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Journal Articles

Preliminary evaluation of local structure and speciation of lanthanoids in aqueous solution, iron hydroxide, manganese dioxide, and calcite using the L$$_{3}$$-Edge X-ray absorption near edge structure spectra

Ota, Atsuyuki*; Tanaka, Kazuya; Tsuno, Hiroshi*

Journal of Physical Chemistry A, 122(41), p.8152 - 8161, 2018/10

 Times Cited Count:1 Percentile:3.42(Chemistry, Physical)

We investigated the application of L$$_{3}$$-edge XANES spectra to the local structural analysis of lanthanoids in aqueous solution, iron hydroxide, manganese dioxide, and calcium carbonate. For each lanthanoid, the full width at half maximum (FWHM) values of lanthanoid compounds roughly decreased with increasing coordination numbers. However, they did not strictly reflect the local coordination sphere of the lanthanoid complex, but were rather sensitive to their chemical forms. The relationship between the magnitude of the FWHM values was determined by the crystal field splitting or degeneracy of 5d orbitals. The systematic variation of FWHM can be explained by the ligand strength of the ligand molecules (-H$$_{2}$$O$$^{0}$$, -O$$^{-}$$, -OH$$^{-}$$, -CO$$_{3}$$$$^{2-}$$, -Cl$$^{-}$$, and -O$$^{2-}$$) that cause the crystal field splitting. Therefore, the FWHM values of L$$_{3}$$-edge XANES of lanthanoid compounds may be more useful in speciation analysis rather than structural analysis such as EXAFS.

JAEA Reports

Fuel and core design studies on metal fuel sodium-cooled fast reactor (4), (5) and (6); Joint research report for JFY2009 - 2012

Uematsu, Mari Mariannu; Sugino, Kazuteru; Kawashima, Katsuyuki; Okano, Yasushi; Yamaji, Akifumi; Naganuma, Masayuki; Oki, Shigeo; Okubo, Tsutomu; Ota, Hirokazu*; Ogata, Takanari*; et al.

JAEA-Research 2012-041, 126 Pages, 2013/02

JAEA-Research-2012-041.pdf:16.49MB

The characteristics of sodium-cooled metal fuel core compared to MOX fuel core are given by its higher heavy metal density and superior neutron economy. By taking advantage of these characteristics and allowing flexibility in metal fuel specification and core design conditions as sodium void reactivity and bundle pressure drop, core design with high burnup, high breeding ratio and low fuel inventory features will be achievable. On ground of the major achievements in metal fuels utilization as driver fuels in sodium fast reactors in U.S., the metal fuel core concept is selected as a possible alternative of MOX fuel core concept in FaCT project. This report describes the following items as a result of the joint study on "Reactor core and fuel design of metal fuel core of sodium-cooled fast reactor" conducted by JAEA and CRIEPI during 4 years from fiscal year 2009 to 2012.

JAEA Reports

User's guide of parallel program development environment (PPDE), The 2nd edition

Ueno, Koichi*; Ota, Hirofumi*; Takemiya, Hiroshi*; Imamura, Toshiyuki; Koide, Hiroshi; Matsuda, Katsuyuki*; Higuchi, Kenji; Hirayama, Toshio

JAERI-Data/Code 2000-023, p.287 - 0, 2000/03

JAERI-Data-Code-2000-023.pdf:34.96MB

no abstracts in English

JAEA Reports

User's guide of parallel program development environment (PPDE)

Ueno, Koichi*; Ota, Hirofumi*; Takemiya, Hiroshi*; Imamura, Toshiyuki; Koide, Hiroshi; Matsuda, Katsuyuki*; Higuchi, Kenji; Hirayama, Toshio

JAERI-Data/Code 2000-012, p.125 - 0, 2000/03

JAERI-Data-Code-2000-012.pdf:19.49MB

no abstracts in English

JAEA Reports

Assessment on the mechanical stability of underground excavations

; Taniguchi, Wataru; Koo, Shigeru*; Hasegawa, Hiroshi; Sugino, Hiroyuki; Kubota, Shigeru*; Dewa, Katsuyuki*

JNC TN8400 99-037, 281 Pages, 1999/11

JNC-TN8400-99-037.pdf:15.51MB

It is planned to construct the tunnels and emplace waste packages at several hundred meters to 1,000 meters under the ground for the repository of high-level radioactive waste based on a policy to assure the safe life environment. It is required to be mechanically stable for the tunnels to assure the work safety throughout the construction, operation and closure phase. In this report, the mechanical stability of tunnels, that is a factor of design requisites, was evaluated by the analyses to present an outline of the technical reliability of geological disposal. To put it concretely, the tunnel sections were determined to have the required areas and shapes, and the analyses on the mechanical stability at tunnel excavations and earthquake, at tunnel intersections were conducted by the theoretical analysis and finite element method. The results obtained by these investigations are shown below: (1)It will be able to construct the tunnels with present techniques. The mechanical stability of tunnels will be assured if proper supports are given, and adequate tunnel spacing and disposal-pit pitches are set. (2)The mechanical stability will be assured at the tunnels intersections if proper reinforcement measures are taken. The reinforcement will be required for the intersection areas over the distance of 1D (D: diameter of tunnels) on the obtuse angle side, and 4D on the acute angle side, when intersection angle is set at 30 degrees. (3)The investigations were conducted on the assumption that the experienced big earthquake occurred. The results show that the effect of earthquake on the mechanical stability of tunnels is small, and tunnels are stable at the earthquake when the mechanical stability at tunnel excavations is assured.

Journal Articles

Distributed parallel scientific computing environment; SSP

Takemiya, Hiroshi; Ota, Hirofumi; Imamura, Toshiyuki; Koide, Hiroshi; Matsuda, Katsuyuki; Higuchi, Kenji; Hirayama, Toshio; Kasahara, Hironori*

Keisan Kogaku Koenkai Rombunshu, 4(1), p.333 - 336, 1999/05

no abstracts in English

Journal Articles

Present status and prospects of NUCEF project; Fuel cycle safety engineering research

Takeshita, Isao; Maeda, Mitsuru; Miyoshi, Yoshinori; Ono, Akio; Okazaki, Shuji; Nakajima, Ken; Fujine, Sachio; Kubota, Masumitsu; Muraoka, Susumu; Ara, Katsuyuki; et al.

Genshiryoku Kogyo, 43(9), p.1 - 37, 1997/09

no abstracts in English

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