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JAEA Reports

Horonobe Underground Research Laboratory Project Investigation report for the 2024 fiscal year

Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Fukatsu, Yuta; Mochizuki, Akihito; Ozaki, Yusuke; et al.

JAEA-Review 2025-042, 136 Pages, 2025/12

JAEA-Review-2025-042.pdf:12.95MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe-cho in Hokkaido, north Japan. In the fiscal year 2024, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on near-field system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100$$^{circ}$$C" were addressed for "Demonstration of repository design options". The validation of a method for assessing permeability using the Ductility Index and a method for estimating the state of in-situ ground pressure from hydraulic perturbation tests were investigated as part of the study "Understanding of buffering behaviour of sedimentary rock to natural perturbations". In FY2024, we continued construction of the East Access Shaft and the Ventilation Shaft, and construction of these shafts were completed to a depth of 500 m. After the completion of the East Access Shaft, excavation of the West Access Shaft and 500 m gallery has began. As of the end of FY2024, excavation progress is as follows, the East Access Shaft and the Ventilation Shaft were 500 m depth, the West Access Shaft was 472 m depth, 500 m gallery was 112.9 m, respectively. In the Horonobe International Project (HIP), Management Board and Joint Task Meeting was held at the Horonobe URL in June 2024 to review the progress of construction of galleries and preparations of experiments. Task Meetings to review the implementation plan for in-situ testing and analysis were also held. HIP will be implemented in two phases: Phase 1 (from FY2022 to FY2024) and Phase 2 (from FY2025 to FY2028), the research results of Phase 1 were compiled in FY2024.

Journal Articles

Metallization and pressure-induced superconductivity in carrier doped excitonic insulator (Ta$$_{1-x}$$Ti$$_x$$)$$_2$$NiSe$$_5$$

Tsuchida, Shun*; Hirose, Yusuke; Sekikawa, Takuya; Ono, Yoshiaki*; Hirahara, Takuya*; Sano, Sumika*; Kawaguchi, Shogo*; Kobayashi, Shintaro*; Uwatoko, Yoshiya*; Settai, Rikio*

Journal of the Physical Society of Japan, 94(11), p.114703_1 - 114703_7, 2025/10

We investigated the carrier doping effect on an excitonic insulator Ta$$_2$$NiSe$$_5$$ by means of the electrical resistivity $$rho$$ and Hall coefficient $$R_{rm H}$$ using single crystals of (Ta$$_{1-x}$$Ti$$_x$$)$$_2$$NiSe$$_5$$, and band calculation. The excitonic transition temperature $$T_{rm c}$$ is continuously suppressed to 83 K at $$x$$ = 0.104 while preserving the crystal structure. With increasing substitution concentration $$x$$, a semiconducting increment of $$rho$$ and $$R_{rm H}$$ is strongly suppressed and a metallic behavior is observed at $$x$$ > 0.06. Ti substitution can realize an excitonic correlated metallic state. This metallization is explained by the hole doping effect based on the band calculations. Applying pressure to the carrier doped (Ta$$_{1-x}$$Ti$$_x$$)$$_2$$NiSe$$_5$$, we found superconductivity above 2.6 GPa, which is much smaller than that of Ta$$_2$$NiSe$$_5$$ around 8 GPa. The carrier doping induced by Ti substitution favors superconductivity in this compound.

JAEA Reports

Horonobe Underground Research Laboratory Project Investigation Program for the Fiscal Year 2025

Nakayama, Masashi; Ishii, Eiichi; Hayano, Akira; Aoyagi, Kazuhei; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Mochizuki, Akihito; Ozaki, Yusuke; Kimura, Shun; et al.

JAEA-Review 2025-027, 80 Pages, 2025/09

JAEA-Review-2025-027.pdf:6.22MB

The Horonobe Underground Research Laboratory Project is being pursued by the Japan Atomic Energy Agency to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2025, we continue R&D on "Study on near-field system performance in geological environment" and "Demonstration of repository design options". These are identified as key R&D challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. In the "Study on near-field system performance in geological environment", we continue to obtain data from the full-scale engineered barrier system performance experiment, and work on the specifics of the full-scale engineered barrier system dismantling experiment. As for "Demonstration of repository design options", the investigation, design, and evaluation techniques are to be systemized at various scales, from the tunnel to the pit, by means of an organized set of evaluation methodologies for confinement performance at these respective scales. Preliminary borehole investigations will be conducted within a 500 m gallery, with the objectives of obtaining rock strength and rock permeability data, as well as surveying the extent of the excavation damaged zone surrounding the test tunnel via tomographic analysis. A planning study for the in-situ construction test will be conducted to investigate the construction of backfill material and watertight plugs. The volume of water inflow associated with the excavation of the 500 m gallery will be observed, and its magnitude will be compared with the range of water inflow predicted in the analysis. The test plan to determine the extent of the excavation damaged zone around the pit, which is planned to be constructed in the 500 m gallery, will be studied to determine the in-situ excavation damaged zone. In addition, the investigation and evaluation methods for the amount of water inflow from fractures and the extent of the excavation damaged zone around the pit will be organized. Concerning the construction and maintenance of the subsurface facilities, excavation of the West Access Shaft and the 500 m gallery will continue. It is anticipated that the construction of the facilities will be completed by the end of the fiscal year 2025. In addition, we continue R&D on the following three tasks in the Horonobe International Project; Task A: Solute transport experiment with model testing, Task B: Systematic integration of repository technology options, and Task C: Full-scale engineered barrier system dismantling experiment.

Journal Articles

Speciation of cesium in a radiocesium-bearing microparticle emitted from Unit 1 during the Fukushima nuclear accident by XANES spectroscopy using transition edge sensor

Takahashi, Yoshio*; Miura, Hikaru*; Yamada, Shinya*; Sekizawa, Oki*; Nitta, Kiyofumi*; Hashimoto, Tadashi*; Yomogida, Takumi; Yamaguchi, Akiko; Okada, Shinji*; Itai, Takaaki*; et al.

Journal of Hazardous Materials, 495, p.139031_1 - 139031_19, 2025/09

In this presentation, we analyzed the chemical state of cesium in radiocesium-bearing microparticles (CsMPs) released during the 2011 Fukushima Daiichi Nuclear Power Plant accident using high-resolution X-ray absorption spectroscopy (XANES) and micro X-ray fluorescence ($$mu$$-XRF). The results identified two forms of cesium: one dissolved in glass and the other enriched on the surfaces of internal voids. The latter is considered to have originally existed as a gas and became concentrated during the cooling and solidification of the molten glass. These findings are crucial for understanding the formation process of CsMPs during the accident, as well as for future decommissioning and safety assessments.

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste stored at the Waste Storage Facility L as compressed packages

Aono, Ryuji; Goto, Katsunori*; Kinase, Akari; Sato, Yoshiyuki; Haraga, Tomoko; Iseda, Hirokatsu

JAEA-Data/Code 2025-006, 24 Pages, 2025/07

JAEA-Data-Code-2025-006.pdf:1.05MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planned to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples stored at the waste storage facility L. In this report, we summarized the radioactivity concentrations of 12 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{60}$$Co, $$^{90}$$Sr, $$^{94}$$Nb, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am) which were obtained from radiochemical analysis of the samples in fiscal year 2020.

Journal Articles

Spontaneous magnetic field and disorder effects in BaPtAs$$_{1-x}$$Sb$$_x$$ with a honeycomb network

Adachi, Tadashi*; Ogawa, Taiki*; Komiyama, Yota*; Sumura, Takuya*; Saito-Tsuboi, Yuki*; Takeuchi, Takaaki*; Mano, Kohei*; Manabe, Kaoru*; Kawabata, Koki*; Imazu, Tsuyoshi*; et al.

Physical Review B, 111(10), p.L100508_1 - L100508_6, 2025/03

 Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-2 and JRR-3 and Stored at the Waste Storage Facility L as compressed packages

Kinase, Akari; Goto, Katsunori*; Aono, Ryuji; Konda, Miki; Sato, Yoshiyuki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2024-004, 60 Pages, 2024/07

JAEA-Data-Code-2024-004.pdf:2.05MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2 and JRR-3 and stored at the waste storage facility L. In this report, we summarized the radioactivity concentrations of 20 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2022.

Journal Articles

Development of nuclear data processing code FRENDY version 2

Tada, Kenichi; Yamamoto, Akio*; Kunieda, Satoshi; Konno, Chikara; Kondo, Ryoichi; Endo, Tomohiro*; Chiba, Go*; Ono, Michitaka*; Tojo, Masayuki*

Journal of Nuclear Science and Technology, 61(6), p.830 - 839, 2024/06

 Times Cited Count:10 Percentile:91.89(Nuclear Science & Technology)

Nuclear data processing code is important to connect evaluated nuclear data libraries and radiation transport codes. The nuclear data processing code FRENDY version 1 was released in 2019 to generate ACE formatted cross section files with simple input data. After we released FRENDY version 1, many functions were developed, e.g., neutron multi-group cross section generation, explicit consideration of the resonance interference effect among different nuclides in a material, consideration of the resonance upscattering, ACE file perturbation, and modification of ENDF-6 formatted file. FRENDY version 2 was released including these new functions. It generates GENDF and MATXS formatted neutron multi-group cross section files from an ACE formatted cross section file or an evaluated nuclear data file. This paper explains the features of the new functions implemented in FRENDY version 2 and the verification of the neutron multigroup cross section generation function of this code.

Journal Articles

Feasibility of using BeO rods as secondary neutron sources in the long-life fuel cycle high-temperature gas-cooled reactor

Ho, H. Q.; Ishii, Toshiaki; Nagasumi, Satoru; Ono, Masato; Shimazaki, Yosuke; Ishitsuka, Etsuo; Sawahata, Hiroaki; Goto, Minoru; Simanullang, I. L.*; Fujimoto, Nozomu*; et al.

Nuclear Engineering and Design, 417, p.112795_1 - 112795_6, 2024/02

 Times Cited Count:1 Percentile:16.48(Nuclear Science & Technology)

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities, 2

Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro

JAEA-Data/Code 2023-011, 32 Pages, 2023/11

JAEA-Data-Code-2023-011.pdf:0.93MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{235}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.

JAEA Reports

Analysis work report on removal of spent fuel sheared powder for decommissioning of main plant

Aoya, Juri; Mori, Amami; Sato, Hinata; Kono, Soma; Morokado, Shiori; Horigome, Kazushi; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo

JAEA-Technology 2023-008, 34 Pages, 2023/06

JAEA-Technology-2023-008.pdf:1.92MB

Flush-out, by which nuclear materials in the Tokai Reprocessing Plant process are recovered, has been started in June 2022 as the first step of decommissioning. Flush-out consists of removal of spent fuel sheared powder, plutonium solution, uranium solution, and the other nuclear materials. Removal of spent fuel sheared powder has been completed in September 2022. During removal of spent fuel sheared powder, uranium concentration, plutonium concentration, acid concentration, radioactivity concentration, and solution density have been analyzed for process control. For nuclear material accountancy, uranium concentration, plutonium concentration, isotope ratio, and solution density have been analyzed. Analysis work including sample pretreatment before transportation to IAEA analytical facility for safeguards, and the other operations related to Flush-out such as calibration of analytical instruments, education, and training of operators are reported.

Journal Articles

Magnetic and transport properties of the pseudobrookite Al$$_{1-x}$$Ti$$_{2+x}$$O$$_{5}$$ single crystals

Takahama, Ryusei*; Arizono, Mitsutoshi*; Indo, Daigo*; Yoshinaga, Taisei*; Terakura, Chieko*; Takeshita, Nao*; Shirasaki, Takumi*; Noda, Masaaki*; Kuwahara, Hideki*; Kajimoto, Ryoichi; et al.

JPS Conference Proceedings (Internet), 38, p.011114_1 - 011114_6, 2023/05

JAEA Reports

Development of "MOX weighing and Ball-mill blending" based on experience in operation and maintenance of MOX fuel manufacturing equipment

Kawasaki, Kohei; Ono, Takanori; Shibanuma, Kimikazu; Goto, Kenta; Aita, Takahiro; Okamoto, Naritoshi; Shinada, Kenta; Ichige, Hidekazu; Takase, Tatsuya; Osaka, Yuki; et al.

JAEA-Technology 2022-031, 91 Pages, 2023/02

JAEA-Technology-2022-031.pdf:6.57MB

The document for back-end policy opened to the public in 2018 by Japan Atomic Energy Agency (hereafter, JAEA) states the decommissioning of facilities of Nuclear Fuel Cycle Engineering Laboratories and JAEA have started gathering up nuclear fuel material of the facilities into Plutonium Fuel Production Facilities (hereafter, PFPF) in order to put it long-term, stable and safe storage. Because we planned to manufacture scrap assemblies almost same with Monju fuel assembly using unsealed plutonium-uranium mixed-oxide (hereafter, MOX) powder held in PFPF and transfer them to storage facilities as part of this "concentration" task of nuclear fuel material, we obtained permission to change the use of nuclear fuel material in response to the new regulatory Requirements in Japan for that. The amount of plutonium (which is neither sintered pellets nor in a lidded powder-transport container) that could be handled in the pellet-manufacturing process was limited to 50 kg Pu or less in order to decrease the facility risk in this manufacture. Therefore, we developed and installed the "MOX weighing and blending equipment" corresponding with small batch sizes that functioned in a starting process and the equipment would decrease handling amounts of plutonium on its downstream processes. The failure data based on our operation and maintenance experiences of MOX fuel production facilities was reflected in the design of the equipment to further improve reliability and maintainability in this development. The completed equipment started its operation using MOX powder in February 2022 and the design has been validated through this half-a-year operation. This report organizes the knowledge obtained through the development of the equipment, the evaluation of the design based on the half-a-year operation results and the issues in future equipment development.

Journal Articles

Restoration of oxygen vacancies on an anatase TiO$$_{2}$$(001) surface with supersonic seeded oxygen molecular beam

Katsube, Daiki*; Ono, Shinya*; Inami, Eiichi*; Yoshigoe, Akitaka; Abe, Masayuki*

Vacuum and Surface Science, 65(11), p.526 - 530, 2022/11

The oxidation of oxygen vacancies at the surface of anatase TiO$$_{2}$$ (001) was investigated by synchrotron radiation photoelectron spectroscopy and supersonic O$$_{2}$$ beam (SSMB). The oxygen vacancies at the top surface and subsurface could be eliminated by the supply of hyperthermal oxygen molecules. Oxygen vacancies are present on the surface of anatase TiO$$_{2}$$(001) when it is untreated before transfer to a vacuum chamber. These vacancies, which are stable in the ambient condition, could also be effectively eliminated by using oxygen SSMB. This result is promising as a surface processing for various functional oxides.

Journal Articles

Cr doping-induced ferromagnetism in the spin-glass Cd$$_{1-x}$$Mn$$_x$$Te studied by X-ray magnetic circular dichroism

Verma, V.*; Sakamoto, Shoya*; Ishikawa, Koichiro*; Singh, V. R.*; Ishigami, Keisuke*; Shibata, Goro; Kadono, Toshiharu*; Koide, Tsuneharu*; Kuroda, Shinji*; Fujimori, Atsushi*

Physica B; Condensed Matter, 642, p.414129_1 - 414129_5, 2022/10

 Times Cited Count:5 Percentile:36.01(Physics, Condensed Matter)

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:8 Percentile:71.12(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Calculation of shutdown gamma distribution in the high temperature engineering test reactor

Ho, H. Q.; Ishii, Toshiaki; Nagasumi, Satoru; Ono, Masato; Shimazaki, Yosuke; Ishitsuka, Etsuo; Goto, Minoru; Simanullang, I. L.*; Fujimoto, Nozomu*; Iigaki, Kazuhiko

Nuclear Engineering and Design, 396, p.111913_1 - 111913_9, 2022/09

 Times Cited Count:1 Percentile:11.24(Nuclear Science & Technology)

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Development of nuclear data processing code FRENDY version 2

Tada, Kenichi; Yamamoto, Akio*; Endo, Tomohiro*; Chiba, Go*; Ono, Michitaka*; Tojo, Masayuki*

Proceedings of International Conference on Physics of Reactors 2022 (PHYSOR 2022) (Internet), 10 Pages, 2022/05

Nuclear data processing is an important interface between an evaluated nuclear data library and nuclear transport calculation codes. JAEA has developed a new nuclear data processing code FRENDY from 2013. FRENDY version 1 generates ACE files which are used for the continuous-energy Monte Carlo codes including PHITS, Serpent, and MCNP; it was released as an open-source software under the 2-clause BSD license in 2019. After FRENDY version 1 was released, many functions are developed: the multi-group neutron cross-section library generation, the statistical uncertainty quantification for the probability tables for unresolved resonance cross-section, the perturbation of the ACE file, and the modification of the ENDF-6 formatted nuclear data file, etc. We released FRENDY version 2 including these functions. This presentation explains the overview of FRENDY and features of the new functions implemented in FRENDY version 2.

Journal Articles

Structural phase transition in cobalt oxyfluoride Co$$_{3}$$Sb$$_{4}$$O$$_{6}$$F$$_{6}$$ observed by high-resolution synchrotron and neutron diffraction

Shimono, Seiya*; Ishibashi, Hiroki*; Nagayoshi, Yusuke*; Ikeno, Hidekazu*; Kawaguchi, Shogo*; Hagihara, Masato; Torii, Shuki*; Kamiyama, Takashi*; Ichihashi, Katsuya*; Nishihara, Sadafumi*; et al.

Journal of Physics and Chemistry of Solids, 163, p.110568_1 - 110568_7, 2022/04

 Times Cited Count:2 Percentile:11.13(Chemistry, Multidisciplinary)

274 (Records 1-20 displayed on this page)