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probed by anisotropic low-energy excitationsIshihara, Kota*; Roppongi, Masaki*; Kobayashi, Masayuki*; Imamura, Kumpei*; Mizukami, Yuta*; Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Hashimoto, Kenichiro*; et al.
Nature Communications (Internet), 14, p.2966_1 - 2966_7, 2023/05
Times Cited Count：1 Percentile：77.02(Multidisciplinary Sciences)The superconducting symmetry of the heavy fermion uranium-based superconductor UTe is investigated using low temperature penetration depth measurements. The anisotropic low-energy quasiparticle excitations indicates multiple superconducting components in a chiral complex form. The most consistent is a chiral non-unitary state.
along hard magnetic axisSakai, Hironori; Tokiwa, Yoshifumi; Opletal, P.; Kimata, Motoi*; Awaji, Satoshi*; Sasaki, Takahiko*; Aoki, Dai*; Kambe, Shinsaku; Tokunaga, Yo; Haga, Yoshinori
Physical Review Letters, 130(19), p.196002_1 - 196002_6, 2023/05
Times Cited Count：0 Percentile：90.94(Physics, Multidisciplinary)The superconducting (SC) phase diagram in uranium ditelluride is explored under magnetic fields (
) along the hard magnetic 
-axis using a high-quality single crystal with 
= 2.1 K. Simultaneous electrical resistivity and AC magnetic susceptibility measurements discern low- and high-field SC (LFSC and HFSC, respectively) phases with contrasting field-angular dependence. Crystal quality increases the upper critical field of the LFSC phase, but the 
of 
T, at which the HFSC phase appears, is always the same through the various crystals. A phase boundary signature is also observed inside the LFSC phase near , indicating an intermediate SC phase characterized by small flux pinning forces.
Ishihara, Kota*; Kobayashi, Masayuki*; Imamura, Kumpei*; Konczykowski, M.*; Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Hashimoto, Kenichiro*; Shibauchi, Takasada*
Physical Review Research (Internet), 5(2), p.L022002_1 - L022002_6, 2023/04
Lower superconducting critical fields 
of UTe have been determined. Orthorhombic UTe has magnetic easy axis along the 
-axis. We found perpendicular to showed anomalous enhancement. By comparing with anisotropy of upper critical fields, effect of magnetic fluctuations on superconductivity is suggested.
Te
Opletal, P.; Sakai, Hironori; Haga, Yoshinori; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo
Journal of the Physical Society of Japan, 92(3), p.034704_1 - 034704_5, 2023/03
Times Cited Count：0 Percentile：0.01(Physics, Multidisciplinary)We investigate the physical properties of a single crystal of uranium telluride UTe. We have confirmed that UTe crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1 
per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at 
= 48 K, where the in-plane magnetization increases sharply, whereas the out of-plane component does not increase significantly. With decreasing temperature further below under field-cooling conditions, the out-of-plane component increases rapidly around T
= 26 K. In contrast, the in-plane component hardly changes at T. Specific heat measurement indicates no 
-type anomaly around T, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.
Rh
SnOpletal, P.; Duverger-N
dellec, E.*; Miliyanchuk, K.*; Malick, S.*; Hossain, Z.*; Custers, J.*
Journal of Alloys and Compounds, 927, p.166941_1 - 166941_7, 2022/12
Times Cited Count：0 Percentile：46.51(Chemistry, Physical)Aoki, Dai*; Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Ishizuka, Jun*; Yanase, Yoichi*; Harima, Hisatomo*; Nakamura, Ai*; Li, D.*; Homma, Yoshiya*; et al.
Journal of the Physical Society of Japan, 91(8), p.083704_1 - 083704_5, 2022/08
Times Cited Count：15 Percentile：97.13(Physics, Multidisciplinary) by molten salt flux methodSakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Tokunaga, Yo; Kambe, Shinsaku; Haga, Yoshinori
Physical Review Materials (Internet), 6(7), p.073401_1 - 073401_10, 2022/07
Times Cited Count：9 Percentile：87.97(Materials Science, Multidisciplinary)The molten salt flux method is applied as a new synthetic route for the single crystals of the spin-triplet superconductor UTe. The single crystals under an optimized growth condition with excess uranium exhibit a superconducting transition at 
K, which is the highest reported for this compound. The obtained crystals show a remarkably large residual resistivity ratio with respect to the room temperature value and a small residual electronic contribution in specific heat well below . These results indicate that the increase of in UTe can be achieved by reducing the disorder associated with uranium vacancies. The excess uranium in the molten salt acts as a reducing agent, preventing tetravalent uranium from becoming pentavalent and suppressing creation of uranium vacancies. At the same time, the relatively low growth temperature can suppress Te volatilization.
Haga, Yoshinori; Opletal, P.; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Tokunaga, Yo; Kambe, Shinsaku; Sakai, Hironori
Journal of Physics; Condensed Matter, 34(17), p.175601_1 - 175601_7, 2022/04
Times Cited Count：14 Percentile：92.94(Physics, Condensed Matter)Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Haga, Yoshinori; Tokiwa, Yoshifumi; Opletal, P.; Fujibayashi, Hiroyuki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; et al.
Journal of the Physical Society of Japan, 91(2), p.023707_1 - 023707_5, 2022/02
Times Cited Count：11 Percentile：95.05(Physics, Multidisciplinary)
Te NMR experiments in field () applied along the easy magnetization axis (the -axis) revealed slow electronic dynamics developing in the paramagnetic state of UTe. The observed slow fluctuations are concerned with a successive growth of long-range electronic correlations below 30
40 K, where the spin susceptibility along the hard magnetization axis (the -axis) shows a broad maximum. The experiments also imply that tiny amounts of disorder or defects locally disturb the long-range electronic correlations and develop an inhomogeneous electronic state at low temperatures, leading to a low temperature upturn observed in the bulk-susceptibility in 
. We suggest that UTe would be located on the paramagnetic side near an electronic phase boundary, where either the magnetic or Fermi-surface instability would be the origin of the characteristic fluctuations.
Ru
Al studied in single crystalsPospisil, J.; Opletal, P.*; Vali
ka, M.*; Tokunaga, Yo; Stunault, A.*; Haga, Yoshinori; Tateiwa, Naoyuki; Gillon, B.*; Honda, Fuminori*; Yamamura, Tomoo*; et al.
Journal of the Physical Society of Japan, 85(3), p.034710_1 - 034710_10, 2016/03
Times Cited Count：9 Percentile：56.39(Physics, Multidisciplinary)Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori
no journal, ,
no abstracts in English
Opletal, P.; Sakai, Hironori; Haga, Yoshinori; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo; Tokiwa, Yoshifumi
no journal, ,
Opletal, P.; Sakai, Hironori; Haga, Yoshinori; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo; Tokiwa, Yoshifumi
no journal, ,
and its effect on physical propertiesHaga, Yoshinori; Opletal, P.; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Tokunaga, Yo; Kambe, Shinsaku; Sakai, Hironori
no journal, ,
no abstracts in English
Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Fujibayashi, Hiroyuki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; et al.
no journal, ,
We report the results of Te NMR measurements in field () applied along the easy magnetization axis (the -axis). The experiments revealed slow electronic dynamics developing in the paramagnetic state of UTe. The observed slow fluctuations are concerned with a successive growth of long-range electronic correlations below 3040 K, where the spin susceptibility along the hard magnetization axis (the -axis) shows a broad maximum. The experiments also imply that tiny amounts of disorder or defects locally disturb the long-range electronic correlations and develop an inhomogeneous electronic state at low temperatures, leading to a low temperature upturn observed in the bulk-susceptibility in .
Opletal, P.; Sakai, Hironori; Tokiwa, Yoshifumi; Haga, Yoshinori; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo
no journal, ,
Opletal, P.; Sakai, Hironori; Tokiwa, Yoshifumi; Haga, Yoshinori; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo
no journal, ,
Haga, Yoshinori; Opletal, P.; Sakai, Hironori; Yamamoto, Etsuji; Kambe, Shinsaku; Tokunaga, Yo; Tokiwa, Yoshifumi
no journal, ,
Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Haga, Yoshinori; Tokiwa, Yoshifumi; Opletal, P.; Fujibayashi, Hiroyuki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; et al.
no journal, ,
; NMR studyTokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori
no journal, ,
no abstracts in English
