Tracer diffusion coefficient measurements on NASICON-type Lithium-ion conductor LAGP using neutron radiography between 25C and 500C

Takagi, Honoka*; Yabutsuka, Takeshi*; Hayashida, Hirotoshi*; Song, F.; Kai, Tetsuya; Shinohara, Takenao; Kurita, Keisuke; Iikura, Hiroshi; Yamamoto, Norio*; Nakajima, Minoru*; et al.

Solid State Ionics, 417, p.116716_1 - 116716_7, 2024/12

https://doi.org/10.1016/j.ssi.2024.116716

In situ neutron imaging of lithium-ion batteries during heating to thermal runaway

Nozaki, Hiroshi*; Kondo, Hiroki*; Shinohara, Takenao; Setoyama, Daigo*; Matsumoto, Yoshihiro*; Sasaki, Tsuyoshi*; Isegawa, Kazuhisa*; Hayashida, Hirotoshi*

Scientific Reports (Internet), 13, p.22082_1 - 22082_8, 2023/12

https://doi.org/10.1038/s41598-023-49399-1

3D water management in polymer electrolyte fuel cells toward fuel cell electric vehicles

Yoshimune, Wataru*; Higuchi, Yuki*; Kato, Akihiko*; Hibi, Shogo*; Yamaguchi, Satoshi*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Shinohara, Takenao; Kato, Satoru*

ACS Energy Letters (Internet), 8(8), p.3485 - 3487, 2023/08

https://doi.org/10.1021/acsenergylett.3c01096

Development of spin-contrast-variation neutron powder diffractometry for extracting the structure factor of hydrogen atoms

Miura, Daisuke*; Kumada, Takayuki; Sekine, Yurina; Motokawa, Ryuhei; Nakagawa, Hiroshi; Oba, Yojiro; Ohara, Takashi; Takata, Shinichi; Hiroi, Kosuke; Morikawa, Toshiaki*; et al.

Journal of Applied Crystallography, 54(2), p.454 - 460, 2021/04

AA2020-0724.pdf:2.05MB

https://doi.org/10.1107/S1600576721000303

We developed a spin-contrast-variation neutron powder diffractometry technique that extracts the structure factor of hydrogen atoms, namely, the contribution of hydrogen atoms to a crystal structure factor. Crystals of L-glutamic acid were dispersed in a dpolystyrene matrix containing 4-methacryloyloxy-2,2,6,6,-tetramethyl-1-piperidinyloxy (TEMPO methacrylate) to polarize their proton spins dynamically. The intensities of the diffraction peaks of the sample changed according to the proton polarization, and the structure factor of the hydrogen atoms was extracted from the proton-polarization dependent intensities. This technique is expected to enable analyses of the structures of hydrogen-containing materials that are difficult to determine with conventional powder diffractometry.

Development and application of a He neutron spin filter at J-PARC

Okudaira, Takuya; Oku, Takayuki; Ino, Takashi*; Hayashida, Hirotoshi*; Kira, Hiroshi*; Sakai, Kenji; Hiroi, Kosuke; Takahashi, Shingo*; Aizawa, Kazuya; Endo, Hitoshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

https://doi.org/10.1016/j.nima.2020.164301

Atmospheric modeling of Cs plumes from the Fukushima Daiichi Nuclear Power Plant; Evaluation of the model intercomparison data of the Science Council of Japan

Kitayama, Kyo*; Morino, Yu*; Takigawa, Masayuki*; Nakajima, Teruyuki*; Hayami, Hiroshi*; Nagai, Haruyasu; Terada, Hiroaki; Saito, Kazuo*; Shimbori, Toshiki*; Kajino, Mizuo*; et al.

Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07

https://doi.org/10.1029/2017JD028230

We compared seven atmospheric transport model results for Cs released during the Fukushima Daiichi Nuclear Power Plant accident. All the results had been submitted for a model intercomparison project of the Science Council of Japan in 2014. We assessed model performance by comparing model results with observed hourly atmospheric concentrations of Cs, focusing on nine plumes over the Tohoku and Kanto regions. The results showed that model performance for Cs concentrations was highly variable among models and plumes. We also assessed model performance for accumulated Cs deposition. Simulated areas of high deposition were consistent with the plume pathways, though the models that best simulated Cs concentrations were different from those that best simulated deposition. The ensemble mean of all models consistently reproduced Cs concentrations and deposition well, suggesting that use of a multimodel ensemble results in more effective and consistent model performance.

Deformation analysis of reinforced concrete using neutron imaging technique

Koyama, Taku*; Ueno, Kazuki*; Sekine, Mariko*; Matsumoto, Yoshihiro*; Kai, Tetsuya; Shinohara, Takenao; Iikura, Hiroshi; Suzuki, Hiroshi; Kanematsu, Manabu*

Materials Research Proceedings, Vol.4, p.155 - 160, 2018/05

https://doi.org/10.21741/9781945291678-24

Non-aqueous selective synthesis of orthosilicic acid and its oligomers

Igarashi, Masayasu*; Matsumoto, Tomohiro*; Yagihashi, Fujio*; Yamashita, Hiroshi*; Ohara, Takashi; Hanashima, Takayasu*; Nakao, Akiko*; Moyoshi, Taketo*; Sato, Kazuhiko*; Shimada, Shigeru*

Nature Communications (Internet), 8, p.140_1 - 140_8, 2017/07

https://doi.org/10.1038/s41467-017-00168-5

A Study of the evaluation of the excavation damaged zone in the Horonobe Underground Research Laboratory, 2; Investigation in the 250 m gallery (Joint research)

Aoyagi, Kazuhei; Kubota, Kenji*; Nakata, Eiji*; Suenaga, Hiroshi*; Nohara, Shintaro*

JAEA-Research 2017-004, 91 Pages, 2017/06

JAEA-Research-2017-004.pdf:6.07MB

In this study, we performed seismic tomography, seismic refraction survey, resistivity tomography, and hydraulic tests to investigate the hydro-mechanical property of the excavation damaged zone (EDZ) in the 250 m gallery of the Horonobe Underground Research Laboratory. As a result of seismic tomography, seismic velocity is significantly decreased within 1 m from the gallery wall. The decrease of seismic velocity is related to the density of fracture induced around the gallery wall as a result of the gallery excavation. Thus the extent of the fractures induced by gallery excavation, i.e., EDZ fractures is clarified to be within 1.0 m from the gallery wall. The enhanced hydraulic conductivity was detected within 0.5 to 1.0 m from the gallery wall on the basis of the result of hydraulic tests. This is almost consistent with the extent of the region that seismic velocity is significantly decreased. Therefore, it is estimated that EDZ fractures induced around the gallery leads to the increase of hydraulic conductivity. In addition, the desaturation zone around the gallery is not induced as a result of resistivity tomography. From these results, the hydro-mechanical property of the EDZ is clarified in detail. Also, the in situ tests and evaluation method applied in this study are appropriate to investigate the EDZ in detail.

Corium stratification test using intermediate products of degraded core materials in severe accident of BWR

Tokushima, Kazuyuki; Shirasu, Noriko; Hoshino, Kuniyoshi*; Ohara, Hiroshi*; Kurata, Masaki

Proceedings of Annual Topical Meeting on LWR Fuels with Enhanced Safety and Performance (TopFuel 2016) (USB Flash Drive), p.1055 - 1063, 2016/09

At the fuel assembly degradation stage in severe accidents, chemical features of the intermediate products are expected to be changed depending upon the accident progressions. These differences are originated from the differences in oxygen potential and temperature, and are highly important for evaluating the relocation and stratification progress of the fuel debris. Two types of sim-test with the different oxygen potentials were performed to investigate these tendencies. The chemical features of the intermediate materials used in the tests were determined from the observations for the control blade and channel box degradation in our previous study. The present results indicate that the U concentration in the metallic layer is largely varied depending upon the oxygen potential of the atmosphere. Also, when the BC-Fe alloy, as of a typical intermediate product, coexists with UO and Zr, the apparent red-ox reaction rate between UO and Zr are mitigated.