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Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Kitamura, Akira; Yoshikawa, Hideki; Oda, Chie; Ishidera, Takamitsu; et al.
JAEA-Research 2014-030, 457 Pages, 2015/03
JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and post-closure performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, based on some examples of developing method of hydro-geological structure model, acquired knowledge are arranged using the tree diagram, and model uncertainty and its influence on the evaluation items were discussed. With regard to (2) study on scenario development, the developed approach for "defining conditions" has been reevaluated and improved from practical viewpoints. In addition, the uncertainty evaluation for the effect of use of cementitious material, as well as glass dissolution model, was conducted with analytical evaluation. With regard to (3) study on setting radionuclide migration parameters, based on survey of precedent procedures, multiple-approach for distribution coefficient of rocks was established, and the adequacy of the approach was confirmed though its application to sedimentary rock and granitic rock. Besides, an approach for solubility setting was developed including the procedure of selection of solubility limiting solid phase. The adequacy of the approach was confirmed though its application to key radionuclides.
Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Hayano, Akira; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.
JAEA-Research 2013-037, 455 Pages, 2013/12
Following FY2011, JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, the tree diagram of methodology of groundwater travel time has been extended for crystalline rock, in addition, tree diagram for sedimentary rock newly has been organized. With regard to (2) study on scenario development, the existing approach has been improved in terms of a practical task, and applied and tested for near field focusing on the buffer. In addition, the uncertainty of some important processes and its impact on safety functions are discussed though analysis. With regard to (3) study on setting radionuclide migration parameters, the approaches for parameter setting have been developed for sorption for rocks and solubility, and applied and tested through parameter setting exercises for key radionuclides.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.
no journal, ,
Spontaneous fissions of Fm, Fm, and Lr have been measured using an Es target at the JAEA Tandem Accelerator Facility. These three nuclei show different fission properties: the asymmetric fission, the high total-kinetic-energy (TKE) symmetric fission, and the low TKE symmetric fission, and the mechanisms of these three fissions should be very different. It is of great interest to elucidate how these differences occur. We have produced Fm in multinucleon-transfer reactions with a Es target and O projectiles, and produced Lr in the Cm(N,4n) fusion-evaporation reaction. The reaction products were mass-separated with a gas-jet-coupled on-line isotope separator, and were delivered into a rotating wheel alpha- and fission-fragment detection system. By comparing the mass and TKE distributions deduced from the present experimental data, we will discuss the differences in fission mechanism among Fm, Fm, and Lr.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi; Tomitsuka, Tomohiro; Chiera, N. M.; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro; Nishio, Katsuhisa; et al.
no journal, ,
Spontaneous fissions of neutron-rich heavy actinide isotopes Fm, Fm, and Lr have been measured at the JAEA Tandem accelerator facility. Fm and Fm were produced in a multinucleon transfer reaction with an O beam and an extremely rare Es target with a half-life of 276 days. Reaction products were mass-separated with an on-line isotope separator (ISOL). A transition between the typical asymmetric mass distribution and a very sharp symmetric one was clearly observed between Fm and Fm, while the spontaneous fission of Lr was found to exhibit mixture of three different fission modes.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi*; Tomitsuka, Tomohiro*; Chiera, N. M.*; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro*; Nishio, Katsuhisa; et al.
no journal, ,
Neutron-rich fermium isotopes Fm and Fm and lawrencium isotope Lr were produced in the multinucleon transfer reaction on Es target with heavy-ion beam and in the heavy-ion fusion reaction on Cm target with N beam, respectively. Reaction products were mass-separated with an on-line isotope separator (ISOL), and spontaneous fission (SF) of these isotopes were measured. It was found that the mass distribution of the SF of Fm was asymmetric, while that of Fm was sharp symmetric, which confirmed the previous experimental results. On the other hand, the SF of Lr seemed to contain both symmetric and asymmetric mass distributions. On the basis of the present results of the mass and total kinetic energy distributions, we discussed the mechanism of fission for these isotopes.
Asai, Masato; Tsukada, Kazuaki; Hirose, Kentaro; Toyoshima, Atsushi*; Tomitsuka, Tomohiro*; Chiera, N. M.*; Ito, Yuta; Makii, Hiroyuki; Nagame, Yuichiro*; Nishio, Katsuhisa; et al.
no journal, ,
We have studied spontaneous fission of neutron-rich Fm and Lr isotopes. The neutron-rich Fm isotopes were produced with the Es target and the O beam delivered by the JAEA tandem accelerator. The neutron-rich Lr isotope were produced with the Cm target and the N beam. Reaction products were mass-separated with an on-line isotope separator (ISOL), which enabled us to obtain non-contaminated samples and to measure fission fragments precisely. From the deduced fission-fragment mass and total kinetic energy distributions, we have obtained a new insight into the competition between the symmetric and asymmetric fission which is characteristic in this neutron-rich region.