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Sueoka, Shigeru; Iwano, Hideki*; Danhara, Toru*; Niwa, Masakazu; Kanno, Mizuho; Kohn, B. P.*; Kawamura, Makoto; Yokoyama, Tatsunori; Kagami, Saya; Ogita, Yasuhiro; et al.
Earth, Planets and Space (Internet), 75(1), p.177_1 - 177_24, 2023/12
Times Cited Count：0 Percentile：0(Geosciences, Multidisciplinary)Fluid-inclusion and thermochronometric analyses have been applied to hydrothermal alteration zones and their host rocks outcropping in the Hongu area of the Kii Peninsula, southwestern Japan in an attempt to detect thermal anomalies related to hydrothermal events and quantify the thermal effects on the host rocks. Hydrothermal events at ca 150 deg. C and ca 200 deg. C were identified by fluid-inclusion microthermometry of quartz veins in the alteration zones. For the host rocks and alteration zones, in the youngest population zircon yielded U-Pb dates ranging between ca 74.7-59.2 Ma, fission-track dates of ca 27.2-16.6 Ma, and (U-Th)/He single-grain dates of ca 23.6-8.7 Ma. Apatite yielded pooled fission-track ages of ca 14.9-9.0 Ma. The zircon U-Pb dates constrain the maximum depositional ages of the sedimentary samples. However, the fission-track and (U-Th)/He dates show no clear trend as a function of distance from the alteration zones. Hence, no thermal anomaly was detected in the surrounding host rocks based on the thermochronometric data patterns. The fission-track and (U-Th)/He dates are rather thought to record regional thermal and exhumation histories rather than a direct thermal imprint of fluid flow, probably because the duration of such activity was too short or because fluid flow occurred before regional cooling events and were later thermally overprinted. Apatite fission-track ages of ca 10 Ma may reflect regional mountain uplift and exhumation related to the obduction of the SW Japan lithospheric sliver onto the Shikoku Basin, or the rapid subduction of the Philippine Sea slab associated with the clockwise rotation of the Southwest Japan Arc.
Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Fujita, Natsuko; Yokoyama, Tatsunori; Ogita, Yasuhiro; Fukuda, Shoma; Nakajima, Toru; Kagami, Saya; Ogata, Manabu; et al.
JAEA-Review 2023-017, 27 Pages, 2023/10
JAEA-Review-2023-017.pdf:0.94MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2023. The objectives and contents in fiscal year 2023 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.
Niwa, Masakazu; Shimada, Koji; Sueoka, Shigeru; Ishihara, Takanori; Ogawa, Hiroki; Hakoiwa, Hiroaki; Watanabe, Tsuyoshi; Nishiyama, Nariaki; Yokoyama, Tatsunori; Ogata, Manabu; et al.
JAEA-Research 2023-005, 78 Pages, 2023/10
JAEA-Research-2023-005.pdf:6.51MB
This annual report documents the progress of research and development (R&D) in the 1st fiscal year of the Japan Atomic Energy Agency 4th Medium- and Long-term Plan (fiscal years 2022-2028) to provide the scientific base for assessing geosphere stability for long-term isolation of high-level radioactive waste. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.
Yuguchi, Takashi*; Ito, Daichi*; Yokoyama, Tatsunori; Sakata, Shuhei*; Suzuki, Satoshi*; Ogita, Yasuhiro; Yagi, Koshi*; Imura, Takumi*; Motai, Satoko*; Ono, Takeshi*
Lithos, 440-441, p.107026_1 - 107026_14, 2023/03
Times Cited Count：0 Percentile：0.02(Geochemistry & Geophysics)We propose a new method for elucidating zircon growth in granitic plutons, based on variations in three-dimensional 3D cathodoluminescence (CL) patterns, U-Pb ages, titanium concentration, and Th/U ratios. We focused on the zircon growth processes in the Okueyama granite (OKG) in central Kyushu, Japan, to obtain interpretations of magma chamber processes that result in the formation of granitic plutons. The OKG consists of three lithofacies: biotite granite (BG), hornblende granite (HG), and hornblende granodiorite (HGD). To determine the 3D internal structure and growth pattern of a zircon crystal, we performed CL observations for multi-sections of the samples. Simultaneously, we also determined the zircon U-Pb age and titanium concentration of the center sections of the samples. The 3D distribution of the oscillatory zoning can be used to determine the crystal nucleus. The simultaneous determination of zircon U-Pb ages and Ti concentrations of the granite samples indicates the time-temperature (t-T) history of granitic magma before its solidification. The t-T histories of the BG, HG, and HGD represented similar cooling behaviors within the magma chamber: rapid cooling from the zircon crystallization temperature to the closure temperature of the biotite K-Ar system between 16 Ma and 10 Ma. The variations in the Th/U ratios against temperature also demonstrate a different trend at the boundary of approximately 670 
C. Fractional crystallization in the magma chamber progressed significantly at temperatures above 670 C; below 670 C, crystallization progressed slowly, indicating only minimal changes in the magma composition. The variations in the Th/U ratio against temperature in the BG, HG, and HGD portrayed common tendencies, indicating the same behavior in the progression of fractional crystallization among the three lithofacies, which in turn, represented the same behavior within the entire magma chamber.
Harada, Takuya*; Nagata, Mitsuhiro; Ogita, Yasuhiro; Kagami, Saya; Yokoyama, Tatsunori
Chigaku Zasshi, 132(1), p.57 - 65, 2023/02
The Harachiyama Formation is Lower Cretaceous volcanic rocks, distributed in the eastern margin of the Kitakami Mountains in northeastern Japan. We performed whole-rock chemical analysis, zircon U-Pb dating and Hf isotope analysis from the Harachiyama Formation to constrain the formation age and discuss the origin of magma. The lava and tuff samples of the Harachiyama Formation from the Omoto and Tsukue areas support island-arc rhyolitic rocks (SiO
content 
70%), and yielded the weighted mean U-Pb ages of 127.8 
3.4 Ma and 129.2 2.6 Ma (2
), respectively. Eighteen zircon grains from two samples, dated between 141.6 Ma and 123.9 Ma, yielded positive 
Hf(t) values between +5.0 and +8.7. These ages and values are consistent with those of the Kitakami Granititods reported in previous studies. Therefore, it is suggested that the Harachiyama Formation have the same magmatic origin as the Kitakami Granitoid.
Sasao, Eiji; Ishimaru, Tsuneari; Niwa, Masakazu; Shimada, Akiomi; Shimada, Koji; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.
JAEA-Review 2022-022, 29 Pages, 2022/09
JAEA-Review-2022-022.pdf:0.97MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2022. The objectives and contents in fiscal year 2022 are described in detail based on the JAEA 4th Medium- and Long-term Plan (fiscal years 2022-2028). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques
Yuguchi, Takashi*; Yamazaki, Hayato*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Suzuki, Satoshi*; Ogita, Yasuhiro; Sando, Kazusa*; Imura, Takumi*; Ono, Takeshi*
Journal of Asian Earth Sciences, 226, p.105075_1 - 105075_9, 2022/04
Times Cited Count：4 Percentile：49.4(Geosciences, Multidisciplinary)Simultaneous determination of the U-Pb age of zircon and concentration of titanium in a single analysis spot, using inductively coupled plasma mass spectrometry with laser ablation sample introduction, produces paired age and temperature data of zircon crystallisation, potentially revealing time-temperature (
) histories for evolved magma. The Kurobegawa granite, central Japan, contains abundant mafic magmatic enclaves (MMEs). We applied this method to evaluate MMEs and their host (enclosing) granites. Cooling behaviour common to both MMEs and host rocks was found between 1.5 and 0.5 Ma. Rapid cooling from the zircon crystallisation temperature to the closure temperature of biotite K-Ar system was within 
1 million year. Combining the obtained paths of MMEs and host rocks with petrological information can provide insights into magma chamber processes. This suggests that MME flotation, migration, and spread through the magma chamber ceased at 1.5-0.5 Ma, indicating the emplacement age of the Kurobegawa granitic pluton, as no large-scale reheating episodes have occurred since then.
Minami, Saki*; Nagata, Mitsuhiro; Sueoka, Shigeru; Fukuda, Shoma; Kajita, Yuya*; Ogita, Yasuhiro; Kagami, Saya; Yokoyama, Tatsunori; Tagami, Takahiro*
Earth, Planets and Space (Internet), 73(1), p.231_1 - 231_7, 2021/12
Times Cited Count：1 Percentile：8.23(Geosciences, Multidisciplinary)Minami, Saki*; Nagata, Mitsuhiro; Sueoka, Shigeru; Fukuda, Shoma; Kajita, Yuya*; Ogita, Yasuhiro; Yokoyama, Tatsunori; Kagami, Saya; Tagami, Takahiro*
Fisshion, Torakku Nyusureta, (34), p.4 - 8, 2021/12
This study employed U-Pb dating for determining the intrusive age of young (several Ma) granitoids in Tanigawa-dake area, where rapid and intense uplift/denudation has probably occurred in Japan. As results, U-Pb age of 109 Ma for the Cretaceous granodiorite and 3.95-3.19 Ma about 3 samples of the Pliocene granodiorites were obtained. These U-Pb ages showed consistent with previously reported ages based on thermochronometers having lower closure temperatures such as K-Ar or zircon fission-track methods. All previous data indicated younger ages than U-Pb ones in this study. Therefore, our U-Pb data can be interpreted as intrusive ages of young granitoids, inferring multiple events possibly occurred at least twice and contributed to the formation in young granitoids in the Tanigawa-dake area.
Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Niwa, Masakazu; Shimada, Akiomi; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; et al.
JAEA-Research 2021-007, 65 Pages, 2021/10
JAEA-Research-2021-007.pdf:4.21MB
This annual report documents the progress of research and development (R&D) in the 6th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.
Ishimaru, Tsuneari; Kokubu, Yoko; Shimada, Koji; Shimada, Akiomi; Niwa, Masakazu; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.
JAEA-Review 2021-012, 48 Pages, 2021/08
JAEA-Review-2021-012.pdf:1.64MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2021. The objectives and contents in fiscal year 2021 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.
Yonaga, Yusuke; Sano, Naomi*; Amamiya, Hiroki*; Ogita, Yasuhiro; Niwa, Masakazu; Yasue, Kenichi*
Oyo Chishitsu, 62(1), p.2 - 12, 2021/04
Provenance analysis based on quick identification of heavy minerals using an electron probe microanalyzer (EPMA) was applied to samples from Pleistocene sediments in Horonobe region, Hokkaido, where major provenance rocks can be sedimentary and mafic igneous rocks. The concentrations of 16 elements were measured in individual grains to identify the mineral species based on their chemical composition. In addition, microscopic observation of thin sections and gravel composition analysis were conducted to confirm the validity of the quick identification of heavy minerals. These analyses clarify that combinations of several heavy mineral species can be a useful index of provenance rocks from the Soya Hill and Teshio Mountains, and suggest that uplift of the Soya Hill after ca. 1.5 Ma constrained supply of sediments from the Teshio Mountains. On the other hand, minerals uncommon both in the Soya Hill and Teshio Mountains, such as hornblende, are included in the Pleistocene sediments. This suggests that a sediment supply from distant area was also significant, like transportation by the Teshio River. The method for quick identification of heavy minerals using EPMA can provide an information about provenance rocks difficult to identify only by gravel composition analysis.
Sueoka, Shigeru; Shimada, Koji; Terusawa, Shuji*; Iwano, Hideki*; Danhara, Toru*; Ogita, Yasuhiro; Hirata, Takafumi*
Chishitsugaku Zasshi, 127(1), p.25 - 39, 2021/01
no abstracts in English
Yuguchi, Takashi*; Ishibashi, Kozue*; Sakata, Shuhei*; Yokoyama, Tatsunori; Ito, Daichi*; Ogita, Yasuhiro; Yagi, Koshi*; Ono, Takeshi*
Lithos, 372-373, p.105682_1 - 105682_9, 2020/11
Times Cited Count：3 Percentile：14.2(Geochemistry & Geophysics)Simultaneous determination of zircon U-Pb age and titanium concentration for a single analysis spot gives both the crystallization age and temperature. The crystallization age and temperature pairs in granitic zircons map the time-temperature () path of granitic magma before its solidification. In laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) analysis, it is challenging to quantitatively analyse a low level of titanium concentration. This study employed two approaches using a Quadrupole mass spectrometer equipped with a collision/reaction cell (CRC). The methods were applied to zircon samples of the Kurobegawa granite (KRG), the Okueyama granite (OKG), the Toki granite (TKG), and the Tono plutonic complex (TPC) and provided U-Pb ages and titanium concentrations consistent with previous studies. The crystallization ages and temperatures collected from individual analysis spots of zircon samples in the KRG, OKG, TKG, and TPC are plotted in the diagrams and enable us to characterize the rapid cooling paths at thermal conditions of zircon crystallization at the sampling sites.
Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Hanamuro, Takahiro; Shimada, Akiomi; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; et al.
JAEA-Research 2020-011, 67 Pages, 2020/10
JAEA-Research-2020-011.pdf:3.87MB
This annual report documents the progress of research and development (R&D) in the 5th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.
Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.
JAEA-Review 2020-010, 46 Pages, 2020/07
JAEA-Review-2020-010.pdf:1.89MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.
Niwa, Masakazu; Amamiya, Hiroki*; Yonaga, Yusuke; Ogita, Yasuhiro; Yasue, Kenichi*; Iwano, Hideki*; Danhara, Toru*; Hirata, Takafumi*
Chishitsugaku Zasshi, 126(5), p.267 - 283, 2020/05
U-Pb and fission-track (FT) ages from single zircon grain were measured for three tephra samples (TKB3, TKB6, and TKB7) intercalated in Neogene to Quaternary in Horonobe area, Hokkaido, to understand their depositional ages. In TKB3 and TKB6, weighed average U-Pb and FT ages for zircon grains within the youngest age range are coincident within a range of error 2 each other, which suggest that their ages correspond to the eruption ages. In TKB7, FT ages for most zircons are reset to their U-Pb ages or younger. The weighed average FT age for all analyzed zircons and weighed average U-Pb age for zircon grains within the youngest age range are coincident within a range of error 2 each other. Thus, their ages could also show the eruption age.
Yuguchi, Takashi*; Ogita, Yasuhiro; Kato, Takenori*; Yokota, Rintaro*; Sasao, Eiji; Nishiyama, Tadao*
Journal of Asian Earth Sciences, 192, p.104289_1 - 104289_16, 2020/05
Times Cited Count：5 Percentile：32.38(Geosciences, Multidisciplinary)Quartz from a granitic pluton is found to have formed through sequential growth events under different mechanisms and crystallization temperatures, which can provide new insights into magmatic processes of granitic magmas that were eventually consolidified into plutons. The events were identified using (1) the description of crystal shape and occurrence, (2) the study of the internal structure with cathodoluminescence (CL), and (3) derivation of the crystallization temperatures based on TitaniQ thermometry. The magmatic quartz crystals from the Toki granite, central Japan, are characterized as having the following internal structures: oscillatory zonation, no-oscillatory zonation with luminescence graduation (gradational zonation), and heterogeneous CL. The quartz crystals with oscillatory zonation were formed in the temperature range of about 800 C to below 700 C, which is referred to as oscillatory zoning temperature (OZT) conditions. The CL zonation pattern was controlled by the temperature conditions and titanium diffusivity in the melt (magma). The crystallization process of quartz within the Toki granite reveals the cooling processes of the granitic pluton; the lithofacies with a high frequency of oscillatory-zoned quartz underwent slower cooling under the OZT conditions than those in other lithofacies.
Ishimaru, Tsuneari; Ogata, Nobuhisa; Hanamuro, Takahiro; Shimada, Akiomi; Kokubu, Yoko; Asamori, Koichi; Niwa, Masakazu; Shimada, Koji; Watanabe, Takahiro; Sueoka, Shigeru; et al.
JAEA-Review 2019-010, 46 Pages, 2019/09
JAEA-Review-2019-010.pdf:2.45MB
This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency, in fiscal year 2019. The objectives and contents in fiscal year 2019 are described in detail based on the outline of 7 years plan (fiscal years 2015-2021). Background of this research is clarified with the necessity and the significance for site investigation and safety assessment, and the past progress in this report. In addition, the plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.
Yuguchi, Takashi*; Shobuzawa, Kaho*; Ogita, Yasuhiro*; Yagi, Koshi*; Ishibashi, Masayuki; Sasao, Eiji; Nishiyama, Tadao*
American Mineralogist, 104(4), p.536 - 556, 2019/04
Times Cited Count：17 Percentile：72.93(Geochemistry & Geophysics)This study describes the plagioclase alteration process with a focus on the role of micropores, mass transfer and reaction rate in the Toki granitic pluton, central Japan. The plagioclase alteration process involves albitization, K-feldspathization, and the formation of illite, calcite, fluorite and epidote. Such secondary minerals of hydrothermal origin in plagioclase within granitic rocks record the chemical characteristics of the hydrothermal fluid. Our results highlight (1) the nature of micropores such as distribution and volume in plagioclase, (2) the reaction nature of plagioclase alteration inferred by petrography and chemistry, (3) the physical conditions including alteration age and temperature, (4) the sequential variations of the fluid chemistry and (5) the mass transfer rate and reaction rate in the plagioclase alteration.
