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Schnabel, G.*; Kunieda, Satoshi; Konno, Chikara; Nakayama, Shinsuke; 27 of others*
Nuclear Data Sheets, 193, p.1 - 78, 2024/02
Fusion Evaluated Nuclear Data Library (FENDL), which has been coordinated by International Atomic Energy Agency (IAEA), was updated for the neutronics analysis on the fusion reactors and related applications. The main sources of data files are the national nuclear data libraries such as ENDF, JEFF and JENDL, where the best data was selected for each isotope through comparisons of the evaluated cross-sections and a number of benchmark analyses. Large differences from the previous library (FENDL-2.1) are extension of the upper energy limit from 20 MeV to 200 MeV and inclusion of the charged-particle reaction data, which had been requested by accelerator-based studies on structural materials for the fusion reactors. This paper gives a comprehensive description on the latest version FENDL-3.2b. A number of validations on the neutronics analysis show that the performance of FENDL-3.2b is better than FENDL-2.1.
Nakayama, Shinsuke
Journal of Nuclear Science and Technology, 60(12), p.1447 - 1453, 2023/12
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)The d+Be neutron source is a candidate for transportable neutron source for on-site nondestructive inspection of infrastructure facilities such as bridges, tunnels and so on. The applicability of the d+Be neutron source to a transportable fast neutron source is explored by Monte Carlo particle transport simulations with PHITS and JENDL-5. The simulation results show that by increasing the shielding thickness by about 1.5 times, it is possible to realize the d+Be neutron source with the comparable performance to another candidate, the 2.5-MeV p+Li neutron source, at lower beam energy.
Fukahori, Tokio; Nakayama, Shinsuke; Katabuchi, Tatsuya*; Shigyo, Nobuhiro*
Nihon Genshiryoku Gakkai-Shi ATOMO
, 65(12), p.726 - 727, 2023/12
The Investigative Committee on Nuclear Data investigates and observes global trends in nuclear research and development and conducts comprehensive examinations of Japanese nuclear data activities from a broader perspective, as well as cooperation with domestic and foreign academic institutions in a wide range of fields other than the Atomic Energy Society. We aim to establish a system for communication, information exchange, and interdisciplinary cooperation. In this report, we will report on three of the main activities for the 2021-2022 term: a request list site for nuclear data, human resource development, and roadmap production.
Zr + d reaction cross sections measured at 28 MeV/nucleonChillery, T.*; Hwang, J.*; Dozono, Masanori*; Imai, Nobuaki*; Michimasa, Shinichiro*; Sumikama, Toshiyuki*; Chiga, Nobuyuki*; Ota, Shinsuke*; Nakayama, Shinsuke; 49 of others*
Progress of Theoretical and Experimental Physics (Internet), 2023(12), p.121D01_1 - 121D01_11, 2023/12
Times Cited Count：0 Percentile：0.01(Physics, Multidisciplinary)The deuteron is a loosely bound system which can easily break up into its constituent proton and neutron whilst in the presence of Coulomb and nuclear fields. Previous experimental studies have shown that this breakup process has a significant impact on residual nucleus production from deuteron bombardment in the high energy range of 50 - 210 MeV/nucleon. However, there remains a lack of cross-section data at energies below 50 MeV/nucleon. The current study determined Zr + d reaction cross sections under inverse kinematics at approximately 28 MeV/nucleon using the BigRIPS separator, OEDO beamline, and SHARAQ spectrometer. Cross sections from this research were compared with previous measurements and theoretical calculations. The experimental results show a large enhancement of the production cross sections of residual nuclei, especially those produced from a small number of particle emissions, compared to the proton-induced reaction data at similar bombarding energy. The DEURACS calculation, which quantitatively takes deuteron-breakup effects into account, reproduces the data well. As a long-lived fission product, Zr remains a challenge for nuclear waste disposal and treatment. This study's low-energy data may assist future consideration of nuclear-waste treatment facilities, where Zr + d may feasibly transmute the waste into short-lived/stable nuclei.
Liu, H.*; Nakayama, Shinsuke; Lei, J.*; Ren, Z.*
Physical Review C, 108(1), p.014617_1 - 014617_8, 2023/07
In this paper, we study deuteron-induced inclusive breakup reaction and explore the 
and 
reactions for light and medium mass nuclei. Using the models of Ichimura, Austern, and Vincent and Glauber, we scrutinize the double differential cross-section of nonelastic breakup and compare the results for various reaction systems. Our findings indicate that the Glauber model, combined with a quantum 
-matrix, produces remarkable results in the deuteron-induced inclusive breakup reaction. While both models are proficient in predicting the outcomes of light and medium mass nuclei, the reaction showcases higher consistency than the reaction. Nevertheless, there are still significant discrepancies between experimental and theoretical cross-sections that require further investigation and analysis. This study opens up a new realm of possibilities for future research in the field.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Nagaya, Yasunobu; Tada, Kenichi; et al.
EPJ Web of Conferences, 284, p.14001_1 - 14001_7, 2023/05
Times Cited Count：0 Percentile：0.21(Nuclear Science & Technology)Nakayama, Shinsuke; Iwamoto, Osamu; Sublet, J.-Ch.*
EPJ Web of Conferences, 284, p.14011_1 - 14011_4, 2023/05
JENDL-5, the latest version of the Japanese evaluated nuclear data library, includes several sub-libraries to contribute to various applications. In this paper, we outline the evaluation and validation of the deuteron reaction sub-library developed mainly for the design of accelerator-based neutron sources and the alpha-particle reaction sub-library developed mainly for use in the back-end field. As for the deuteron sub-library, the data for 
Li, 
Be, and 
C from JENDL/DEU-2020 were partially modified and adopted. The data up to 200 MeV for 
Al, 
Cu, and Nb, which are important as accelerator structural materials, were newly evaluated based on the calculations with the DEURACS code. As for the alpha-particle sub-library, the data up to 15 MeV for 18 light nuclides from Li to Si isotopes were evaluated based on the calculations with the CCONE code, and then only the neutron production cross sections were replaced with the data of JENDL/AN-2005. Validation on neutron yield by Monte Carlo transport simulations was performed for both sub-libraries. As a result, it was confirmed that the simulations based on the sub-libraries showed good agreement with experimental data.
Watanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei; Nakano, Keita; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.
EPJ Web of Conferences, 284, p.01041_1 - 01041_4, 2023/05
Times Cited Count：0 Percentile：0.21(Nuclear Science & Technology)Intensive fast neutron sources using deuteron accelerators have been proposed for the study of medical RI production, radiation damage for fusion reactor materials, nuclear transmutation of radioactive waste, and so on. Neutron production data from various materials bombarded by deuterons are required for the design of such neutron sources. In the present work, we have conducted a systematic measurement of double-differential neutron production cross sections (DDXs) for a wide atomic number range of targets (Li, Be, C, Al, Cu, Nb, In, Ta, and Au) at an incident energy of 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin target foil. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0
to 25). The neutron energy was determined by a conventional time-of-flight (TOF) method. The measured DDXs were compared with theoretical model calculations by the DEUteron-induced Reaction Analysis Code System (DEURACS) and PHITS. The result indicated that the DEURACS calculation provides better agreement with the measured DDXs than the PHITS calculation.
Tada, Kenichi; Nagaya, Yasunobu; Taninaka, Hiroshi; Yokoyama, Kenji; Okita, Shoichiro; Oizumi, Akito; Fukushima, Masahiro; Nakayama, Shinsuke
Journal of Nuclear Science and Technology, 21 Pages, 2023/04
Times Cited Count：6 Percentile：98.92(Nuclear Science & Technology)The new version of the Japanese evaluated nuclear data library, JENDL-5, was released in December 2021. This paper demonstrates the validation of JENDL-5 for fission reactor applications. Benchmark calculations are performed with the continuous-energy Monte Carlo codes MVP and MCNP and the deterministic code system MARBLE. The benchmark calculation results indicate that the performance of JENDL-5 for fission reactor applications is better than that of the former library JENDL-4.0.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Abe, Yutaka*; Tsubakihara, Kosuke*; Okumura, Shin*; Ishizuka, Chikako*; Yoshida, Tadashi*; et al.
Journal of Nuclear Science and Technology, 60(1), p.1 - 60, 2023/01
Times Cited Count：64 Percentile：99.99(Nuclear Science & Technology)Nakayama, Shinsuke
Kaku Deta Nyusu (Internet), (133), p.88 - 99, 2022/10
The content of the paper that received the Paper Award of Atomic Energy Society of Japan in 2021 is outlined. Although the use of deuteron accelerator-based neutron sources has been proposed in various fields, deuteron nuclear database accurate enough to be applied to the design study of such neutron sources had not been developed. Under these situations, we had developed a deuteron nuclear database, JENDL/DEU-2020. It contains evaluated deuteron nuclear data for light nuclei (Li, Be, C), which are candidates for deuteron beam irradiation targets of the neutron sources. Evaluation of JENDL/DEU-2020 was performed by using the code system DEURACS with further modifications. In order to validate the accuracy of the database, simulations using the particle transport code were performed under various conditions with different target nuclides and incident deuteron energies, and the results were compared with the available experimental data. As a result, it was found that JENDL/DEU-2020 significantly improves the prediction accuracy of experimental data under a wider range of conditions than other nuclear reaction databases or the nuclear reaction models implemented in transport calculation codes.
Nakayama, Shinsuke; Furutachi, Naoya; Iwamoto, Osamu; Watanabe, Yukinobu*
NEA/NSC/R(2020)4 (Internet), p.345 - 349, 2022/10
Long-lived fission products (LLFPs) generated in nuclear reactors are strongly desired to be converted to stable or short-lived nuclides. Recently, it has been considered to transmute LLFPs by spallation reactions with high energy particles, and some experimental studies revealed that spallation reaction cross-sections induced by deuteron are larger than proton-induced ones. These results suggest the possibility that nuclear transmutation of LLFPs using deuteron beams is more efficient than one using proton beams. On the other hand, we have been developing a code system dedicated for deuteron-induced reactions, called DEURACS. DEURACS has been originally developed to contribute to the design of deuteron accelerator neutron sources. In the present study, we apply DEURACS to calculation of deuteron-induced spallation reactions on LLFPs. Through comparison with measured data, the applicability of DEURACS will be discussed.
Fukahori, Tokio; Nakayama, Shinsuke; Katabuchi, Tatsuya*; Shigyo, Nobuhiro*
Nihon Genshiryoku Gakkai-Shi ATOMO, 64(7), p.413 - 414, 2022/07
The Investigation Advisory Committee on Nuclear Data monitors global nuclear research and development trends, and conducts collaborative nuclear data activities with domestic and foreign academic institutions in a wide range of fields. The aims are to contact, to exchange information, and to build an interdisciplinary cooperation system. Reported are the activities on the request list site, human resources development, and roadmap creation regarding nuclear data directly related to future nuclear data research activities, among the main activities in the 2019-2020 period.
Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*; Ogata, Kazuyuki*
Few-Body Systems, 63(1), p.4_1 - 4_6, 2022/03
Times Cited Count：0 Percentile：0(Physics, Multidisciplinary)Intensive neutron sources using deuteron accelerators have been proposed for not only science and engineering fields but also medical applications. For the engineering design of such facilities, accurate and comprehensive nuclear data of deuteron-induced reactions are indispensable. However, it is difficult to meet the requirement by employing experimental data alone. Thus, theoretical model calculations play a key role in completing the necessary nuclear data by interpolation and extrapolation of experimental data. Under the above situations, we have been developing a code system dedicated for deuteron-induced reactions, called DEURACS. In the present work, calculations using DEURACS are compared with available experimental data and validation of the present modelling in DEURACS is discussed. Moreover, the importance of consideration of the breakup processes for accurate prediction of deuteron-induced reactions is also presented.
Nakayama, Shinsuke
JAEA-Conf 2021-001, p.65 - 70, 2022/03
Since deuteron is a weakly bound system consisting of a proton and a neutron, it easily breaks up and emits a neutron through interaction with a target nucleus. Utilizing this property, intensive neutron sources using deuteron accelerators have been proposed for not only science and engineering fields but also medical applications. For design studies of such facilities, accurate and comprehensive nuclear data of deuteron-induced reactions are indispensable. Toward evaluation of deuteron nuclear data, we have developed a code system dedicated for deuteron-induced reactions, called DEURACS. In DEURACS, breakup processes of incident deuteron are taken into account. DEURACS was so far successfully applied to analyses of production of nucleons, composite particles up to 
= 4, and residual nuclei. In this talk, we will present the results of these analyses and discuss how important it is to consider the breakup processes for accurate prediction of deuteron-induced reactions. Moreover, we have recently developed JENDL/DEU-2020, a deuteron nuclear database for Li, Be, and C up to 200 MeV. DEURACS was employed for evaluation of JENDL/DEU-2020. Validation of JENDL/DEU-2020 was carried out by the simulation with the Monte Carlo transport codes. These validation results will also be presented.
Nakayama, Shinsuke
Kaku Deta Nyusu (Internet), (130), p.25 - 28, 2021/10
The outline of the presentation at the joint session of Research Committee for Nuclear Data and Subcommittee on Nuclear Data in the Atomic Energy Society of Japan 2021 Autumn Meeting was contributed to Nuclear Data News. Research Committee for Nuclear Data has been preparing the nuclear data roadmap aiming for completion by the end of FY 2022. The contents of the presentation such as the background, progress, and future plan of the roadmap are described. In addition, impressions regarding the roadmap development policy obtained from the discussions on the presentation are also described.
Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*; Ogata, Kazuyuki*
Journal of Nuclear Science and Technology, 58(7), p.805 - 821, 2021/07
Times Cited Count：20 Percentile：96.99(Nuclear Science & Technology)Intensive fast neutron sources using deuteron accelerators have been proposed for various applications. To contribute to the design study of such neutron sources, a deuteron nuclear data library for Li, Be, and C up to 200 MeV, JENDL/DEU-2020 is developed. The evaluation of JENDL/DEU-2020 are performed by employing the code system DEURACS with particular attention to neutron production data. Toward the evaluation of JENDL/DEU-2020, some modifications are made to DEURACS. The validation of the library is performed though simulation with the Monte Carlo transport calculation codes. From the simulation, it is shown that the calculation results based on JENDL/DEU-2020 reproduce the measured neutron production data well in the incident energies up to 200 MeV. The new library is expected to make a large contribution to diverse design studies of deuteron accelerator neutron sources.
) reaction at 12, 20, and 30 MeVPatwary, M. K. A*; Kin, Tadahiro*; Aoki, Katsumi*; Yoshinami, Kosuke*; Yamaguchi, Masaya*; Watanabe, Yukinobu*; Tsukada, Kazuaki; Sato, Nozomi*; Asai, Masato; Sato, Tetsuya; et al.
Journal of Nuclear Science and Technology, 58(2), p.252 - 258, 2021/02
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)While designing deuteron accelerator neutron sources for radioisotopes production, nuclear data for light elements such as Li, Be, and C have been systematically measured in the deuteron energy range from a few MeV to around 50 MeV. Currently, the experimental data available on double-differential thick-target neutron yields (DDTTNYs) is insufficient, especially for deuteron energies between 18 and 33 MeV. In this study, we measured the DDTTNYs of () reactions on 
C target for incident deuteron energies of 12, 20, and 30 MeV using the multiple-foils activation method to improve nuclear data insufficiency. We applied the GRAVEL code for the unfolding process to derive the DDTTNYs. The results were compared with the calculation by DEURACS. The present data were also used to confirm the systematics of the differential neutron yields at 0 and total neutron yield per incident deuteron in the wide range of deuteron energy.
) reaction for the development of accelerator-based neutron sourcesWatanabe, Yukinobu*; Sadamatsu, Hiroki*; Araki, Shohei*; Nakano, Keita*; Kawase, Shoichiro*; Kin, Tadahiro*; Iwamoto, Yosuke; Satoh, Daiki; Hagiwara, Masayuki*; Yashima, Hiroshi*; et al.
EPJ Web of Conferences, 239, p.20012_1 - 20012_4, 2020/09
Times Cited Count：2 Percentile：86.93(Nuclear Science & Technology)Accelerator-based neutron sources induced by deuteron beams are attractive for study of nuclear transmutation of radioactive waste as well as radiation damage for fusion reactor materials. In the present work, we have carried out a Double Differential cross section (DDX) measurement for Li at 200 MeV in the Research Center for Nuclear Physics (RCNP), Osaka University. A deuteron beam accelerated to 200 MeV was transported to the neutron experimental hall and focused on a thin Li target. Emitted neutrons from the target were detected by two different-size EJ301 liquid organic scintillators located at two distances of 7 m and 20 m, respectively. The neutron DDXs were measured at six angles from 0 to 25). The neutron detection efficiencies of the detectors were calculated by SCINFUL-QMD code. We will present the results of the present DDX measurement and compare them with theoretical model calculations with DEURACS and PHITS.
Nakayama, Shinsuke; Iwamoto, Osamu; Watanabe, Yukinobu*
EPJ Web of Conferences, 239, p.03014_1 - 03014_4, 2020/09
Times Cited Count：2 Percentile：86.93(Nuclear Science & Technology)Intensive neutron sources using deuteron accelerators have been proposed for various applications such as irradiation test for fusion reactor materials and production of radioisotopes for medical use. In addition, transmutation system using deuteron-induced spallation reactions has been recently proposed for LLFPs. Accurate and comprehensive deuteron nuclear data are indispensable in the design study of such facilities. Under the above situations, we have been developing a code system dedicated for deuteron-induced reactions, which is called DEURACS. In the present work, calculations using DEURACS are compared with available experimental data up to 200 MeV such as DDXs for emission of neutron or light charged particles. We also analyze isotopic production cross sections of residual nuclei. Validation of the present modelling in DEURACS is discussed through comparison with the experimental data.
