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Ikeuchi, Hirotomo; Sasaki, Shinji; Onishi, Takashi; Nakayoshi, Akira; Arai, Yoichi; Sato, Takumi; Ohgi, Hiroshi; Sekio, Yoshihiro; Yamaguchi, Yukako; Morishita, Kazuki; et al.
JAEA-Data/Code 2023-005, 418 Pages, 2023/12
JAEA-Data-Code-2023-005-01.pdf:24.59MBJAEA-Data-Code-2023-005-02.pdf:32.18MB
For safe and steady decommissioning of Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station (1F), information concerning composition and physical/chemical properties of fuel debris generated in the reactors should be estimated and provided to other projects conducting the decommissioning work including the retrieval of fuel debris and the subsequent storage. For this purpose, in FY2021, samples of contaminants (the wiped smear samples and the deposits) obtained through the internal investigation of the 1F Unit 2 were analyzed to clarify the components and to characterize the micro-particles containing uranium originated from fuel (U-bearing particles) in detail. This report summarized the results of analyses performed in FY2021, including the microscopic analysis by SEM and TEM, radiation analysis, and elemental analysis by ICP-MS, as a database for evaluating the main features of each sample and the probable formation mechanism of the U-bearing particles.
Ikeuchi, Hirotomo; Koyama, Shinichi; Osaka, Masahiko; Takano, Masahide; Nakamura, Satoshi; Onozawa, Atsushi; Sasaki, Shinji; Onishi, Takashi; Maeda, Koji; Kirishima, Akira*; et al.
JAEA-Technology 2022-021, 224 Pages, 2022/10
JAEA-Technology-2022-021.pdf:12.32MB
A set of technology, including acid dissolving, has to be established for the analysis of content of elements/nuclides in the fuel debris samples. In this project, a blind test was performed for the purpose of clarifying the current level of analytical accuracy and establishing the alternative methods in case that the insoluble residue remains. Overall composition of the simulated fuel debris (homogenized powder having a specific composition) were quantitatively determined in the four analytical institutions in Japan by using their own dissolving and analytical techniques. The merit and drawback for each technique were then evaluated, based on which a tentative flow of the analyses of fuel debris was constructed.
= 
one-dimensional Ising-like antiferromagnet BaCo
VO
Kimura, Shojiro*; Onishi, Hiroaki; Okutani, Akira*; Akaki, Mitsuru*; Narumi, Yasuo*; Hagiwara, Masayuki*; Okunishi, Koichi*; Kindo, Koichi*; He, Z.*; Taniyama, Tomoyasu*; et al.
Physical Review B, 105(1), p.014417_1 - 014417_9, 2022/01
Times Cited Count：3 Percentile：34.67(Materials Science, Multidisciplinary)Koyama, Shinichi; Nakagiri, Toshio; Osaka, Masahiko; Yoshida, Hiroyuki; Kurata, Masaki; Ikeuchi, Hirotomo; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Takano, Masahide; et al.
Hairo, Osensui Taisaku jigyo jimukyoku Homu Peji (Internet), 144 Pages, 2021/08
JAEA performed the subsidy program for the "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy and Thermal Behavior Estimation of Fuel Debris))" in 2020JFY. This presentation summarized briefly the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning and Contaminated Water Management.
=1/2 one-dimensional Ising-like antiferromagnet BaCoVO in transverse magnetic fieldsOkutani, Akira*; Onishi, Hiroaki; Kimura, Shojiro*; Takeuchi, Tetsuya*; Kida, Takanori*; Mori, Michiyasu; Miyake, Atsushi*; Tokunaga, Masashi*; Kindo, Koichi*; Hagiwara, Masayuki*
Journal of the Physical Society of Japan, 90(4), p.044704_1 - 044704_9, 2021/04
Times Cited Count：3 Percentile：30.35(Physics, Multidisciplinary)Taya, Hidetoshi*; Park, A.*; Cho, S.*; Gubler, P.; Hattori, Koichi*; Hong, J.*; Huang, X.-G.*; Lee, S. H.*; Monnai, Akihiko*; Onishi, Akira*; et al.
Physical Review C, 102(2), p.021901_1 - 021901_6, 2020/08
Times Cited Count：8 Percentile：69.78(Physics, Nuclear)
resonances in a boxOno, Akira*; Xu, J.*; Colonna, M.*; Danielewicz, P.*; Ko, C. M.*; Tsang, M. B.*; Wang, Y,-J.*; Wolter, H.*; Zhang, Y.-X.*; Chen, L.-W.*; et al.
Physical Review C, 100(4), p.044617_1 - 044617_35, 2019/10
Times Cited Count：58 Percentile：98.56(Physics, Nuclear)International comparison of heavy-ion induced reaction models were discussed in the international conference "Transport2017" held in April 2017. Owing to their importance for safety assessment of heavy-ion accelerators and dosimetry of astronauts, various models to simulate heavy-ion induced reaction models are developed. This study is intended to clarify the difference among them to pinpoint their problems. In the comparison study, 320 protons and neutrons were packed in a 20-fm-large cube to calculate the number and energies of collisions during the time evolution. The author contributed to this study by running calculation using JQMD (JAERI Quantum Molecular Dynamics). This study showed that time step in the calculation is one of the biggest causes of the discrepancies. For example, the calculation by JQMD comprises 1-fm/c time steps, each of which is composed of transport, scattering and decay phases. Therefore a sequence of scattering, and decay followed by another scattering in 1 fm/c cannot be considered. Moreover, in JQMD particles are labeled by sequential numbers and scattering reactions are simulated by the order. Therefore scattering between low ID numbers, that between high ID numbers and that between the first (low ID) pair is overlooked in JQMD. Above indications obtained in this study must be kept in our mind for future JQMD upgrades.
Ni
Mn
CoO in a lithium-ion batteryKonishi, Hiroaki*; Hirano, Tatsumi*; Takamatsu, Daiko*; Gunji, Akira*; Feng, X.*; Furutsuki, Sho*; Okumura, Takafumi*; Terada, Shohei*; Tamura, Kazuhisa
Journal of Solid State Chemistry, 262, p.294 - 300, 2018/06
Times Cited Count：9 Percentile：49.17(Chemistry, Inorganic & Nuclear)The potential in each state of charge (SOC) during charging of LiNiMnCoO is higher than that during discharging. To clarify the effect of chargedischarge operating conditions on the electrochemical reaction, LiNiMnCoO was charged and discharged under various charge-discharge operating ranges, and OCP, crystal structure, and oxidation states of the ransition metals were evaluated by electrochemical measurement, XRD, and XAFS. These results indicate that OCP, lattice parameters, and oxidation states of the transition metals of LiNiMnCoO in each SOC are not constant. The XRD results indicate that two phases, namely, LiNi
MnCoO-like and LiMnO
-like, exist in LiNiMnCoO.
Zhang, Y.-X.*; Wang, Y,-J.*; Colonna, M.*; Danielewicz, P.*; Ono, Akira*; Tsang, M. B.*; Wolter, H.*; Xu, J.*; Chen, L.-W.*; Cozma, D.*; et al.
Physical Review C, 97(3), p.034625_1 - 034625_20, 2018/03
Times Cited Count：98 Percentile：99.11(Physics, Nuclear)International comparison of heavy-ion induced reaction models were discussed in the international conference "Transport2017" held in April 2017. Owing to their importance for safety assessment of heavy-ion accelerators and dosimetry of astronauts, various models to simulate heavy-ion induced reaction models are developed. This study is intended to clarify the difference among them to pinpoint their problems. In the comparison study, 320 protons and 320 neutrons were packed in a 20-fm-large cube to calculate the number of particle-particle collisions as well as the energies of collisions during the time evolution. In addition to the calculation, their algorithms were compared. The author contributed to this study by running calculation using JQMD (JAERI Quantum Molecular Dynamics). The results were compared with those calculated by the other 15 codes from over the world. Algorithm comparison showed that JQMD calculates collision probabilities from protons at first and collisions by neutrons are simulated later, which might be unreasonable. On the other hand, it was clarified that the calculation by JQMD agrees with those by the others. Despite the fact that some codes deviate from the average by a factor of 2, JQMD exhibited stable performance.
NiMnCoO used for lithium ion batteriesKonishi, Hiroaki*; Hirano, Tatsumi*; Takamatsu, Daiko*; Gunji, Akira*; Feng, X.*; Furutsuki, Sho*; Okumura, Takafumi*; Terada, Shohei*; Tamura, Kazuhisa
Journal of Solid State Chemistry, 258, p.225 - 231, 2018/02
Times Cited Count：8 Percentile：44.83(Chemistry, Inorganic & Nuclear)LiNiMnCoO is known as one of the cathode electrode material for Li ion batteries and its structure during charge and discharge process was investigated using electrochemical method and X-ray diffraction. It was found that in the charge process the structure changes in the order of LiMnO, LiNiMnCoO, and LiMnO. On the other hand, in the discharge process, the structure changes in the order of LiMnO and LiNiMnCoO.
=1/2 quasi-one-dimensional Ising-like antiferromagnet BaCoVO in a transverse magnetic fieldMatsuda, Masaaki*; Onishi, Hiroaki; Okutani, Akira*; Ma, J.*; Agrawal, H.*; Hong, T.*; Pajerowski, D. M.*; Copley, J. R. D.*; Okunishi, Koichi*; Mori, Michiyasu; et al.
Physical Review B, 96(2), p.024439_1 - 024439_8, 2017/07
Times Cited Count：12 Percentile：51.46(Materials Science, Multidisciplinary)Cho, S.*; Hyodo, Tetsuo*; Jido, Daisuke*; Ko, C. M.*; Lee, S. H.*; Maeda, Saori*; Miyahara, Kenta*; Morita, Kenji*; Nielsen, M.*; Onishi, Akira*; et al.
Progress in Particle and Nuclear Physics, 95, p.279 - 322, 2017/07
Times Cited Count：93 Percentile：89.92(Physics, Nuclear)With upgraded detectors at the Relativistic Heavy Ion Collider (RHIC) and the Large Hadron Collider (LHC), it has become possible to measure hadrons beyond their ground states in high energy heavy ion collisions. Therefore, heavy ion collisions provide a new method for studying exotic hadrons that are either molecular states made of various hadrons or compact system consisting of muliquarks. Because their structures are related to the fundamental properties of Quantum Chromodynamics (QCD), studying exotic hadrons is currently one of the most active areas of research in hadron physics. The present review is a summary of the current understanding of a selected set of exotic candidate particles that can be potentially measured in heavy ion collisions.
Naito, Fujio*; Anami, Shozo*; Ikegami, Kiyoshi*; Uota, Masahiko*; Ouchi, Toshikatsu*; Onishi, Takahiro*; Oba, Toshiyuki*; Obina, Takashi*; Kawamura, Masato*; Kumada, Hiroaki*; et al.
Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1244 - 1246, 2016/11
The proton linac installed in the Ibaraki Neutron Medical Research Center is used for production of the intense neutron flux for the Boron Neutron Capture Therapy (BNCT). The linac consists of the 3-MeV RFQ and the 8-MeV DTL. Design average beam current is 10mA. Target is made of Beryllium. First neutron production from the Beryllium target was observed at the end of 2015 with the low intensity beam as a demonstration. After the observation of neutron production, a lot of improvement s was carried out in order to increase the proton beam intensity for the real beam commissioning. The beam commissioning has been started on May 2016. The status of the commissioning is summarized in this report.
Sasaki, Akira; Nishimura, Hiroaki*; Onishi, Naofumi*
Purazuma, Kaku Yugo Gakkai-Shi, 91(2), p.166 - 167, 2015/02
no abstracts in English
Onishi, Yuki*; Takata, Takashi*; Yamaguchi, Akira*; Uchibori, Akihiro; Kikuchi, Shin; Kurihara, Akikazu; Ohshima, Hiroyuki
Proceedings of 8th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-8) (USB Flash Drive), 8 Pages, 2012/12
In the steam generator of sodium-cooled fast reactor (SFR), self-wastage phenomena is a crack enlargement on the heat transfer tube itself caused by sodium-water reaction, a quantification of the self-wastage phenomenon is of importance from the viewpoint of safety assessment. In this study, we propose a numerical approach to evaluate the self-wastage phenomena and investigate a crack enlargement using SERAPHIM code. In the analysis, two-dimensional initial crack is assumed based on SWAT-4 experiment. The wastage rate was estimated by Arrhenius type equation, and re-meshing arrangement was performed by cut down from a part of tube in the initial model with the wastage amount. After simulated again using the re-meshing models, the resulting SWR products were distributed not only circumferential direction but also radial direction.
Seki, Yohji; Onishi, Yoichi*; Yoshikawa, Akira; Tanigawa, Hisashi; Hirose, Takanori; Ozu, Akira; Ezato, Koichiro; Tsuru, Daigo; Suzuki, Satoshi; Yokoyama, Kenji; et al.
Progress in Nuclear Science and Technology (Internet), 2, p.139 - 142, 2011/10
R&D of a test blanket module (TBM) with a water-cooled solid breeder has been performed for ITER. For our design, the temperature of a coolant pressurized up to 15 MPa is designed as 598 K in an outlet of the TBM, respectively. Establishment of estimation methods of the flow phenomena is important for designs of the channel network and predictions of the material corrosion and erosion. A purpose of our research is to establish and verify the method for the prediction of the flow phenomena. The Large-eddy simulation and Reynolds averaged Navier-Stokes simulation have been performed to predict the pressure drop and flow rates in the channels of the side wall. It results the inhomogeneous flow rates in each channel. At viewpoint of the heat removal capability, however, the smallest flow-rates near the first wall are evaluated with satisfying acceptance criteria. Moreover, the results of the numerical simulation correspond with those of experiment performed for the real size mock-up.
OKirishima, Akira*; Mitsugashira, Toshiaki*; Onishi, Takashi; Sato, Nobuaki*
Journal of Nuclear Science and Technology, 48(6), p.958 - 966, 2011/06
Times Cited Count：3 Percentile：26.02(Nuclear Science & Technology)A novel reprocessing process based on the selective sulfurization of fission products (FP) has been proposed, where FP and minor actinides (MA) are first sulfurized by CS gas, and then, dissolved by a dilute nitric acid solution. Consequently, the fuel elements are recovered as UO and PuO. As a basic research of this new concept, the sulfurization and dissolution behaviors of U, Pu, Np, Am, Eu, Cs and Sr were investigated in this paper using 
Pu, 
Np, 
Am, 
Eu, 
Cs and 
Sr doped UO sample by 
ray and 
spectrometries. The dependence of the dissolution ratio of each element on the sulfurization temperature was studied and reasonably explained by combining the information of the sulfide phase analysis and the chemical thermodynamics of the dissolution reaction. The sulfurization temperature ranging from 350 to 450 
C seems to be promising for the separation of FP and MA from U and Pu.
Seki, Yohji; Onishi, Yoichi*; Yoshikawa, Akira; Tanigawa, Hisashi; Hirose, Takanori; Ozu, Akira; Ezato, Koichiro; Tsuru, Daigo; Suzuki, Satoshi; Yokoyama, Kenji; et al.
Proceedings of Joint International Conference of 7th Supercomputing in Nuclear Application and 3rd Monte Carlo (SNA + MC 2010) (USB Flash Drive), 4 Pages, 2010/10
R&D of a test blanket module (TBM) with a water-cooled solid breeder has been performed for ITER. For our design, the temperature of a coolant pressurized up to 15 MPa is designed as 598 K in an outlet of the TBM, respectively. Establishment of estimation methods of the flow phenomena is important for designs of the channel network and predictions of the material corrosion and erosion. A purpose of our research is to establish and verify the method for the prediction of the flow phenomena. The Large-eddy simulation and Reynolds averaged Navier-Stokes simulation have been performed to predict the pressure drop and flow rates in the channels of the side wall. It results the inhomogeneous flow rates in each channel. At viewpoint of the heat removal capability, however, the smallest flow-rates near the first wall are evaluated with satisfying acceptance criteria. Moreover, the results of the numerical simulation correspond with those of experiment performed for the real size mockup.
Okamura, Masachika*; Shimizu, Akira*; Onishi, Noboru*; Hase, Yoshihiro; Yoshihara, Ryohei; Narumi, Issei
JAEA-Review 2008-055, JAEA Takasaki Annual Report 2007, P. 62, 2008/11
no abstracts in English
Uehara, Shinichi*; Kobayashi, Akira*; Chijimatsu, Masakazu*; Onishi, Yuzo*; Fujita, Tomoo; Rejeb, A.*
Proceedings of 3rd International Conference on Coupled T-H-M-C Processes in Geo-systems; Fundamentals, Modeling, Experiments and Applications (GeoProc 2008), p.419 - 425, 2008/06
