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Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*
Mechanical Engineering Journal (Internet), 11(2), p.23-00444_1 - 23-00444_7, 2024/04
Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*
Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 4 Pages, 2023/05
Applicability of temperature swing extraction technology employing monoamides was examined for uranium contaminated waste treatment procedure. Separation experiments on simulated target solution with three kinds of monoamides with different structure showed that Ce(IV) in the solution was selectively recovered by the temperature swing extraction operation. Based on the experiments, an appropriate monoamide for the procedure was selected.
Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*
no journal, ,
The sludge generated production of nuclear fuel contained uranium has been storage. The sludge is immersed in some kinds of solution. After immersion, uranium is recovered from the solution. Cerium extractive tests using thermoresponsive polymer was carried out on two kinds of extractants. C14-BAMA was found to be superior, and we plan to conduct a uranium study on this extractant.
Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*
no journal, ,
The sludge contained uranium generated production of nuclear fuel has been storage. The sludge is immersed in some kinds of solution. After immersion, uranium is recovered from the solution. Solvent extraction method, extraction chromatography and gelling extraction method were conducted on uranyl nitrate solution using monoamide extractant to compare on amount of waste and running cost on each methods. The gelling extraction method was superior to other two methods.
Kai, Masao; Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Nakamura, Masahiro; Tsukahara, Takehiko*; Itoda, Naokazu*; Naruse, Atsuki*
no journal, ,
The sludges containing uranium are generated in nuclear fuel fabrication process and have been stored in nuclear fuel fabrication facilities. Uranium is suggested to be selectively recovered from the solution in which the sludges are immersed. In this study, the oxide conversion tests were carried out with the gel obtained by the temperature swing extraction tests with cerium. The most effective heating temperature for the oxide conversion of was determined as 1000 degree Celsius. Based on the results of tests with cerium, the oxide conversion tests with uranium gel were also carried out. The gel was heated at 1000, and products were specified according to analysis data.
Kai, Masao; Sato, Takanori*; Iwamoto, Toshihiro; Saito, Madoka*; Nakahara, Masaumi; Takahatake, Yoko; Watanabe, So; Nakamura, Masahiro; Naruse, Atsuki*; Itoda, Naokazu*; et al.
no journal, ,
The sludges containing uranium are generated in the nuclear fuel fabrication facilities. Uranium is planned to be selectively recovered from the sludge leachate. The temperature swing extraction method was selected for the selective recovery of uranium. In this study, a small-scale testing system was developed, and the performances of the agitation, the transportation of the gel-containing solution, and the separation of the gel were experimentally examined. Cerium(IV) was used instead of uranium, and agitator blades were selected to agitate the gel solution effectively. The gel solution was transferred through the self-feeding pump and was successfully separated into the gel and the solution using the spin dryer with a filter cloth.