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Abe, Takumi; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
Progress in Nuclear Science and Technology (Internet), 7, p.299 - 304, 2025/05
Currently, much research continues on stable energy sources that do not emit CO in order to achieve a carbon-neutral and sustainable society. Nuclear energy is one of the such sources, and various new reactors and reprocessing technologies are being developed. In order to implement the nuclear fuel cycle with these technologies, a nuclear fuel cycle simulator is required to quantitatively evaluate various quantities, such as the distribution of nuclear fuel materials and the scale of waste loading. For this purpose, NMB4.0 was developed in collaboration with Tokyo Institute of Technology and Japan Atomic Energy Agency. This code calculates the material balance of 179 nuclides including actinides and fission products (FPs) from the front-end to the back-end and simulates the nuclear fuel cycle in an integrated manner. Unlike other nuclear fuel cycle simulators, the code is capable of performing precise back-end analyses such as the number of radioactive wastes and the scale of the geological repository considering heat generation of waste package under diverse nuclear energy scenario, and is an open source code that runs on Microsoft Excel. By these features, it is possible to quantitatively study nuclear energy utilization strategies with various stakeholders. The presentation will detail the numerical model used in NMB4.0.
Pyeon, C. H.*; Oizumi, Akito; Katano, Ryota; Fukushima, Masahiro
Nuclear Science and Engineering, 199(3), p.429 - 444, 2025/03
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Experimental analyses of neptunium-237 (Np), americium-241 (
Am), and
Am fission and
Np capture reaction rates are conducted by the Serpent 2 code together with ENDF/B-VIII.0 and JENDL-5, using experimental data at neutron spectra of thermal and intermediate regions obtained in the solid-moderated and solid-reflected cores with highly-enriched uranium fuel at the Kyoto University Critical Assembly. Also, uncertainty quantification of fission and capture reaction rate ratios of test samples of
Np,
Am and
Am with reference samples of uranium-235 (
U) and gold-197 (
Au) are evaluated by the MARBLE code system. In terms of fission reaction rate ratios of
Np/
U,
Am/
U and
Am/
U, a comparison between experiments and Serpent 2 calculations shows an accuracy about 5, 15 and 10%, respectively, together with ENDF/B-VIII.0 and JENDL-5. For capture reaction rate ratios of
Np/
Au, Serpent 2 calculations reveal a fairly good accuracy at the thermal neutron spectrum. The total uncertainties of
Np/
U,
Am/
U and
Am/
U fission reaction rate ratios by MARBLE with the covariance data of ENDF/B-VIII.0 and JENDL-5 are found to be about 4% at most in all cores, except for about 8% of
Am/
U with ENDF/B-VIII.0 at the intermediate neutron spectrum.
Oizumi, Akito
Dai-45-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2024/11
When a domestic reprocessing plant starts operation, differences in the estimated Pu amount between the electric utility that manages the discharge of spent MOX fuel from LWRs and the reprocessing plant that received it may affect safeguards reliability. In this study, the uncertainties in the estimated Pu amount caused by nuclear data covariance were quantitatively determined by burn-up sensitivity analysis. In addition, the recommended verification frequency of the Pu amount was discussed by estimating the Pu amount that may be undeclared, using the quantified uncertainty caused by nuclear data covariance. As a result, the quantified uncertainty of the Pu amount caused by the nuclear data covariance was estimated to be 1.58%, and the verification frequency based on this was evaluated once every two weeks or more. More discussion including measurement error is necessary to estimate a more effective verification frequency.
Oizumi, Akito; Fukushima, Masahiro; Gunji, Satoshi; McKenzie, G.*; Amundson, K.*
International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook (2022/23 edition) (Internet) , 313 Pages, 2024/11
This benchmark report was compiled to register a critical experiment using the lower-enriched uranium (LEU) system core to the International Criticality Safety Evaluation Project (ICSBEP). The LEU experiment was one of a series of joint experimental project with the Los Alamos Laboratory in the United States from 2015 to 2019 aimed at improving the design accuracy of the accelerator driven system (ADS). This core was loaded alternating highly-enriched uranium (HEU) and natural uranium (NU) to simulate LEU. In addition, a fast neutron spectrum system was constructed with not only HEU and NU but also lead which is part of coolant in the ADS. In this evaluation, it was clarified that the experimental uncertainty for the effective multiplication factor was almost 100 pcm. Moreover, the C/E-1 values of almost -70 pcm and -145 pcm were obtained by the calculation with the continuous energy Monte Carlo code MCNP and the nuclear data ENDF/B-VIII.0 and JENDL-4.0, respectively.
Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro; Pyeon, C. H.*; Yamamoto, Akio*; Endo, Tomohiro*
Nuclear Science and Engineering, 198(6), p.1215 - 1234, 2024/06
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)In this study, we have demonstrated that data assimilation using lead and bismuth sample reactivities measured in the Kyoto University Critical Assembly A-core can successfully reduce the uncertainty of the coolant void reactivity in accelerator-driven systems derived from inelastic-scattering cross-sections of lead and bismuth. We re-evaluated and highlighted the experimental uncertainties and correlations of the sample reactivities for the data assimilation formula. We used the MCNP6.2 code to evaluate the sample reactivities and their uncertainties, and performed data assimilation using the reactor analysis code system MARBLE. The high-sensitivity coefficients of the sample reactivities to lead and bismuth allowed us to reduce the cross-section-induced uncertainty of the void reactivity of the accelerator-driven system from 6.3% to 4.8%, achieving a provisional target accuracy of 5% in this study. Furthermore, we demonstrated that the uncertainties arising from other dominant factors, such as minor actinides and steel, can be effectively reduced by using integral experimental data sets for the unified cross-section dataset ADJ2017.
Tada, Kenichi; Nagaya, Yasunobu; Taninaka, Hiroshi; Yokoyama, Kenji; Okita, Shoichiro; Oizumi, Akito; Fukushima, Masahiro; Nakayama, Shinsuke
Journal of Nuclear Science and Technology, 61(1), p.2 - 22, 2024/01
Times Cited Count:12 Percentile:96.41(Nuclear Science & Technology)The new version of the Japanese evaluated nuclear data library, JENDL-5, was released in December 2021. This paper demonstrates the validation of JENDL-5 for fission reactor applications. Benchmark calculations are performed with the continuous-energy Monte Carlo codes MVP and MCNP and the deterministic code system MARBLE. The benchmark calculation results indicate that the performance of JENDL-5 for fission reactor applications is better than that of the former library JENDL-4.0.
Oizumi, Akito; Akie, Hiroshi
JAEA-Technology 2023-017, 93 Pages, 2023/12
After the decision of decommissioning JMTR (Japan Materials Testing Reactor), Japan Atomic Energy Agency investigated the possibility to construct a new irradiation test reactor to succeed JMTR (post-JMTR), and the final report of the investigated result was submitted to the Ministry of Education, Culture, Sports, Science and Technology on March 30th 2021. This investigation was carried out in 4 steps of (1) selection of reactor type, (2) reactor core plans studies, (3) neutronic studies, (4) thermal studies, and was finally (5) considered and evaluated. This JAEA-Technology report summarizes the process and the results of (3) neutronic studies. Neutron fluxes were calculated at irradiation sample positions in the investigated cores, the standard core and the compact core, and the calculated fluxes satisfied the required irradiation capability. It was also evaluated the two investigated cores' continuous reactor operation time in days in one refueling cycle, and the results guaranteed an operation days equality with that of existing JMTR. In addition, neutronic characteristics of the cores were estimated, such as power distribution in the core, control rod reactivity worth, reactivity coefficients, distribution of fuel burnup rate of each fuel element, and kinetics parameters. The evaluated neutronic characteristics were used in the post-JMTR final investigation report to confirm the neutronic feasibility by comparing with the neutronic limiting values of existing JMTR, and to estimate the cooling capability to make the core thermally feasible.
Oizumi, Akito; Sagara, Hiroshi*
Dai-44-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2023/11
Research and development of transuranium (TRU) fuel cycles with accelerator drive systems (ADSs) transmuting minor actinides separated from the commercial cycles has been continuously conducted to reduce the high-level radioactive waste contained in spent fuel discharged from nuclear power plants. Since ADS could be misused to illegally produce Pu by using neutrons generated by the accelerator, a different approach from a conventional nuclear reactor would be needed. In this study, we have analyzed possible misuse scenarios of ADS quantitatively evaluated Pu that can be illegally produced within the design tolerance of ADS, and evaluated the effects of the Dual Containment and Surveillance(C/S) and the design information verification methods. As a result, it was quantitatively clarified that 10-60 kg of Pu could be generated clandestinely, and the dual C/S and design information verification with monitoring of the operation history of both accelerators and reactors could detect and prevent all the misuse scenarios effectively.
Pyeon, C. H.*; Katano, Ryota; Oizumi, Akito; Fukushima, Masahiro
Nuclear Science and Engineering, 197(11), p.2902 - 2919, 2023/11
Times Cited Count:2 Percentile:46.61(Nuclear Science & Technology)Sample reactivity and void reactivity experiments are carried out in the solid-moderated and solid-reflected cores at the Kyoto University Critical Assembly (KUCA) with the combined use of aluminum (Al), lead (Pb) and bismuth (Bi) samples, and Al spacers simulating the void. MCNP6.2 eigenvalue calculations together with JENDL-4.0 provide good accuracy of sample reactivity with the comparison of experimental results; also experimental void reactivity is attained by using MCNP6.2 together with JENDL-4.0 and ENDF/B-VII.1 with a marked accuracy of relative difference between experiments and calculations. Uncertainty quantification of sample reactivity and void reactivity is acquired by using the sensitivity coefficients based on MCNP6.2/ksen and covariance library data of SCALE6.2 together with ENDF/B-VII.1, arising from the impact of uncertainty induced by Al, Pb and Bi cross sections. A series of reactivity analyses with the Al spacer simulating the void demonstrates the means of analyzing the void in the solid-moderated and solid-reflected cores at KUCA
Oizumi, Akito
Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 10 Pages, 2023/10
Research and development of the transuranium fuel cycle with accelerator-drive systems (ADSs) transmuting minor actinides (MAs) separated from commercial cycles has been continuously conducted by the Japan Atomic Energy Agency (JAEA) to reduce the high-level radioactive waste contained in the spent fuel discharged from nuclear power plants. To transmute MA with high efficiency, the ADS fuel contains a large amount of MA. The criticality safety design of facilities within the ADS cycle must rely on calculated values using the nuclear data library because there are no experimental or measured values for the critical mass of many MAs. Thus, it is crucial to figure out the impact of updating the evaluated nuclear data library on the critical mass calculation. This study compared the differences in the calculated critical masses of a bare metal sphere (BCMs) for each actinide isotope between two version of Japanese Evaluated Nuclear Data Library, JENDL-5 (released in December 2021) and JENDL-4.0 as a basic assessment. The study found that the differences in BCMs between JENDL-5 and JENDL-4.0 were less than 1% for U,
U,
Np, and
Pu, which have the integral experimental data for metallic spheres registered in the International Criticality Safety Benchmark Evaluation Project (ICSBEP). On the other hands, the difference in BCMs between two nuclear data libraries was found to be almost 7-40% for nuclides such as
Am,
Am,
Cm, and
Cm, which have relatively limited or no integral experimental data registered in ICSBEP and International Handbook of Evaluated Reactor Physics Benchmark Experiments (IRPhEP). Furthermore, as a result of analyzing the nuclear data that influenced the difference in BCM, for example in the case of
Cm, it was clarified that the update of fission reaction and prompt
gave a significant contribution.
Okamura, Tomohiro*; Katano, Ryota; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
Journal of Nuclear Science and Technology, 60(6), p.632 - 641, 2023/06
Times Cited Count:3 Percentile:42.88(Nuclear Science & Technology)The Okamura explicit method (OEM) for depletion calculation was developed by modifying the matrix exponential method for dynamic nuclear fuel cycle simulation. The OEM suppressed the divergence of the calculation for short half-life nuclides, even for long time steps. The computational cost of the OEM was small, equivalent to the Euler method, and it maintained sufficient accuracy for the fuel cycle simulation.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Nagaya, Yasunobu; Tada, Kenichi; et al.
EPJ Web of Conferences, 284, p.14001_1 - 14001_7, 2023/05
Times Cited Count:2 Percentile:86.54(Nuclear Science & Technology)Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.
EPJ Web of Conferences, 284, p.01023_1 - 01023_4, 2023/05
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron, lead, and bismuth have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics. The measured TTNYs and DDXs were compared with calculations by the Monte Carlo transport code PHITS with its default physics model of INCL version 4.6 combined with GEM and those with the JENDL-4.0/HE nuclear data library.
Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.
Journal of Nuclear Science and Technology, 60(4), p.435 - 449, 2023/04
Times Cited Count:4 Percentile:53.26(Nuclear Science & Technology)Double-differential thick target neutron yields (TTNYs) for Fe, Pb, and Bi targets induced by 107-MeV protons were measured using the fixed-field alternating gradient accelerator at Kyoto University for research and development of accelerator-driven systems (ADSs) and fundamental ADS reactor physics research at the Kyoto University Critical Assembly (KUCA). Note that TTNYs were obtained with the time-of-flight method using a neutron detector system comprising eight neutron detectors; each detector has a small NE213 liquid organic scintillator and photomultiplier tube. The TTNYs obtained were compared with calculation results using Monte Carlo-based spallation models (i.e., INCL4.6/GEM, Bertini/GEM, JQMD/GEM, and JQMD/SMM/GEM) and the evaluated high-energy nuclear data library, i.e., JENDL-4.0/HE, implemented in the particle and heavy iontransport code system (PHITS). All models, including JENDL-4.0/HE, failed to predict high-energy peaks at a detector angle of 5. Comparing the energy- and angle-integrated spallation neutron yields at energies of
20 MeV estimated using the measured TTNYs and the PHITS indicated that INCL4.6/GEM would be suitable for the Monte Carlo transport simulation of ADS reactor physics experiments at the KUCA.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Abe, Yutaka*; Tsubakihara, Kosuke*; Okumura, Shin*; Ishizuka, Chikako*; Yoshida, Tadashi*; et al.
Journal of Nuclear Science and Technology, 60(1), p.1 - 60, 2023/01
Times Cited Count:202 Percentile:99.98(Nuclear Science & Technology)Iwamoto, Hiroki; Meigo, Shinichiro; Nakano, Keita*; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; et al.
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.404 - 409, 2023/01
no abstracts in English
Oizumi, Akito; Sagara, Hiroshi*
Dai-43-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2022/11
Research and development of partitioning and transmutation cycle with accelerator drive systems (ADSs) transmuting minor actinides separated from the commercial cycles has been continuously conducted to reduce the high-level radioactive waste contained in spent fuel discharged from nuclear power plants. Since the chemical form and composition of the fuels are different from those of the current commercial cycles, it is necessary to examine the inspection goal of the safeguards and the design level of physical protections which are required for the partitioning and transmutation (P&T) cycle. In previous studies, the (
) of the uranium (U) in the ADS fuel with a unique isotopic composition was evaluated as 2, the second highest on a 4-point scale, assuming state actors. In this study, reduction methods of potential nuclear proliferation were examined for the rationalization of the P&T cycle design considering nuclear non-proliferation. The amount of recovered U (RepU) added to the ADS fuel, which was required to increase the bare critical mass of U, was quantitatively evaluated as one of the reduction methods of potential nuclear proliferation risk. As a result, the addition of RepU, which was about 1.3- 2.7 times U in the ADS fuel, lowered the
to 3 - 4. The rationalization of the P&T cycle design based on the safeguards by design can be expected by reviewing the U decontamination standards in the reprocessing steps of the commercial cycle based on these quantitative data.
Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; Nishio, Katsuhisa; et al.
JAEA-Conf 2022-001, p.129 - 133, 2022/11
For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors composed of the NE213 liquid organic scintillators and photomultiplier tubes, which were connected to a multi-channel digitizer mounted with a field-programmable gate array (FPGA), for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination applying the gate integration method to the FPGA. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics.
Oizumi, Akito; Sugawara, Takanori; Sagara, Hiroshi*
Annals of Nuclear Energy, 169, p.108951_1 - 108951_9, 2022/05
Times Cited Count:2 Percentile:29.47(Nuclear Science & Technology)Research and development of the partitioning and transmutation (P&T) cycle with accelerator-drive systems (ADSs) transmuting minor actinides separated from the commercial cycles have been continuously conducted to reduce the amount of high-level radioactive waste contained in spent fuel discharged from nuclear power plants. Because the chemical form and composition of the fuels are different from those of the current commercial cycles, it is necessary to examine the inspection goal of the safeguards (SGs) and the design level of physical protections (PPs) that are required for the P&T cycle. In this study, the material attractiveness was evaluated assuming the theft or diversion of fuel assemblies from the fuel storage pool of the ADS facility in terms of nuclear security and non-proliferation. According to the results, quantitative components based on the fundamental fuel property were created as an important factor to decide the inspection goal for SGs and the design level for PPs required for the ADS facility. Additionally, the attractiveness of mixed oxide (MOX) fuel assemblies stored in the commercial boiling water reactor (BWR) facility was compared with that of the ADS. With regard to nuclear security, the ADS fuel was less attractive than the BWR MOX in every cycle. Regarding nuclear non-proliferation, the ADS fuel assembly had less attractive plutonium (Pu) than the BWR MOX, and the uranium (U) in the ADS fuel assembly was as attractive as (or slightly more attractive than) that of the BWR MOX owing to low spontaneous fission neutron. Furthermore, new issues were identified through this evaluation. With the current regulations, it was difficult to decide whether the ADS fuel before irradiation should be treated as fresh or spent, because the ADS fresh fuel contained more transuranium and rare earth than U and contained U whose main component was U-234 instead of U-238.
Okamura, Tomohiro*; Nishihara, Kenji; Katano, Ryota; Oizumi, Akito; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
JAEA-Data/Code 2021-016, 43 Pages, 2022/03
The quantitative prediction and analysis of the future nuclear energy utilization scenarios are required in order to establish the advanced nuclear fuel cycle. However, the nuclear fuel cycle consists of various processes from front- to back-end, and it is difficult to analyze the scenarios due to the complexity of modeling and the variety of scenarios. Japan Atomic Energy Agency and Tokyo Institute of Technology have jointly developed the NMB code as a tool for integrated analysis of mass balance from natural uranium needs to radionuclide migration of geological disposal. This user manual describes how to create a database and scenario input for the NMB version 4.0.