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Developing accelerator mass spectrometry capabilities for anthropogenic radionuclide analysis to extend the set of oceanographic tracers

Hain, K.*; Martschini, M.*; G$"u$lce, F.*; 本多 真紀; Lachner, J.*; Kern, M.*; Pitters, J.*; Quinto, F.*; 坂口 綾*; Steier, P.*; et al.

Frontiers in Marine Science (Internet), 9, p.837515_1 - 837515_17, 2022/03

Vienna Environmental Research Accelerator (VERA)における加速器質量分析(AMS)の最近の大きな進歩は、検出効率向上とアイソバー抑制向上であり、環境中の極微量の長寿命放射性核種を分析する可能性を開くものである。これらの核種は$$^{233}$$U, $$^{135}$$Cs, $$^{99}$$Tc及び$$^{90}$$Srであり、通常は安定して海水中に溶存していることから、海洋混合・循環や放射性物質の広がりを研究する海洋トレーサーへの適応が重要になる。特に、同位体比$$^{233}$$U/$$^{236}$$Uと$$^{137}$$Cs/$$^{135}$$Csは元素分別の影響を受けないため、放出源の特定に有力なフィンガープリントであることが我々の研究によって実証されている。検出効率の向上により、10Lの海水試料で主要長寿命アクチニド$$^{236}$$U, $$^{237}$$Np, $$^{239,240}$$Pu, $$^{241}$$Amに加え、非常に稀な$$^{233}$$Uを分析することが可能となり、北西太平洋におけるアクチノイドの典型的な深度プロファイルを得ることに成功した。特に$$^{90}$$Sr分析に関しては、IAEAの標準物質(例えばIAEA-A-12)を用いて我々の新しいアプローチが海洋学的研究へ応用可能であることを示した。我々の推定では、$$^{90}$$Srと$$^{135}$$Csそれぞれの分析に必要な海水はわずか(1-3)Lである。


Interaction between surface acoustic waves and spin waves in a ferromagnetic thin film

山本 慧; Xu, M.*; Puebla, J.*; 大谷 義近*; 前川 禎通*

Journal of Magnetism and Magnetic Materials, 545, p.168672_1 - 168672_10, 2022/03

We present a theoretical description of magnon-phonon interactions in a multi-layer structure containing a ferromagnetic thin film. The formalism is applicable to an arbitrary direction of external magnetic field and various types of acoustic waves including Rayleigh and Love surface modes. A particular attention is paid to the spatial profile of the acoustic wave modes and analytical expressions for the effective coupling coefficients are derived taking into account the degree of mode profile overlap between spin waves and acoustic waves. The results are applied to reproduce a strongly anisotropic and non-reciprocal linewidth of acoustic ferromagnetic resonance reported in a recent experiment.


A Comparative CFD exercise on bubble hydrodynamics using Euler-Euler and interface tracking approaches

Dehbi, A.*; Cheng, X.*; Liao, Y.*; 岡垣 百合亜; Pellegrini, M.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 15 Pages, 2022/03

Nuclear degraded cores produce fission product aerosols that may reach the environment if not removed by natural processes and/or filtering equipment. The transport paths of aerosols usually include transits through stagnant water pools. It is therefore essential to develop computational tools to predict the aerosols retention by water pools. Currently, this is mostly done with 1-D lumped-parameter codes that are too simplistic to capture the physics. It is hence worthwhile to attempt the CFD approach, which has recently become reasonably mature to address bubble hydrodynamics in low momentum two-phase flows. In this first comparative exercise, we restrict the investigation to a hypothetical parallelepiped water pool (2$$times$$2$$times$$8 cm$$^{3}$$) into which air is injected through a circular 4 mm ID orifice at low velocity of 0.2 m/s. We present predictions of the gas phase dynamics (void and velocity profiles) for both Euler-Euler and Interface Tracking (IT, Volume-of-Fluid (VOF)) methodologies. In addition, we compare bubble shape, volume and detachment frequency from various IT simulation codes (CFX, Fluent, Star-CCM+, OpenFOAM). Reasonable agreement is found between IT simulations near the injector, but discrepancies increase as one moves towards the free surface. The disagreement between the Euler-Euler and IT results is substantial throughout the domain. Future studies will consist of validation exercises against experimental data to highlight potential model deficiencies and point to ways of remedying them.


Overview and main outcomes of the pool scrubbing lumped-parameter code benchmark on hydrodynamic aspects in IPRESCA project

Marchetto, C.*; Ha, K. S*; Herranz, L. E.*; 廣瀬 意育; Jankowski, T.*; Lee, Y.*; Nowack, H.*; Pellegrini, M.*; Sun, X.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 17 Pages, 2022/03

After the Fukushima Daiichi accident of March 2011, one of the main concerns of the nuclear industry has been the research works for improving atmospheric radioactive release mitigation systems. Pool scrubbing is an important process in reactors that mitigates radioactive release. It is based on the injection of gases containing fission products through a water pool. Bubble hydrodynamics, as a result of gas injection and the associated water pool thermal-hydraulics, is an important aspect of the process since the bubble size, shape, velocity, etc. influence the fission product trapping at the bubble interface with the water. Computer codes dedicated to the pool scrubbing have been mainly developed in the 90's last century and modelling drawbacks have been identified in particular for bubble hydrodynamics. One of IPRESCA project objectives is to improve the pool scrubbing modelling. In order to highlight the main modelling issues, a benchmark exercise has been performed focusing on the bubble hydrodynamics. This benchmark, performed by nine organisations coming from six countries, aims at simulating a basic configuration, a single upward injector in ambient conditions, experimentally characterized in the RSE tests carried out in the European PASSAM project. In this paper, a short description of the code modelling and a comparison between the code results and the experimental data are presented and discussed. Then, outcomes from the benchmark result analysis and proposals of improvements are emphasized.


Integration of pool scrubbing research to enhance source-term calculations (IPRESCA) project

Gupta, S.*; Herranz, L. E.*; Lebel, L. S.*; Sonnenkalb, M.*; Pellegrini, M.*; Marchetto, C.*; 丸山 結; Dehbi, A.*; Suckow, D.*; K$"a$rkel$"a$, T.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Pool scrubbing is a major topic in water cooled nuclear reactor technology as it is one of the means for mitigating the source-term to the environment during a severe accident. Pool scrubbing phenomena include coupled interactions between bubble hydrodynamics, aerosols and gaseous radionuclides retention mechanisms under a broad range of thermal-hydraulic conditions as per accident scenarios. Modeling pool scrubbing in some relevant accident scenarios has shown to be affected by substantial uncertainties. In this context, IPRESCA (Integration of Pool scrubbing Research to Enhance Source-term CAlculations) project aims to promote a better integration of international research activities related to pool scrubbing by providing support in experimental research to broaden the current knowledge and database, and by supporting analytical research to facilitate systematic validation and model enhancement of the existing pool scrubbing codes. The project consortium includes more than 30 organisations from 15 countries involving research institutes, universities, TSOs, and industry. For IPRESCA activities, partners join the project with in-kind contributions. IPRESCA operates under NUGENIA Technical Area 2/SARNET (Severe Accident) - Sub Technical Area 2.4 (Source-term). The present paper provides an introduction and overview of the IPRESCA project, including its objectives, organizational structure and the main outcomes of completed activities. Furthermore, key activities currently ongoing or planned in the project framework are also discussed.


Nanosecond structural dynamics of intrinsically disordered $$beta$$-casein micelles by neutron spectroscopy

中川 洋; Appavou, M.-S.*; Wuttke, J.*; Zamponi, M.*; Holderer, O.*; Schrader, T. E.*; Richter, D.*; Doster, W.*

Biophysical Journal, 120(23), p.5408 - 5420, 2021/12



An Approach toward evaluation of long-term fission product distributions in the Fukushima Daiichi Nuclear Power Plant after the severe accident

内田 俊介; 唐澤 英年; 木野 千晶*; Pellegrini, M.*; 内藤 正則*; 逢坂 正彦

Nuclear Engineering and Design, 380, p.111256_1 - 111256_19, 2021/08

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)



Conversion factors bridging radioactive fission product distributions in the primary containment vessel of Fukushima Daiichi NPP and dose rates measured by the containment atmosphere monitoring system

内田 俊介; Pellegrini, M.*; 内藤 正則*

Nuclear Engineering and Design, 380, p.111303_1 - 111303_11, 2021/08

 被引用回数:1 パーセンタイル:81.22(Nuclear Science & Technology)

福島第一原子力発電所(1F)の事故進展解析と同時に廃炉計画立案のためには、プラント全体にわたるFP分布の定量化が必須で、このために多期間FP挙動解析手法を開発している。この解析手法の妥当性は、プラントで測定されたデータに基づいて立証する必要がある。この妥当性立証の有効な手法のひとつがCAMSでの線量率測定データの適用である。しかし、FPの分布(kg, Bq)と線量率(Sv/h)という特性、単位次元の異なるデータを比較するためには、両者を適切につなぐ手段が必要となる。線量率解析が可能な、迅速で、取り扱いが容易で、かつトレーサブルな手法として、多くの線源位置、多核種に関しての線量率換算係数を求めた。この線量率換算係数を用いると、多期間FP挙動解析手法で求めたFP分布から容易に線量率が算出可能である。


Numerical investigations on the coolability and the re-criticality of a debris bed with the density-stratified configuration

Li, C.; 内堀 昭寛; 高田 孝; Pellegrini, M.*; Erkan, N.*; 岡本 孝司*

第25回動力・エネルギー技術シンポジウム講演論文集(インターネット), 4 Pages, 2021/07



Expansion of agriculture in northern cold-climate regions; A Cross-sectoral perspective on opportunities and challenges

Unc, A.*; Altdorff, D.*; Abakumov, E.*; Adl, S.*; Baldursson, S.*; Bechtold, M.*; Cattani, D. J.*; Firbank, L. G.*; Grand, S.*; Gudjonsdottir, M.*; et al.

Frontiers in Sustainable Food Systems (Internet), 5, p.663448_1 - 663448_11, 2021/07

 被引用回数:0 パーセンタイル:0(Food Science & Technology)



Overview and outcomes of the OECD/NEA benchmark study of the accident at the Fukushima Daiichi NPS (BSAF), Phase 2; Results of severe accident analyses for unit 3

Lind, T.*; Pellegrini, M.*; Herranz, L. E.*; Sonnenkalb, M.*; 西 義久*; 玉置 等史; Cousin, F.*; Fernandez Moguel, L.*; Andrews, N.*; Sevon, T.*

Nuclear Engineering and Design, 376, p.111138_1 - 111138_12, 2021/05

 被引用回数:3 パーセンタイル:81.22(Nuclear Science & Technology)



$$^{60}$$Fe and $$^{244}$$Pu deposited on Earth constrain the r-process yields of recent nearby supernovae

Wallner, A.*; Froehlich, M. B.*; Hotchkis, M. A. C.*; 木下 哲一*; Paul, M.*; Martschini, M.*; Pavetich, S.*; Tims, S. G.*; Kivel, N.*; Schumann, D.*; et al.

Science, 372(6543), p.742 - 745, 2021/05

 被引用回数:1 パーセンタイル:63.46(Multidisciplinary Sciences)



Development of a reference database for beta-delayed neutron emission

Dimitriou, P.*; Dillmann, I.*; Singh, B.*; Piksaikin, V.*; Rykaczewski, K. P.*; Tain, J. L.*; Algora, A.*; Banerjee, K.*; Borzov, I. N.*; Cano-Ott, D.*; et al.

Nuclear Data Sheets, 173, p.144 - 238, 2021/03

 被引用回数:1 パーセンタイル:0.03(Physics, Nuclear)

核分裂の発見以降、核分裂片から放出される遅発中性子の存在には、数多くの関心が集められてきた。原子力発電では、遅発中性子は原子炉動特性の計算や炉の安全運転において非常に重要な役割を演じている。それに加え、遅発中性子は、核構造や天体核、特に新世代のRIビーム施設の中心課題である安定線から離れた原子核でも、大きなインパクトをもっている。現在、ベータ崩壊半減期と遅発中性子分岐比に関するいくつかの文献が利用可能であるが、測定と評価によって実施されるべき十分な考証は、それらの文献ではしばしば抜けている。この欠落部に注目し、遅発中性子の核データ評価とそれに関する新しい文献作成の作業が、国際原子力機関(IAEA)の援助の基に着手され、「ベータ遅発中性子用データベースの開発」に関するCoordinated Research Project (CRP)が結成された。本論文では、CRPで行われたこれまでの結果について報告をする。


Morphological reproductive characteristics of testes and fertilization capacity of cryopreserved sperm after the Fukushima accident in raccoon (${it Procyon lotor}$)

小松 一樹*; 岩崎 亜美*; 村田 康輔*; 山城 秀昭*; Goh, V. S. T.*; 中山 亮*; 藤嶋 洋平*; 小野 拓実*; 木野 康志*; 清水 良央*; et al.

Reproduction in Domestic Animals, 56(3), p.484 - 497, 2021/03



Discovery of a new low energy neutron resonance of $$^{89}$$Y

片渕 竜也*; 藤 暢輔; 水本 元治*; 齋藤 辰宏*; 寺田 和司*; 木村 敦; 中村 詔司; Huang, M.*; Rovira Leveroni, G.; 井頭 政之*

European Physical Journal A, 57(1), p.4_1 - 4_4, 2021/01

 被引用回数:0 パーセンタイル:0.03(Physics, Nuclear)

A new neutron resonance of $$^{89}$$Y was found in time-of-flight (TOF) neutron capture experiments using a pulsed neutron beam from a spallation neutron source of the Japan Proton Accelerator Research Complex. The observed resonance energy was 19.7 eV that is much lower than the lowest energy (2.60 keV) of the previous reported resonances. In addition to the TOF measurement, nuclide identification of the resonance was made by prompt $$gamma$$-ray analysis. Neutron capture $$gamma$$-rays from $$^{89}$$Y were clearly observed only on the resonance. Resonance analysis was applied to the experimental results and the resonance parameters of the new resonance are given.


Review of Fukushima Daiichi Nuclear Power Station debris endstate location in OECD/NEA preparatory study on analysis of fuel debris (PreADES) project

仲吉 彬; Rempe, J. L.*; Barrachin, M.*; Bottomley, D.; Jacquemain, D.*; Journeau, C.*; Krasnov, V.; Lind, T.*; Lee, R.*; Marksberry, D.*; et al.

Nuclear Engineering and Design, 369, p.110857_1 - 110857_15, 2020/12

 被引用回数:0 パーセンタイル:0.33(Nuclear Science & Technology)



Overview and outcomes of the OECD/NEA benchmark study of the accident at the Fukushima Daiichi NPS (BSAF) Phase 2; Results of severe accident analyses for Unit 1

Herranz, L. E.*; Pellegrini, M.*; Lind, T.*; Sonnenkalb, M.*; Godin-Jacqmin, L.*; L$'o$pez, C.*; Dolganov, K.*; Cousin, F.*; 玉置 等史; Kim, T. W.*; et al.

Nuclear Engineering and Design, 369, p.110849_1 - 110849_7, 2020/12

 被引用回数:5 パーセンタイル:76.41(Nuclear Science & Technology)



Overview and outcomes of the OECD/NEA benchmark study of the accident at the Fukushima Daiichi NPS (BSAF), Phase 2; Results of severe accident analyses for Unit 2

Sonnenkalb, M.*; Pellegrini, M.*; Herranz, L. E.*; Lind, T.*; Morreale, A. C.*; 神田 憲一*; 玉置 等史; Kim, S. I.*; Cousin, F.*; Fernandez Moguel, L.*; et al.

Nuclear Engineering and Design, 369, p.110840_1 - 110840_10, 2020/12

 被引用回数:6 パーセンタイル:84.6(Nuclear Science & Technology)



Cathodoluminescence of cerium dioxide; Combined effects of the electron beam energy and sample temperature

Constantini, J.-M.*; Seo, P.*; 安田 和弘*; Bhuian, AKM S. I.*; 小川 達彦; Gourier, D.*

Journal of Luminescence, 226, p.117379_1 - 117379_10, 2020/10

 被引用回数:2 パーセンタイル:52.45(Optics)



Comprehensive analysis and evaluation of Fukushima Daiichi Nuclear Power Station Unit 2

山下 拓哉; 佐藤 一憲; 本多 剛*; 野崎 謙一朗*; 鈴木 博之*; Pellegrini, M.*; 酒井 健*; 溝上 伸也*

Nuclear Technology, 206(10), p.1517 - 1537, 2020/10

 被引用回数:5 パーセンタイル:89.87(Nuclear Science & Technology)

The estimation and understanding of the state of fuel debris and fission products inside the plant is an essential step in the decommissioning of the TEPCO Fukushima Daiichi Nuclear Power Station (1F). However, the direct observation of the plant interior, which is under a high radiation environment. Therefore, in order to understand the plant interior conditions, the comprehensive analysis and evaluation is necessary, based on various measurement data from the plant, analysis of plant data during the accident progression phase and information obtained from computer simulations for this phase. These evaluations can be used to estimate the conditions of the interior of the reactor pressure vessel (RPV) and the primary containment vessel (PCV). Herein, 1F Unit 2 was addressed as the subject to produce an estimated map of the fuel debris distribution from data obtained about the RPV and PCV based on the comprehensive evaluation of various measurement data and information obtained from the accident progression analysis, which were released to the public in June 2018.

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