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JAEA Reports

Technical note for the cavitation damage inspection for interior surface of the mercury target vessel, 2; Damage depth measurement for cavitation erosion

Naoe, Takashi; Wakui, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Teshigawara, Makoto; Haga, Katsuhiro

JAEA-Technology 2023-022, 81 Pages, 2024/01

JAEA-Technology-2023-022.pdf:9.87MB

In the liquid mercury target system for the pulsed spallation neutron source of Materials and Life Science Experimental Facility (MLF) in the Japan Proton Accelerator Research Complex (J-PARC), pressure waves that is generated by the high-energy proton beam injection simultaneously with the spallation reaction, resulting severe cavitation erosion damage on the interior surface of the mercury target vessel. Because the bubble of pressure wave-induced cavitation collapsing near the interior surface of the mercury target vessel with applying the large amplitude of localized impact on the surface. Since the wall thickness of the beam entrance portion of the target vessel is designed to be 3 mm to reduce thermal stress due to the internal heating, the erosion damage has the possibility to cause the vessel fatigue failure and mercury leakage originated from erosion pits during operation. To reduce the erosion damage by cavitation, a technique of gas microbubble injection into the mercury for pressure wave mitigation, and double-walled structure of the beam window of the target vessel has been applied. A specimen was cut from the beam window of the used mercury target vessel in order to investigate the effect of the damage mitigation technologies on the vessel, and to reflect the consideration of operation condition for the next target. We have observed cavitation damage on interior surface of the used mercury target vessel by cutting out the disk shape specimens. Damage morphology and depth of damaged surface were evaluated and correlation between the damage depth and operational condition was examined. The result showed that the erosion damage by cavitation is extremely reduced by injecting gas microbubbles and the damage not formed inside narrow channel of the double-walled structure for relatively high-power operated target vessels.

Journal Articles

Beam separation experiment with prototype non-destructive electrostatic septum and study for device improvement

Nagayama, Shota; Harada, Hiroyuki; Shimogawa, Tetsushi*; Sato, Atsushi*; Yamada, Ippei; Chimura, Motoki; Kojima, Kunihiro; Yamamoto, Kazami; Kinsho, Michikazu

Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.526 - 530, 2023/11

We have been developing "Non-destructive electrostatic septum" for a slow extraction. This septum has multiple electrodes placed around the region without the beam hitting and separate the beam by its electric field. To evaluate its electric field, we have built a prototype septum and a test machine, which consists of an electron gun and monitors. This test machine can measure the electric field indirectly by using a narrow electron beam. The experiment results of prototype septum is good agreement with the calculation one. However, this electric field distribution is not enough to separate the beam. A step function-like electric field distribution is ideal for the beam separation with minimal negative effect on the beam. We have studied to improve the electrode configuration to match the beam shape. In this paper, we present the result of the electric field measurements and the septum improvement. Additionally, we describe the future plan of this development.

Journal Articles

Effect of inner wall cracking on the cavitation bubble formation in the mercury spallation target at J-PARC

Ariyoshi, Gen; Saruta, Koichi; Kogawa, Hiroyuki; Futakawa, Masatoshi; Maeno, Koki*; Li, Y.*; Tsutsui, Kihei*

Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.1407 - 1420, 2023/08

Cavitation damage on a target vessel due to proton beam-induced pressure waves is one of the crucial issues for the pulsed neutron source using a mercury spallation target. As a mitigation technique for the damage, the helium microbubble injection into the mercury has been carried out by using a swirl bubbler in order to utilize compressibility of bubbles. Moreover, double-walled structure, which consists of an outer wall and an inner wall, has been applied as the target head structure. In this study, we aim to develop an abnormality diagnostic technology to detect the inner wall cracking, which is caused by such cavitation damage, from the outside of the target vessel. The mercury flow fields in the case with the cracking are evaluated by computational fluid dynamics analysis based on finite element method. And then, effect of the cracking on the flow field is discussed from the point of view of the flow-induced vibration and the acoustic vibration.

Journal Articles

Study of non-destructive slow beam extraction method in particle accelerator

Nagayama, Shota; Harada, Hiroyuki; Shimogawa, Tetsushi*; Yamada, Ippei; Chimura, Motoki; Yamamoto, Kazami; Kinsho, Michikazu

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.503 - 507, 2023/01

Synchrotron accelerators realize physics experiments and radiation cancer treatment using the slow extraction technique, in which beams are stored in the ring and gradually delivered. We have devised and are currently developing a "non-destructive electrostatic septum" based on a new method, which in principle cannot be solved by conventional methods and is a cause of equipment failure and output limitation. It is ideal to generate a force distribution similar to a staircase function with discontinuous gaps at the boundary. In this presentation, we will show the calculation method for optimizing the electrode and wire configuration to generate a Lorentz force with a distribution similar to a staircase function in vacuum, and the calculation results of the beam breakup due to the generated Lorentz force. The compact proof-of-principle machine developed for the ongoing demonstration of this method will also be introduced.

JAEA Reports

Optimization of mercury flow with microbubbles in the target-vessel design by means of machine learning

Kogawa, Hiroyuki; Futakawa, Masatoshi; Haga, Katsuhiro; Tsuzuki, Takayuki*; Murai, Tetsuro*

JAEA-Technology 2022-023, 128 Pages, 2022/11

JAEA-Technology-2022-023.pdf:9.0MB

In a mercury target of the J-PARC (Japan Proton Accelerator Research Complex), pulsed proton beams repeatedly bombard the flowing mercury which is confined in a stainless-steel vessel (target vessel). Cavitation damage caused by the propagation of the pressure waves is a factor of the life of the target vessel. As a measure to reduce damages, we developed a bubbler to inject the gas microbubbles into the flowing mercury, which can reduce the pressure waves. To operate the mercury target vessel stably with the 1 MW high-intensity proton beams, further reduction of the damage is required. The bubbler setting position should be closer to the beam window to increase the bubble population, which could enhance the reduction effect on the pressure waves and damage. However, the space at the beam window of the target vessel is restricted. The bubbler design and setting position as well as the vane design for the mercury flowing pattern are optimized by means of a machine learning technique to get more suitable bubble distribution, increasing in bubble population and optimizing bubble size nearby the beam window of the target vessel. The results of CFD analyses performed with 1000 cases were used for machine learning. Since the flow rate of mercury affects the temperature of the target vessel, this was used for the constraint condition. As a result, we found a design of mercury target vessel that can increase the bubble population by ca. 20% higher than the current design.

JAEA Reports

Technical note for the cavitation damage inspection for interior surface of the mercury target vessel, 1; Development of specimen cutting machine for remote handling

Naoe, Takashi; Kinoshita, Hidetaka; Wakui, Takashi; Kogawa, Hiroyuki; Haga, Katsuhiro

JAEA-Technology 2022-018, 43 Pages, 2022/08

JAEA-Technology-2022-018.pdf:7.84MB

In the liquid mercury target system for the pulsed spallation neutron source of Materials and Life science experimental Facility (MLF) at the Japan in the Japan Proton Accelerator Research Complex (J-PARC), cavitation that is generated by the high-energy proton beam-induced pressure waves, resulting severe erosion damage on the interior surface of the mercury target vessel. The erosion damage is increased with increasing the proton beam power, and has the possibility to cause the leakage of mercury by the penetrated damage and/or the fatigue failure originated from erosion pits during operation. To achieve the long term stable operation under high-power proton beam, the mitigation technologies for cavitation erosion consisting of surface modification on the vessel interior surface, helium gas microbubble injection, double-walled beam window structure has been applied. The damage on interior surface of the vessel is never observed during the beam operation. Therefore, after the target operation term ends, we have cut out specimen from the target nose of the target vessel to inspect damaged surface in detail for verification of the cavitation damage mitigation technologies and lifetime estimation. We have developed the techniques of specimen cutting out by remote handling under high-radiation environment. Cutting method was gradually updated based on experience in actual cutting for the used target vessel. In this report, techniques of specimen cutting out for the beam entrance portion of the target vessel in high-radiation environment and overview of the results of specimen cutting from actual target vessels are described.

Journal Articles

Development of the high-power spallation neutron target of J-PARC

Haga, Katsuhiro; Kogawa, Hiroyuki; Naoe, Takashi; Wakui, Takashi; Wakai, Eiichi; Futakawa, Masatoshi

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 13 Pages, 2022/03

The cross-flow type target was developed as the basic design of mercury target in J-PARC, and the design has been improved to realize the MW-class pulsed spallation neutron source. When the high-power and short-pulsed proton beam is injected into the mercury target, pressure waves are generated in mercury by rapid heat generation. The pressure waves induce the cavitation damages on the target vessel. Two countermeasures were adopted, namely, the injection of microbubbles into mercury and the double walled structure at the beam window. The bubble generator was installed in the target vessel to absorb the volume inflation of mercury and mitigate the pressure waves. Also, the double walled target vessel was designed to suppress the cavitation damage by the large velocity gradient of rapid mercury flow in the narrow channel of double wall. Finally, we could attain 1 MW beam operation with the duration time of 36.5 hours in 2020, and achieved the long term stable operation with 740 kW from April in 2021. This report shows the technical development of the high-power mercury target vessel in view of thermal hydraulics to attain 1 MW operation.

Journal Articles

Multilayered lamellar materials and thin films by instant self-assembly of amphiphilic random copolymers

Ikami, Takaya*; Watanabe, Yuki*; Ogawa, Hiroki*; Takenaka, Mikihito*; Yamada, Norifumi*; Ouchi, Makoto*; Aoki, Hiroyuki; Terashima, Takaya*

ACS Macro Lett (Internet), 10(12), p.1524 - 1528, 2021/12

JAEA Reports

Interim activity status report of "the group for investigation of reasonable safety assurance based on graded approach" (from September, 2019 to September, 2020)

Yonomoto, Taisuke; Nakashima, Hiroshi*; Sono, Hiroki; Kishimoto, Katsumi; Izawa, Kazuhiko; Kinase, Masami; Osa, Akihiko; Ogawa, Kazuhiko; Horiguchi, Hironori; Inoi, Hiroyuki; et al.

JAEA-Review 2020-056, 51 Pages, 2021/03

JAEA-Review-2020-056.pdf:3.26MB

A group named as "The group for investigation of reasonable safety assurance based on graded approach", which consists of about 10 staffs from Sector of Nuclear Science Research, Safety and Nuclear Security Administration Department, departments for management of nuclear facility, Sector of Nuclear Safety Research and Emergency Preparedness, aims to realize effective graded approach (GA) about management of facilities and regulatory compliance of JAEA. The group started its activities in September, 2019 and has had discussions through 10 meetings and email communications. In the meetings, basic ideas of GA, status of compliance with new regulatory standards at each facility, new inspection system, etc were discussed, while individual investigation at each facility were shared among the members. This report is compiled with expectation that it will help promote rational and effective safety management based on GA by sharing contents of the activity widely inside and outside JAEA.

Journal Articles

Effect of gas microbubble injection and narrow channel structure on cavitation damage in mercury target vessel

Naoe, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Wakui, Takashi; Wakai, Eiichi; Haga, Katsuhiro; Takada, Hiroshi

Materials Science Forum, 1024, p.111 - 120, 2021/03

The mercury target vessel for the at the J-PARC neutron source is severely damaged by the cavitation caused by proton beam-induced pressure waves in mercury. To mitigate the cavitation damage, we adopted a double-walled structure with a narrow channel for the mercury at the beam window of the vessel. In addition, gas microbubbles were injected into the mercury to suppress the pressure waves. The front end of the vessel was cut out to inspect the effect of the damage mitigation technologies on the interior surface. The results showed that the double-walled target facing the mercury with gas microbubbles operating at 1812 MWh for an average power of 434 kW had equivalent damage to the single-walled target without microbubbles operating 1048 MWh for average power of 181 kW. The erosion depth due to cavitation in the narrow channel was clearly smaller than it was on the wall facing the bubbling mercury

Journal Articles

New design of high power mercury target vessel of J-PARC

Wakui, Takashi; Wakai, Eiichi; Kogawa, Hiroyuki; Naoe, Takashi; Hanano, Kohei*; Haga, Katsuhiro; Shimada, Tsubasa*; Kanomata, Kenichi*

Materials Science Forum, 1024, p.145 - 150, 2021/03

To realize a high beam power operation at the J-PARC, a mercury target vessel covered with water shroud was developed. In the first step, to realize an operation at 500 kW, the basic structure of the initial design was followed and the connection method between the mercury vessel and the water shroud was changed. Additionally, the operation at a beam power of 500 kW was realized in approximately eight months. In the second step, to realize the operation at 1 MW, the new structure in which only rear ends of vessels were connected was investigated. Cooling of the mercury vessel is used to reduce thermal stress and thick vessels of the water shroud are used to increase stiffness for the internal pressure; therefore, it was adopted. The stress in each vessel was lower than the allowable stress based on the pressure vessel code criteria prescribed in the Japan Industrial Standard, and confirmation was obtained that the operation with a beam power of 1 MW could be conducted.

Journal Articles

Neutron reflectometry tomography for imaging and depth structure analysis of thin films with in-plane inhomogeneity

Aoki, Hiroyuki; Ogawa, Hiroki*; Takenaka, Mikihito*

Langmuir, 37(1), p.196 - 203, 2021/01

 Times Cited Count:2 Percentile:15.56(Chemistry, Multidisciplinary)

Journal Articles

Corrosion resistance of a cast steel overpack for high-level radioactive waste disposal in Japan

Ogawa, Yusuke*; Suzuki, Satoru*; Taniguchi, Naoki; Kawasaki, Manabu*; Suzuki, Hiroyuki*; Takahashi, Rieko*

Materials and Corrosion, 72(1-2), p.52 - 66, 2021/01

 Times Cited Count:2 Percentile:13.1(Materials Science, Multidisciplinary)

Cast steel is one of the promising alternative to forged steel that is the current reference material for carbon steel overpack. In this study, the full-scale cast steel overpack was produced experimentally and the distribution of casting defects were investigated. The corrosion test regarding corrosion rate and stress corrosion cracking (SCC) susceptibility were also conducted using samples taken from the full-scale cast steel overpack and the corrosion resistance of cast steel was compared with that of forged steel. From above two corrosion tests, it can be said that the corrosion resistance of cast steel is mostly the same as that of forged steel.

Journal Articles

Pressure wave induced sound measurement for diagnosing the operation status of the J-PARC pulsed spallation neutron source

Naoe, Takashi; Kogawa, Hiroyuki; Wakui, Takashi; Teshigawara, Makoto; Haga, Katsuhiro; Futakawa, Masatoshi

Nuclear Instruments and Methods in Physics Research A, 982, p.164566_1 - 164566_6, 2020/12

 Times Cited Count:1 Percentile:26.45(Instruments & Instrumentation)

A liquid mercury target for the spallation neutron source is installed in the J-PARC. The liquid mercury is enclosed with the multi-walled stainless steel vessel. At the time of highly intense proton beams hits the target at a repetition rate of 25 Hz, pressure waves, that causes cavitation erosion, are generated owing the rapidly thermal expansion of mercury. We have installed the target diagnostic system consisting of a laser Doppler vibrometer (LDV) and a dynamic microphone to remotely investigate the structural integrity of the target under high-radiation environment. In this study, aiming to understand correlation between the acoustic vibration and the operation conditions such as the proton beam power and beam profile, proton beam induced acoustic vibration was measured by parametrically changing the target operation conditions. The result showed that the sound is well correlated with the operation conditions.

Journal Articles

Water leakage due to the welding defect and improvement to reach 1-MW beam operation in the mercury target of J-PARC

Kogawa, Hiroyuki; Wakui, Takashi; Naoe, Takashi; Haga, Katsuhiro; Takada, Hiroshi; Futakawa, Masatoshi

Journal of Nuclear Science and Technology, 57(5), p.487 - 494, 2020/05

 Times Cited Count:1 Percentile:12.47(Nuclear Science & Technology)

Neutron flux per pulse reached world record at neutron source in the J-PARC. In the J-PARC, mercury target system is used as a spallation neutron source. A target vessel has the multi-walled protection system that comprises a mercury vessel enclosed with a double-walled water shroud. This is to prevent the leakage of the mercury outside the mercury vessel. The multi-walled structure needed to be complicated with a lot of welding lines. However, during the operation, we faced an unscheduled shutdown due to water leakage to the intermediate layer between the mercury vessel and water shroud. An investigation on the cause of the leakage was carried out. It is deduced that the leakage path was formed due to the crack propagation from welding defects that is caused by the complicated multi-walled structure. The crack propagation is attributed to the repeated stress by pressure waves generated in the mercury target. Based on the investigation results, the design was improved to remove the welding line on the complicated structure and to realize the stable operation with 1 MW proton beam.

Journal Articles

Mitigation of cavitation damage in J-PARC mercury target vessel

Naoe, Takashi; Kinoshita, Hidetaka; Kogawa, Hiroyuki; Wakui, Takashi; Wakai, Eiichi; Haga, Katsuhiro; Takada, Hiroshi

JPS Conference Proceedings (Internet), 28, p.081004_1 - 081004_6, 2020/02

The beam window of the mercury target vessel in J-PARC is severely damaged by the cavitation. The cavitation damage is a crucial factor to limit lifetime of the target because it increases with the beam power. Therefore, mitigating cavitation damage is an important issue to operate the target stably for long time at 1 MW. At J-PARC, to mitigate the cavitation damage: gas microbubbles are injected into mercury for suppressing pressure waves, and double-walled structure with a narrow channel of 2 mm in width to form high-speed mercury flow ($$sim$$4m/s) has been adopted. After operation, the beam window was cut to inspect the effect of the cavitation damage mitigation on inner wall. We optimized cutting conditions through the cold cutting tests, succeeding in cutting the target No.2 (without damage mitigation technologies) smoothly in 2017, and target No.8 with damage mitigation technologies. In the workshop, progress of cavitation damage observation for the target vessel will be presented.

Journal Articles

New design and fabrication technology applied in mercury target vessel #8 of J-PARC

Wakui, Takashi; Wakai, Eiichi; Kogawa, Hiroyuki; Naoe, Takashi; Hanano, Kohei; Haga, Katsuhiro; Takada, Hiroshi; Shimada, Tsubasa*; Kanomata, Kenichi*

JPS Conference Proceedings (Internet), 28, p.081002_1 - 081002_6, 2020/02

A mercury target vessel of J-PRAC is designed with a triple-walled structure consisting of the mercury vessel and a double-walled water shroud with internal and external vessels. During the beam operation at 500 kW in 2015, small water leakages from a water shroud of the mercury target vessel occurred twice. Design, fabrication and inspection processes were improved based on the lessons learned from the target failures. The total length of welding lines at the front of the mercury target vessel decreases drastically to approximately 55% by adopting monolithic structure cut out from a block of stainless steel by the wire-electrical discharge machining. Thorough testing of welds by radiographic testing and ultrasonic testing was conducted. The fabrication of the mercury target vessel #8 was finished on September 2017 and the beam operation using it started. Stable beam operation at 500 kW has been achieved and it could experience the maximum beam power of 1 MW during a beam test.

Journal Articles

Effects of the nuclear structure of fission fragments on the high-energy prompt fission $$gamma$$-ray spectrum in $$^{235}$$U($$n_{rm th},f$$)

Makii, Hiroyuki; Nishio, Katsuhisa; Hirose, Kentaro; Orlandi, R.; L$'e$guillon, R.; Ogawa, Tatsuhiko; Soldner, T.*; K$"o$ster, U.*; Pollitt, A.*; Hambsch, F.-J.*; et al.

Physical Review C, 100(4), p.044610_1 - 044610_7, 2019/10

 Times Cited Count:11 Percentile:75.05(Physics, Nuclear)

Journal Articles

Pulsed pressure induced cavitation erosion in mercury narrow channel under flowing conditions

Naoe, Takashi; Kogawa, Hiroyuki; Tanaka, Nobuatsu*; Futakawa, Masatoshi

Advanced Experimental Mechanics, 4, p.17 - 21, 2019/08

We have introduced the following two techniques to mitigate the pressure wave-induced cavitation damage in the mercury target. One is the gas microbubble injection into the flowing mercury, and the other is the double-walled structure with a narrow gap channel at the proton beam entrance portion of the mercury vessel. The latter is expected to mitigate the cavitation damage due to the high-speed liquid flow ($$sim$$ 4 m/s) and the narrow gap boundary (2 mm). To quantitatively investigate the effect of double-walled structure on cavitation damage, cavitation damage tests were conducted by parametrically changing mercury flow velocity and gap width of the channel wall. The results showed that the damage evaluated as a surface roughness was reduced by increasing the flow velocity. By contrast, the effect of gap width on cavitation damage was hardly observed under flowing conditions.

Journal Articles

Proposal of non-destructive device for slow extraction

Shimogawa, Tetsushi*; Harada, Hiroyuki

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1156 - 1158, 2019/07

A particle beam from accelerators has been applied not only to physics experiments but also medical applications. In the slow extraction which extract beam from a synchrotron during a large number of turns, the accelerated beam is blown up and extracted by the electrostatic septum. The septum consists of electrode and septum for separating between extraction and circulating beam. Generally, the wire and plate are used for septum. In this case, the beam hits on septum. Consequently, the extraction efficiency and the beam power are limited. We propose the non-destructive electrostatic septum. The multiple electrodes arrange surround the beam and produce the electric field for separation and deflect the beam. There are no materials in the beam orbit area. This will be reported introduction of our proposed non-destructive electrostatic septum.

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