoshimi*; Tsuruta, Tadahiko
JAEA-Research 2022-010, 134 Pages, 2023/02
An accident occurred at the TEPCO's Fukushima Daiichi Nuclear Power Station (1F) in 2011 and a large amount of radioactive materials were deposited around the 1F. Japan Atomic Energy Agency has continued to conduct research on the dynamics of radioactive materials after the accident. This report summarizes the results of the survey conducted in FY 2021 on the status of marine monitoring survey on radioactive substances. Furthermore, a seabed topography and sediments distribution survey was conducted in the coastal area off the Mano River from the Ohta River to understand the topography and sediment distribution. Furthermore, in order to evaluate the inflow of radioactive Cs from the river, the horizontal distribution of the radioactive Cs concentration on the surface sediment in front of the rivers was measured. As basic information on the effects of radioactive materials on marine products, the distribution status of fish was investigated. In addition, a demonstration test of water sampling and sediment sampling was conducted using an unmanned observation vessel. From these results, we estimated the distribution and its dynamics of radioactive Cs in the sediments in the front area on the 1F.
Misono, Toshiharu; Nakanishi, Takahiro; Shiribiki, Takehiko; Nagao, Seiya*; Ochiai, Shinya*; Sanada, Yukihisa; Tsuruta, Tadahiko
Gekkan Kaiyo, 54(11), p.558 - 561, 2022/11
Sediment traps were set up around estuaries and in coastal areas to collect sinking particles at the time of river discharge. Around the estuary, changes in radiocesium concentration and mass flux of sinking particles linked to the discharge of radiocesium from the river were observed.
Battulga, B.; Atarashi-Andoh, Mariko; Nakanishi, Takahiro; Koarashi, Jun
Science of the Total Environment, 849, p.157758_1 - 157758_11, 2022/11
Times Cited Count:7 Percentile:48.42(Environmental Sciences)Characterizing plastic-associated biofilms is key to the better understanding of organic material and mineral cycling in the "Plastisphere"-the thin layer of microbial life on plastics. In this study, we propose a new method to extract biofilms from environmental plastics, in order to evaluate the properties of biofilm-derived organic matter through stable carbon (C) and nitrogen (
N) isotope signatures and their interactions with radionuclides especially radiocesium (
Cs). After ultrasound-assisted separation from the plastics, biofilm samples were successfully collected via a sequence of syringe treatments. Biofilm-derived organic matter samples (14.5-65.4 mg) from four river mouths in Japan showed
Cs activity concentrations of
75 to 820 Bq kg
biofilm (dw), providing evidence that environmental plastics, mediated by developed biofilms, serve as a carrier for
Cs in the coastal environment. Significant differences in the (
C and
N signatures were also obtained for the biofilms, indicating the different sources, pathways, and development processes of biofilms on plastics.
Tatsuno, Takahiro*; Waki, Hiromichi*; Kakuma, Minato*; Nihei, Naoto*; Wada, Toshihiro*; Yoshimura, Kazuya; Nakanishi, Takahiro; Ote, Nobuhito*
Radiation Protection Dosimetry, 198(13-15), p.1052 - 1057, 2022/09
Times Cited Count:2 Percentile:30.61(Environmental Sciences)Kitamura, Akihisa*; Okazaki, Sota*; Kondo, Mitsuru*; Watanabe, Takahiro; Nakanishi, Toshimichi*; Hori, Rie*; Ikeda, Masayuki*; Ichimura, Koji*; Nakagawa, Yuki*; Mori, Hideki*
Shizuoka Daigaku Chikyu Kagaku Kenkyu Hokoku, (49), p.73 - 86, 2022/07
On July 3 2021, a debris flow caused by a landslide from a landfill occurred along the Aizome River in the Izusan area of Atami City, Shizuoka. In this study, debris flow deposits and soil samples were characterized in terms of their sedimentology and geochemically analyzed.
Misono, Toshiharu; Nakanishi, Takahiro; Tsuruta, Tadahiko; Shiribiki, Takehiko; Sanada, Yukihisa
Marine Pollution Bulletin, 178, p.113597_1 - 113597_9, 2022/05
Times Cited Count:5 Percentile:51.60(Environmental Sciences)It is essential to evaluate secondary migration caused by riverine input and resuspension from seabed sediments to estimate the future distribution of radioactive cesium (Cs) in the coastal area off Fukushima Prefecture. In particular, the inflow from rivers cannot be ignored because most of the
Cs inflow from rivers is deposited on the coast without elute into seawater. Two mooring systems were installed near the Ukedo River's mouth (Fukushima Prefecture) from February 2017 to February 2018. The first contained a sediment trap system, collecting sinking particles during the period. The second comprised a turbidity sensor and a current sensor. The contribution of resuspension and inflow from the river to the mass flux was quantitatively evaluated using multiple regression equations. The results showed that resuspension caused 79%-83% of secondary
Cs migration in nearshore areas, whereas the influence of riverine
Cs input on the sediment was only 7% per year.
Funaki, Hironori; Tsuji, Hideki*; Nakanishi, Takahiro; Yoshimura, Kazuya; Sakuma, Kazuyuki; Hayashi, Seiji*
Science of the Total Environment, 812, p.152534_1 - 152534_10, 2022/03
Times Cited Count:21 Percentile:70.72(Environmental Sciences)Reservoir sediments generally act as a sink for radionuclides derived from nuclear accidents, but under anaerobic conditions, several radionuclides remobilise in bioavailable form from sediment to water columns, which may contribute to a long-term contamination in aquatic products. This study systematically investigated the Cs activities between sediment and pore water, which is a direct evidence of the remobilisation of bioavailable
Cs from sediments, in two highly contaminated reservoirs affected by the Fukushima Dai-ichi Nuclear Power Plant accident. Our results strongly indicate a competitive ion exchange process between
Cs and NH
via a highly selective interaction with the frayed edges sites of phyllosilicate minerals to be the major reason for the variability of the Kd values between sediment and pore water, even in the Fukushima case.