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Toyoda, Shin*; Inoue, Kazuhiko*; Yamaguchi, Ichiro*; Hoshi, Masaharu*; Hirota, Seiko*; Oka, Toshitaka; Shimazaki, Tatsuya*; Mizuno, Hideyuki*; Tani, Atsushi*; Yasuda, Hiroshi*; et al.
Radiation Protection Dosimetry, 199(14), p.1557 - 1564, 2023/09
Times Cited Count：2 Percentile：25.59(Environmental Sciences)Interlaboratory comparison studies are important for radiation dosimetry in order to demonstrate how the technique is universally available. The set of standard samples are examined in each participating laboratory in the present study. After a set of standard samples together with the samples with unknown doses, which were prepared in the same laboratory as the standard samples, are measured at a participating laboratory, those samples are sent to another participating laboratory for next measurement. There is some small difference observed in the sensitivity (the slope of the dose response line) of the standard samples while the differences in the obtained doses for the samples with unknown doses are rather systematic, implying that the difference is mostly due to the samples but not to measurements.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
Radiation Protection Dosimetry, 199(14), p.1620 - 1625, 2023/09
Times Cited Count：2 Percentile：25.59(Environmental Sciences)We have been conducting dose assessments for Japanese macaques captured in Fukushima to reveal radiobiological effects on the low-dose expose animals. To accurately determine the external exposure dose, it is desirable to examine the analysis of the CO
radical intensity. We examined ESR spectra of teeth of 10 macaques captured in Fukushima by two spectrum-decomposition algorithms.
Okutsu, Kenichi*; Yamashita, Takuma*; Kino, Yasushi*; Miyashita, Konan*; Yasuda, Kazuhiro*; Oka, Toshitaka; Okada, Shinji*; Sato, Motoyasu*
JJAP Conference Proceedings (Internet), 9, p.011003_1 - 011003_7, 2023/00
Muon catalyzed fusion (
CF) is a cyclic reaction where a negatively charged muon itself acts like a catalyst of nuclear fusion between hydrogen isotopes. In the CF reaction, muon transfer from deuteron to triton and muonic molecular formation are rate-limiting processes. In this work, we have investigated the role of resonance states of muonic molecule in the CF which affects the muonic deuterium atom population. Solving simultaneous rate equations numerically by the fourth-order Runge-Kutta method, we determined the muonic molecular formation rate so that the number of fusion events reproduces a latest experimental result. It is revealed that the resonance states play a role to enhance the fusion rate by accelerating the de-excitation of the muonic atoms.
Ishikawa, Ryoya*; Suzuki, Masatoshi*; Kino, Yasushi*; Endo, Satoru*; Nakajima, Hiroo*; Oka, Toshitaka; Takahashi, Atsushi*; Shimizu, Yoshinaka*; Suzuki, Toshihiko*; Shinoda, Hisashi*; et al.
KEK Proceedings 2022-2, p.61 - 66, 2022/11
The balance between oxidative stress and antioxidant activity, which is a defense mechanism against oxidative stress, was investigated in the liver and bladder of wild Japanese macaques captured in Fukushima Prefecture. No significant induction of oxidative stress by exposure to environmental radionuclides after the Fukushima nuclear accident was observed, suggesting that the stress defense mechanism of the organism is activated in some organs.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
KEK Proceedings 2022-2, p.120 - 125, 2022/11
We investigate the effect of sample's anisotropy and measurement condition to obtain the higher reproducibility for the shape of the ESR spectrum and the intensity of CO radical.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2021-2, p.91 - 96, 2021/12
We examined whether the ESR dose estimation method could be applied to wild Japanese macaque. In this work, we investigated the enamel preparation protocol and the analytical method of the ESR spectra.
Okutsu, Kenichi*; Yamashita, Takuma*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
Fusion Engineering and Design, 170, p.112712_1 - 112712_4, 2021/09
Times Cited Count：5 Percentile：38.44(Nuclear Science & Technology)A muonic molecule which consists of two hydrogen isotope nuclei (deuteron (d) or tritium (t)) and a muon decays immediately via nuclear fusion and the muon will be released as a recycling muon, and start to find another hydrogen isotope nucleus. The reaction cycle continues until the muon ends up its lifetime of 2.2 s. Since the muon does not participate in the nuclear reaction, the reaction is so called a muon catalyzed fusion (CF). The recycling muon has a particular kinetic energy (KE) of the muon molecular orbital when the nuclear reaction occurs. Since the KE is based on the unified atom limit where distance between two nuclei is zero. A precise few-body calculation estimating KE distribution (KED) is also in progress, which could be compared with the experimental results. In the present work, we observed recycling muons after CF reaction.
Yamashita, Takuma*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
Fusion Engineering and Design, 169, p.112580_1 - 112580_5, 2021/08
Times Cited Count：4 Percentile：31.16(Nuclear Science & Technology)A muon () having 207 times larger mass of electron and the same charge as the electron has been known to catalyze a nuclear fusion between deuteron (d) and triton (t). These two nuclei are bound by and form a muonic hydrogen molecular ion, dt. Due to the short inter-nuclear distance of dt, the nuclear fusion, d +t
+ n + 17.6 MeV, occurs inside the molecule. This reaction is called muon catalyzed fusion (CF). Recently, the interest on CF is renewed from the viewpoint of applications, such as a source of high-resolution muon beam and mono-energetic neutron beam. In this work, we report a time evolution calculation of CF in a two-layered hydrogen isotope target.
Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I.-H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.
IEEE Transactions on Applied Superconductivity, 31(5), p.2101704_1 - 2101704_4, 2021/08
Times Cited Count：4 Percentile：21.43(Engineering, Electrical & Electronic)A superconducting transition-edge sensor (TES) microcalorimeter is an ideal X-ray detector for experiments at accelerator facilities because of good energy resolution and high efficiency. To study the performance of the TES detector with a high-intensity pulsed charged-particle beam, we measured X-ray spectra with a pulsed muon beam at the Japan Proton Accelerator Research Complex (J-PARC) in Japan. We found substantial temporal shifts of the X-ray energy correlated with the arrival time of the pulsed muon beam, which was reasonably explained by pulse pileup due to the incidence of energetic particles from the initial pulsed beam.
X raysOkumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.
Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07
Times Cited Count：24 Percentile：78.88(Physics, Multidisciplinary)We observed electronic X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic 
and 
X rays together with the hypersatellite X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the 
-shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic - and -shell hole production and their temporal evolution during the muon cascade process.
Miyashita, Konan*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
To observe a kinetic energy distribution of a recycling muon emitted after CF reaction, it is necessary to guide the recycling muons to a detector. In this work, we simulated the muon transportation using PHITS code and designed an experimental system.
Nakashima, Ryota*; Okutsu, Kenichi*; Kino, Yasushi*; Miyashita, Konan*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
The recycling muon emitted after the muon catalized fusion (CF) has a kinetic energy between a few keV to 10 keV. To observed the kinetic energy distribution of the recycling muon, we have to guide and inject muons to Ti foil, and measure the muonic X-ray. In this work, we utilized SIMION code to calculate the electric field and the trajectory of muons from deuteron target to Ti foil.
Miyashita, Konan*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
To measure the kinetic energy of a recycling muon, we discussed how to reduce the background radiation and the trajectory of the transported recycling muons by simulation code.
Nakashima, Ryota*; Okutsu, Kenichi*; Kino, Yasushi*; Miyashita, Konan*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
To detect a recycling muon emitted after muon catalyzed fusion reaction, it is necessary to guide the recycling muons from the target to a detector in a low background area. In this work, we simulated the muon transportation using SIMONS and PHITS codes and designed an experimental system.
Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
A muon is one of elementary particles which is known to weight 207 times more than an electron. A nuclear fusion reaction occurs in a muonic molecule which consists of two hydrogen isotope nuclei and a muon because the muon binds more tightly than electron. Since the muon does not directly participate in the fusion reaction, the reaction is called muon catalyzed fusion (CF). The muon released after the reaction is called a "recycling muon", and maintains the molecular orbital information when the muonic molecule formed. Therefore, information of the muon wavefunction can be investigated by observing the energy distribution of the recycling muon. We will report the experimental setup for measuring the energy distribution of the recycling muons after the nuclear reaction.
Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Fujiwara, Kenso; Terashima, Motoki; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Yamashita, Takuma*; et al.
no journal, ,
We demonstrated a method of 
Sr measurement in small pieces of hard tissues with radioactivity measurement or ICP-MS measurement. Interference elements of the measurements were removed by chemical separation. We could determine Sr in 0.1 g of hard tissues by radioactivity measurement method and ICP-MS method. Limit of detection of the ICP-MS method was lower than that of the radioactivity measurement. The ICP-MS method is adequate method for distribution analysis of Sr in the hard tissues.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
no journal, ,
The Fukushima Daiichi Nuclear Power Plant (FDNPP) accident in 2011 resulted in a release of radionuclides into the environment and caused chronic low-dose-rate exposure to wildlife there. Studies of the radiobiological effects by the chronic low-dose-rate exposure was limited and there is a need for accurate determination of exposure doses and further studies of radiation effects by FDNPP accident. We determined dose of wild animals mainly captured in Namie Town, Fukushima Prefecture from the CO
radical intensities in tooth enamel by an electron spin resonance dosimetry.
Yamashita, Takuma*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
A muon () having 207 times larger mass of electron and the same charge as the electron has been known to catalyze a nuclear fusion (CF) between deuteron (d) and triton (t). In this work, we have solved simultaneous reaction rate equations by the 4th-order Runge-Kutta method for the jointed CF cycles in the two layers (H/D and D/T). The T concentration to maximize the intensities of fusion neutrons and muons emitted to the vacuum will be discussed.
CF experiment at J-PARC MLFNatori, Hiroaki*; Doiuchi, Shogo*; Ishida, Katsuhiko*; Kino, Yasushi*; Miyake, Yasuhiro*; Miyashita, Konan*; Nakashima, Ryota*; Nagatani, Yukinori*; Nishimura, Shoichiro*; Oka, Toshitaka; et al.
no journal, ,
A muonic molecule which consists of muon and two hydrogen isotope nuclei (deuteron (d) or tritium (t)) decays immediately via nuclear fusion (
CF) and the muon will be released as a recycling muon. We attempted to use these muons to develop the scanning muon microscope. In this work, we will report the detection of neutron which emits during the CF reaction.
Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Yamashita, Takuma*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
no journal, ,
Muon catalized fusion (CF) is expected to be a high-quality muon beam source for undestructive measurement and a monoenergetic neutron source. In this work, we attemped to observe a released muon after intermolecular nuclear reaction using muonic X-ray.
